利用场关联效应抑制瑞利型非简并四波混频的热背底

瑞利型非简并四波混频是测量物质超快纵向弛豫时间的有效手段,将场关联原理应用于具有热吸收的样品中瑞利型非简并四波混频的热背底抑制，给出了抑制热背底的条件，并通过数值模拟证明了其可行性. 关键词： 四波混频 场关联 超快测量     

布里渊增强非简并四波混频

在CS₂介质中观测到由声波引起的布里渊增强非简并四波混频(NFWM)和由分子取向栅产生的瑞利型NFWM.研究发现,分子取向栅与声波之间并不是相互独立的,声波的存在会破坏瑞利型NFWM和布里渊增强NFWM极化之间的相位关系. 关键词： 四波混频 布里渊散射 瑞利散射     

应用波分复用技术实现飞秒级超快动态过程的脉冲数字显微全息记录

采用波分复用方法实现飞秒级超快动态过程的脉冲数字显微全息记录和再现。在全息记录过程中,利用BBO倍频晶体对入射激光进行倍频,将基波和谐波分光,并经时间延迟后进入迈克耳孙干涉仪,从而可应用波分复用技术,先后在CCD的一帧图像上记录两张具有不同空间频率的子全息图。采用这种方法,实现了对单脉冲飞秒激光激发空气电离的超快动态过程的全息记录,并通过数字傅里叶变换和数字滤波的方法,分别再现出每张子全息图记录的波前,从而获得了具有飞秒时间分辨的空气等离子体形成和传播过程的动态振幅和相位图像,其单次曝光时间为50 fs,曝光时间间隔为400 fs,相应的曝光频率约为2.5×1012f/s。     

引入量子干涉的双光子共振非简并四波混频

研究了级联四能级系统中双光子共振非简并四波混频(NFWM)由于加入耦合光场而产生的量子干涉效应，发现在强耦合场作用下NFWM频谱呈现AT劈裂，它反映的是两个缀饰态的能级.量子干涉还使NFWM信号被抑制或增强.此方法牵涉到三光子共振，因此可以成为研究原子或分子高激发态的有效光谱学工具. 关键词： 四波混频 量子干涉     

Precursor states for charge carrier generation in conjugated polymers probed by ultrafast spectroscopy

Photocurrent experiments using two femtosecond laser pulses are performed on a photodiode using a ladder-type conjugated polymer as the active layer. With a photon energy of 3.1 eV the first pulse excites singlet excitons. A time-delayed second pulse with a photon energy of 2.49 eV leads to a decrease of the photocurrent by exciton depletion due to stimulated emission. S1 excitons being dissociated during their entire lifetime are identified as the only relevant channel for charge carrier generation. Intrachain polaron pairs are also formed on an ultrafast time scale with a yield of approximately 10%. They can be efficiently dissociated by reexcitation with photons of an energy of 1.9 eV.     

Atomic coherence in nondegenerate four-wave mixing

Two-photon resonant nondegenerate four-wave mixing (NFWM) with the addition of a coupling field in Ba atomic vapour has been studied. We find that coherence of the atomic level transitions leads to suppression of the NFWM signal, giving rise to a dip with a linewidth that is linearly proportional to the intensity of the coupling field.     

双光子共振非简并四波混频测量钡原子里德伯态碰撞展宽中的伴线研究

研究了采用双光子共振非简并四波混频技术测量原子里德伯态碰撞展宽时出现的伴线现象, 测量了不同缓冲气压下的钡原子里德伯态6snd ¹D₂ (n=16, 22, 36) 的四波混频谱线, 研究了伴线随主量子数n 的变化曲线以及伴线信号强度随缓冲气压压强的变化曲线, 分析了伴线对NFWM谱线的线宽的影响, 发现考虑伴线对四波混频谱线线宽的贡献, 可以对NFWM模型下测量到的碰撞展宽系数进行修正.     

Logical stochastic resonance in bistable system under α-stable noise

An autonomous stochastic system with nonlinear time-delayed feedback is investigated employing the stochastic simulation method. In the autonomous stochastic system with quadratic time-delayed feedback or under positive feedback, the nonlinear delay time fails to possess the role improving the noisy state of the system. In the autonomous stochastic system with cubic time-delayed feedback and under negative feedback, the nonlinear delay time can improve the noisy state, tuning the signal output, and generating incoherence and coherence maximization. We reveal a new kind of anti-coherence and coherence resonance phenomena induced by the nonlinear time delay in the autonomous stochastic system without external periodic force, discussing further the effects of the noise strength, the control parameter, and the feedback strength on anti-coherence and coherence resonance.     

