Observation of magnetoplasma type surface polaritons on n-InSb

Surface polariton dispersion curves have been obtained for an n-InSb—air interface in a magnetic field using the ATR method and are found to be in qualitative agreement with theory. In particular the curves show the predicted non-reciprocal nature of the surface polariton propagation, and the appearance of virtual excitation type branches of the dispersion curves. On the basis of data obtained in zero magnetic field on etched surfaces, the quantitative differences between experimental and theoretical dispersion curves are attributed to surface damage.     

Quantum theory of the polariton of the bounded semiconductor

The quantization of the polariton field is carried out for the semiconductor bounded by the surface. The orthonormalized set of the normal mode of the vacuum-semiconductor system is explicitly given for the case of the excitonic polarization field with the standard form of the spatial dispersion and the additional boundary condition of the elastic type. The scheme is employed to interpret the several experiments: optical reflectance and transmission, resonant Raman and Brillouin scattering, and the induced absorption of the polariton. Particularly, a recent experiment on CuCl which shows the existence of correlation among the polaritons and reflected light is discussed in view of the quantum picture.     

Theory of nonlinear excitation of surface polaritons in lossy media

The purpose of this paper is to study the nonlinear excitation of surface polaritons taking fully into account the damping of the active medium and the finite cross-section of the nonlinear polarization on the interface. This problem is solved using the guided wave calculation techniques where the EM field at the surface polariton frequency is expanded over a complete set of normal modes of the unperturbed interface. Using a “table method” we find that this set includes one guided mode, which is the surface polariton mode, and two classes of radiation modes. The expressions of all these modes are derived and interpreted physically. We then get the expression of the EM field excited at the surface polariton frequency inside and outside the pumped region and show that, in the general case, it is a mixture of all these normal modes. The end of the paper is mainly devoted to the study of the surface term occurring in the expression of the EM field at the surface polariton frequency: we point out the existence of a resonance phenomenon with two kinds of surface polariton modes: the “spatial” one and the “temporal” one. The corresponding dispersion curves, or resonance curves, are given and it is explained how each of them can be obtained experimentally.     

Suppression of radiative losses of surface polaritons on nanostructured thin metal films

The strong electromagnetic coupling between surface plasmon polariton modes on opposite interfaces of a finite thickness periodically nanostructured metal film has been studied. Surface polariton dispersion and associated electromagnetic field distributions have been analyzed. It was shown that at a frequency that corresponds to the crossing of film Bloch modes of different symmetries, the radiative losses of surface polaritons that are related to the polaritons' coupling to light during propagation on the structured surface are suppressed.     

Quantum Theory of Surface Polaritons on a Rough Surface

In this paper, we present the quantum field theory of the surface phonon-polaritolis on a rough polar crystal surface. The dispersion relations of the surface phonon-polaritons and the dispersion relations of polariton leaking modes owing to the interaction between bulk TO mode with the surface effect and photons are derived. We also study the k-dependence of the electric field strength in each polariton branch. The numerical calculations for the dispersion relations and the k-dependence of the electric field strength are carried out for a stepped Gap surface. The results show that the surface roughness depressed the frequency of the surface phonon-polariton below its values in the absence of the surface roughness. For the frequencies of the polariton leaking modes, the photon-like one is enhanced by the surface roughness and the phonon-like one b depressed. Our evaluations also illustrate that the surface roughness introduces a strong dependence on the k-dependence of the electric field strength in each polariton branch.     

Exciton-polaritons in halfspace

A rigorous method is presented describing the coupling between an exciton polariton in a halfspace semiconductor and the external driving field. The method is based on density matrix theory. It allows to consider realistic electron-hole interactions, spatial dispersion and extrinsic surface potentials. Without invoking additional boundary conditions or an artificial subdivision of the semiconductor it is shown that the influence of the surface can be isolated from the bulk behaviour. This is accomplished by a symmetric continuation of the restricted configuration space to bulk geometry inspired by the image source method in electrostatics. As a demonstration the solution is worked out for a simplified polariton model. The results are compared with other theories and with experimental reflection spectra.     

