Electronic and Optical Properties of a Lens Shaped Quantum Dot under Magnetic Field：Second and Third-Harmonic Generation

In the present work, we have studied electronic and optical properties of a lens-shaped quantum dot under an external magnetic field. For this goal, we have calculated the energy levels and wave functions using the finite element method (FEM) for different values of magnetic field. We have also studied effect of magnetic field on second harmonic generation (SHG) and third-harmonic generation (THG) in the lens-shaped quantum dot. In this regard, we have obtained an analytic expression for the SHG and THG by a compact density matrix approach and an iterative procedure. According to the obtained results, it is found that the presence of the magnetic field affects the symmetry of the system. The SHG and THG are decreased with increasing the magnetic field. The magnetic field has a great influence on the energy levels, wave functions, the SHG and THG in a lens shaped quantum dot.     

Electronic and Optical Properties of a Lens Shaped Quantum Dot under Magnetic Field: Second and Third-Harmonic Generation

In the present work, we have studied electronic and optical properties of a lens-shaped quantum dot under an external magnetic field. For this goal, we have calculated the energy levels and wave functions using the finite element method(FEM) for different values of magnetic field. We have also studied effect of magnetic field on second harmonic generation(SHG) and third-harmonic generation(THG) in the lens-shaped quantum dot. In this regard, we have obtained an analytic expression for the SHG and THG by a compact density matrix approach and an iterative procedure. According to the obtained results, it is found that the presence of the magnetic field affects the symmetry of the system. The SHG and THG are decreased with increasing the magnetic field. The magnetic field has a great influence on the energy levels, wave functions, the SHG and THG in a lens shaped quantum dot.     

Imaging theory of nonlinear second harmonic and third harmonic generations in confocal microscopy

ItisreportedrecentlythatnonlinearopticalphenomenonofSHGandTHGhasbeenobservedinmanybiologicaltissues[16].SHGandTHGhavebeenusedtoperformthethree-dimensionalimaginginlivingtissuesandhaveattractedmuchattentionrecently.TherearemanyadvantagesofusingSHGandTHGtoperformthethree-dimensionalimaginginlivingtissues,suchasnoninvasiveandnophotobleaching,inadditiontotheimagingpropertiesofmulti-photonfluorescenceimaging[7—9].Firstly,unlikeinthesingle-andmulti-photonfluorescenceprocesses,onlyvirtualstat…     

Nonlinear Optical Rectification,Second and Third Harmonic Generations in Square-Step and Graded-Step Quantum Wells under Intense Laser Field

For square-step quantum wells(SSQWs) and graded-step quantum wells(GSQWs), the nonlinear optical rectification(NOR), second harmonic generation(SHG) and third harmonic generation(THG) coefficients under an intense laser field(ILF) are analyzed. The found results indicate that ILF can ensure a vital influence on the shape and height of the confined potential profile of both SSQWs and GSQWs, and alterations of the dipole moment matrix elements and the energy levels are adhered on the profile of the confined potential. According to the results, the potential profile and height of the GSQWs are affected more significantly by ILF intensity compared to SSQWs. These results indicate that NOR, SHG and THG coefficients of SSQWs and GSQWs may be calibrated in a preferred energy range and the magnitude of the resonance peak(RP) by tuning the ILF parameter. It is feasible to classify blue or red shifts in RP locations of NOR, SHG and THG coefficients by varying the ILF parameter. Our results can be useful in investigating new ways of manipulating the opto-electronic properties of semiconductor QW devices.     

