A high-average-power diode-pumped Nd:YVO4 regenerative laser amplifier for picosecond-pulses

A 5.3 W average output power at a pulse repetition-rate of 40 kHz was achieved with a diode-end-pumped Nd:YVO₄ regenerative amplifier. In a continuous-wave operation an optical efficiency of 43% was reached. The output pulse duration is 19 ps, if seeded by a 7-ps-oscillator. A maximum pulse repetition-rate of 80 kHz and a maximum pulse energy of 350 J were generated by the entire laser system. PACS 42.65.Re; 42.79.Kr; 42.79.Hp     

Q-switched Yb 3+ :YVO 4 laser with Raman self-conversion

We report the efficient continuous-wave (CW) and Q-switched laser operation of a diode-pumped Yb:YVO₄ laser. A CW output power of 1 W with a slope efficiency of 59% with respect to absorbed pump power was demonstrated. Passively Q-switched with a Cr⁴⁺:YAG saturable absorber, a Yb:YVO₄ laser with Raman conversion was demonstrated. Q-switched 18.7- J pulses with a pulse duration of 17 ns and a peak power up to 1 kW were obtained at 1018-nm fundamental wavelength and 3.6- J pulses with a pulse duration of 6 ns and a peak power of about 0.6 kW were obtained at 1119.5-nm first-Stokes wavelength.This revised version was published online in March 2005. In the previous version, the published online date was missing     

Bismuth triborate (BiB3O6) optical parametric oscillators

We report the phase matching of parametric frequency conversion in the nonlinear material BiB₃O₆ (BiBO) and on an investigation of optical parametric oscillators (OPOs) of this new crystal. Based on the calculation of collinear type I and type II phase matching within the refractive-index planes, the most favorable directions for phase matching are identified for OPOs pumped by the fundamental or the harmonics of 1064-nm Nd-doped lasers. Based on these results, pulsed 532-nm-pumped ns OPOs are realized. The pump source is either a Q-switched high repetition rate (10 kHz) Nd:YVO₄ laser (with a pulse energy of 24 J) or a low repetition rate (10 Hz), high pulse energy (120 mJ) Nd:YAG laser system. The BiBO OPO pumped by the Nd:YVO₄ laser showed a very low threshold of 0.047 J/cm². At an average pump power of 2.4 W the total OPO output power was 630 mW. By changing the phase-matching angle within the yz plane from 0 to 11.6° the signal wavelength was tuned from 735 nm to 970 nm, while the spectral width changed from 0.2 nm to 1.4 nm. By pumping the OPO with the Nd:YAG laser, the OPO had a threshold of 0.12 J/cm², a steep slope (59%) and a high total efficiency (of up to 48%). Due to divergence broadening the spectral width changes from 8.5 nm at 800 nm to 70 nm near degeneracy. The properties of BiBO determined from the experimental results are compared with those of well-known nonlinear materials such as BBO, LBO and KTP. PACS 42.65.-k; 42.65.Yj; 42.70.-a; 42.70.Mp     

Experiment and modeling of a diode-pumped 1.3 μm Nd:YVO<Subscript>4</Subscript> laser passively Q-switched with PbS-doped glass

A diode-pumped 1.34 m Nd:YVO₄ laser passively Q-switched with PbS quantum dots doped glass is presented. An average output power of 24 mW with a Q-switching efficiency of 13% and a Q-switched pulse width of 15 ns was obtained. A four level spectroscopic model of a PbS quantum dots doped glass saturable absorber is applied to numerically simulate passively Q-switched Nd:YVO₄ laser operation. It has been shown that for the simulation of passive Q-switching of 1.3 m Nd:YVO₄ lasers with PbS doped glasses as the saturable absorbers, it is necessary to take into account intensity dependence of bleaching relaxation times. PACS 42.60.Gd; 42.55.Xi; 42.70.Hj     

