Differential measurement of the ultracold Cs radiative escape and fine structure changing collision rates

We present direct measurements of the overall trap loss rate and the fine structure changing collision rate for ultracold cesium atom confined in a magneto-optical trap over an intensity range of 5 mW/cm² to 200 mW/cm². This set of simultaneous measurements allows the accurate extraction and separation of the fine structure changing rate and the radiative escape rate as these two processes compete with one another to determine the overall trap loss rate. Received 4 December 1998 and Received in final form 18 March 1999     

Flux enhancement model for cold cesium fine-structure changing collisions

The measurements of fine-structure changing collisions in a cesium magneto-optical trap, reported in a previous work [A. Fioretti et al., Phys. Rev. A 55, R3999 (1997)], are reanalyzed within a model based on the flux enhancement effect, which takes place in cold atomic collisions. In the present analysis, we consider the cooperative effect of the long-range and the shorter-range excitation by the strong trap laser. We evidence also the important role of the hyperfine structure of the Cs₂ molecular levels asymptotically connected to the ground-state and excited-state dissociation limits. Received 22 July 1999 and Received in final form 4 May 2000     

Two body loss rate in a magneto-optical trap of metastable He

We have measured the two body loss rate in a magneto-optical trap containing triplet metastable He atoms. We find a rate constant cm³/s at a -8 MHz detuning, with an uncertainty of a factor 2. This measurement is in disagreement with a recent experiment which measures the absolute, ion-producing collision rate, but agrees with several other published measurements. Received 20 April 1999 and Received in final form 12 July 1999     

Cold inelastic collisions between lithium and cesium in a two-species magneto-optical trap

We investigate collisional properties of lithium and cesium which are simultaneously confined in a combined magneto-optical trap. Trap-loss collisions between the two species are comprehensively studied. Different inelastic collision channels are identified, and inter-species rate coefficients as well as cross-sections are determined. It is found that loss rates are independent of the optical excitation of Li, as a consequence of the repulsive Li^*-Cs interaction. Li and Cs loss by inelastic inter-species collisions can completely be attributed to processes involving optically excited cesium (fine-structure changing collisions and radiative escape). By lowering the trap depth for Li, an additional loss channel of Li is observed which results from ground-state Li-Cs collisions changing the hyperfine state of cesium. Received 28 December 1998 and Received in final form 16 February 1999     

Cold rubidium molecule formation through photoassociation: A spectroscopic study of the 0 g - long-range state of 87 Rb 2

We report the detailed analysis of translationally cold rubidium molecule formation through photoassociation. Cold molecules are formed after spontaneous decay of photoexcited molecules from a laser cooled atomic sample, and are detected by selective mass spectroscopy after two-photon ionization into Rb ₂ ⁺ ions. A spectroscopic study of the 0 _g ^- (5 S + 5 P _3/2 ) pure long-range state of ⁸⁷Rb₂ is performed by detecting the ion yield as a function of the photoassociation laser frequency; the spectral data are theoretically analyzed within the semiclassical RKR approach. Molecular ionization is resonantly enhanced through either the 2 ³ Π _g or the 2 ³ Σ ⁺ _g intermediate molecular states. Some vibrational levels of the latter electronic state are observed and assigned here for the first time. Finally, cold molecules formation rates are calculated and compared to the experimentally measured ones, and the vibrational distribution of the formed molecules in the a ³ Σ ⁺ _u ground triplet state is discussed. Received 18 January 2001 and Received in final form 10 April 2001     

Formation of ultracold molecules via photoassociation with blue detuned laser light

We propose a new possibility to form ultracold molecules, via photoassociation of a pair of cold atoms into vibrational levels of the external well of an excited electronic state located at intermediate interatomic distance ( ≈ 20 Bohr radii), and embedded in the dissociation continuum above its dissociation limit. The existence of such a well is demonstrated by conventional free-free absorption spectroscopy at thermal energies. Estimation for cold atom photoassociation and cold molecule formation rates are obtained within a perturbative approach [Drag et al., IEEE J. Quant. Electr. 36, 1378 (2000)], and are found observable for usual conditions of photoassociation experiments. Received 1st March 2001     

