Structure of low-lying levels in91Rb and93Rb

Life-times of low-lying levels in ₃₇ ⁹¹ Rb₅₄ and ₃₇ ⁹³ Rb₅₆ have been determined fromβ ^??γ coincidence measurements at the fission-product separator JOSEF. Values oft _1/2=17.0(8) ns and 2.0(2) ns have been obtained for the levels at 1,134 keV in⁹¹Rb and 267 keV in⁹³Rb, respectively, and upper limits could be deduced for several other states. Calculations in the frame of IBFM/PTQM have been performed for⁹¹Rb, the results of which allow an interpretation of the low-lying levels of this nucleus. For the 1,134 keV level the configuration [πg _9/2?2⁺] 7/2⁺ is suggested which lies close to or even below the 9/2 ₁ ⁺ level. The calculated half-life of 14 ns for the 1,134 keV level reproduces well the experimental value. The half-life of the 267 keV level in⁹³Rb favours the assignment ofI ^π=1/2^? to this state over the alternative 3/2^?.     

First evidence for the 2+ level in the very neutron-rich nucleus102Sr

Evidence for the 2⁺ level in¹⁰²Sr is obtained from theβ-decay of¹⁰²Rb, mass separated at the ISOLDE facility. The energy of 126 keV and the collectivity of the 2⁺→0⁺ transition indicate that¹⁰²Sr is a strongly deformed rigid rotor. In addition, a sizeable lifetime is measured for the 94 keV transition in¹⁰²Y.     

The decay scheme of the 3-s Isomer of100Nb and the properties of levels in100Mo

Theβ ^? decay of the longer-lived isomer in¹⁰⁰Nb has been studied at the fission-product separator JOSEF. Measurements ofγ-ray singles spectra, ofγ-γ coincidences and ofγ-γ angular correlations have been performed. A value oft _1/2=2.99(11)s has been determined for the isomer which probably hasI ^π=4⁺ or 5⁺. A scheme of the levels of¹⁰⁰Mo which are populated in the decay of this isomer has been established. Information on the spins of several states of¹⁰⁰Mo has been obtained. Thus,I=0 levels have been identified at 1,505, 2,038 and 2,087 keV. The mixing ratios have been determined for the 2₂ ⁺→2₁ ⁺ and 2₃ ⁺→2₁ ⁺ transitions. The results provide evidence for a vibrational structure of¹⁰⁰Mo with separate bands based on the ground state and on the first excited 0⁺ level.     

The β-decay of98Y and the level scheme of98Zr

Study of theβ-decay of⁹⁸Y and of the level scheme of⁹⁸Zr was undertaken by the use of the two recoil fission product separators JOSEF and LOHENGRIN. Twoβ-decay modes have been detected for⁹⁸Y, the half-lives of which are 0.65±0.05 s and 2.0±0.2 s. The spins and parities of the two states which undergoβ-decay are proposed to be 1⁺ and 4^?, respectively, with the configurations (π1g _9/2)(ν1g _7/2) and (π2p _1/2 (ν1g _7/2). The measuredQ _β -value is 7300±400 keV for the 0.65 s decay. The level scheme of⁹⁸Zr was deduced fromγ,γ-coincidence data. Absoluteγ-intensities were obtained from two independent measurements. The half-life of the first excited state of⁹⁸Zr at 853.0 keV with spin and parity 0⁺ was determined through delayedγ, e^?-measurements to be 63 ±7ns. No indication of the coexistence of two different nuclear shapes of⁹⁸Zr was found.     

New isomers in83Br,85Rb,85Kr and86Kr

Using methods of in-beam spectroscopy in connection with 35 MeV⁷Li bombardment of⁸²Se targets four new isomers have been identified. They are observed in⁸³Br at 3070 keV (T_1/2=0.6±0.2 μs), in⁸⁵Rb at 2826 keV (T_1/2=12.5±0.6 ns), in⁸⁵Kr at 1991 keV (T_1/2=1.2+ _0.4 ^1.0 μs) and in⁸⁶Kr at 2250 keV (T_1/2=3.1±0.6 ns). Spin and parity 19/2^? have been assigned to the new isomer in⁸⁵Rb that is interpreted as the coupling of a p_3/2 proton to the g ₉ ^2/?2 two-neutron excitation of the N=48 neutron system. Using the TDPAD method an upper limit for the g-factor of ¦g¦≦0.17 has been estimated for this isomer. The same two-neutron excitation is also believed to be responsible for the new isomer in⁸³Br. The new isomers in⁸⁵Kr and⁸⁶Kr are interpreted as configurations containing the two-proton excitation (f ₅ ^2/?1 , p ₃ ^2/?1 ) where in the isomeric 17/2⁺ level of⁸⁵Kr an additional g_9/2 neutron hole is involved.     

