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A novel class of nonlinear optical processes is described in which radiation at the nth harmonic is generated through the use of a (2n+1)-order nonlinearity. Utilizing an odd-order nonlinearity, this process allows for the generation and amplification of both odd- and even-order harmonics in isotropic materials. Additionally, this process can always be phase matched in normal-dispersion materials without the use of birefringence. Experimental results are presented in which conical third-harmonic emission is generated from a sapphire sample. 相似文献
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A.G.M. Maaswinkel 《Optics Communications》1980,35(2):236-238
Second harmonic (SH) generation in a laser produced plasma (NdYAG laser with wavelength 1.06 μm, pulse duration 30 ps, intensity 1013Wcm-2) was investigated experimentally as a function of polarization and angle of incidence of the laser beam. The results are in agreement with theoretical predictions for SH generation in the presence of linear mode conversion in the plasma. 相似文献
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James H. Churnside 《Optics Communications》1984,51(3):207-212
The second harmonic generation process is considered using partially coherent light formed by the superposition of a coherent field and a chaotic field. The conversion efficiency is derived. Expressions are also presented for the variance and for the probability density function of the second harmonic intensity and of the transmitted intensity at the fundamental wavelength. 相似文献
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The wavevector distribution excited by light scattering in opaque materials is calculated and compared to recently observed asymmetrical Brillouin lineshapes. 相似文献
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《中国物理 B》2015,(3)
The intensity of third harmonic emission in air filamentation disturbed by copper fibers and alcohol droplets has been investigated experimentally. Enhancement of the third harmonic emission up to more than one order of magnitude has been observed. The physical mechanism of third harmonic enhancement is attributed to suppression of the destructive interference by comparison of the experimental results and it is closely related to the type, size, and relative position of the obstacles. 相似文献
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提出应用级联倍频方法提高倍频系统输出稳定性,并就该方法的有效性进行了理论分析和模拟计算.分析和计算结果不但证明级联倍频方法能实现倍频系统稳定输出,而且还表明可以通过仔细调节第一块倍频晶体中波矢方向 k 与光轴间夹角、两块倍频晶体间的间隔,能调节改变实现倍频系统最稳输出时所需第二块晶体的理论计算长度,使之与第二块倍频晶体的实际加工长度一致,最终实现系统稳定倍频输出.级联倍频方法在实现高输出稳定性的同时能实现高的倍频转换效率,对应用于光参量啁啾脉冲放大系统的高稳定抽运源系统的设计建造具有重要参考意义.
关键词:
级联倍频
稳定倍频输出
光参量啁啾脉冲放大 相似文献
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Spectra of the second and third optical harmonics generated in epitaxial films of magnetic garnets were studied in the ranges 1.7–3.2 and 2.4–4.2 eV, respectively. A large magnetic contrast was revealed in second-optical-harmonic spectra, which reaches 100% at certain photon energies. By contrast, the symmetry-allowed magnetic contribution to spectra of the third optical harmonic was not found. While linear absorption in ferrite-garnet films grows by two orders of magnitude above the fundamental absorption edge at ~3.2 eV, the intensity of nonlinear spectra did not reveal any noticeable increase over this spectral range. 相似文献
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R. A. Ganeev 《Optics and Spectroscopy》2017,123(1):117-138
A few recently introduced approaches of the high-order harmonic generation in laser-produced plasmas are reviewed. We show how the tuning of odd and even high-order harmonics of ultrashort pulses along the strong resonance of laser-produced indium plasma using optical parametric amplifier of white-light continuum radiation (1250?1400 nm) allows observation of different harmonics enhanced in the vicinity of the transition of In II ions possessing high oscillator strength. We discuss various peculiarities and discuss the theoretical model of the phenomenon of tunable harmonics enhancement in the region of 62 nm using indium plasma. With the theoretical analysis, we present the approach allowing reproduce the experimental observations and characterize the dynamics of the resonant harmonic emissions. We also discuss the resonance enhancement of harmonics using mid-infrared radiation in the tin, chromium, and antimony plasmas and show the calculations of this process. 相似文献
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R.A. Ganeev P.A. Naik H. Singhal J.A. Chakera M. Kumar U. Chakravarty P.D. Gupta 《Optics Communications》2012,285(12):2934-2941
A systematic study of the high-order harmonic generation (HHG) of laser radiation in various carbon-containing plasma plumes (CCPPs) is presented. The materials studied are: graphite, boron carbide, C60, polytetrafluoroethylene, polyethylene, carbon nanotubes, and soot. These studies show that CCPPs present the best plasma media for efficient lower order (from 9th to 19th) harmonic generation, while the harmonic cutoff restricted to the 29th order. The advantages of CCPPs for the harmonic generation are confirmed by comparison of the HHG conversion efficiency with that in Ag and In plasma plumes, where the highest conversion efficiency was reported. Use of two-color pump scheme allows further enhancement of harmonic yield from the CCPPs. 相似文献
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A novel method for generating quadruple-frequency millimeter-wave (MMW) by using an actively mode-locked fiber ring laser is proposed and demonstrated. In this approach, the optical Mach-Zehnder intensity modulator (MZM) is biased to suppress the odd-order optical sidebands, the fiber laser operates in the second-order rational harmonic mode, and a fiber Bragg grating (FBG) notch filter is used to block the optical carrier. When the MZM is driven by a fixed radio-frequency (RF) source of 10 GHz, a stable MMW signal of 40 GHz with the phase noise better than -76 dBc/Hz at 1-kHz offset is generated. 相似文献
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Accurate molecular imaging via high-order harmonic generation relies on comparing harmonic emission from a laser-irradiated molecule and an adequate reference system. However, an ideal reference atom with the same ionization properties as the molecule is not always available. We show that for suitably designed, very short laser pulses, a one-to-one mapping from high-order harmonic frequencies to electron momenta in above-threshold ionization exists. Comparing molecular and atomic momentum distributions then provides the electron recollision amplitude in the molecule for enhanced molecular imaging. The method retrieves the molecular recombination transition moments highly accurately, even with suboptimal reference atoms. 相似文献
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The high-order harmonic generation using ellipticity-modulated laser field is investigated experimentally and theoretically. The laser field with time-varying ellipticity is obtained using two quarter wave plates. The harmonic spectral intensity peaks appear periodic for the localization induced by the ellipticity modulation of the laser pulse. We calculate the single-atom response to the driving laser field using the Lewenstein model and compare the calculated and measured harmonic spectra generated with ellipticity-modulated driving laser pulses. The theoretical simulation and the experiment results agree well with each other. 相似文献
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Surface second harmonic generation of chiral molecules using three-coupled-oscillator model
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Based on the three-coupled-oscillator molecular model we proposed, the
relation between the second-order susceptibilities of a chiral film and the
molecular hyperpolarizabilities is given. The effect of microscopic
parameters on the second-order susceptibilities is simulated numerically and
the difference between the efficiencies of s-polarized second-harmonic
fields induced by the left- and the right-handed circularly-polarized
fundamental beams is discussed. The theoretical basis for studying
second-order nonlinear optical properties of the chiral molecular media with
a tripod-like structure is provided in this paper. 相似文献
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数值研究了啁啾激光驱动H_2~+辐射谐波的特点.结果表明,(1)在低强度和高强度激光驱动下,谐波光谱分别呈现红移和蓝移现象.引入正负向啁啾参数后,谐波频移和谐波辐射强度都可以得到调控.(2)谐波光谱在高强度激光驱动下呈现非奇次谐波.理论分析表明,非奇次谐波产生的原因是双H核频移不一致所导致的不对称相消干涉引起的. 相似文献