Interaction of 11 MeV neutrons with Y

Differential cross section for scattering of 11 MeV neutrons by ⁸⁹Y were measured using the Ohio University beam swinger time-of-flight facility. Measurements were taken in the angular range between 15° and 145°. Empirical optical model parameters have been obtained from the measured elastic scattering data. Deformation parameters were obtained for low-lying excited states using these optical-model parameters in a DWBA collective formalism. A comparison with deformation parameters in neighboring even-even nuclei ⁸⁸Sr and ⁹⁰Zr is presented. The weak-coupling model is used to describe neutron scattering to low-lying states in ⁸⁹Y.     

Nuclear reactions between oxygen isotopes

Elastic and inelastic cross sections have been measured for the system ¹⁶O + ¹⁷O at c.m. energies from 12.5 to 15.5 MeV, and for ¹⁶O + ¹⁸O at c.m. energies from 12 to 20 MeV, at angles between 60° and 125°. Position-sensitive detectors were employed, using the kinematic coincidence technique. The data have been analyzed with particular attention to the contributions of multiple-exchange processes.     

Quadrupole interactions in pionic and muonic tantalum and rhenium

The hyperfine splitting of pionic and muonic X-rays in natural Re has been studied using the known ratio (accurate to 1.6 parts in 10⁵) of the quadrupole moments of the two naturally occurring ¹⁸⁵Re and ¹⁸⁷Re isotopes. From the hyperfine splitting of the ⁵g → 4f and 4f → 3d pionic X-rays the effective quadrupole hyperfine constants were determined to be ¹⁸⁷A₂^eff(4f) = 1.163 ± 0.010 keV and ¹⁸⁷A₂^eff(3d) = 5.39 ± 0.63 keV, giving strong interaction quadrupole shifts ₂(4f) = 46 ± 10 eV and ₂(3d) = 1.3 ± 0.6 keV. The strong interaction monopole shifts ₀ and widths Γ₀ of the 5g, 4f and 3d levels have also been measured. For the two higher orbits, standard optical-potential calculations fit the measured shifts and widths quite well. The observed deeper-lying 3d state, however, has shifts and widths that differ by a factor of 2 or more from the predictions. From the measured quadrupole hyperfine constants of the 4f level we calculate the spectroscopic quadrupole moments to be ¹⁸⁷Q^μ(gm) = 2.09 ± 0.04 b, ¹⁸⁷Q^π = 2.07 ± 0.02 b, ¹⁸⁵Q^μ = 2.21 ± 0.04 b, and ¹⁸⁵Q^π = 2.1 addition, muonic X-rays from ¹⁸¹Ta were observed; using the same methods for determining the quadrupole moment as above, a value of ¹⁸¹Q^μ = 3.28 ± 0.06 b was obtained, in good agreement with earlier published data.     

Nucleon-nucleon final-state interactions in the reactions He(p, d)2p, He(p, t)2p and He(p, He)pn

The energy spectra of deuterons, tritons and ³He particles from the reactions ³He(p, d)2p, ⁴He(p, t)2p and ⁴He(p, ³He)pn have been measured at angles between 6° and 60° lab. The ³He(p, d)2p reaction was studied at both 30.5 and 49.5 MeV incident proton energies, while the other two reactions were studied at 49.5 MeV only. The energy spectra are compared with calculations based on the Watson-Migdal model of final-state interactions.     

Measurement of some gamma-ray energies suitable for routine energy calibration

The energies of several gamma-ray transitions have been measured using a Ge(Li) spectrometer. The isotopes and the corresponding transition energy measurements in keV are ¹⁴¹Ce(145.44±0.05), ¹³⁹Ce(165.85±0.05), ⁵¹Cr(320.07±0.05), ⁷Be(477.57±0.05), ⁸⁵Sr(513.95±0.07), ⁹⁵Nb(765.83±0.07), ⁵⁴Mn(834.84±0.07), ⁴⁶Sc±889.25±0.07, 1120.50±0.07), ⁸⁸Y(898.01±0.07, 1836.08±0.07), ⁹²Nb(934.51±0.07), ²⁰⁷Bi(1063.63±0.07), ⁶⁵Zn(1115.51±0.07) and ²²Na(1274.52±0.07).     

