类镍等电子系列离子M1,M2,E2禁戒跃迁特性的理论研究

利用基于全相对论框架下的多组态Dirac-Fock理论方法发展起来的程序包GRASP92和新发展的处理辐射跃迁过程的程序REOS99，计算了类镍等电子系列离子(Z=45—95)的基组态3s²3p⁶3d¹⁰¹S₀以及低激发组态3s²3p⁶3d⁹4l,3s²3p⁵3d¹⁰4l和3s3p⁶3d¹⁰4l(l=s,p,d,f)的能级及其向基态的M1,M2,E2禁戒跃迁概率.通过分析高离化类镍离子在特定的原子序数范围内由于存在能级交叉而产生的强组态相互作用，解释了高离化类镍离子禁戒跃迁概率的反常变化现象，探讨了禁戒跃迁概率受强组态相互作用影响而变化的一般规律.     

New cross-section measurements for the (n, 2n), (n, p), and (n, α) reactions on bromine in the 14 MeV region with detailed uncertainty quantification

Measurement of the cross-sections of the ⁷⁹Br(n, 2n)⁷⁸Br, ⁸¹Br(n, p)^81mSe, ⁸¹Br(n, α)⁷⁸As, and ⁷⁹Br(n, α)⁷⁶As reactions was performed at specific neutron energies, precisely, 13.5±0.2, 14.1±0.2, 14.4±0.2, and 14.8±0.2 MeV, relative to the standard ⁹³Nb(n, 2n)^92mNb and ²⁷Al(n, α)²⁴Na reference reactions using offline γ-ray spectrometry and neutron activation. Monoenergetic neutrons were generated at the China Academy of Engineering Physics via a ³H(d, n)⁴He reaction using the K-400 Neutron Generator equipped with a solid ³H-Ti based target. The activity of the reaction produce was obtained using a high-purity germanium detector. The cross-sections of the (n, 2n), (n, p), and (n, α) reactions on the bromine isotopes were measured in the 13–15 MeV neutron energy range. The covariance analysis approach was employed for a thorough inspection of any uncertainties within the measured cross-section data. A discussion and comparison of the observed outcome were carried out with previously published data, especially with the results of the JENDL-4.0, JEFF-3.3, TENDL-2019, and ENDF/B-VIII.0 data libraries, along with the theoretical excitation function curve derived by employing the TALYS-1.95 program. Improved cross-section restrictions for the investigated processes in the 13–15 MeV neutron energy range will be obtained using the current findings, which will help to raise the caliber of associated databases. Furthermore, the parameters of relevant nuclear reaction models can be verified using this data.     

The p/π ratio pT dependence in the RHIC range of baryo-chemical potential

The BRAHMS measurement of proton-to-pion ratios in Au+Au and p+p collisions at $ \sqrt {s_{NN} } $ \sqrt {s_{NN} } = 62.4 GeV and $ \sqrt {s_{NN} } $ \sqrt {s_{NN} } = 200 GeV is presented as a function of transverse momentum and collision centrality within the pseudorapidity range 0 ≤ η ≤ 3. The baryo-chemical potential, μ _B , for the indicated data spans from μ _B ≈ 26 MeV ($ \sqrt {s_{NN} } $ \sqrt {s_{NN} } 200 GeV, η ≈ 0) to μ _B ∼ 260 MeV ($ \sqrt {s_{NN} } $ \sqrt {s_{NN} } = 62.4 GeV, η ≈ 3) [1]. The p/πratio measured for Au+Au system at $ \sqrt {s_{NN} } $ \sqrt {s_{NN} } 62.4 GeV, η ≈ 3 reaches astounding value of 8–10 at p _T > 1.5 GeV/c. For these energy and pseudorapidity interval no centrality dependency of p/π ratio is observed. Moreover, the baryon-to-meson ratio of nucleus-nucleus data are consistent with results obtained for p+p interactions.     

