Yields and cross sections of the 241Am(γ, n)240mfAm and 243Am(γ, n)242mf-Am reactions in the E1 giant resonance region

The ratio of delayed to prompt fission yields has been measured for ²⁴¹Am and ²⁴³Am samples irradiated by a bremsstrahlung photon pulsed beam over the energy range E_γmax = 10–80 MeV. The relative probabilities of ^240mfAm and ^242mfAm isomer production and the cross sections of the ²⁴¹Am(γ, n)^240mfAm and ^243Am(γ, n)^242mfAm reactions were deduced from the yields measured in the E1 giant resonance region.     

Hyperfine shifts for cesium in Argon at high density

An optical pumping experiment was performed to obtain precise hfs shifts for Cs in Argon. The shifts measured include a term quadratic in the densityρ and a large temperature coefficient. The coefficients of the expansionδv/v ₀=a ρ+bρ ₂ area(80 °C)=?29.8(6)x10^?9(Torr^?1(0°C))b(80 °C)=+11(2)x10^?14(Torr^?2(0 °C)). The shift grows more negative with increasing temperature by 0.37 (2)%/°C.     

Lebensdauer- und Spinrotationsmessungen an den ersten angeregten Zuständen in197Pt und197Hg

The magnetic moment of the 134 keV state of¹⁹⁷Hg was measured by the differential angular correlation method. The half life of the state was redetermined and the half life of the 53 keV state in¹⁹⁷Pt was determined. The results are:μ(134 keV state in¹⁹⁷Hg)=+0.950(65) nmT _1/2(134 keV state in¹⁹⁷Hg)=7.3(2) nsT _1/2(53 keV state in¹⁹⁷Pt)=16.5(1.5) ns.     

Core vibration of99Tc

The gyromagnetic ratios and the half-lifes of the 141 keV and 181 keV states of⁹⁹Tc have been remeasured. The results,g(141 keV)=+1.280(44);g(181 keV)=+1.446(20) andT _1/2(141 keV)=0.205(4)ns;T _1/2(181 keV)=3.44(3) ns are in only fair agreement with prior published data but more precise. They confirm that both states are members of the ground state core vibration multiplet. The hyperfine field of TcFe has been determined asB _hf ^10K (TcFe)=30.42 (30)T;B _hf ^290K (TcFe)=29.47 (29)T     

The gyromagnetic ratio of the 589 keV 3/2− state of117In

Theg-factor of the 589 keV state of¹¹⁷In has been determined by a measurement of the rotation of the 1,303–273 keVγ —γ directional correlation in an external magnetic field of 9.55(1) T. The result,g _3/2(589 keV)=+0.068(39), contradicts the usual interpretation of the state as the 2p _3/2 single proton hole configuration for which the Schmidt value isg _3/2-(Schmidt)=+2.53. It favours the interpretation as the first rotational state built up on the single proton [301] 1/2^? Nilsson orbit in a strongly deformed core of prolate shape.     

Winkelverteilung der Polarisation der Neutronen aus der Reaktion14C(d,n 0)15N bei Deuteronenenergien zwischen 1,3 und 1,9 MeV

Polarization distributions of ground state neutrons emitted from the¹⁴C(d,n ₀)¹⁵N reaction were investigated over the angular range from 15 ° (lab) to 150 ° (lab) at bombarding energies of 1.28, 1.55 and 1.88 MeV. Scattering of neutrons from helium served as polarization analyzer. The experimental results show a large variation with energy of the polarization ranging betweenP(Θ_lab=130 °)=?21% andP(Θ_lab=130 °)=+50% at 1.28 and 1.88 MeV respectively.     

Photofission of americium isotopes in the energy range 6–12 MeV

By means of the reference method, the cross sections for the fission of the ²⁴¹Am, ^242m Am, and ²⁴³Am isotopes were measured at the microtron of the Institute of Physics and Power Engineering (Obninsk). These measurements, which employed the cross section for ²³⁸U photofission as a reference, covered the energy range 6–12 MeV scanned with a variable step of 50 to 200 keV. Data on ^242m Am photofission in the energy range 6–12 MeV and ²⁴³Am photofission in the region between 6 and 7 MeV were obtained for the first time. New results for ²⁴¹Am reveal that the cross sections for ²⁴¹Am photofission from previous studies of the present author were exaggerated. The new results for this isotope comply well with data of other authors. It is not confirmed that the fissility of ²⁴¹Am is less than the fissility of ²⁴³Am. The energy dependences of the fissilities of the americium isotopes from photofission data are compared with those that were obtained for these fissilities from data on direct reactions like ²⁴⁰Pu(³He, df)²⁴¹Am. The results of this comparison show that the observed fission thresholds and the plateaulike dependences at energies above 7.5 MeV from the two types of studies comply well. The present data show evidence that, in the energy region around 6 MeV, the photofission cross section has a maximum, which is associated, in all probability, with the low-energy resonance structure in the cross section for dipole photoabsorption.     