Decay schemes and total decay energies of89Br and90Br

Spectroscopical investigations of⁸⁹Br and⁹⁰Br have been performed, utilizing the formation of the molecular ion AlBr⁺ in the ion-source of an isotope separator on-line a reactor. Detailed level schemes have been constructed for⁸⁹Kr and⁹⁰Kr, and theβ-strength function of⁸⁹Br and⁹⁰Br below the neutron binding energy is presented. The total decay energy of^89,90Br, as well as of⁸⁹Kr, have been measured by means ofβ γ-coincidences, and the population of excited states in⁸⁹Kr via⁹⁰Br delayed neutrons has been deduced.     

The Gamow-Teller beta decay of100Cd

Neutron-deficient isotopes of cadmium were produced in thep(600 MeV)+^natSn spallation reaction. The ISOLDE facility provided mass-separated beams of these isotopes. The production yield was 10³ to 10⁴ atoms/s for¹⁰⁰Cd and roughly two orders of magnitude less for⁹⁸Cd. The properties of the¹⁰⁰Cd→¹⁰⁰Ag decay were studied in detail by X-ray,γ-ray and conversion electron spectroscopy. Forty nineγ-transitions were assigned to this decay, and all but five of them were placed in the decay scheme. The half-life was determined to be 49.1±0.5 s. TheQ _EC value of 3890±70 keV was deduced from a comparison of experimental and theoreticalβ ⁺/(EC+β ⁺ probability ratios. Seven 0⁺→1⁺ Gamow-Teller transitions with log ft values between 3.5 and 4.9 were identified. The total (summed) strength is about five times smaller than predicted by the shell model for the transformation of ag _9/2 proton into ag _7/2 neutron. The quenching of the Gamow-Teller strength and other questions of nuclear structure are discussed for the¹⁰⁰Cd decay. The properties of⁹⁸Cd are inferred by extrapolation of^104,102,100Cd data, and some preliminary experimental results on⁹⁸Cd decay are presented.     

Penetration effects in111Cd

Penetration effects in the conversion process of the 7/2⁺→5/2⁺, 171 keV and 5/2⁺→1/2⁺, 245 keV transitions in¹¹¹Cd have been investigated. The decay of¹¹¹In has been studied to deduce the relative intensity of theK-conversion lines I_K(171)/I_K(245) and the ratioI _K(245)/I _L+M... (245). The values obtained for the penetration parameters of the two transitions are 0≦λ(171)≦2.3 and ?0.4≦λ ₁(245)≦1.9.     

Levels in182W populated in the decay of182Ta

Theγ-rays emitted in theβ-decay of¹⁸²Ta have been reinvestigated with improved statistics in attempting to clarify the reported new levels at 1460.41, 1592.98, 1620.36, 1712.29 and 1762.91 keV in¹⁸²W observed in theβ-decay of¹⁸²Ta. The present study demonstrated that the fifteen newγ-rays, which were used to support the existence of the five new levels, are not relevant to theγ-decay of¹⁸²Ta. Therefore the five new levels are not populated in this decay. Additionally, theγ-ray with an energy of 1035.6 keV (0 ₂ ⁺ →2 ₁ ⁺ ) deexciting theβ-band head in¹⁸²W is observed for the first time in the present decay study and the previous tentative placement of the 351.0 keVγ-ray in the level scheme is confirmed by the present coincidence measurements.     

Excited states in the doubly closed shell nucleus 50 132 Sn82

New excited states in the nucleus¹³²Sn have been identified fromγγ coincidence measurements. Strong beta feeding to a state at 7,210 keV was established. This level is interpreted as a 6^? state formed after aπg ₉ ^2/?1 →vg ₇ ^2/?1 GTβ ^? transition from the 7^? ground state of¹³²In. The deexcitation of the 7,210 keV state passes through a 4,351 keV state, providing support for a 3^? assignment of this level.     