Inversion analysis of K 2 coupled electronic states with the Fourier grid method

We present a new determination of the potential curves and interactions of the coupled electronic states A ¹ Σ ⁺ _u and b ³ Π _u of the potassium dimer, based on new laser spectroscopy measurements within a molecular beam, combined with data available in the literature. We used a new global deperturbation approach, involving the Fourier Grid Hamiltonian method for energy level calculation. A standard deviation of 1.2 is obtained corresponding to a variance of 7.5×10 ^-3 cm^-1, representing a significant improvement compared to the standard deviation of 4 yielded by the traditional local deperturbation approach. Received 12 June 2001 and Received in final form 3 September 2001     

Penning collisions of laser-cooled metastable helium atoms

We present experimental results on the two-body loss rates in a magneto-optical trap of metastable helium atoms. Absolute rates are measured in a systematic way for several laser detunings ranging from -5 to -30 MHz and at different intensities, by monitoring the decay of the trap fluorescence. The dependence of the two-body loss rate coefficient β on the excited state ( 2³ P ₂) and metastable state ( 2³ S ₁) populations is also investigated. From these results we infer a rather uniform rate constant K _sp = (1±0.4)×10^-7 cm³/s. Received 8 September 2000 and Received in final form 19 December 2000     

Detection by two-photon ionization and magnetic trapping of cold Rb2 triplet state molecules

We present detailed experimental spectra and accurate theoretical interpretation of resonance-enhanced two-photon ionization of ultracold rubidium molecules in the 14000–17000 cm^-1 transition energy range. The dimers are formed in a magneto-optical trap by photoassociation followed by radiative decay into the a ³Σ_u⁺ lowest triplet state. The theoretical treatment of the process, which reproduces the main features of the spectra, takes into account the photoassociation and decay steps as well as the resonant ionization through the manifold of intermediate gerade states correlated to the 5S + 4D limit. In particular, the energy of the v=1 level of the potential well has been determined for the first time. In addition, a tight constraint has been put on the position of the a ³Σ_u⁺ repulsive wall. Finally, magnetic trapping of rubidium molecules in the a ³Σ_u⁺ state is demonstrated. Electronic supplementary material Online Material     

Photo induced collisions with laser cooled He* atoms

This paper presents an experimental investigation of cold collisions between metastable helium atoms in an optical trap at 1 mK. Penning (PI) and associative (AI) ionization reactions are distinguished using a mass spectrometer and studied under influence of near resonant laser light. Dramatic enhancement, by more than a factor 15, of the ion rate is observed when the laser is tuned close to resonance. Experimental findings are well-described, on an absolute scale, by model predictions. Received: 9 February 1998 / Revised: 4 May 1998 / Accepted: 14 May 1998     

Cross-section for collisions of ultracold Li with Na

In a magneto-optical trap (MOT) we are able to simultaneously trap and cool ⁷Li and Na. We investigated the loading behavior of the cloud of Li atoms in presence of the overlapped cloud of cold Na atoms, and, by blocking the weak repumping beam for Na, compared it with the loading curve for Li atoms only. Out of these loading curves we calculated the collision cross-section of Na on Li to be 10^-11 cm ³ /s. Received 11 January 2002 / Received in final form 5 April 2002 Published online 24 September 2002     

Comparative investigation of <Emphasis Type="Bold">39</Emphasis>K and <Emphasis Type="Bold">40</Emphasis>K trap loss rates: alternative loss channel at low light intensities

We report a comparative investigation of trap loss rates in a magneto-optical trap for two potassium isotopes, ³⁹K and ⁴⁰K, as a function of trap light intensity. The isotopes present a quite similar behavior for the loss rates at high intensities, and a sudden increase of the loss rates at low intensities is present in both cases. While for ³⁹K such increase can be explained assuming that the major contribution to the losses comes from hyperfine changing collisions, a different loss mechanism must be considered for ⁴⁰K, which has an inverted ground state hyperfine structure. The experimental results of both isotopes are well reproduced by an alternative model based on radiative escape as the dominant loss mechanism. Received 1st May 2002 / Received in final form 19 October 2002 Published online 4 March 2003 RID="a" ID="a"Alternative address: Dipartimento di Fisica, Universitá di Trento, 38050 Povo (Tn), Italy. RID="b" ID="b"e-mail: marcassa@if.sc.usp.br     