Structure and M?ssbauer studies of manganese monosulfide solid solutions MxMn1 ? xS (M = Cr, Fe)

This paper reports on the results of the synthesis and study of the diffraction patterns and M?ssbauer spectra of single crystals of homogeneous M xMn_{1 − x} S solid solutions with a cubic NaCl structure prepared by the cation substitution of 3d elements for divalent manganese ions in manganese monosulfide. It has been shown that, similarly to the hydrostatic pressure, the substitution of 3d ions with a smaller ionic radius is accompanied by the contraction of the MnS cubic cell. The calculated lattice parameters agree with the experimental data. The homogeneous region of the formation of homogeneous solid solutions is limited in composition x, which depends on the choice of a substitutional cation.     

General SU(2)L × SU(2)R × U(1)EM Sigma Model with External Sources, Dynamical Breaking and Spontaneous Vacuum Symmetry Breaking

We give a general SU(2) _L × SU(2) _R × U(1) _EM sigma model with external sources, dynamical breaking and spontaneous vacuum symmetry breaking, and present the general formulation of the model. It is found that σ and π⁰ without electric charges have electromagnetic interaction effects coming from their internal structures. A general Lorentz transformation relative to external sources is derived, using the general Lorentz transformation and the four-dimensional current of nuclear matter of the ground state with J _gauge = 0, we give the four-dimensional general relations between the different currents of nuclear matter systems with J _gauge≠ 0 and those with J _gauge = 0. The relation of the density’s coupling with external magnetic field is derived, which conforms well to dense nuclear matter in a strong magnetic field. We show different condensed effects in strong interaction about fermions and antifermions, and give the concrete scalar and pseudoscalar condensed expressions of σ₀ and π₀ bosons. About different dynamical breaking and spontaneous vacuum symmetry breaking, the concrete expressions of different mass spectra are obtained in field theory. This paper acquires the running spontaneous vacuum breaking value σ′₀, and obtains the spontaneous vacuum breaking in terms of the running σ′₀, which make nucleon, σ and π particles gain effective masses. We achieve both the effect of external sources and nonvanishing value of the condensed scalar and pseudoscalar paticles. It is deduced that the masses of nucleons, σ and π generally depend on different external sources. PACA numbers: 24.10.-i, 11.30.Qc     

Transition probabilities for two-photon H(1s–2s) and He(11s–21s) transitions: A partial-closure approach

Transition amplitudes and transition probabilities for the two-photon 1s–2s transition in the hydrogen atom and 1¹ s–2¹ s transition in helium atom have been calculated using a partial-closure approach. The dominant term is calculated exactly and the remaining sum over intermediate states is calculated using a mean excitation energy. Our value of the transition amplitudes agree within 2% with the exact results for the hydrogen case. Our value of the transition probability for hydrogen is 8.50 s⁻¹ which is in good accord with its known value 8.226 s⁻¹. For helium, the photon energy distribution of the metastable 2¹ s state is in good agreement with the accurate values. The corresponding transition probability is 53.7 s⁻¹ which is in good agreement with the accurate value 51.3 s⁻¹.     

AlxOy(x=1—2,y=1—3)分子几何结构与稳定性的DFT研究

用密度泛函理论(DFT)的B31yp方法在6-311++g^水平上对Al_xO_y(x=1—2,y=2—3)分子的几何构型、电子结构、振动频率等性质进行了理论研究. 通过对基态结构的几何参数分析发现，它们的基态结构趋于直线或平面结构. 对基态结构的绝热电离能讨论表明，金属铝原子数一定时，氧原子数从1增加到3，其气态分子越来越稳定，铝原子数少的分子体系更稳定. 系统给出了该系列分子基态的几何参数、电子结构、光谱性质. Al₂O₃的C_2V三重态是该分子的能量最低结构. 关键词： xO_y分子')" href="#">Al_xO_y分子 密度泛函理论 结构与稳定性     

Structure and analytical potential energy function for the ground state of the BCx (x=0, －1)

In this paper, the electronic states of the ground states and dissociation limits of BC and BC- are correctly determined based on group theory and atomic and molecular reaction statics. The equilibrium geometries, harmonic frequencies and dissociation energies of the ground state of BC and BC- are calculated by using density function theory and quadratic CI method including single and double substitutions. The analytical potential energy functions of these states have been fitted with Murrell-Sorbie potential energy function from our ab initio calculation results. The spectroscopic data （αe, ωe and ωeχe） of each state is calculated via the relation between analytical potential energy function and spectroscopic data. All the calculations are in good agreement with the experimental data.     