PräziseQ β -Wert-Messungen mit einem Intrinsic-Germanium Detektor an leichten,neutronenreichen Spaltprodukten

An intrinsic Germanium detector of 10 mm depth and 300 mm² sensitive area has been used to determineβ-endpoint energies for Rb, Sr and Y fission products. It was calibrated with monoenergetic electrons supplied by a magnetic conversion electron spectrometer for the energy range from 1.6 to 8 MeV. The energy calibration of the detector is linear with deviations less than 2 · 10^?4, and the detector was recalibrated daily using precisely known gamma rays of⁹⁰Rb. At the on-line fission product separator OSTIS at the ILL, Grenoble the endpoints ofβ-singles-spectra have been determined andQ-values deduced if possible also from beta-gamma coincidence measurements. The obtainedQ-values are:⁸⁸Rb:(5 318±4) keV,⁸⁹Rb: (4 510 ± 8) keV,⁹⁰Rb: (6 578 ± 15) keV,⁹¹Rb: (5 857 ± 8) keV,⁹¹Sr: (2 704.5 ±3) keV,⁹²Rb: (8 111 + 15) keV,⁹³Rb:(7 485 ± 15) keV,⁹⁴Rb: (10 304 ± 30) keV,⁹⁴Sr: (3 512 ± 5) keV,⁹⁴Y: (4 920 ±5)keV,⁹⁵Rb: (8 947 ±100) keV,⁹⁵Y: (4 445±5) keV,⁹⁶Rb: (11 303±250) keV,⁹⁶Sr: (5 413±20) keV,⁹⁶Y: (7 120 ±50) keV,⁹⁷Rb: (10 020 ±50) keV.     

The Gamow-Teller transitions in the96Pd→96Rh decay

Using the⁴⁰Ca(4.2 MeV/u) +⁶⁰Ni reaction and on-line mass separation, the decay properties of ₄₆ ⁹⁶ Pd₅₀ were reinvestigated. From a comparison of experimental and theoreticalβ ⁺/(EC +β ⁺) probability ratios, theQ _EC value was deduced to be 3,450 ± 150 keV. The strength was determined for four 0⁺→1⁺ Gamow-Teller beta transitions and found to be quenched as compared to predictions of the single-particle shell model. For⁹⁶Pd and⁹⁴Ru the sources of this quenching are discussed.     

Atomic mass of145Eu derived from relative PK-ratios

The level scheme of⁹³Ru has been studied in⁴⁰Ca induced reactions on Ni and Fe targets. Two new levels feeding the known 17/2⁺ state have been established: an isomeric level (T_1/2=2.6 us) at 2081.5 keV with J=21/2⁺ and a level at 2103 keV, presumably a 17/2^? state. The B(E2; 21/2⁺→17/2⁺) value and the level scheme are compared to shell model predictions.     

Study of the radioactive decay of192Ir

Theβ ^? and electron capture decays of¹⁹²Ir to the levels of¹⁹²Pt and¹⁹²Os respectively have been investigated to verify the existence of some of weak gamma transitions reported earlier. Gamma-gamma directional correlation measurements have been done for 13-cascades. Multipole admixture of 201, 283, 485 keV gamma transitions in¹⁹²Os and 296, 308, 416, 604 keV gamma transitions in¹⁹²Pt have been deduced. A spin value of 4⁺ has been reaffirmed on the basis of almost zero intensity of 1201 keV gamma ray (4⁺→0⁺) and 416→(468)→316 keV cascade directional correlation measurements.     

The decay of105Tc to levels in105Ru

Theβ ^?-decay of 7.6-min¹⁰⁵Tc has been investigated byβ- andγ-ray singles and coincidence measurements. The activities have been produced by thermal-neutron-induced fission of²³⁵U or²³⁹Pu and subsequent chemical separation of the technetium fraction from the fission product mixture. AQ _β-value of 3.2±0.2 MeV has been determined. In a delayed coincidence experiment the lifetime of the first excited state in¹⁰⁵Ru at 20.55 keV has been measured to be 340±15 nsec. A level scheme of¹⁰⁵Ru is proposed and compared with the results of recent nuclear reaction studies like¹⁰⁴Ru(d, p) and¹⁰⁴Ru(n, γ). From beta branching ratios to levels in¹⁰⁵Ru, ground state spin and parity of 5/2⁺ can be suggested for¹⁰⁵Tc in accordance with the trend observed in neutron rich technetium isotopes.     

