在BBO中获得230.8—223.2nm高功率和频输出

用Q-YAG泵浦的Rh·6G染料激光在一块45°切割的β-BaB₂O₄(BBO)晶体中倍频,产生294.8—282.5nm范围的连续调谐输出,其能量为8mJ(在285nm处)。用这个倍频光与泵浦染料后剩余基波(1064nm)在另一块45°切割的BBO中和频,已获得230.8—223.2nm范围的连续调谐输出,其能量为120μJ,相应的峰值功率为12kW。还简述了获得高功率和频输出的关键技术。     

Collinear and non-collinear sum-frequency mixing inβ-BBO for a tunable 195–198 nm all-solid-state laser system

We attained tunable UV laser radiation between 195 and 198 nm by sum-frequency mixing two synchronized flashlamp-pumped solid-state Q-switch lasers, a Nd:YAG laser frequency quadrupled to 266 nm and a tunable (730–770 nm) alexandrite laser. UV pulse energies of 0.12 mJ with repetition rates of 10 Hz were attained in collinear, as well as non-collinear sum-frequency interaction in a-Barium Borate (BBO) crystal with a conversion efficiency of 2.5%. Theoretical models for the non-collinear phase-matching interaction were investigated at UV wavelengths below 200 nm.     

Tunable sub-100 femtosecond dye-laser pulses generated with a nanosecond pulsed pumping

Subpicosecond pulses at a fixed wavelength produced with a low-Q cavity dye laser pumped by a single, nanosecond laser (Q-switched Nd:YAG) are converted into tunable high-power sub-100 femtosecond pulses by generation, spectral selection, amplification and compression of a supercontinuum. The tunable, chirped, high-energy pulses obtained are compressed with a prism pair. Energies up to 50 J in sub-100 fs pulses were obtained in the 540 to 650 nm range using 40 mJ of the Nd: YAG-laser pumping pulses at 532 nm. The whole sub-100 fs system including the low-Q dye laser uses only one Nd:YAG laser as a pump source.     

在BBO晶体中获得271—281.5nm和频输出

本文用自制的Q-YAG的倍频光泵浦Rh·6G染料,用调谐的染料激光束(562—598nm)与YAG的倍频光束在B-BaB2O4(BBO)晶体中和频,获得的连续可调谐范围是271-281.5nm,和频输出能量大子200μJ,最高转换效率为5%.我们用陈创天等人和K.Kato所给BB0晶体的Sellmetier方程计算了和频调谐曲线,它们之间的相位匹配角大约有一度之差.实验曲线与两条理论曲线都有不同程度的偏差.但是,与K.Kato的理论曲线更为接近.我们还讨论了BBO晶体的长度对输出能量的影响,并解释了产生这种影响的原因。     

Harmonic and sum-frequency generation of pulsed laser radiation in BBO,LBO, and KD*P

The optical properties of the nonlinear crystals lithium borate (LBO), barium borate (BBO) and deuterated potassium phosphate (KD*P) are compared for second and third harmonic generation of Nd:YAG laser radiation. In an experimental investigation the conversion efficiency has been measured as a function of the energy density of 8 ns long laser pulses, generated by a commercial Nd:YAG oscillator-amplifier system. In LBO and BBO the second harmonic generation saturates at an energy density of about 1.5 J cm^–2 at efficiencies of 55–60%. In KD*P comparable efficiencies (40–55%) require energy densities of 2–2.6 J cm^–2. Similar results are obtained for frequency tripling. In LBO and BBO saturated efficiencies of 20–25% are measured at an energy density of about 1.5 J cm^–2. In KD*P efficiencies of 20% are obtained at energy densities exceeding 2 J cm^–2. Besides for doubling and tripling of Nd:YAG laser radiation the phase-matching is calculated for frequency conversion of tunable laser light. The results demonstrate that in LBO and BBO phase-matched sum-frequency mixing of UV and infrared laser light generates tunable radiation at wavelengths as short as the transmission cut-off at 160 nm and 190 nm, respectively.     

Generation of coherent tunable deep UV radiation for detection and absorption studies of explosives RDX and TNT

We report a technique for the efficient generation of tunable coherent deep UV radiation and its application in studies of RDX and TNT at the ppm level on the basis of their absorption characteristics. The obtained experimental absorption data are compared with conventional spectrophotometric data. The UV radiation in the range 200–260 nm has been generated by the type-I noncollinear third harmonic of the dye laser radiation (600–700 nm) and also by sum frequency mixing (SFM) of Nd:YAG output (1064 nm) with the second harmonic of the dye laser in β-barium borate (BBO) crystal. The maximum conversion efficiency of the generated signal is estimated to be 57.5% at λ = 218.9 nm wavelength. Apart from measurements of the absorbance of RDX and TNT at different concentrations in their respective solutions, the minimum detection concentrations have also been ascertained. The estimated minimum detectable concentration of RDX is 8.47·10⁻⁹ M, whereas that for TNT is 35.7·10⁻⁹ M. The data were obtained using only ∼100 μJ/pulse of laser energy. Published in Zhurnal Prikladnoi Spektroskopii, Vol. 74, No. 6, pp. 516–521, July–August, 2007.     