Determination of the probability of existence of pair interactions in the formation of M2tX2t?1Superstructures in MXy nonstoichiometric compounds

An analytical method has been proposed for calculating the probabilities P _i ^(2)(s) of existence of X-X, X−□, and □−□ pair interactions in the nonmetal sublattice of M _2tX_2t−1 superstructures formed in strongly nonstoichiometric compounds MX _y (MX _y □_1−y) and M ₂X _y (MX_y/2□_1−y/2) with a high content of structural vacancies □. The main characteristics necessary for the quantitative determination of the probabilities P_i(2)(s) as functions of the composition, degree of long-range order, symmetry, and structure type have been determined for all the known superstructures M _2tX_2t−1.     

Eu3+在M3La2(BO3)4(M=Ca,Sr,Ba)中的发光性质

本文报导了M3La2(BO3)4:Eu3+(M=Ca,Sr,Ba)磷光体的制备方法及晶体结构。三种磷光体均属正交晶系。研究了Eu3+离子的光谱特征与基质化合物的关系。发现在三种磷光体中,被Eu3+所取代的La3+离子均只有一种格位,且在此格位上不具备反演操作的对称性;Eu3+在Ca3La2(BO3)4:Eu3+中所处格位的局部对称性最低,属C1,C2和Cs中之一种,在M3La2(BO3)4:Eu3+(M=Sr,Ba)中Eu3+所处格位的局部对称性可能为C2v。     

One-loop formulas for H → Zνlνl for l = e, μ, τ in 't Hooft-Veltman gauge

In this paper, we present analytical results for one-loop contributions to the decay processes \begin{document}$ H\rightarrow Z \nu_l\bar{\nu}_l $\end{document} (for \begin{document}$ l = e, \mu, \tau $\end{document}). The calculations are performed within the Standard Model framework in the 't Hooft-Veltman gauge. One-loop form factors are then written in terms of scalar one-loop functions in the standard notations of \begin{document}$ {\tt LoopTools}$\end{document}. As a result, one-loop decay rates for the decay channels can be evaluated numerically by using the package. Furthermore, we analyze the signals of \begin{document}$ H\rightarrow Z \nu_l\bar{\nu}_l $\end{document} via the production processes \begin{document}$ e^-e^+ \rightarrow ZH^* \rightarrow Z (H^* \rightarrow Z \nu_l\bar{\nu}_l) $\end{document}, including the initial beam polarizations at future lepton colliders. The Standard Model backgrounds, such as the processes \begin{document}$ e^-e^+ \rightarrow \nu_l\bar{\nu}_l ZZ $\end{document}, are also examined in this study. Numerical results indicate that one-loop corrections make contributions of approximately 10% to the decay rates. These are sizeable contributions and should be taken into account at future colliders. We show that the signals \begin{document}$ H\rightarrow Z\nu_l\bar{\nu}_l $\end{document} are clearly visible at the center-of-mass energy \begin{document}$ \sqrt{s}=250 $\end{document} GeV and are difficult to probe in higher-energy regions owing to the dominant backgrounds.     

The absorption spectrum of the (1, 0), (3, 1) and (4, 2) bands in the cΣg–aΣu system of He2 eximer

The near-infrared absorption spectrum of He₂ has been recorded in the range of 12 090–13 300 cm⁻¹ using the optical heterodyne concentration modulation spectroscopy. Fifty-nine He₂ spectral lines were assigned to the (1, 0), (2, 0), (3, 1) and (4, 2) bands in the c³Σ_g⁺–a³Σ_u⁺ system and a non-linear least-squares fitting was performed to get the improved molecular constants for the levels (υ = 1, 3 and 4) in the upper electronic state.     