Atomic beam magnetic resonance investigations in the 2p 2 3 P ground multiplet of the stable carbon isotopes12C and13C

The hyperfine structure seperations Δv andg _J -factors have been measured in the 2p ^{2 3} P states of¹³C(I=1/2) and¹²C(I=0), respectively, using the atomic beam magnetic resonance method. The results are Δv(³ P ₁,¹³C)=4.200 (25) MHz, Δv(³ P ₂,¹³C)=372.593 (25) MHz,g _J (³ P ₁,¹²C)=1.501052 (13), andg _J (³ P ₂,¹²C)=1.501039 (15). After applying corrections due to perturbations by neighbouring fine structure levels one deduces the constants of the magnetic dipole interactionA(³ P ₁,¹³C)=+2.838 (17) MHz, A(³ P ₂,¹³C)=+149.055 (10) MHz. No signs of theA-factors were determined by the experiment; they follow from the known positive sign of the nuclear magnetic moment μ _I of¹³C. CombiningA(³ P ₂,¹³C) with the results of other measurements on¹¹C, yields μ _I (¹¹C)=?0.964 (1) nm.     

g-factor of the 4 1 + rotational state of160Dy

By use of Ge-detectors of the OSIRIS-collaboration [1] in connection with the 12 detector IPAC apparatus of our laboratory [2] a precise measurement of theg-factor of the 4 ₁ ⁺ rotational state of¹⁶⁰Dy was performed. The directional correlations of the threeγ-γ cascades, 1003-197 keV, 1103-197 keV and 1115-197 keV, which are weakly populated in the decay of 72.3 d¹⁶⁰Tb were observed simultaneously. The integral rotations in the static hyperfine field of DyTb at 4.2 K were measured. Theg-factorg(4 ₁ ⁺ )=+0.350(20) was derived. By comparison with the magnetic splitting of the 2 ₁ ⁺ rotational state observed in the same environment by a Mössbauer experiment [3] the ratio of the twog-factors was derived as g(4 ₁ ⁺ )/g(2 ₁ ⁺ )=+ 0.91(5). For the high energy lines we derived from the measured directional correlations the E1/M2 mixing parameters: δ(1003 keV)=+0.005(4); δ(1103 keV)=?0.020(22), and δ(1115 keV)=+0.010(4)     

Die elektrischen Kernquadrupolmomente von Cäsium 131 und Cäsium 132 aus Doppelresonanzmessungen am 72 P 3/2-Term

The hyperfine splitting of the 7² P _3/2-state of the radioactive isotopes¹³¹Cs and¹³²Cs has been investigated by optical double resonance. The hyperfine interaction constants deduced from the measured hfs transition frequencies are¹³¹Cs¹³²CsA(7² P _3/2)+31.73(6) MHz +25.03(12) MHzB(7² P _3/2)?28.63(35) MHz + 23.60(60) MHz These values yield spectroscopic nuclear quadrupole momentsQ _s (corrected for the Sternheimer effect) ofQ _s (¹³¹Cs)=?0.57(1) barnQ _s (¹³²Cs)=+0.47(1) barn. The magnetic interaction constantA of¹³²Cs results in a slightly improved precision of the nuclear magnetic dipole momentμ ₁ (¹³²Cs)=+2.22(1)μ _K . The Cesium isotopes have been produced by (d, xn)-reactions on natural Xenon. Total cross sections of the reactions¹³²Xe(d, 2n)¹³²Cs;¹³⁴Xe(d, 4n)¹³²Cs;¹³⁴Xe(d, 2n)¹³⁴Cs;¹³⁶Xe(d, 4n)¹³⁴Cs;¹³⁶Xe(d, 2n)¹³⁶Cs have been measured between 10 and 29 MeV.     

