Cavityless optical bistability in a thin semiconductor film upon the resonant excitation of excitons and biexcitons

The bistable properties of a thin semiconductor film under conditions of resonant excitation of coherent excitons and biexcitons by photons in one or two different pulses are studied theoretically. Fiz. Tverd. Tela (St. Petersburg) 40, 932–933 (May 1998)     

Level-anticrossing effect on the magnetoluminescence of the triplet indirect bound exciton in GaSe

The presence of level-anticrossing in the triplet state of the indirect impurity-bound exciton in GaSe has been found for the first time in the magnetic field of 1.5 kOe applied along the c-axis. Measurements on the magnetic circular dichroism (MCD) of the photoluminescence and on the spin dependent formation rate (SDFR) show that the |S_z| = 1 level lies 0.016 meV higher than the S_z = 0 level in the absence of the magnetic field. The resonance-like behavior in these two types of polarization correlation measurements may be explained in terms of weak perturbation between |S_z| = 1 and S_z = 0 levels.     

Influence of two-pair continuum correlations following resonant excitation of excitons

The memory structure induced by coherent transitions to the exciton-exciton scattering continuum is shown to have significant influence on spectrally resolved four-wave-mixing signals even under selective excitation of 1s excitons. Comparisons between experiments and calculations that account nonperturbatively for these quantum kinetic Coulomb correlations demonstrate large compensations between mean-field contributions and transitions to the two-pair continuum. Experiments with different polarizations of the laser pulses show that two-pair continuum correlations are responsible for delay-time dependent shifts of the excitonic emission as well as for substantial deformations of the line shape.     

Optical spin orientation of excitons in GaSe under longitudinal magnetic field

The degree of circular polarization of the free-exciton luminescence line has been measured in GaSe excited by circularly polarized light at 4.2 K under longitudinal magnetic field. The result shows that the spin relaxation time of exciton is field-dependent but the spin memory before reaching the exciton ground state is almost unaffected by the applied longitudinal magnetic field.     

Resonant optical orientation and alignment of excitons in superlattices

Exciton states in short-period GaAs/AlGaAs superlattices have been studied by optical orientation and optical dipole-moment alignment methods. The effect of magnetic field in the Faraday and Voigt geometries on the degree of linear and circular polarization of photoluminescence have been studied under resonant and nonresonant excitation. The constants of electron-hole exchange interaction in the exciton have been determined. Fiz. Tverd. Tela (St. Petersburg) 40, 2229–2235 (December 1998)     

Spontaneous and stimulated emission in GaSe under intense excitation

Emission spectra have been investigated in GaSe at 80 K under nitrogen laser excitation. In the case of intense excitation, an additional broad band appears at 5970 Å, and is considered to be due to an exciton-exciton collision process. This process leads to stimulated emission.     

Optical and thermal orientation of localized excitons in solid solutions under resonant excitation in a longitudinal magnetic field

A theoretical and experimental study of the effect of a longitudinal magnetic field on optical orientation and magneto-circular polarization of the luminescence of localized excitons in semiconducting solid solutions is reported. It is shown that recombination takes place through two types of emitting states differing substantially in the degree of anisotropy, g factor, and spin relaxation time. Estimates are made of the g factors, anisotropic and exchange splittings, lifetime, and spin relaxation time of localized states in a CdS_0.96Se_0.04/GaAs solidsolution epitaxial layer. Fiz. Tverd. Tela (St. Petersburg) 40, 900–902 (May 1998)     

Dynamics of optical sine-Gordon solitons under double coherent pulse excitation

On the basis of a numerical simulation of the sine-Gordon equation the conclusion is made that the number of solitary waves is invariant with respect to the input pulse separation interval. But the value of this interval affects the form of the pulses: either 2π and a breather or 2π and a (± 2π) pair.     