High-repetition-rate, intracavity-pumped KTP OPO at 1572 nm

An efficient, eye-safe, high-repetition-rate, intracavity optical parametric oscillator (IOPO) inside an acousto-optically Q-switched Nd:YVO₄ laser end pumped by a 30-W fiber-coupled diode laser was demonstrated. The pumping, acousto-optically Q-switched Nd:YVO₄ laser gives 3-W average output power at 1064-nm wavelength at 40-kHz repetition rate. An additional separating mirror, x-cut KTP crystal and output coupler highly reflective at 1064-nm and partially transparent at 1572-nm wavelengths form a flat–flat IOPO resonator of 35-mm length. We have achieved 3-ns-duration pulses for 20-mm-long KTP and 4-ns-duration pulses for 30-mm-long KTP, respectively. More than 8-kW-peak-power pulses with an average power of 1.5 W at the signal wavelength for 40-kHz repetition rate were demonstrated. Due to the intracavity spatial cleaning effect, a near diffraction limited signal beam was achieved despite a relatively worse beam quality of the pumping beam. Conversion efficiencies of 50% with respect to Q-switched output at 1064-nm wavelength and 11% with respect to diode pump power were achieved. PACS 42.55.Xi; 42.60.Gd; 42.65.Yj     

Efficient amplification of sub-picosecond pulses of a non-CW dye laser

Efficient amplification in a dye laser amplifier is investigated theoretically and experimentally. A five-level rate equation approach is considered including rotational relaxation of the dye molecules. The effects of the pump pulse duration and of the parameters of the input pulse are discussed. The results are compared with experimental data for 0.5 ps pulses of a pulsed dye laser. Conversion efficiencies >10% are achieved for a single pass amplifier using Nd:YAG pump pulses of 2 ns while an effective fluorescence lifetime of 1.7±0.2 ns is determined for the gain medium rhodamine 6G. The triple pass amplifier stage of the laser system achieves an energy conversion of 4% with 40 J output pulses.     

A comprehensive study of Nd:YAG,Nd:YAlO<Subscript>3</Subscript>, Nd:YVO<Subscript>4</Subscript> and Nd:YGdVO<Subscript>4</Subscript> lasers operating at wavelengths of 0.9 and 1.3 μm. Part 2: passively mode locked-operation

This paper reports on the generation of picosecond (ps) laser pulses by self-phase-adjusting additive-pulse-mode-locking (PSA) at wavelengths of 0.9 and 1.3 μm. The main objective of this work was to investigate and compare the characteristic optical properties of ps lasers based on different Nd-doped laser crystals like Nd:YAG, Nd:YAlO₃, Nd:YVO₄ and Nd:GdVO₄. As a result of these investigations a mode-locked Nd:YVO₄ laser for example, generated, ps pulses at 1.3 μm with a duration of 7 ps, a repetition rate of 160 MHz and an average power of 4.7 W. At 0.9 μm pulses with a duration of 1.9 ps were obtained at a repetition rate of 158 MHz and an average power of 2.8 W. PACS  42.70.Hj; 42.65.Re; 42.65.Ky     

Reflective carbon nanotube as the saturable absorber for mode-locked 1064 nm laser

With a reflective single-walled carbon nanotube as the saturable absorber, a laser diode-pumped passively mode-locked Nd:YVO₄ laser at 1064 nm was realized for the first time. The pulse duration of 12 ps was produced with a repetition rate of 83.7 MHz. The peak power and the single pulse energy of the mode-locking laser were 1.28 kW and 15.4 nJ, respectively.     

