Hyper-Raman scattering in the LiNbO3 crystal

The hyper-Raman spectra in non-centrosvmmetric LiNbO₃ crystal were obtained using the multichannel recording technique. The hyper-Raman cross-section and non-linear susceptibility for the 151 cm^-1 band were measured.     

Nonvolatile hologram storage properties of tri-doped Zn:Ce:Cu:LiNbO3 crystals

Congruent Zn(7 mol%):Ce:Cu:LiNbO₃ single crystal was grown by the Czochralski method in air. The occupation mechanism of the Zn²⁺ was discussed by an infrared transmittance spectrum. The nonvolatile holographic recording in Zn(7 mol%):Ce:Cu:LiNbO₃ single crystal was measured by two-photon fixed method. Zn(7 mol%):Ce:Cu:LiNbO₃ single crystals present the faster recording time and higher light-induced scattering resistance ability comparing with Ce:Cu:LiNbO₃ single crystals.     

One-dimensional steady-state bright photovoltaic solitons in LiNbO3:Fe crystal with background illumination

We investigate theoretically and experimentally one-dimensional bright photovoltaic solitons in LiNbO₃:Fe crystal by use of the background illumination. We find that, in LiNbO₃:Fe crystal, bright photovoltaic solitons can be obtained with background illumination for κ>1, where κ is the ratio of the background illumination photovoltaic constant to the soliton optical beam's photovoltaic constant. For κ<1, dark photovoltaic solitons are generated. On the other hand, our experiments show good agreement with theoretical prediction for the soliton existence curve in a special intensity ratio.     

Lateral-field-excitation properties of LiNbO3 single crystal

LiNbO 3 has been found attractive for lateral field excitation (LFE) applications due to its high piezoelectric coupling. In this paper, bulk acoustic wave propagation properties for LiNbO 3 single crystal excited by a lateral electric field have been investigated using the extended Christoffel-Bechmann method. It is found that the LFE piezoelectric coupling factor for c mode reaches its maximum value of 95.46% when ψ = 0 for both (yxl)-58 and (yxwl)±60 /58 LiNbO 3 . The acoustic wave phase velocity of c mode TSM (thickness shear mode) changes from 3456 m/s to 3983 m/s as a function of ψ. Here ψ represents the angle between the lateral electric field and the crystallographic X-axis in the substrate major surface. A 5 MHz LFE device of (yxl)-58 LiNbO 3 with ψ = 0 was designed and tested in air. A major resonance peak was observed with the motional resistance as low as 17 and the Q-factor value up to 10353. The test result is well in agreement with the theoretical analysis, and suggests that the LFE LiNbO 3 device can be a good platform for high performance resonator or sensor applications.     

LiNbO3晶体中屏蔽光伏孤子自偏转的 时空演化与可控因素

基于带输运模型理论建立了 LiNbO₃ 晶体屏蔽光伏孤子的时空演化动力学方程, 用有限差分方法求解发现, LiNbO₃ 晶体中明、暗屏蔽光伏孤子存在大的自偏转, 并且光孤子形状变得具有不对称性, 偏转方向的曲线斜率绝对值变大, 偏转反方向的曲线斜率绝对值变小. 分析研究表明影响其自偏转度和形变的因素包括受主浓度 N_A, 暗辐射强度 I_d 和外加电场 E₀ . 其他条件不变的情况下N_A 越大, 明孤子的自偏转度与形变越小, 暗孤子的自偏转度与形变反而越大; 对于 I_d , 它对明暗孤子的影响是相同的, I_d 越小, 晶体里诱导出的空间电荷场越容易达到饱和, 当信号光中心光强与暗辐射强度之比为 10^-1时无饱和现象产生; 随着 E₀ 数值的增大, 明孤子的自偏转度和形变减小, 而暗孤子的自偏转度和形变反而增大.     

Application of interference microscopy to the study of hologram build-up in LiNbO3 crystals

Interference microscopy was applied to direct microscopic observation of temporal evolution of phase holograms in LiNbO₃:Fe photorefractive crystals. First a hologram was recorded in the sample, and diffraction efficiency was monitored during hologram build-up using inactinic laser light. Thus kinetics of hologram build-up could be determined. The initial hologram was erased using white light. Then a series of write-erase cycles were performed with increasing exposure times. Holograms were observed by interference microscope after each exposure. The time elapsed between the exposure and the microscopic observation was negligible compared to the relaxation time of the hologram. The obtained temporal evolution of the grating profile gives a deeper insight into the physical mechanism of hologram formation in photorefractive materials than simple diffraction efficiency measurements. A congruently grown sample of LiNbO₃ doped with 10⁻³ mol/mol Fe in melting was studied by this method. Sample thickness was set to 300 μm to allow correct microscopic observation. Plane-wave holograms were recorded in the samples using an Ar-ion laser at λ = 488.0 nm of grating constants of 3, 6.5 and 8.8 μm.     