π Meson interaction on He at 120, 145 and 165 MeV

The total cross sections and the differential cross sections of π⁺-⁴He elastic and inelastic reactions at E_π=120, 145 and 165 MeV have been measured using a 38 cm diffusion cloud chamber in a magnetic field exposed to the Frascati Laboratories' pion beam. Total π⁺ track lengths of (2141 ± 10) × 10³ cm, (3435 ± 10) × 10³ cm and (2413 ± 10) × 10³ cm were measured at the three considered energies, respectively. The elastic cross-section data are in good agreement with the results of the Dubna-Torino collaboration. The total inelastic cross sections have been obtained taking into account the contributions from all the inelastic channels. The analysis of the various inelastic processes has allowed us to distinguish five main reaction mechanisms, which compare reasonably with the existing data and with the models for pion-light-nuclei interactions.     

Intermediate energy proton scattering and nuclear transition densities in nickel isotopes

Using the high-resolution spectrometer SPES-I, the angular distribution of 1.047 GeV protons scattered from ⁵⁸Ni, ⁶⁰Ni, ⁶²Ni, ⁶⁴Ni have been measured in the angular range 4–18°, up to 4.8 MeV excitation energy. The data are analyzed within the framework of Glauber multiple scattering theory using a spin-dependent NN scattering amplitude. The parameters of the neutron density distributions have been determined by a χ² analysis of elastic scattering. The inelastic data corresponding to the first 2⁺ and 3⁻ states are analyzed with the collective model and an attempt has been made to extract information about the corresponding neutron transition densities.     

Polarisation circulaire du rayonnement gamma de Sb, Cs et Ag

The βγ circular polarization correlation of the 3⁻(β⁻ 621 keV)3⁻(γ 1692)2⁺ cascade in ¹²⁴Sb, the 4⁺(β⁻ 662)4⁺ (γ 796)2⁺ (γ 605)0⁺ in ^13Z4Cs and the 6⁺(β⁻529)6⁺ (γ 937)4⁺ (γ 885)2⁺ (γ 658)0⁺ in ^110mAg have been studied by using a Compton effect polarimeter. The measured asymmetry parameters are 0.172±0.004, −0.0702 ±0.0024 and 0.0549±0.0013 respectively.     

Polarization of protons from the Be(d, p)Be reaction

The polarization of protons from the ⁹Be(d, p)¹⁰Be reaction has been measured for deuteron energies between 1 and 6 MeV. Angular distributions of the polarization for the ground state proton group (Q=4.59 MeV) have been measured for laboratory angles 10° and 135° at 2.5, 4.0 and 5.5 MeV. The polarization at a laboratory angle of 30° was measured in 0.2 MeV steps between 1 and 6 MeV. In addition the polarization of protons leaving ¹⁰Be in its first excited state (Q=1.22 MeV) was measured between 10° and 90° for a deuteron bombarding energy of 5.5 MeV. Measurements were made by conventional double-scattering techniques using elastic scattering from helium at 45° as the analyser. The results show a strong energy dependence contrary to what one might expect on the basis of the lack of structure in the cross section. The maximum polarization observed at each energy is about 0.35.     

Defect versus nanocrystal luminescence emitted from room temperature and hot-implanted SiO2 layers

Silicon nanocrystals have been synthesized in SiO₂ matrix using Si ion implantation. Si ions were implanted into 300-nm-thick SiO₂ films grown on crystalline Si at energies of 30–55 keV, and with doses of 5×10¹⁵, 3×10¹⁶, and 1×10¹⁷ cm⁻². Implanted samples were subsequently annealed in an N₂ ambient at 500–1100°C during various periods. Photoluminescence spectra for the sample implanted with 1×10¹⁷ cm⁻² at 55 keV show that red luminescence (750 nm) related to Si-nanocrystals clearly increases with annealing temperature and time in intensity, and that weak orange luminescence (600 nm) is observed after annealing at low temperatures of 500°C and 800°C. The luminescence around 600 nm becomes very intense when a thin SiO₂ sample is implanted at a substrate temperature of 400°C with an energy of 30 keV and a low dose of 5×10¹⁵ cm⁻². It vanishes after annealing at 800°C for 30 min. We conclude that this luminescence observed around 600 nm is caused by some radiative defects formed in Si-implanted SiO₂.     