双波长双脉冲激光三次谐波的产生方法

提出双波长双脉冲激光产生三次谐波的方法。波长不同的两脉冲激光束由反射使它们合拢后通过两块非线性的BBO晶体 ,激光脉冲第一次通过BBO晶体产生两波长的二次谐波 (SHG) ,它们由各自的反射镜反射再次通过BBO又产生了二次谐波 ,这两次产生的二次谐波和基波通过用于产生三次谐波的BBO晶体可产生双波长的三次谐波 ,它们由 45°斜置的耦合镜输出。文中分析了满足二次谐波和三次谐波的四个相位匹配的条件 ,该方法也可用于腔内双波长双脉冲的三次谐波激光的产生 ,给出了相应的实验结果。     

In vivo polarization dependant Second and Third harmonic generation imaging of Caenorhabditis elegans pharyngeal muscles

In this study Second and Third harmonic generation (SHG-THG) imaging measurements were performed to the pharyngeal muscles of the nematode Caenorhabditis elegans, in vivo with linearly polarized laser beam. Complementary information about the anatomy of the pharynx and the morphology of the anterior part of the worm were extracted. THG signals proved to have no dependence on incident light polarization, while SHG images are highly sensitive to the changes of the incident linearly polarized light.     

In vivo imaging of cell morphology and cellular processes in Caenorhabditis elegans, using non-linear phenomena

We present the detailed imaging of structures and processes of the nematode Caenorhabditis elegans (C. elegans) using non-linear microscopy. Complementary information about the anatomy of the nematode was collected by implementing a combination of two photon excitation fluorescence (TPEF), second and third harmonic generation (SHG and THG) image contrast modes on the same microscope. Three-dimensional (3D) reconstructions of TPEF, SHG and THG images were also performed. Moreover, THG imaging technique has been tested as a potential, novel, non-destructive diagnostic tool for monitoring cellular processes in vivo, such as neuronal degeneration.     

Intense laser-induced electronic and optical properties in double finite oscillator potential

In the present paper, a theoretically study of the non-resonant laser field effect on the optical response, such as nonlinear optical rectification (NOR), second (SHG) and third harmonic generation (THG) coefficients in double finite oscillator potential (DFO) quantum wells is performed in the framework of the effective mass approximation. The obtained results reveal that, energy states and optical response is significantly affected by the non-resonant intense laser field (ILF) intensity and symmetry of the structure. Also it was found that the laser field is more effective on the optical response in the DFO potential when the asymmetric character of the confinement potential is strong. Thus, the NOR, SHG and THG coefficients with designated values can be obtained by using a properly adjusted ILF intensity and symmetry parameter of confinement potential.     

Tuning third harmonic generation of impurity doped quantum dots in the presence of Gaussian white noise

We perform a broad exploration of profiles of third harmonic generation (THG) susceptibility of impurity doped quantum dots (QDs) in the presence and absence of noise. We have invoked Gaussian white noise in the present study. A Gaussian impurity has been introduced into the QD. Noise has been applied to the system additively and multiplicatively. A perpendicular magnetic field emerges out as a confinement source and a static external electric field has been applied. The THG profiles have been pursued as a function of incident photon energy when several important parameters such as electric field strength, magnetic field strength, confinement energy, dopant location, Al concentration, dopant potential, relaxation time and noise strength assume different values. Moreover, the role of the pathway through which noise is applied (additive/multiplicative) on the THG profiles has also been deciphered. The THG profiles are found to be decorated with interesting observations such as shift of THG peak position and maximization/minimization of THG peak intensity. Presence of noise alters the characteristics of THG profiles and sometimes enhances the THG peak intensity. Furthermore, the mode of application of noise (additive/multiplicative) also regulates the THG profiles in a few occasions in contrasting manners. The observations highlight the possible scope of tuning the THG coefficient of doped QD systems in the presence of noise and bears tremendous technological importance.     

光合色素分子吸附膜的非线性增强效应

吸附在光学表面上的细菌叶绿素和藻兰素生物分子膜.在基波(λ=1.06μm)激光作用下,观察到谐波效应.文中对藻兰素只产生三次谐波而不产生二次谐波做了分析.     