Picosecond Self-modelocked Wavelength Tunable Ti:Al_2O_3 Laser

1.IntroductionTi:Alzoscrystalasabroadtunablesolid--statelasermaterialbasedonvibronicallybroadenedtransitionsinmetalions,hasseenaresurgenceofresearchanddevelopmentrecently.TheadvantagesofTi:A12O3crystalincludebroadabsorptionandemissionspectrumbandwidth,highbeamqualityandcapabilityofallsolid--stateoperation.KerrlensmodelockedTi:sapphirelaserspumpedbyCWargon--ionlasersarewidelyusedasasourceoffemtosecondopticalpulsesll~'j.KerrlensmodelockingutlizestheorstiealKerreffecttoproduceafastpulse--shor…     

Development of a dual-wavelength dye-laser system for the UV and its application to simultaneous multi-element detection

In this paper, the design and performance characteristics of a pulsed tunable dye laser system for the simultaneous generation of two UV wavelengths are presented. The system is composed of an oscillator and an amplifier stage, pumped by the second harmonic of a commercial Nd:YAG laser. Dual-wavelength operation is achieved with one additional tuning mirror introduced to the prism expanded grazing incidence oscillator. The two obtained wavelengths are independently tunable, their separation is only limited by the gain profile of the dye. Both wavelengths are frequency doubled by Second-Harmonic Generation (SHG) in two KDP or BBO crystals. Performance characteristics such as bandwidth, efficiency, tuning range and wavelength separation are reported. As application two such systems are used for the simultaneous detection of the four elements cadmium, nickel, manganese and lead by Laser-Excited Atomic Fluorescence Spectrometry in a graphite furnace (ETA-LEAFS).     

Continuously tunable VUV radiation (129–210 nm) by anti-Stokes Raman scattering in cooled H2

The generation of tunable vacuum ultraviolet radiation by anti-Stokes Raman scattering of tunable ultraviolet dye-laser radiation in cold hydrogen has been investigated. The scattering efficiency of XeCl laser and Nd:YAG laser pumped commercial dye lasers and the influence of different beam profiles has been studied. Up to 12 anti-Stokes orders down to 129 nm were observed with output powers between about 20 kW at =191 nm and somewhat less than 100 W at =129 nm. The efficiency of transversely pumped lasers with an intensity peaked in the center of the beam profile was found to be higher than doughnut shaped intensity distributions. The cooling of the active gas to liquid nitrogen temperatures improved the output pulse energies 3 to 5 times on average. It was found that this intensity increase was caused mainly by the narrowing of the Raman linewidth upon cooling.     

Highly efficient deep ultraviolet generation by sum-frequency mixing in a BBO crystal pair

Generation of deep ultraviolet radiation at 210 nm by Type-I third harmonic generation is achieved in a pair of BBO crystals with conversion efficiency as high as 36%. The fundamental source is the dye laser radiation pumped by the second harmonic of a Q-switched Nd: YAG laser. A walk-off compensated configuration with the BBO crystal pair has enabled us to realize such a high conversion efficiency in the interaction.     

A Narrow Bandwidth BBO Optical Parametric Oscillator Injection－seeded by a Tunable Pulsed Ti：Sapphire Laser

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Sum and difference frequency generation of white light continuum with the ps pulses of Nd:YAG laser in a thick BBO crystal

The white light continuum (WLC) generated in water/D₂O mixture by pumping with the fundamental of ps Nd⁺³:YAG laser has been used as a variable frequency source for the sum frequency generation as well as for its amplification. 35 ps long pulses with 8 mJ energy at 1064 nm were mixed collinearly with the WLC generated by the same laser beam in a 20 mm thick BBO crystal. The obtained tunable output has been identified as the sum frequency between the fundamental and a portion of the WLC with the required phase matching. Theoretical simulations are also given along with a few initial experiments to use this combination for the difference frequency generation (optical parametric amplification) under non-collinear geometry.     