Pionic K X-rays in liquid He

Energies and lorentzian widths of pionic K X-ray transitions have been measured in liquid ³He with improved accuracy. The strong interaction on the π³He 1s level is found to be attractive and to produce an increase in the K transition energies of 34 ± 4 eV; the measured lorentzian width is 36 ±7 eV. Measured values are also presented for K X-ray energies in liquid π⁴He and μ⁴He, the lorentzian width of the 1s level in π⁴He, and relative intensities of K X-ray transitions in π³He, π⁴He and μ⁴He. The measurements are compared with those of others and with recent theoretical calculations.     

The (He, t) reaction at intermediate energies : Spin-isospin multipole transitions

Data for the (³He, t) reaction at 900 MeV and 2 GeV on the targets ²⁶Mg, ⁴⁰Ca, ⁴⁸Ca, ⁵⁴Fe, ⁹⁰Zr and ²⁰⁸Pb are presented. A multipole decomposition for the data at 900 MeV has been made and the different distributions have been analysed. From the L = 0 cross section the Gamow-Teller strength distributions are extracted and compared with (p, n) data. The L = 1 and 2 distributions are analysed in a schematic model which describes the general systematics fairly well. The spectra at 2 GeV and Θ = 4° show for all targets a well-developed quasi-elastic peak. The A-dependence of the cross section is analysed in a simple model.     

Measurement of the average polarization of B produced by polarized muons in the μ + C → νμ + B reaction

The average polarization of ¹²B produced by the capture of polarized muons in ¹²C has been measured using recoil implantation techniques. From the result we deduce the average polarization of the ¹²B ground state ¹²B(0) corresponding to the ¹²C → ¹²B(0) Gamow-Teller reaction: J_μ(0) = 0.43 ± 0.10. The sizeable deviation of this polarization from the value of 2/3, characteristic of a “bare” 0⁺ → 1⁺ process, is a fair evidence for induced axial-vector interaction(s) in muon capture. The ratio of the induced pseudoscalar and the axial-vector coupling constants is deduced to be: g^μ_P/g^μ_A = 12 ± 5.     

Spectroscopy of C

The ¹⁴C(t, p)¹⁶C reaction locates five new states in ¹⁶C, at excitation energies of 3120 ± 15, 3983 ± 10, 4136 ± 10 and 6109 ± 15 keV, in addition to the g.s. and 1.76 MeV states. The 3.02 and 3.98 MeV states appear to be the second 0⁺ and 2⁺ 2p-2h states, respectively. The 4.14 MeV state has J^π = 4⁺ and the 6.11 MeV state has J^π = 2⁺, 3⁻, or 4⁺.     

A study of the level structure in Fe from the (d, p) reaction on Fe

The reaction ⁵⁶Fe(d, p)⁵⁷Fe is investigated at 12 MeV using the Aldermaston multi-channel magnetic spectrograph. The angular distributions of protons leading to various states in ⁵⁷Fe upto an excitation of 6.7 MeV are measured over an angular range 5°–175°. The data are analysed with the distorted wave Born approximation calculations; a satisfactory agreement is found in most cases upto about 100°. Spin, parity and the spectroscopic factors for various states are obtained and the positions of the single-quasiparticle energies determined. The results are compared with those for the isotonic nuclei ⁵⁵Cr and ⁵⁹Ni and with the pairing theory.     

Electro-pion production on O to bou nd states of the residual nuclei

Differential cross sections for the reactions 16O(γ, π−π+−)16F16F to the sum of the four lowest lying states in 16F and 16N have been measured as a function of angle for pions with a kinetic energy of 30 MeV. The extracted ratios R = σ(γ, π−)/σ(γ, π+), the first ones to discrete final states as a function of angle, are in fair agreement with results obtained for the nucleon. For positive pions the energy dependence of the cross section has been measured at the angles of 45° and 90°. Distorted wave impulse approximation calculations fail to describe the energy dependence.     