Picosecond transient photoconductivity in functionalized pentacene molecular crystals probed by terahertz pulse spectroscopy

We have measured transient photoconductivity in functionalized pentacene molecular crystals using ultrafast optical pump-terahertz probe techniques. The single crystal samples were excited using 800 nm, 100 fs pulses, and the change in transmission of time-delayed, subpicosecond terahertz pulses was used to probe the photoconducting state over a temperature range from 10 to 300 K. A subpicosecond rise in photoconductivity is observed, suggesting that mobile carriers are a primary photoexcitation. At times longer than 4 ps, a power-law decay is observed consistent with dispersive transport.     

Correlation Functions of an Autonomous Stochastic System with Nonlinear Time Delays

The auto-correlation function and the cross-correlation of an autonomous stochastic system with nonlinear time-delayed feedback are investigated by using the stochastic simulation method. There are prominent differences between the roles of quadratic time-delayed feedback and cubic time-delayed feedback on the correlations of an autonomous stochastic system. Under quadratic time-delayed feedback, the nonlinear time delay fails to improve the noisy state of the autonomous stochastic system, the auto-correlation decreases monotonously to zero, and the cross-correlation increases monotonously to zero with the decay time. Under cubic time-delayed feedback, the nonlinear time delay can improve the noisy state of the autonomous stochastic system; the auto-correlation and the cross-correlation show periodical oscillation and attenuation, finally tending to zero with the decay time. Comparing the correlations of the system between with nonlinear time-delayed feedback and linear time-delayed feedback, we find that nonlinear time-delayed feedback lowers the correlation strength of the autonomous stochastic system.     

Ultrafast three-dimensional submicrometer-resolution readout of coherent optical-phonon oscillations with shaped unamplified laser pulses at 20 MHz

An ultrafast three-dimensional readout of coherent optical-phonon oscillations from a diamond film is demonstrated using temporally and spectrally shaped ultrashort laser pulses, delivered by a compact, oscillator-only laser system. This system integrates a long-cavity ytterbium-fiber-laser-pumped 30?fs Cr:forsterite oscillator with a photonic-crystal-fiber soliton frequency shifter and a periodically poled lithium niobate spectrum compressor, providing coherent Raman excitation and time-delayed interrogation of optical phonons in diamond at a 20?MHz repetition rate with a submicrometer spatial resolution.     

应用双光子共振非简并四波混频测量Ba原子里德伯态

使用具有中间态的双光子共振非简并四波混频(NFWM)测量了Ba原子J＝0和J＝2的偶宇称里德伯线系，与现代实验方法不同，本方法是纯光学的方法，其光路简单，检测的是相干光，而不是电子或离子信号.当用窄带宽的激光时，本技术对里德伯能级的窄光谱结构可以获得消多普勒的分辨率. 关键词： 四波混频 里德伯态     

The effect of time-delayed feedback on logical stochastic resonance

We examine the possibility of obtaining logic operation in a quartic-bistable system with linear time-delayed feedback subjected to Gaussian noise. The effect of time-delayed feedback on the effective potential well is investigated, and explicit numerical stimulation is conducted to study the influence of delay time and strength of the time-delayed feedback on the responses of the system. Although the response deteriorates slightly at low values of noise intensity with time-delayed feedback and the peak correct probability decreases from 100% when the delay time is too long, the reliability of obtaining the desired logic output is enhanced in the higher noise boundary with the help of moderate time-delayed feedback. We also found that increasing the linear factor of the system can shift the optimal noise intensity to a higher level.     