High Efficient C6H12 Raman Laser Enhanced by DCM Fluorescence

We report the first-order Stokes output （wavelength of 627.6 nm） from C6H12 enhanced by DCM dye fluorescence with high energy conversion efficiency of 47.9%, quantum conversion efficiency of 56.5%. To our knowledge, it is the highest conversion efficiency of stimulated Raman scattering obtained from liquid Raman laser. A 532nm frequency doubled Nd：YAG laser with 8 Hz repetition rate is employed as the pump source, and the enhancement medium is DCM dye solution in ethanol. The conversion efficiencies at various pump energies and various pump repetition rates are measured and analysed. The enhancement mechanism of SRS together with its potential application is discussed.     

Synchronously pumped femtosecond dye oscillator-amplifier system at 815 nm

A tunable dye oscillator-amplifier system that produces 0.25 mJ, 105 fs pulses at 815 nm is demonstrated. The system consists of a synchronously pumped femtosecond dye laser followed by a dye amplifier that is quasi-longitudinally pumped using the frequency-doubled output from a Nd:YAG regenerative amplifier.     

LD端面泵浦Nd:YAG/BIBO单模蓝光激光器

从理论上分析了准三能级系统946 nmNd:YAG全固态激光器运转的条件,并比较了几种不同的倍频晶体的特性,给出内腔倍频获得473 nm蓝光发射的方案。用波长808 nm、输出功率为2.2 W的半导体激光器泵浦Nd:YAG,采用内腔倍频的方法,在一定的温度下,用Ⅰ类临界相位匹配B IBO晶体倍频获得了473 nm 26.5 mW的单模连续蓝色激光输出,功率波动小于±5%。     

全固态多波长飞秒脉冲激光系统

利用棱镜对引进频谱空间啁啾来补偿飞秒脉冲激光二次谐波产生中的相位失配,提高了倍频效率建立了一套全固态、多波长(1065nm, 532nm,823.1nm, 402nm)飞秒脉冲激光系统自制的Nd:YVO4激光器输出532nm绿光激光,最高平均功率可达5.6W当用2.5W绿光激光泵浦时,从自制的钛宝石激光器及经BBO倍频可分别输出中心波长为823.1nm和402nm,平均功率300mW和73mW,谱宽32.3nm和5.1nm,脉宽22fs和33.3fs、重复率108MHz的近红外和蓝光激光整个系统具有结构紧凑、倍频效率高、运行稳定的特点.     

Noncollinear ultraviolet generation in a lithium borate crystal

Nd:YAG and a Nd:YAG-pumped dye laser are used to generate tunable deep ultraviolet radiation down to 240 nm in a lithium triborate crystal (LBO) by noncollinear sum-frequency mixing. All longer wavelengths can be generated by a combination of harmonic generation of the dye laser and sum-frequency mixing, 240 nm being the near noncritical limit. A set of versatile Sellmeier dispersion equations is derived to satisfactorily predict phase-matching in LBO.     

Generation of short-pulse VUV and XUV radiation

Starting from intense short-pulse KrF (248 nm, 25 mJ, 400 fs), ArF (193 nm, 10 mJ, 1 ps), and Ti:sapphire (810 nm, 100 mJ, 150 fs) laser systems, schemes for the generation of fixed-frequency and tunable VUV and XUV radiation by nonlinear optical techniques are investigated. With the KrF system, a four-wave mixing process in xenon yields tunable radiation in the range of 130–200 nm with output energies of, so far, 100 J in less than 1 ps. For the XUV spectral range below 100 nm, nonperturbative high-order harmonic generation and frequency mixing processes in noble gas jets are considered. To achieve tunability, the intense fixed-frequency pump laser radiation is mixed with less intense but broadly tunable radiation from short-pulse dye lasers or optical parametric generator-amplifier systems. In this way, tunability down to wavelengths of less than 40 nm has been demonstrated.     

All-solid-state continuous-wave frequency-doubled Nd:YAG-BiBO laser with 2.8-W output power at 473 nm

We report on a diode-pumped Nd:YAG laser with 4.6 W of linear polarized continuous-wave (cw) output power on the 4F3/2 --> 4I9/2 transitions at 946 nm. Three different crystals, cut for critical type I phase matching at room temperature, are used for the intracavity frequency doubling of the laser: 10-mm-long LiBaO5 (LBO), an 8-mm-long beta-BaB2O4 (BBO), and a 10.4-mm-long BiB3O6 (BiBO) grown by FEE GmbH. Up to 2.8 W of cw output power in the blue spectral range at 473 nm has been achieved with the BiBO crystal (2.1 W with BBO and 1.5 W with LBO).     

在BBO中产生217.3-2 21.4nm高功率和频输出

用Q-YAG激光的三次谐波(355nm)与调谐的Rh·6G染料激光在β-BaB2O4(BBO)晶体中和频,获得217.3～221.4nm连续调谐输出,和频输出的最大能量为250μJ,转换效率为11%.我们还讨论了获取最大和频输出能量的一些实验条件.