Defect structure and nonvolatile hologram storage properties in Hf:Fe:Mn:LiNbO3 crystals

A series of Hf:Fe:Mn:LiNbO₃ crystals with various levels of HfO₂ doping were grown by Czochralski technique. The infrared spectra and ultraviolet spectra were measured and discussed to investigate their structure and defects. The optical damage resistance was characterized by the transmitted beam pattern distortion method. The nonvolatile two-color holographic recording experimental results showed that the recording speed was faster with the increase of HfO₂ doping concentration and at the same time little loss of nonvolatile diffraction efficiencies could be achieved.     

二维LiNbO3非线性光子晶体

制备了周期为13.64 μm方形格子二维周期性极化的LiNbO₃，利用二阶准相位匹 配实现了波长为1.064μm二倍频，二次谐波的内部转换效率高达42％. 测量了二次谐波输出功率随晶体温度及入射光入射方向的变化，实验值与模拟计算一致. 制备二阶准相位匹配掩模板，解决了在制备一阶准相位匹配掩模板中遇到周期尺寸太小、数据量大的难题，同时还降低了因周期太小造成的极化难度. 关键词： 二维 准相位匹配 二次谐波     

光折变晶体LiNbO_3:Fe中的特殊散射现象

用柱面透镜把经针孔滤波器扩束的激光束沿某一个方向聚焦成细丝状(或长条状),细丝状光束垂直入射到LiNbO_3:Fe晶体上,在远场位置观察散射光.我们发现光散射的方向与晶体的c轴方向不一致,不仅沿着晶体的c轴方向有散射光出现,沿光束的条形方向也出现很强的散射光.     

Optical waveguide engraving in a LiNbO3 crystal fiber

This paper reports the engraving of an optical waveguide inside a LiNbO₃ crystal fiber via the photorefractive effect and an optical vortex. Afterwards this waveguide was successfully tested and its properties evidenced.     

Cu-diffused layers in LiNbO3 for reversible holographic storage

Some holographic recording characteristics of Cu-diffused layers fabricated in Rh-doped LiNbO₃ have been examined in comparison with those fabricated in undoped lithium niobate.The diffusion layers, whose thickness depends on the diffusion temperature, are found to be enormously susceptible to optically-induced refractive index changes and to be able to attain a high diffraction efficiency. A distinguished difference is found between the persistence of holograms stored in Rh-doped and undoped LiNbO₃.     

Investigation of nonvolatile holographic storage in LiNbO3:Mn:Ce:Fe crystal

We investigate the persistent holographic recording in triply doped LiNbO₃:Mn:Ce:Fe crystals at different oxidation/reduction states. The experimental results show that there is an optimum oxidation/reduction state, which results in the best dynamic range M/#. Compared with doubly doped LiNbO₃:Ce:Fe, we found that the nonvolatile diffraction efficiency and the best dynamic range M/# obtained in triply doped samples are larger than that obtained in doubly doped samples. The reason for the increase of the crystal about the nonvolatile diffraction efficiency and the dynamic range M/# was also explained.     

Improved nonvolatile holographic storage sensitivity of near-stoichiometric LiNbO3:Fe:Mn crystals

We investigate the nonvolatile holographic storage characteristics of near-stoichiometric LiNbO3 :Fe:Mn crystals with different Li2O contents. Experimental results indicate that the optimal value of Li2O content is about 49.6 mol%. Nonvolatile sensitivity S considerably improved to 0.15 cm/J because of the use of near-stoichiometric LiNbO3 :Fe:Mn with 49.6 mol% Li2O.     

Transient energy transfer during hologram formation in LiNbO3 in external electric field

Volume phase hologram recording in pure LiNbO₃ crystals with applied electric field E ≈ 5 kV/cm is accompanied by considerable intensity redistribution of the writing beams by transient energy transfer. Practically the whole intensity of the donor beam may be transferred into the weak acceptor beam with initial intensity 3% from total incident intensity. This effect originates from transient phase mismatch of the recorded phase grating and fringe pattern in the applied electric field when the interacting beams have different intensities.     