Contribution of hexadecapole alignment to the polarization of quadrupole emission under laser excitation conditions

The linear polarization of quadrupole emission by the J=2-J ₀=0 transition under conditions of laser excitation in a gas medium is studied. Cases of excitation through dipole and quadrupole absorption of monochromatic laser radiation are considered. Taking into account the anisotropy of collisional relaxation, the contributions of polarization moments of the second and fourth ranks, i.e., those with usual and hexadecapole alignments, to the signal of linear polarization of quadrupole emission are calculated. The dependence of this signal on the laser frequency, the density of the gas medium, and the angles determining the orientation of the system of axes of observation of light polarization relative to a laser ray is studied. The numerical calculations of contributions of usual and hexadecapole alignment to the signal of linear polarization are made for the magnetic quadrupole transition J=2-J ₀=0 between the states 2p ⁵(² P ₁ ^2/0 )3p′[3/2]₂ and 2p ⁵(² P ₁ ^2/0 )3s 3s′[1/2]⁰ of neon atoms in the xenon atmosphere.     

Anisotropy of photoconductivity and nonlinear effects in GaSe monocrystals at high optical excitation

In this work, the photoelectric properties of gallium selenide (GaSe) monocrystals in the edge absorption region, with various configurations of current contacts, at low and high optical excitation levels are investigated. The photoconductivity spectrum behavior is determined by localized electronic and excitonic states along c-axis. It is shown that the localization of electronic and excitonic states in one-dimensional fluctuation potential along c-axis results to an anisotropy in photoconductivity spectrum at various current contacts configurations. At E⊥c the photoconductivity is observed in the hν < E_g and hν > E_g regions. In the case of hv < E_g, the maximum photoconductivity, in the impurity and exciton absorption region are observed at 1.975 eV and 2.102 eV, respectively. With rising of excitation energy level, suppression of photoconductivity in the exciton absorption region and increases in impurity absorption region is observed. At E||c contact configuration, the considerable photoconductivity is observed only in the impurity absorption region, which also increases with rising of excitation level. It is supposed that, suppression of photoconductivity in the exciton absorption region at high excitation levels is connected with exciton-exciton interaction, which results to a nonlinear light absorption. The results are compared with the absorption and photoluminescence measurements.     

Quantum optical studies on individual acceptor bound excitons in a semiconductor

We demonstrate the generation of triggered single photons at a predetermined and well defined energy using the radiative recombination of single nitrogen-bound excitons in a semiconductor. The nitrogen atoms are embedded in a ZnSe quantum well structure and were excited by nonresonant optical pumping (82 MHz) at low temperature (4 K). We find resolution-limited photoluminescence lines (280 micro eV) which display photon antibunching under continuous optical pumping. Our results also suggest that single nitrogen-bound excitons are well suited for cavity quantum electrodynamics experiments.     

Non-markovian dynamics of spectral narrowing for excitons in the layered semiconductor GaSe observed using optical four-wave mixing spectroscopy

We have investigated non-markovian dephasing by using time-resolved and spectrally resolved four-wave mixing measurements in a layered semiconductor GaSe. When the time interval between the first and second excitation pulses is increased, photon echo spectra exhibit narrowing only in a regime of a few picoseconds. In the initial dephasing of these signals, fast damping is observed. The narrowing of the spectrally resolved signal is consistent with the Fourier transformation of the time-resolved signals. Spectral narrowing is crucial evidence of the transition from non-markovian to markovian dynamics. By comparing experimental data with calculation results based on the non-markovian theory, we have found that the correlation time of the exciton-phonon interaction is 1.1 ps.     

Free and bound excitons in silver bromide under hydrostatic pressure

Abstract

Employing resonant Raman and luminescence spectroscopy, various exciton states and phonon modes are studied at low temperature in AgBr under hydrostatic pressure up to 0.7 GPa. The deformation potential for the indirect free exciton gap and mode Grüneisen parameters for various phonons are determined. Excitons bound to neutral donors and isoelectronic iodine are found to essentially derive from L-point valence band states.     

Theory of four-photon scattering in conditions of intense resonant excitation

Journal of Applied Spectroscopy -