Research progress of femtosecond surface plasmon polariton

As the combination of surface plasmon polariton and femtosecond laser pulse,femtosecond surface plasmon polariton has both nanoscale spatial resolution and femtosecond temporal resolution,and thus provides promising methods for light field manipulation and light-matter interaction in extreme small spatiotemporal scales.Nowadays,the research on femtosecond surface plasmon polariton is mainly concentrated on two aspects:one is investigation and characterization of excitation,propagation,and dispersion properties of femtosecond surface plasmon polariton in different structures or materials;the other one is developing new applications based on its unique properties in the fields of nonlinear enhancement,pulse shaping,spatiotemporal super-resolved imaging,and others.Here,we introduce the research progress of properties and applications of femtosecond surface plasmon polariton,and prospect its future research trends.With the further development of femtosecond surface plasmon polariton research,it will have a profound impact on nano-optoelectronics,molecular dynamics,biomedicine and other fields.     

The Investigation of Plasmon-Longitudinal Optical Phonon Coupling and Surface Polariton Modes in Donor Doped GaAs-Al0.33Ga0.67As Multi Quantum Wells

Infrared Fourier transform spectroscopy has been used to investigate phonon, plasmon, surface polariton and plasma-longitudinal optical phonon coupling in highly donor doped multi quantum wells (GaAs/Al_0.33Ga_0.67As) and direct band gap n- type Al_XGa_1-XAs thin layer on GaAs substrate. Using different samples with different concentration of free carriers. The dispersion equation of coupling modes have been calculated by using the condition which the dielectric functions of samples are zero for longitudinal coupled modes and experimental papameters which have been obtained from the best fit p-polarized oblique incidence far infrared reflection spectra. In MQW samples, the free carriers confined to the well and carriers are quasi two dimensional. So, plasmon- LO phonon coupling occur in the well (GaAs). In n- type Al_XGa_1-XAs thin layer, the coupled modes consist of three branches of the high, intermediate and low frequency modes. Their frequencies depend on both concentration and alloy composition. To analyses the surface polariton modes we carry out attenuated total reflection (ATR) measurements. In order to support our assignment the magnetic field profiles and surface polariton dispersion curves have been calculated.     

Back-propagating surface polaritons of a one-dimensional photonic crystal containing single negative metamaterials

The existence of the surface polaritons at the interface separating a semi-infinite uniform left-handed metamaterial and a one-dimensional photonic crystal composed of alternating layers of two kinds of single-negative materials is theoretically investigated. The dispersion characteristics of the surface polaritons are analyzed and demonstrated that in the presence of metamaterial, the surface polaritons are sensitive to light polarization, so that there exist only backward TM-polarized (or TE-polarized) kind of the surface polaritons depending on the ratio of the thicknesses of the two periodic stacking layers. The existence regions of the surface polariton modes are determined for both TM-polarized and TE-polarized surface polariton modes.     

Dispersion relation of LT mixed mode polaritons

Simple equations are presented for polariton dispersion relations in anisotropic medium for an arbitrary direction of wave vector, where LT (longitudinal-transverse) mixed modes occur in general. The use of the polarizability tensor defined for pure external (not for the total) field is essentially important to obtain the simple result. The relation between all the tensor components of the polarizability and dielectric function is also explicitly given. The result can be used for any elementary excitations relevant to dielectric function. In the case of multi-component excitons of LT mixed mode character, the dispersion equation is rewritten in a matrix form, which is useful to obtain the allowed values of polariton wave vector for a given frequency.     

太赫兹表面极化激元

作为束缚于表面或界面的电磁波与极性元激发的耦合模量子,表面极化激元是克服衍射极限的核心物理.在紫外、可见以及近红外波段,表面等离子极化激元展现出了亚波长特性,具有高分辨成像等应用,并发展成为"表面等离子极化激元亚波长光学"学科;在中红外波段,表面声子极化激元发挥着同样的作用.太赫兹波段曾是人类认识的空白区域,近三十年来得以高速发展,其战略意义重大.具有克服衍射极限能力的太赫兹表面极化激元同样是小型化与集成化太赫兹器件,以及太赫兹超高分辨成像的重要物理基础.近几年来,对以石墨烯为代表的二维材料的研究突飞猛进,诞生了"石墨烯表面等离子极化激元亚波长光学"这门学科,并贡献于太赫兹领域.本文对可在太赫兹波段工作的人工超构材料、掺杂半导体、二维电子气、二维材料、拓扑绝缘体等结构材料的表面极化激元进行了较为全面的总结与介绍,为研制克服衍射极限的太赫兹集成光子学器件提供可资借鉴的物理基础.     