The Ratio Rdp of the quasielastic nd → p(nn) to the elastic np → pn charge-exchange-process yields at the proton emitting angle θp,lab = 0° over 0.55–2.0 GeV neutron-beam energy region. Comparison of the results with the model-dependent calculations

Our new experimental results (see, e.g., Preprint JINR no. E1-2008-61 (Dubna, 2008)) on ratio R _dp of the quasielastic charge-exchange yield at the proton emitting angle θ _p,lab = 0° for the nd → p(nn) reaction to the elastic np → pn charge-exchange yield were presented. The measurements were carried out at the Nuclotron of the Veksler and Baldin Laboratory of High Energies of the JINR (Dubna) at the neutron-beam kinetic energies of 0.55, 0.8, 1.0, 1.2, 1.4, 1.8, and 2.0 GeV. In this paper the comparison of the experimental R _dp data with the obtained R _dp calculations within the impulse approximation by using the invariant-amplitude sets from the GW/VPI phase-shift analysis is made. The R _dp values calculated using the set of invariant amplitude data for the elastic np → pn charge exchange at θ _p,CM = 0°, agree with the experimental data. This confirmed the nd → p(nn) process yield at θ _p,CM = 0° is caused by the contribution of the spin-dependent part of the elastic np → pn charge-exchange reaction. Thus, it has been shown that the obtained experimental R _dp results can be used for the Delta-Sigma experimental program to reduce the total ambiguity in the extraction of the amplitude real parts. The text was submitted by the authors in English.     

(G′/G)展开法和(2+1)维非对称Nizhnik-Novikov-Veselov系统的新精确解

通过引入并扩展 （G′/G）展开法, 构造出（2+1）维非对称Nizhnik-Novikov-Veselov系统的三种形式的新精确通解: 双曲函数通解, 三角函数通解, 有理函数通解. 当双曲函数通解中的常数取特定值时, 通解变为相应孤立波解. 关键词： G′/G）展开法')" href="#">（G′/G）展开法 （2+1）维非对称Nizhnik-Novikov-Veselov系统 精确解 孤立波解     

Mo,Ta, W在NixAl1-x(x=0.25,0.5,0.75) 中的择优占位

用多体势结合分子动力学计算了L1₂型NiAl₃, L1₂型Ni₃Al, L1₀型NiAl和B₂ 型NiAl的晶格常数, 结合能以及合金形成热; 分析了结构性点缺陷在上述四种合金中的存在形式; 在此基础上研究了合金化元素Mo, Ta, W在Ni_xAl_1-x(x=0.25,0.5,0.75)中的择优占位行为. 计算结果表明: 对于四种结构的Ni-Al合金, 偏离理想化学配比时,主要的结构缺陷形式是反位置; 根据占位能最小化, 第三组元元素Mo, Ta, W在上述四种Ni-Al中都显著优先占据Al格位. 关键词： 多体势 Ni-Al合金 占位     

Electrical conductivity and magnetic properties of La1 ? xCaxMn1 ? yFeyO3 ceramic samples (x = 0.67, y = 0, 0.05)