Temperature-dependent Sellmeier equation in the MIR for the extraordinary refractive index of 5% MgO doped congruent LiNbO<Subscript>3</Subscript>

We present a temperature-dependent Sellmeier equation for the extraordinary refractive index of 5 mol % MgO doped congruent lithium niobate. This equation is adapted for wavelengths in the range of 1.3–5 μm and temperatures between 40 °C and 200 °C. The calculation of the appropriate Sellmeier coefficients is based on the wavelengths of the signal and idler radiation measured for quasi-phase-matched optical parametric generators excited by 10-ns-long, 1064-nm pulses of a Q-switched Nd:YVO₄ laser. PACS 42.65.Ky; 42.70.Mp; 42.65.Yj     

Compact efficient self-frequency Raman conversion in diode-pumped passively Q-switched Nd:GdVO<Subscript>4</Subscript> laser

I report the first demonstration of the generation of efficient sub-nanosecond self-stimulated Raman pulses by a diode-pumped passively Q-switched Nd:GdVO₄/Cr⁴⁺:YAG laser. The conversion efficiency for the average power is 7% from pump diode input to self-Raman output and the slope efficiency is up to 14%. At an incident pump power of 2.0 W, the pulse duration, pulse energy, and peak power for the Stokes wavelength of 1175.6 nm were found to be 750 ps, 6.3 J, and 8.4 kW, respectively, with a pulse-repetition rate of 22 kHz. PACS 42.55.Ye; 42.55.Xi; 42.60.Gd     

High-power source of coherent picosecond light pulses tunable from 0.41 to 12.9 μm

We report a high-power source of coherent picosecond light pulses based on optical parametric generation and amplification in LiB₃O₅ and AgGaS₂ crystals. The spectral range of this continuously tunable source covers the visible, near-infrared and medium-infrared spectrum from 0.41 to 12.9 m. An optical parametric generator and amplifier, consisting of two type-I phase-matched LiB₃O₅ crystals and a diffraction grating, is pumped by the third harmonic of a picosecond Nd:YAG laser and provides spectrally narrow, high-power pulses from 0.41 to 2.4 m. Energy conversion efficiencies up to 16 percent are achieved. The pulse duration is about 14 ps, the bandwidth between 10 and 30 cm^–1. The tuning range is extended to 12.9 m by mixing the infrared output between 1.16 and 2.13 m with the fundamental of the Nd:YAG laser in type-I-phase-matched AgGaS₂ crystals. Up to 25 percent of the pulse energy at 1.064 m is converted into parametric infrared pulses. Bandwidths between 3 and 8 cm^–1 and a pulse duration of approximately 19 ps are measured for these pulses. We also observe a retracing behaviour in the tuning curve of AgGaS₂ not reported before.     

High-energy single longitudinal mode 1 ns all-solid-state 266 nm lasers

A single longitudinal mode (SLM) short pulse high energy all-solid-state ultraviolet laser is demonstrated in this paper. Through the use of a master oscillator power amplifier (MOPA) architecture, we have been able to provide high-energy outputs with the combination of short pulses, good beam quality and SLM typically produced by a 1064 nm Nd:YAG laser. The passively Q-switched SLM Nd:YAG laser in a twisted-mode cavity is operated as the seed source. After the seed is amplified by a double-pass pre-amplifier and a single-pass main-amplifier, the 100 μJ, 1064 nm, ∼1 ns seeding pulse was amplified up to 400 mJ energy in the total pulse train. Using a KTP crystal for second-harmonic generation and a CLBO for fourth-harmonic generation, we successfully obtained a short pulse, high energy ultraviolet laser of 266 nm, with the output energy of 108 mJ, pulse width 1 ns and M²<5. PACS 42.65.Ky; 42.72.Bj; 42.60.Da     

High-power picosecond LiB3O5 optical parametric oscillators tunable in the blue spectral range