Groove depth dependence of surface plasmon luminescence from bare silver gratings: Experimental study

We have observed luminescence of surface plasmon polariton from bare silver gratings of variable groove depths. The intensity of the surface plasmon polariton luminescence has been measured versus the groove depth of the gratings: we report the existence of an optimum groove depth for which the luminescence peak intensity is maximum.     

Enhanced backscattering in a magnetic field

By means of numerical simulations the authors study the scattering of a beam of p-polarized light from a small RMS slope one-dimensional random surface on a semi-infinite metal or n-type semiconductor to which a constant magnetic field is applied. The surface is defined by the equation x₃=ξ(x₁), where the surface profile function ξ(x₁) is a stationary stochastic Gaussian process. The plane of incidence is the x₁x₃ plane, and the magnetic field is directed along the x₂-axis. In the presence of the magnetic field the dispersion curve for the surface polaritons supported by the surface in the absence of the random roughness becomes non-reciprocal, i.e. the wavenumber k₊(ω) for a surface polariton of frequency ω propagating in the +x₁-direction is unequal to the (magnitude of the) wavenumber k_-(ω) for a surface polariton of the same frequency propagating in the -x₁-direction. As a consequence of this they find that the peak in the angular distribution of the intensity of the incoherent component of the scattered light that is observed in the retroreflection direction in the absence of the magnetic field—enhanced backscattering—is shifted in the direction of larger scattering angles with increasing magnetic field strength. At the same time the width of the peak increases and its amplitude decreases. When the frequency of the incident light is high enough that the dispersion curve for surface polaritons on the planar surface becomes completely non-reciprocal, i.e. the surface polariton propagates only in the +x₁-direction but not in the -x₁-direction, the enhanced backscattering is completely suppressed. These results are interpreted as being due to the breakdown of the coherency between a given light/surface polariton path that contributes to backscattering and its time-reversed partner, caused by the removal of time-reversal symmetry from the scattering system by the application of the external magnetic field. They provide strong evidence for the fundamenlal role played by surface polaritons in the enhanced backscattering of light from small RMS slope random surfaces.     

Virtual excitation type surface polaritons on anisotropic media

We discuss the nature of a new type of surface polariton which occurs on anisotropic media, involving a photon coupled to a surface virtual excitation. Dispersion curves are calculated for α-quartz, where both real excitation type and virtual excitation type surface polaritons are predicted. The dispersion curves for virtual excitation surface polaritons are found to remain at small wavevector, and the endpoints of the dispersion curves terminate on the bulk polariton dispersion curves in the two media. The virtual excitation surface polaritons which occur on gyromagnetic and gyrodielectric media are also noted.     

Optical properties of microcavity polaritons

This work contains a theoretical analysis of the optical properties of semiconductor quantum wells embedded in planar Fabry-Perot microcavities. In particular, the properties of the system in correspondence to the excitonic transition are studied by means of the polariton formalism. The polariton states in microcavities are derived and the polar-iton dispersion is presented. Particular emphasis is put on the existence of two well distinct regimes depending on the exciton and cavity parameters: strong coupling and weak coupling regime. The main experimental results are reviewed and compared with the prediction of the theory. After the polariton states have been characterized, the optical response of the system is discussed, with particular attention to the photoluminescence measurements. The polariton formation and relaxation through phonon scattering and the effect of the exciton inhomogeneous broadening are considered and, finally, a phe-nomenological model for the polariton photoluminescence spectra is presented.     