Second- and third-harmonic generations for a nondilute suspension of coated particles with radial dielectric anisotropy

We derive expressions for the effective nonlinear susceptibility tensors for both the second harmonic generation (SHG) and induced third harmonic generation (THG) of nonlinear composite materials, in which nondilute coated particles with radial dielectric anisotropy are randomly embedded in the linear host. Two types of coated particles are considered. The first is that the core possesses a second order nonlinear susceptibility and the shell is linear and radially anisotropic, while the second is that the core is linear with radial anisotropy and the shell has a second order nonlinear susceptibility. We observe greatly enhanced SHG and THG susceptibilities at several surface plasmon resonant frequencies. For the second model, due to the coating material being metallic, there exists two fundamental resonant frequencies ω_c1 and ω_c2, whose difference ω_c2-ω_c1 is strongly dependent on the interfacial parameter and the radial dielectric anisotropy. Furthermore, in both systems, the adjustment of the dielectric anisotropy results in larger enhancement of both SHG and induced THG susceptibilities at surface plasmon resonant frequencies than the corresponding isotropic systems. Therefore, both the core-shell structure and the dielectric anisotropy play important roles in determining the nonlinear enhancement and the surface resonant frequencies.     

LD泵浦全固态355nm紫外皮秒脉冲激光器

利用激光二极管（LD）端面抽运Nd∶YVO4激光晶体皮秒三倍频355nm全固态紫外激光器,采用半导体可饱和吸收镜（SESAM）锁模技术及皮秒再生放大技术,对1 064 nm基波采用Ⅰ类相位匹配Li3B3O5（LBO）晶体二倍频和Ⅱ类相位匹配LBO晶体三倍频,获得了稳定性好、倍频效率较高的355 nm紫外激光输出。当二极管泵浦功率为5 W时,获得了脉宽为17 ps、重复频率为1 Hz、单脉冲能量为129.6 J的稳定三倍频紫外激光输出,基频光到二倍频光和三倍频光的转换效率分别达到60.3%和16.6%,3 h输出单脉冲能量的抖动在0.58%以下。     

Harmonic generation in bismuth triborate (BiB3O6)

We report a study of second- and third-harmonic generation in BiB₃O₆ (BiBO). The effective nonlinearity, phase-matching angle, acceptance bandwidth, and walk-off are calculated and analyzed within the principal planes of the optical indicatrix. In the experiment, the phase-matched harmonic generation is investigated within the xz and yz planes. Also, the temperature dependence of the noncritical phase matching for laser radiation propagating along the z axis is measured for second-harmonic generation (SHG) at crystal temperatures of 25–265^∘C. The corresponding wavelengths of the laser radiation are in the range of 1.16 to 1.34μm. In addition, SHG of 1342-nm radiation of a q-switched Nd:YVO₄ laser system is investigated for noncritical and critical phase matching. The achieved conversion efficiencies are 59% and 20%, respectively. Besides SHG, third-harmonic generation (THG) of 1064-nm, ns laser pulses is investigated. The measured conversion efficiency is as high as 34%. For THG the properties of BiBO are compared with those of BBO and LBO.     

Effects of weak localization of photons in nonlinear optics: Second harmonic generation

The angular distribution of the second harmonic generation (SHG) in disordered nonlinear media is shown to exhibit sharp peaks due to the weak localization of photons. The shape of these peaks is related to the spatial structure of the electric field for strongly scattered second harmonic (SH) radiation and is sensitive to the Anderson localization effects. The angular distribution of the second harmonic energy flux is calculated for the case of steady state and pulse generation in a slab of thickness d ≫ l (l is the elastic mean free path). For the case of pulse generation the time dependence of the SHG is discussed.     