Muon Knight shift in palladium

The Knight shift at positive muons implanted in pure palladium has been measured as a function of temperature from 19.8 to 883 K. The Knight shift variation is strictly proportional to the Pd magnetic susceptibility with ΔK^μ/Δ_x=-(0.43±0.02) mole/emu=-(2.39±0.11)kG/μ_B. A temperature independent term K^μ(x=0)=+45±10 ppm is found. The results are discussed in terms of the electronic structure of H in Pd.     

Isotopieverschiebungskonstanten von Th,U, Pu und Am

The isotope shifts of unperturbed electron configurations have been determined from isotope shift measurements in the spectra of Th, U, Pu, and Am. The screening of the 7s electron charge density at the nucleus by 6d, 7s, and 7p electrons is discussed. It turns out that the same screening factors as for the 6s electron in lighter elements can be used. The screening of the 7s electron charge density at the nucleus by one 5f electron amounts to about 25%: [δT(f ⁿ s)?δT(f ⁿ )]/[δT(f ⁿ }s)?δ(f ^n} )]=0.7₅. The charge density at the nucleus due to the filleds (andp _1/2) shells is considerabely screened by anf electron. The isotope shiftδT(f^n}-1 d ^m +2)?δT(f ⁿ d ^m ) produced by this effect is of the same order of magnitude as the isotope shiftδT(f ⁿ d ^m s)-δT(f ⁿ d ^m ) due to ans electron. The experimental isotope shift constants are found to be:Β C _exp(Th²³⁰–Th²³²)=880±120;Β C _exp(U²³³–U²³⁵)=1000±180;Β C _exp(U²³⁴–U²³⁶)=1070±200;Β C _exp(U²³⁶–U²³⁸)=1080±180;Β C _exp(Pu²³⁸–Pu²⁴⁰)=1200±120;Β C _exp(Pu²³⁹–Pu²⁴¹)=1060±100;Β C _exp(Pu²⁴⁰–Pu242)=900 ±90;Β C _exp(Am²⁴¹–Am²⁴³)=890±50 [10^?3cm^?1]. The ratiosΒ C _exp/C _th are discussed.     

Nuclear orientation and NMR/ON on implanted114mIn in Fe and Co

Nuclear orientation and NMR/ON of^114mIn implanted into Fe at an energy of 80 keV and dose of 3–5×10¹⁴ cm^–2 is reported. The zero applied field resonance frequencyv ₀=203.65(6) MHz is combined with the recently determinedB _hf(InFe) of 286.8(3) kG to yield (^114mIn)=+4.658(14) nm. The nuclear spin-lattice relaxation time for^114mIn in iron is measured to be 88(18) s at 18 mK and the applied field dependence of the NMR/ON resonance frequency gives the Knight shift for the system as –2.4(6)%. The absence of measurable nuclear orientation in similarly prepared^114mInCo sources is discussed.     

Elektrisches Kernquadrupolmoment von Cäsium 134

The hyperfine structure splitting of the 7² P _3/2 state of Cs¹³⁴ has been measured by optical double resonance spectroscopy in zero magnetic field. The following interaction constants have been obtained: Magnetic hfs constantA(7² P _3/2, Cs¹³⁴)=16.851 (16) MHz. Quadrupole coupling constantB(7² P _3/2, Cs¹³⁴)=18.07 (12) MHz. Then the electric quadrupole moment of Cs¹³⁴ can be calculatedQ _hfs(Cs¹³⁴)=+0.436 (3) barn without Sternheimer correction, andQ(Cs¹³⁴)=+0.356(2) barn with Sternheimer correction. A method for the production of alkali resonance cells with quantities of less than 10¹⁴ atoms of the radioactive isotope is described.     

Half-life and magnetic moment of the 1+ first excited state in116Sb

The life-time and the magnetic dipole moment of the 1⁺ isomeric state in¹¹⁶Sb have been measured by the TDPAD method. The state was populated in the reaction¹¹⁶Sn(p, n)¹¹⁶Sb atE _p =15 MeV. The obtained results,μ(1⁺,¹¹⁶Sb)=+2.47(9) n.m. andT _1/2= 194(4) ns, support the pure single particle [πd _5/2*vd _3/2] configuration for the 1⁺ isomeric state.     