The paper reports on an experimental investigation and numerical analysis of noncritically and critically phasematched LiB₃O₅ (LBO) optical parametric oscillators (OPOs) synchronously pumped by the third harmonic of a cw diode-pumped mode-locked Nd:YVO₄ oscillator–amplifier system. The laser system generates 9.0 W of 355-nm mode-locked radiation with a pulse duration of 7.5 ps and a repetition rate of 84 MHz. The LBO OPO, synchronously pumped by the 355-nm pulses, generates a signal wave tunable in the blue spectral range 457–479 nm. With a power of up to 5.0 W at 462 nm and 1.7 W at 1535 nm the conversion efficiency is 74%. The OPO is characterized experimentally by measuring the output power (and its dependence on the pump power, the transmission of the output coupler and the resonator length) and the pulse properties (such as pulse duration and spectral width). Also the beam quality of the resonant and nonresonant waves is investigated. The measured results are compared with the predictions of a numerical analysis for Gaussian laser and OPO beams. In addition to the blue-signal output visible-red 629-nm radiation is generated by sum-frequency mixing of the 1.535-μm infrared idler wave with the residual 1.064-μm laser radiation. A power of 1.25 W of 1.535-μm idler radiation and 5.7 W of 1.064-μm laser light generated a red 629-nm output power of 2.25 W. Received: 2 February 2000 / Revised version: 28 July 2000 / Published online: 22 November 2000     

Laser-diode-pumped Nd:YVO<Subscript>4</Subscript>/Nd:YAG MOPA burst-mode laser

We report a high-repetition-rate, high-peak-power laser diode (LD) pumped burst-mode 1064 nm laser from a Nd:YVO₄/Nd:YAG master oscillator power amplifier. 10–100 kHz pulse burst in a duration up to 2 ms is achieved in LD end-pumped Nd:YVO₄ acousto-optically Q-switched laser. After amplification with LD side-pumped Nd:YAG rod amplifiers, the single pulse energy reaches 73 mJ in 10 kHz pulse burst laser with a peak power of 7.8 MW.     

Tunable mid-infrared,high-energy femtosecond laser source for glyco-protein structure analysis

We have developed a 6–12 μm mid-infrared (MIR) femtosecond laser source for glyco-protein structure analysis. The MIR femtosecond laser pulses are generated by a differential frequency generation (DFG) configuration with a combination of Ti:sapphire based regeneratively amplified femtosecond laser pulses (780 nm, 160 fs, 1 mJ) and a β-BaB₂O₄ (BBO) based optical parametric amplifier (OPA). The MIR pulse energy exceeds 4.5 μJ, where a glyco-protein molecule has resonant absorption lines due to the vibrational–rotational transitions. The pulse width is estimated to be less than 1 ps according to the cross correlation measurement between the two OPA output pulses. Using the MIR femtosecond laser pulses, we demonstrated photo-dissociation of the sialyl Lewis X (sLeX) proton added ion, which is the first time to the best of our knowledge. PACS 42.65.Re; 42.62.-b; 42.60.-b; 42.65.-k; 87.50     

Mid-infrared nonlinear phenomena in polycrystalline semiconductors

We have studied second-harmonic generation by 30 ps and 70 ns 10 m CO₂ laser pulses in nonlinear polycrystalline ZnSe, CdTe and GaAs samples. Second-harmonic generation in these materials can limit the amplification of high-power CO₂-laser pulses in amplifier chains sealed with these polycrystalline IR-transmission materials. On the other hand, we now demonstrate for the first time that these materials are suited as nonliner elements for autocorrelation measurements on short infrared laser pulses. For such pulse-width measurements polycrystalline materials have an advantage over single crystals, e.g. GaAs, because they are insensitive to misalignement. Furthermore, these polycrystalline optical elements are easier and cheaper to manufacture than single crystal devices. With such polycrystalline materials we were able to realize reliable autocorrelation measurements of 30–300 ps 10 m optical-free-induction-decay (OFID) laser pulses.     