Acceleration of cold Rb atoms by frequency modulated light pulses

The displacement of Rb atoms in a magneto-optical trap (MOT) caused by the force of a finite time series of counter-propagating frequency modulated light pulse pairs is measured as a function of the chirp of the pulses. The frequency modulated light pulses induced ⁸⁵Rb 5²S_1/2 F=3 ↔ ⁸⁵Rb 5²P_3/2 F'=2, 3, 4 excitation and de-excitation of the atoms. The result of this excitation de-excitation process is a force causing the acceleration and, consequently, the displacement of the maximum of the spatial distribution of the trap atoms. The time dependence of the populations of the levels of the atom are calculated — including also the ⁸⁵Rb 5²S_1/2 F=2 and F'=1 states — as the result of the interaction with the finite train of counter propagating frequency modulated light pulses by the solution of the Bloch equations. As the result of the measurement the interval of the chirp of the frequency modulated light of given intensity where the transitions take place, are determined. The results of the experiment and the expectation on the basis of model calculations are in qualitative agreement.     

Optical spectroscopy in ion traps

Spectroscopic experiments in static or dynamic ion traps have produced results of extremely high precision. They have been, however, performed mainly on systems with simple electronic level schemes as available in singly charged ions of the earth-alkaline elements. In this contribution the most complex system investigated so far, Eu⁺, is used as example to discuss the possibility of spectroscopy on superheavy elements in traps.     

Light-induced effect on the density distribution in a sample of cold trapped atoms

As it is known [1] an intense laser field can induce atom-atom interaction according to a dipole-dipole R ^–3 law. Such an interaction depends on the angle between light polarization and interatomic vector-position R. This angular dependence may produce an anisotropy in the spatial density distribution of the confined sample of cold atoms. We develop the main relations and apply them to the case of an atomic cloud of cold trapped neutral atoms with the density higher than or of the order of ^–3, where is the wavelength of light. The results presented here show the effect of such an interaction in a density regime of high experimental interest.     

Semi-classical theory of laser cooling in two dimensions

We present a semi-classical theory of the light pressure force for atoms interacting with a two-dimensional laser field. Unlike previous 2D theory, ours is valid for general atomic level and laser field configurations. We show that striking new features appear in the velocity-dependent force arising from the multi-dimensionality. Finally, we describe in detail the novel numerical technique used in the calculation. Received 4 December 1998 and Received in final form 13 February 1999     

Collisions between linear polar molecules trapped in a microwave field

The collisions between linear polar molecules, trapped in a microwave field with circular polarization, are theoretically analyzed. We demonstrate that the collisional dynamics is mostly controlled by two ratios ν/B and x=μ₀E₀/ħ B (ν is the microwave frequency, B is the molecular rotational constant, μ₀ is the dipole moment, and E₀ is the electric field amplitude). We discuss the dependence of collision cross sections on these ratios in order to find an advantageous condition for evaporative cooling.     

Anisotropic velocity distributions in 3D dissipative optical lattices

We present a direct measurement of velocity distributions in two dimensions by using an absorption imaging technique in a 3D near resonant optical lattice. The results show a clear difference in the velocity distributions for the different directions. The experimental results are compared with a numerical 3D semi-classical Monte-Carlo simulation. The numerical simulations are in good qualitative agreement with the experimental results. Received 3 September 2002 / Received in final form 25 October 2002 Published online 11 February 2003     

Blue-Sisyphus cooling in cesium gray molasses and antidot lattices

We present an experimental study of the kinetic temperature of cesium atoms interacting with laser beams tuned on the blue side of the transition. In the case of a three-dimensional four-beam molasses, temperatures as low as 800 nK were found. These low temperatures are compatible with a good capture efficiency. The influence of other hyperfine transitions on the temperature is significant. In the presence of a static magnetic field (antidot lattices), the temperatures are slightly higher but show a much weaker dependence on the other hyperfine transitions. Received: 14 May 1998 / Received in final form: 16 October 1998 / Accepted: 2 November 1998