Ultraviolet laser-induced photovoltaic effects in miscut ferroelectric LiNbO3 single crystals

This paper investigates the photovoltaic properties of miscut LiNbO 3 single crystal with different thicknesses under irradiation of a 248 nm ultraviolet laser pulse with 20 ns duration without an applied bias.Nanosecond photovoltaic response is observed and faster rise time is obtained in thinner samples.In accord with the 248 nm laser duration,the full width at half maximum of the photovoltaic signals keeps a constant of ～ 20 ns.With decrease of the crystal thickness,the photovoltaic sensitivity was improved rapidly at first and then decreased,and the maximum photovoltage occurred at 0.38 mm-thick single crystal.The present results demonstrate that decreasing the LiNbO3 single crystal thickness can obtain faster response time and improve the photovoltaic sensitivity.     

亮暗屏蔽光伏孤子在LiNbO3晶体中的大自偏转

用数值方法证实了亮、暗屏蔽光伏孤子在有外加电场的LiNbO₃晶体中都可以发生大自偏转,并验证了这种自偏转现象不但与晶体中受主浓度N_A有关而且还与外加电场E₀有关. 在E₀相同的条件下,N_A越小这种自偏转现象越明显,在N_A相同的条件下,E₀越大自偏转现象越明显. 还发现亮、暗屏蔽光伏孤子的自偏转现象不同：亮屏蔽光伏孤子整体都发生明显偏转,暗屏蔽光伏孤子的偏转只是发生在一侧,其极值位置和另一侧几乎不发生偏转. 关键词： 自偏转 空间孤子 光折变效应     

Electro-optic modulation analysis of a Y-cut Z-propagation LiNbO3 light modulator: Comparison with an X-cut Z-propagation LiNbO3 light modulator and a dual LiNbO3 crystal type modulator

We analyzed dependence of modulation characteristics on manufacturing errors for a Y-cut Z-propagation (YZ) and an X-cut Z-propagation (XZ) LiNbO₃ (LN) crystal light modulators. We investigated that the modulation of the YZ modulator is hardly affected by small rotation error of Z-axis, while the XZ modulator suffers significant influence. We also analyzed temperature characteristics of modulation of conventional temperature-compensation LN light modulator. These numerical results show that the modulated signal change of the YZ modulator due to temperature variance is not more than 2.5% of that of the temperature-compensation modulator, in the presence of applied electric field of integral times of the half-wave voltage, modulated signal of the YZ modulator is almost independent on the temperature.     

Spectroscopic analysis of Er transition in Mg/Er-codoped LiNbO3 crystal

We present a Judd-Ofelt spectroscopic analysis on the Mg/Er-codoped congruent lithium niobate (LiNbO₃) crystals. The Judd-Ofelt model is applied to the room temperature unpolarized absorption intensities of Er³⁺ ions on eleven transition bands to determine their intensity parameters: Ω₂=2.36×10⁻²⁰ cm², Ω₄=0.76×10⁻²⁰ cm², Ω₆=0.30×10⁻²⁰ cm² in Er:LiNbO₃ crystal heavily codoped with MgO. The radiative lifetime of ²H_9/2 becomes longer when MgO is added into Er:LiNbO₃ crystal. The experimental lifetimes are obtained using microsecond time-resolved spectra at 400 nm femtosecond pulse excitation to predict radiative quantum efficiency. Combining higher radiative quantum efficiency with longer radiative lifetime, we conclude that Mg/Er-codoped LiNbO₃ crystals are more suitable than Er: LiNbO₃ ones in laser materials.     

Effect of the parameters on diffraction efficiency after thermal fixing for reflection geometry hologram storage in LiNbO3:Fe

For reflection geometry hologram storage in LiNbO₃:Fe, we have shown that the diffraction efficiency increases with doping level and thickness of storage material monotonically. When the acute angle between reference and z-axis is large enough for getting a relative small Bragg angle that is needed for angle multiplexing, smaller angle does good to diffraction efficiency after thermal fixing. And for absorption coefficient, there is an appropriate value responding to optimal diffraction efficiency after thermal fixing and we develop a theoretical model that predicts achievable diffraction efficiency after thermal fixing as a function of crystal thickness, doping level, acute angle between reference and z-axis and absorption coefficient. We compare this model with experiment results and get a good agreement.