Third harmonic generation in quantum dot with Rashba spin orbit interaction

Here we have investigated the influence of magnetic field and confinement potential on nonlinear optical property, third harmonic generation (THG) of a parabolically confinement quantum dot in the presence of Rashba spin orbit interaction. We have used density matrix formulation for obtaining optical properties within the effective mass approximation. The results are presented as a function of confining potential, magnetic field, Rashba spin orbit interaction strength and photon energy. Our results indicate that an increase of Rashba spin orbit interaction coefficient produces strong effect on the peak positions of THG. The role of confinement strength and spin orbit interaction strength as control parameters on THG have been demonstrated.     

Effects of hydrostatic pressure and temperature on the nonlinear optical properties of semiparabolic plus semi-inverse squared quantum wells

In this study, the effects of hydrostatic pressure and temperature on nonlinear optical rectification(OR), second-harmonic generation(SHG), third-harmonic generation(THG) and the linear,nonlinear, and total optical absorption coefficients(OACs) of a semiparabolic plus semi-inverse squared quantum well(QW) are theoretically investigated. The results show that hydrostatic pressure and temperature have significant effects on the optical properties of semiparabolic plus semi-inverse squared QWs, and that the energy levels and magnitudes of the resonant peaks of OR, SHG, THG, and the total OACs vary according to the shape of the limiting potential, the hydrostatic pressure, and the temperature. It is easily seen that the peak positions of the resonant peaks of OR, SHG, THG, and the total OACs in the semiparabolic plus semi-inverse squared QW show a red shift with increasing hydrostatic pressure, but a blue shift with increasing temperature. Therefore, the magnitude and position of the resonant peaks of OR, SHG, THG,and the total OACs can be adjusted by changing the hydrostatic pressure and the temperature,which promise a new degree of freedom in the tunability of various electro-optical devices.     

Completely solid-state LD-side-pumped Nd:YAlO<Subscript>3</Subscript> CW blue laser with intracavity frequency tripling

We report a completely solid-state continuous-wave (CW) blue laser operating at 447 nm utilizing intracavity frequency tripling of an LD-side-pumped Nd:YAlO₃ (Nd:YAP) laser operating at 1341.4 nm. An LBO crystal with type-I critical phase matching and a KTP crystal with type-II critical phase matching (CTM) were used for the second harmonic generation (SHG) and the third harmonic generation (THG), respectively. In view of the analysis of the cavity stability, a four-mirror folded cavity was designed and the output characteristics were theoretically analyzed. Experimental characteristics obtained were shown to be in agreement with the theoretical analysis. The maximum output power of the 447 nm CW blue laser reached 114 mW, which corresponds to a red-to-blue conversion efficiency of 9%.     

Design of the Seed Source for High Power KrF Excimer Laser System

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Analysis on dependence of phase matching angle on temperature in KDP crystal

The dependence of the phase matching (PM) angle on temperature in type-I second harmonic generation (SHG) and type-II third harmonic generation (THG) of KDP is experimentally investigated. The experimental results show that as the crystal temperatures vary by 1 °C, the external PM angles of the KDP doubler and tripler change 100 μrad and 220 μrad, respectively. The PM angle of KDP tripler is more sensitive to temperature variation than is that of the KDP doubler. Comparing the numerical calculations and the previous reports, a discrepancy has been found among the different reported results. Based on the analytical solution of the temperature dependence of the SHG process it is shown that a small error in the thermo-optic coefficients of the crystal is the main factor source of the discrepancy.     

Effects temperature,pressure and spin–orbit interaction simultaneously on third harmonic generation of wedge-shaped quantum dots

In the present paper, we have studied the effects of temperature and pressure simultaneously on the third harmonic generation (THG) of a GaAs wedge-shaped quantum dot under the influence of spin–orbit interaction (SOI). For this purpose, we have used analytical expression for THG obtained by the compact-density matrix formalism. THG has been calculated for different temperatures and pressures under SOI. According to the obtained results, it is found that (i) THG shows a red shift of peak position in the presence of SOI. (ii) THG shifts toward higher energies with increasing temperature and considering the SOI. (iii) THG moves to lower energies with increasing pressure and considering the SOI.