Tunable,narrow-band picosecond radiation in the mid-infrared by difference frequency mixing in GaSe and CdSe

We report on the generation of tunable, narrow-band picosecond laser pulses in the mid-IR at 1 kHz repetition rate. An optical parametric oscillator (OPO) seeded optical parametric amplifier (OPA) delivers signal and idler pulses with energies of several hundred microjoule tunable between 1.56 and 3.24 m. Difference frequency mixing of the OPA signal and idler waves permits the generation of mid-IR radiation between 3 and 24 m. The laser system therefore permits full coverage of the wavelength range between 1.6 and 24 m. Conversion efficiencies greater than 50% and pulse energies up to 40 J are obtained with GaSe. PACS 42.65.Re; 42.65.Yj; 42.72.Ai     

Diode-pumped cw and Q-switched Nd:GdVO4 laser operating at 1.34 μm

A diode-pumped 1.34 m Nd:GdVO₄ laser operating in cw and active Q-switching modes has been demonstrated. 4.15 W of cw output power was obtained at the highest attainable pump power of 12.3 W, resulting in an optical conversion efficiency of 33.7%, the slope efficiency was determined to be 37.6%. In Q-switching operation, a maximum average output power of 2.7 W was generated at pulse repetition frequency (PRF) of 50 kHz, with an optical conversion efficiency of 22% and a slope efficiency of 29.2%. The laser pulses with shortest duration, highest energy and peak power were achieved at PRF of 10 kHz, the parameters being 15 ns, 160 J, and 10.7 kW, respectively. By intracavity frequency-doubling with a type II phased-matched KTP crystal, 0.62 W average power at 0.67 m was produced at a PRF of 15 kHz, the resulting pulse energy, peak power, and pulse width being 41.3 J, 2.2 kW, and 19 ns, respectively. A group of analytical formulae, based on rate equations, are presented to evaluate the operational parameters of an actively Q-switched laser. Calculated results were found to be in close consistency with the experimental data.     

Optical parametric chirped pulse amplification based on photonic crystal fibre

A compact two-stage optical parametric chirped pulse amplifier based on photonic crystal fibre is demonstrated.A 1064-nm soliton pulse is obtained in a home-made photonic crystal fibre (PCF) with femtosecond pulse pumping and then amplified to 2 mJ in an Nd:YAG regenerative amplifier.After the amplified pulses pass through the LBO crystal,the 532-nm double-frequency light with an energy of 0.8 mJ and a duration of over 100 ps at 10-Hz repetition rate is generated as a pump source in the following two-stage optical parametric amplification (OPA).The 850-nm chirped signal light gain from the stretcher is 1.5×10 4 in the first-stage OPA while it is 120 in the second-stage OPA.The total signal gain of optical parametric chirped pulse amplification (OPCPA) can reach 1.8×10 6.     

Optical parametric oscillators for high pulse energy and high average power operation based on large aperture periodically poled KTP and RTA

We report on optical parametric oscillators (OPOs) based on large aperture periodically poled KTiOPO₄ (PPKTP) and RbTiOAsO₄ (PPRTA) pumped with high pulse energy and high average power Q-switched solid-state lasers. The OPOs were pumped with 1064-nm pulses of a diode-pumped Nd:YVO₄ laser at 20 kHz repetition rate. The emitted signal wavelengths were 1.72 μm and 1.58 μm and the idler wavelengths were 2.79 μm and 3.26 μm, respectively. Pumping the PPKTP OPO with 7.2 W and the PPRTA OPO with 8 W average power, 2 W and 1.3 W total OPO output powers were generated. Two-dimensional measurements of the total OPO output power, the signal wavelength and the signal bandwidth in dependence on the crystal location indicated a good uniformity of the quasiphasematching structure over the entire 3-mm-thick crystals. This allowed pumping with larger pump beams and therefore with pulse energies of tens of millijoules. Pumping with different flash-lamp-pumped lasers, good OPO performance and high output pulse energies could be achieved for all pump lasers. Maximum input pulse energies of 56 mJ gave output pulse energies of as much as 18 mJ. The temperature tuning behaviors of both OPOs were measured, showing excellent agreement with calculated temperature tuning curves. New equations for temperature dispersion in RTA are presented. These results show that large-aperture PPKTP and PPRTA crystals are well suited for tunable nanosecond OPO operation with multi-watt average pump power and several tens of millijoules pump pulse energies. Received: 7 September 2001 / Published online: 7 November 2001