The temperature dependences of the magnetic susceptibility χ(T) and the electrical resistivity ρ(T) of ceramic samples of La_{1 − x} Ca _x MnO₃ with x = 0.67 (LCMO) and La_{1 − x} Ca _x Mn_{1 − y} Fe _y O₃ with x = 0.67 and y = 0.05 (LCMFO) are investigated in magnetic fields B = 50–10⁵ G and the temperature range T = 4.2–400 K. Both samples undergo a transition from the paramagnetic state to a state with charge (orbital) ordering (CO) at temperatures T _CO ≈ 272 K for LCMO and T _CO ≈ 222 K for LCMFO. The behavior of the paramagnetic phase in the temperature range 320–400 K for LCMO and 260–400 K for LCMFO is described by the Curie-Weiss law with effective Bohr magneton numbers p _eff = 4.83 μ_B (LCMO) and 4.77 μ_B (LCMFO), respectively. The disagreement between the observed positive Weiss temperatures (θ ≈ 175 K (LCMO) and θ ≈ 134 K (LCMFO)) and negative Weiss temperatures required for the antiferromagnetic ground state can be explained by the phase separation and transition to the charge-ordered state. The magnetic irreversibility for T < T _CO is accounted for by the existence of a mixture of the ferromagnetic and antiferromagnetic phases, as well as the cluster glass phase. At low temperatures, doping with iron enhances the frustration of the system, which manifests itself in a more regular behavior of the decay rate of the remanent magnetization with time. The temperature dependence of the electrical resistivity in the range of the charge-ordered phase conforms to the variable-range hopping model. The behavior of the electrical resistivity is governed by the complex structure of the density of localized states near the Fermi level, which includes a soft Coulomb gap Δ = 0.464 eV for LCMO and 0.446 eV for LCMFO. It is established that the ratio between the localization radii of charge carriers a for LCMFO and a _und for LCMO is a/a _und = 0.88. Original Russian Text ? V.S. Zakhvalinskiĭ, R. Laiho, T.S. Orlova, A.V. Khokhulin, 2008, published in Fizika Tverdogo Tela, 2008, Vol. 50, No. 1, pp. 61–68.     

The Second-Order Equation from the (1/2, 0) ⊕ (0, 1/2) Representation of the Poincare Group

On the basis of first principles we derive theBarut-Wilson-Fushchich secondorder equation in the (1/2,0) (0, 1/2) representation. Then we discuss thepossibility of describing various mass and spin states in such a framework.     

Magnetic properties of complex oxides Ba6Ni5 ? xMnxO15 (x = 2, 3, 4) of the A3n + 3mA′nB3m + nO9m + 6n family

The magnetic interactions in the quasi-one-dimensional complex oxides Ba₆NiMn₄O₁₅, Ba₆Ni₂Mn₃O₁₅, and Ba₆Ni₃Mn₂O₁₅ have been investigated using electron paramagnetic resonance and magnetic susceptibility measurements. It has been revealed that, for the Ba₆Ni₂Mn₃O₁₅ and Ba₆Ni₃Mn₂O₁₅ compounds, the magnetic moments are considerably smaller than the theoretical values and depend on the temperature. The results obtained have been interpreted under the assumption that the structure contains Ni³⁺ ions in which the energy level structure can lead to the above anomalies.     

Emission centers in Ca1–xPrxF2+x (x = 0.35) solid solutions

Luminescence spectra of Ca_0.65Pr_0.35F_2.35 solid solutions are studied. It is found that, depending on the excitation energy, different kinds of emission centers appear in these spectra. An interconfigurational 4f ¹5d¹ →4f² luminescence is typical for single Pr³⁺ ions in tetragonal sites. Data on the structure of the solid solutions show that the emission centers involved in ¹S₀ → 4f² transitions can be attributed to Pr³⁺ ions contained in clusters.     

Anomalous enhancement of the thermoelectric power in gallium-doped p-(Bi1 ? xSbx)2Te3 single crystals

The effect of gallium on the temperature dependences (5 K ≤ T ≤ 300 K) of Seebeck coefficient α, electrical conductivity σ, thermal conductivity k, and thermoelectric efficiency Z of mixed p-(Bi_0.5Sb_0.5)₂Te₃ semiconductor single crystals is studied. The hole concentration decreases upon gallium doping; that is, gallium causes a donor effect. The Seebeck coefficient increases anomalously, i.e., much higher than it should be at the detected decrease in the hole concentration. This leads to an enhancement of the thermoelectric power. The observed changes in the Seebeck coefficient indicate a noticeable gallium-induced change in the density of states in the valence band.