光学外差法测量Ba原子的自电离态

提出了把三光子共振非简并六波混频(NSWM)和双光子共振非简并四波混频(NFWM)应用于研究Ba原子自电离态的光学外差探测方法。采用该方法测量了Ba原子的6P_３／２19d自电离态,并观察到了三光子共振 NSWM和双光子共振NFWM信号干涉引起的信号增强。该方法是一种纯非线性光学方法,具有优秀的空间分辨率和简单的光路。其中双光子共振非简并四波混频信号作为本地振荡光束,三光子共振非简并六波混频信号作为信号光束,通过 改变信号光束的频率来达到用光学外差探测法研究Ba原子自电离态的目的。该方法中,实现相位匹配所要求的条件不是很严格,可以在很宽的频率范围内实现相位匹配,而一般的六波混频很难做到相位匹配, 并且所测量的信号是相干光, 当用窄带宽的激光时,可以获得消多普勒的分辨率。     

Control of unstable steady states in neutral time-delayed systems

We present an analysis of time-delayed feedback control used to stabilize an unstable steady state of a neutral delay differential equation. Stability of the controlled system is addressed by studying the eigenvalue spectrum of a corresponding characteristic equation with two time delays. An analytic expression for the stabilizing control strength is derived in terms of original system parameters and the time delay of the control. Theoretical and numerical results show that the interplay between thecontrol strength and two time delays provides a number of regions in the parameter space where the time-delayed feedback control can successfully stabilize an otherwise unstable steady state.     

Experimental investigation of a bistable system in the presence of noise and delay

We experimentally analyze the behavior of a non-Markovian bistable system with noise, using a vertical cavity surface emitting laser with time-delayed optoelectronic feedback. The effects of the delayed feedback are observed in the probability distribution of the residence times of the two orthogonal polarization states, and in the polarization-resolved power spectrum. They agree well with recent theoretical predictions based on a two-state model with transition rates depending on an earlier state of the system. We also observe experimentally and explain theoretically that the residence time probability distribution deviates from exponential decay for residence times close to (and smaller than) the delay time.     

测量原子里德堡态的新方法——双光子共振非简并四波混频

本文介绍了一种测量原子里德堡态的新方法--具有中间态的双光子共振非简并四波混频,与现代实验方法不同,该方法是纯光学的方法,其光路简单,检测的是相干光,而不是电子或离子信号.当用窄带宽的激光时,该技术对里德堡能级的窄光谱结构可以获得消多普勒的分辨率.     

Experimental demonstration of phase control of dispersion effects for an ultrashort pulse train propagating in a resonant medium

We present an experiment in which an ultrashort pulse train propagates resonantly through anoptically dense vapor of atomic rubidium. The sequence obtained from a Fabry-Perot interferometer comprises nearly 10 regularly time-delayed and mode-locked pulses. We show that a sequence with phase shift phi = 0[2pi] between two successive pulses propagates with important temporal distortion, whereas a sequence with phi = pi[2pi] experiences few propagation effects, thus leading for the first time to our knowledge to the possibility of phase control of dispersion effects for an ultrashort pulse train.     

长寿命吸收过程对超快动力学过程测量的影响

使用飞秒时间分辨抽运-探测透射光谱技术,实验研究了GaAs体材料中光激发载流子的超快弛豫动力学的波长依赖.在相同的光激发载流子浓度和抽运/探测比时,发现760 nm和780 nm两中心波长处的瞬态透射变化延迟扫描信号出现负的和振荡的信号.与模拟计算结果对比,判定该实验瞬态信号是错误的.分析探测器输出波形,发现是由于反相波形导致的,而引起反相波形的原因在于样品中存在长寿命的吸收过程.指出通过提高探测器上的抽运/探测比能够矫正反相波形,从而获得正确的瞬态透射变化动力学.提高探测器上的抽运/探测比与目前的应尽量减小抽运光对探测器的散射贡献的观点是对立的.文章的研究结果对应用抽运-探测时间分辨光谱技术正确地测量超快瞬态动力学过程具有重要的参考价值. 关键词： 时间分辨抽运-探测透射光谱 饱和吸收 吸收增强 GaAs体材料     

Optimal signal-to-noise ratio in stochastic time-delayed bistable systems

We study the optimal signal-to-noise ratio in a stochastic time-delayed bistable system.By using the small delay approximation, we transform the time-delayed system intostochastic nondelayed differential equations to obtain the analytic expressions of thesignal-to-noise ratio in different mechanisms. In the valid range of small delayapproximation, we compare the peak values of signal-to-noise ratio curves and obtain theoptimal signal-to-noise ratio. From the results, we find that the interplay of time delayand noise has a great influence on time-delayed bistable systems.