Investigation of statistically perturbed angular correlations of154Gd and156Gd in different liquid sources

The statistical perturbations of γγ-angular correlations involving the first 2⁺ rotational state of¹⁵⁴Gd and¹⁵⁶Gd have been time differentially investigated. We used liquid sources of 3⁺ ions of Gadolinium in lN perchloric acid, 0.5 N and 1N hydrochloric acid, 1.3N and 2.6 N sulfuric acid. Influences of the various chemical surroundings on the ratio λ₄/λ₂ of the attenuation parameters have been found. A simultaneous measurement of the angular correlation of the 874 keV–123 keV cascade and the 2,098 keV–89 keV cascade of¹⁵⁴Gd and¹⁵⁶Gd, respectively, has been performed in perchloric solution. From the ratio of the attenuation parameters λ₂, obtained by this experiment, we have derived the ratio of the magneticg-factors of the first 2⁺ levels of these isotopes asg ¹⁵⁴/g ¹⁵⁶=1.11±0.08.     

Der Zerfall des125m Xe,des127m Xe und des127g Xe

The decay of^125m Xe produced by the reaction¹²²Te(α, n)^125m Xe using a target enriched in¹²²Te (95.4%) and the decay of^127m Xe produced by the reaction¹²⁷J(d, 2n)^127m Xe have been investigated: ^125m Xe decays with a half-life ofT _1/2=(56±3) sec by ayy- cascade withE _γ1=(140.4 ±0.5) keV andE _γ2=(110.5 ±0.5) keV. The experimental conversion coefficients yield multipolarities ofE3 for the 140.4 keV isomeric transition and predominantlyM1 for the 110.5 keV-transition. ^127m Xe decays with a half-life ofT _1/2=(71±2) sec. The decay also proceeds by aγγ-cascade with an isomeric E3 transition ofE _γ1=(172.5±0.3) keV and a predominantlyM1 transition ofE _γ2=(124.6±0.3) keV. In the decay of^127g Xe an additional branching of the electron capture to a level at (618.1±0.3) keV was observed. The relative probability forK-captureP _K618/P_K375=0.40 ±0.07 yields a total transition energyQ _EC=(664 ±4)keV. A spin of 1/2⁺ was assigned to the ground state.     

Low-spin states in151Gd

The level structure of the 87-neutron nucleus¹⁵¹Gd has been investigated by studying the EC- andβ ⁺-decay of¹⁵¹Tb. Gamma-ray and conversion electron spectra as well as gamma-gamma coincidence spectra were measured by using semiconductor spectrometers and a high-capacity two-parameter recording system. The proposed decay scheme contains several new energy levels in¹⁵¹Gd, among them a 5^?/2 state at 427 keV. To explain the low-energy level structure, a small stable deformation is assumed for¹⁵¹Gd. Using a single-particle-plus-rotor model based on a generalized Woods-Saxon potential, complete mixing of the shells 1h _9/2, 2f _7/2 and separately 1i _13/2 is observed. By these mixings the correct level order and approximately correct excitation energies up to 1 MeV are reproduced.     

States of167Ho from the decay of neutron rich nuclide167Dy

Theβ ^?-decay of ₆₆ ¹⁶⁷ Dy produced through the fast neutron reaction¹⁷⁰Er(n, α)¹⁶⁷Dy has been investigated by using several kinds of detectors and a high-capacity two-parameter recording system. The half-life andβ ^?-decay energy of¹⁶⁷Dy were determined to beT _1/2 = 6.20 ± 0.08min andQ _β-=2.35±0.06, respectively. The observed level scheme of ₆₇ ¹⁶⁷ Ho (completely unknown previously) contains 12 states, among them a 6.0±0.1 μsM2 isomer at 259.3 keV. On the basis of theoretical and systematic considerations combined with multipole determinations, the following Nilsson model assignments are proposed for the lowest states of¹⁶⁷Ho: 0 keV (7?/2 [523]), 259.3 keV (3+/2[411]), 319.8 keV (5/2 3+/2[411]), 392.5 keV (1+/2[411]), 410.0 keV (3/2 1+/2[411]), 569.7 keV (3?/2{7?/2[523], 2⁺}). Theβ-decay proceeds mainly to the proposed gamma-vibrational state at 569.7 keV with an anomalously low logft value 5.4, indicating similarity between the microscopic structures of this state and the famous ¦K ₀?2¦ gamma vibration of¹⁶⁵Ho.     

High-spin states in109Sn and their decay to the ground state

An extended level scheme of¹⁰⁹Sn is presented showing high-spin states up to E_x≈ 8 MeV and spins up toJπ=(41/2+). Their decay to the 5/2+ ground state has been observed identifying a 12.8 keV 7/2⁺ → 5/2⁺ transition. A half-life of T_1/2=7(1) ns has been measured for the 17/2⁺ state atE _x =2114 keV. The experimental data are compared with the predictions of shell-model calculations.