Sapphire surface polariton splitting due to resonance with magnesium oxide film phonon

Surface polariton spectra of magnesium oxide films (of thickness ranging from 10 to 300 nm) prepared by chemical vapor deposition technique on sapphire substrates have been studied. The splitting of the dispersion curve of the sapphire surface polariton appears near 700 cm⁻¹ due to the resonance interaction of the sapphire substrate surface polariton with the film optical phonon. This splitting is proportional to the square root of the film thickness. Optical constants of ultrathin magnesium oxide films have been obtained from surface polariton spectra measurements. For the thinnest film (10 nm) they appear to be close to the bulk crystal values.     

Quantum Theory of Surface Polaritons in Semi-Infinite Dielectric Systems

The interaction system of a semi-infinite diatomic dielectric and the electromagnetic field propagating parallelly to the surface is studied. The long-wave optical phonon modes of the semi-infinite dielectric are calculated including the electronic polarizability by a quantum-mechanical theory. Retardation effects are neglected. A quantum field theory method of surface polaritons is developed to calculate the operator describing the interaction between a photon and the phonon polarization fields of the semi-infinite crystal, with explicit inclusion of surface effects. The dispersion relations of the surface phonon-polaritons are derived and discussed. The results are in good agreement with those obtained by the conventional, macroscopic dielectric theory of surface polaritons and experimental ATR (attenuated total reflection) spectra. The dispersion cuwes of polariton leaking modes caused by the interaction between bulk TO mode with surface effect and photons are presented in a graphical form. The k_||-dependence of the electric field strength in each polariton branch is calculated and presented also in a graphical form. We also research the spatial dependence of the field strength in each polariton branch. It is found that these properties are influenced and modulated by the surface phonons because of the interaction between photons and the surface phonon modes of the semi-infinite dielectric system. Hence the divergent nature (diffraction effect) of light propagating along the fib& and waveguides is restrained. We present a method how to use the boundary conditions in the quantum theory, which will be discussed in detail.     

Dispersion relation for surface plasmon polaritons in metal/nonlinear-dielectric/metal slot waveguides

We present the first (to our knowledge) exact dispersion relation for the transverse-magnetic surface plasmon polariton (SPP) modes of a plasmonic slot waveguide, which is formed by a nonlinear Kerr medium sandwiched between two metallic slabs. The obtained relation is then simplified to the case of small field intensities, while retaining nonlinear terms, to derive approximate dispersion equations for the symmetric and antisymmetric SPP modes.     

Ondes solitaires polaritoniques dans un ferroaimant quasi-unidimensionnel

Spin dynamics in an easy plane magnetic chain has been studied in terms of polaritons and solitons, when the coupling between magnons and their induced dipolar electromagnetic field is included. For a moderate external magnetic field in the easy plane, non-topoligical, classical ø⁴ solitons can describe the dynamics of spins dressed with the electromagnetic field. The solitary wave thus produced propagates at phase velocities bounded by the two limiting phase velocities of the polariton dispersion relations.     

Dispersion polaritons on metallized surfaces of optically uniaxial crystals

We have constructed a theory of dispersion polaritons (localized electromagnetic waves) on arbitrarily oriented metallized surfaces of optically uniaxial crystals. The domain of existence of polaritons is defined by the following inequalities for permittivities ε_o and ε_e of the crystal and the angle θ between the optical axis and the surface: ?ε_etan²θ < ε_o < 0. Thus, polaritons exist only in the range of wave frequencies ω ensuring negative values of ε_o(ω) for ε_e > 0. The frequency boundaries of this region are specified for the case when the ε_o(ω) dependence corresponds to the model of a single polar excitation. The azimuthal orientation φ of the optical axis projection onto the surface does not appear in the criterion for polariton existence, but affects (together with angle θ) its main dispersion characteristics, such as the refractive index and partial wave localization parameters. This effect is analytically described in detail. Anomalies in the behavior of polariton parameters are studied in the vicinity of the boundaries of the domain of its existence, where the wave fields are especially sensitive to variations in the angles θ and φ. It is shown that a polariton in the plane of propagation (sagittal plane) passing through the optical axis is transformed into a one-partial bulk wave satisfying the boundary conditions. Accordingly, the wave branch under investigation for close orientations (when the optical axis forms a small angle with the sagittal plane) describes deeply penetrating (quasi-bulk) polaritons.