Particle multiplicities in the fission-like reactions of 340 MeV Si on Th

Pre-scission and post-scission multiplicities of neutrons and alpha particles have been simultaneously measured for the fission-like reactions of 340 MeV ²⁸Si on ²³²Th. Dynamical model calculations using HICOL code predict that about 90% of the observed events are of quasi-fission type while the remaining 10% are from compound nucleus fission decay. Moving source fits were carried out to the observed neutron and alpha particle spectra, measured at different angles with respect to the fragment directions. The pre-scission and post-scission neutron multiplicities are deduced to be 8.7±2.0 and 9.4±2.0, respectively. The corresponding multiplicity values for alpha particles are found to be 0.22±0.08 and 0.1±0.03. From the measured post-scission neutron multiplicity, it is inferred that about 65±20 MeV of the initial excitation energy remains at scission. This may be compared to the value of 85±30 MeV estimated from PACE2 statistical model calculations, adjusted to reproduce the measured pre-scission neutron multiplicity. From a comparison of the Statistical Model predictions with the measured pre-scission neutron multiplicity, the fission delay is estimated to be of 5⁺⁷₋₃×10⁻²⁰ s which overlaps with the average duration of fission-like process from the contact to the scission point (2×10⁻²⁰ s) as determined from HICOL-based dynamical calculations. For the delay time deduced as above, the pre-scission alpha particle multiplicity calculated by the PACE2 code is about a factor two larger than the experimental one, demonstrating the difficulties in modelling the alpha particle emission from highly elongated shapes that characterize the fissioning system from the contact point to scission.     

Elastic scattering of B on B in the energy range from 4 to 15 MeV

Angular distributions (at E_c.m. = 4, 6.5 and 10.5 MeV) and excitation functions (at 30°, 60° and 90°) are given for the elastic scattering of ¹⁰B on ¹⁰B. The results of an optical model (OM) analysis are presented and discussed. In the energy range covered the Sommerfeld parameter η varies from 4.4 to 2.3.     

Multinuclear NMR studies on the sol-gel preparation of sodium aluminophosphate glasses

Sodium aluminophosphate gels and glasses in the system NaPO₃–Al₂O₃ with P/Al ratios ranging from 9:1 to 1:1 have been synthesized by a novel sol–gel route based on the reaction of aluminum lactate with sodium polyphosphate in aqueous solution. The route from the solution to the gel and the final glass was monitored in situ by liquid and solid state NMR techniques, characterizing the influence of composition and pH on the hydrolysis, polymerization, and vitrification processes. The site distribution in the xerogels is strongly influenced by the gel-processing temperature. At temperatures near 150°C ligation with lactate groups can be nearly suppressed, resulting in maximum Al/P connectivity in the gel. Annealing the gels at temperatures near 400°C produces significant structural rearrangements, resulting in a glassy network that has close structural similarity to the glasses derived from the usual melt-cooling procedure at 1100–1450°C. This has been confirmed by extensive ²⁷Al, ³¹P and ²³Na MAS NMR as well as ²⁷Al{³¹P} and ²⁷Al {¹H} double resonance experiments. Compared to melt-cooling, the sol–gel process permits a significant extension of the glass-forming region towards higher alumina contents.     

Crystallographically-dependent ripple formation on Sn surface irradiated with focused ion beam

The metallographically polished polycrystalline Sn surface was sputtered by 30 kV focused Ga⁺ ions at room temperature. The experiment was carried out using various FIB incidence angles (0°, 15°, 30°, and 45°) over a wide range of doses (10¹⁶–10¹⁸ ions/cm²). The surface morphology was carefully characterized under the optical microscope, scanning electron microscope (SEM) and atomic force microscope (AFM). Ripples were observed on the irradiated areas even at the normal FIB incidence angle, which is not consistent with the Bradley–Harper (BH) rippling model. The orientation of ripples relies on crystallographic orientation rather than projected ion beam direction as predicted by BH model. The ripple wavelength is independent of ion dose, while ripple amplitude increases with ion dose. It is found that the ripples are formed by self-organization due to anisotropic surface diffusion in the low melting point metal.