The quadrupole moments of195–197Aum(11/2) and the low temperature thermal relaxation of gold in cadmium

^195,197mHg has been oriented at low temperature in a cadmium single crystal. From the orientation pattern of the 388 keV gamma ray V_ZZ (HgCd) =+1.82(25).10¹⁸ V/cm² has been deduced. Using the dipole-relaxation mechanism on the gold isomeric state, the relaxation constant C_K=0.044(5)Ks, the quadrupole interaction frequencies _Q (195m-AuCd)=+395(18) MHz, _Q (197m-AuCd)=+380(58) MHz and (E2/M1; 261 keV) < 0 are obtained from the orientation pattern of the 261 and 279 keV gamma rays. Using literature electric field gradient of gold in cadmium, Q(195m-Au,11/2)=(+) 1.41(1.0)b and Q(197m-Au,11/2)=(+)1.35(22)b can be deduced.     

Optical determination of the nuclear moments of137La

Using the reactor-produced lanthanum isotope ₅₇ ¹³⁷ La, the hyperfine structure (hfs) of the transition La I, 5d ² 6p z ⁴ G ₁₁ ^2/0 ?5d ² 6s a ⁴ F _9/2, λ=6250 Å and La I, 5d ² 6p z ² H ₁₁ ^2/0 ? 5d ² 6s a ²G_9/2, λ=6266 Å were measured by means of a Fabry-Pérot interferometer. The nuclear spin I (¹³⁷La)=7/2, already theoretically estimated by earlier authors, was confirmed. The nuclear magnetic dipole moment μ_I(¹³⁷La)=+ 2.690 (6) n.m. and the electric quadrupole momentQ(¹³⁷La)=+ 0.26 (8) · 10^?24 cm² were determined from the ratios of the hfs interaction constantsA andB of¹³⁷La and the natural¹³⁹La.     

New measurements of the g factor of the 20Ne(41+) state with fs lifetime

In view of the puzzlingly small g factor, obtained for the ²⁰Ne(4₁⁺) state in previous measurements, in contradiction to all existing theoretical calculations, we have performed a new set of experiments that rigorously test the former results. Besides employing the same nuclear reaction for populating the nuclear states, new experimental features were introduced to exert strict control on the relevant parameters of the transient magnetic hyperfine field technique. The new result, g(4₁⁺)=+0.38(8), is close to theoretical predictions.     

Study of short-lived bromine isotopes

First experiments in the systematic study of the structure of ground states and isomeric states of Br isotopes as function of neutron number at ISOLDE, CERN are reported. The isotopes^{74g.74m,77,78,84g,84m}Br have been implanted into iron and studied with the techniques of low temperature nuclear orientation and nuclear magnetic resonance of oriented nuclei (NMR/ON). The experiments were performed with the NICOLE on-line nuclear orientation set-up using the isotope separator ISOLDE-3. NMR/ON experiments were successful for^74mBr with continuous on-line implantation and for⁷⁷Br. Using as value of the hyperfine field B_hf(BrFe)=+81.3S (3) T we obtain |g (^74mBr)|=0.455 (3) and |g (⁷⁷Br)|=0.6492 (3). Static nuclear orientation data have been measured for all above mentioned isotopes. From these data we derive |μ(⁷⁸Br, I=1)|=0.13 (3) and |μ(^84gBr, I=2)|=1.9 (7). The results are discussed within the systematics of the bromine isotopes.     

Klein paradox in the Breit equation

We demonstrate that in the Breit equation with a central potentialV(r) having the propertyV(r ₀)=E there appears a Klein paradox atr=r ₀. This phenomenon, besides the previously found Klein paradox arr→∞ appearing ifV(r)→∞ atr→∞, seems to indicate that in the Breit equation valid in the singleparticle theory the sea of particle-antiparticle pairs is not well separated from the considered two-body configuration. We conjecture that both phenomena should be absent from the Salpeter equation which is consistent with the hole theory. We prove this conjecture in the limit ofm ⁽¹⁾→∞ andm ⁽²⁾→∞, where we neglect the terms ～1/m ⁽¹⁾ and 1/m ⁽²⁾. In Appendix I we show that in the Breit equation the oscillations accumulating atr=r ₀ in the case ofm ⁽¹⁾≠m ⁽²⁾ are normalizable to the Dirac δ-function. In Appendix II the analogical statement is justified for the nonoscillating singular behaviour appearing atr=r ₀ in the case ofm ⁽¹⁾=m ⁽²⁾.