Intersubband excitations in single-and double-layer electron systems in a parallel magnetic field

The spectrum of neutral intersubband excitations in single and double quantum wells has been studied by the inelastic light scattering method. It is shown that excitation energies in an external magnetic field have an anisotropic component proportional to the dipole moment of excitations along the growth axis of the quantum wells. Consequently, the measurement of excitation energy in a magnetic field makes it possible to experimentally estimate the quantitative measure of asymmetry of the quantum wells (dipole moment of the intersubband transition). In addition, a parallel magnetic field makes it possible to considerably extend the range of momenta studied since it shifts the dispersion curves in the momentum space by the value of the anisotropic component. A new method is proposed for determining the symmetry of double quantum wells. In asymmetric wells, intersubband excitations appear between the layers and have a large dipole moment along the growth axis. In symmetric wells, the magnetic field itself induces the dipole moment of intersubband excitations so that the excitation spectrum does not change upon magnetic field inversion. Analysis of energy anisotropy in intersubband excitations in double quantum wells makes it possible to determine the symmetry of double wells to a high degree of accuracy.     

Minigap plasmons in a two-dimensional electron gas subjected to a one-dimensional periodic potential

We investigate the plasmon excitations in a two-dimensional electron gas subjected to a one-dimensional weak periodic potential. We derive and discuss the dispersion relations for both intrasubband and intersubband excitations within the framework of Bohm-Pines' random-phase approximation. For such an anisotropic system with spatially modulated charge density, we observe a splitting of the 2D plasmon dispersion. The splitting is caused by the superlattice effect of the charge-density modulation on the collective excitation spectrum. We also discuss how the tunneling and the potential amplitude affect the plasmon excitations.     

Many-body effects on intersubband resonances in narrow InAs/AlSb quantum wells

Intersubband polarization couples to collective excitations of the interacting electron gas confined in a semiconductor quantum well (QW) structure. Such excitations include correlated pair excitations (repellons) and intersubband plasmons. The oscillator strength of intersubband resonances (ISBRs) strongly varies with QW parameters and electron density because of this coupling. Using the intersubband semiconductor Bloch equations for a two-conduction-subband model, we show that intersubband absorption spectra for narrow wells are dominated by the Fermi-edge singularity (via coupling to repellons) when the electron gas becomes degenerate and in the presence of large nonparabolicity. Thus the resonance peak position appears at the Fermi edge and the peak is greatly narrowed, enhanced, and red shifted as compared to the free particle result. Our results uncover a new perspective for ISBRs and indicate the necessity of proper many-body theoretical treatment in order for modeling and prediction of ISBR line shape.     

Intersubband spectroscopy of two dimensional electron gases: Coulomb interactions

We have made a direct determination of resonant screening (the depolarization field effect) in the collective intersubband excitations of a dense two dimensional electron gas. The effect was observed, for both odd and even parity transitions, in polarized inelastic light scattering spectra of a modulation-doped GaAs-AlGaAs superlattice. We offer a quantitative interpretation in terms of the Coulomb matrix elements for the transitions. Final state, or exciton-like, many-body effects are considered briefly.     

FTIR-spectroscopy of (GaAS)n/(AlAs)m superlattices

The optical properties of (GaAs)_n/(AlAs)_m superlattices in the infra-red spectral region have been studied. The confinement of optical phonons has been observed in both GaAs and AlAs layers of superlattices under investigation. The superlattice modes caused by the coupling between LO phonons and collective intersubband excitations have been found in doped superlattices. Macroscopic and microscopic calculations have been used for the analysis of experimental results. Good agreement with experiment has been obtained.     

Intersubband transport in quantum wells in strong magnetic fields mediated by single- and two-electron scattering

We show theoretically that in quantum wells subjected to a strong magnetic field the intersubband current peaks at magnetic field values, which reveal the underlying specific intersubband scattering mechanism. We have designed and grown a superlattice structure in which such current oscillations are clearly visible, and in which the transition from the purely single-electron to the mixed single- and two-electron scattering regimes can be observed by tuning the applied voltage bias. The measurements were conducted in ultrahigh magnetic fields (up to 45 T) to obtain the full spectrum of the current oscillations.     

Intersubband radiation in weakly bound superlattice structures with wide quantum wells in a transverse electric field

Long-wavelength IR radiation was detected in a long-period superlattice with wide quantum wells under conditions of electrical injection of charge carriers into lower size-quantization subbands, which was explained by intersubband transitions. The detected radiation probably suggests that there is a strongly nonequilibrium carrier distribution in subbands, caused by the difference between scattering processes into lower subbands with and without involving optical phonons.     

Hyperentanglement source by intersubband two-photon emission from semiconductor quantum wells

We propose an efficient hyperentanglement source emitting photon pairs entangled in both energy and polarization. The compact electrically driven room-temperature source, based on intersubband two-photon emission from semiconductor quantum wells (QWs) exhibits pair generation rates several orders of magnitude higher than alternative conventional schemes. A theoretical formalism is derived for the calculation of photon pair generation spectra and rates. The results are presented for superlattice structures similar to quantum cascade lasers of GaAs/AlGaAs QWs emitting in the mid-IR and far-IR and for InN/AlN QW structures suitable for telecommunication wavelengths.     

Intersubband vs interband-light coupling in semiconductors

This paper presents a direct comparison and contrast of strong light coupling with either interband or intersubband excitations in semiconductors. The approach is based on analytical expressions obtained after a series of systematic approximations starting from Nonequilibrium Greens Functions and Semiconductor Bloch Equations. Numerical results for III–V quantum wells embedded in microcavities are presented.     

Intersubband collective excitations in a quasi-two-dimensional electron system in external magnetic field

The spectrum of collective excitations in a quasi-two-dimensional electron system was studied by the method of Raman scattering spectroscopy. In an applied magnetic field, such systems exhibit collective excitations related to the electron transitions between dimensionally quantized subbands with a change in the Landau level index (intersubband Bernstein modes). It is shown that these modes interact with the fundamental intersubband excitations of the charge and spin densities, the interaction energy being determined by the excitation quasimomentum. Interaction of the intersubband Bernstein modes and the fundamental intersubband excitations with quasi-two-dimensional LO phonons was studied. Behavior of the new branches of collective excitations in a quasi-two-dimensional electron system possessing more than one occupied Landau level was studied and the nature of these branches was determined.     

Two-electron linear intersubband light absorption in a biased quantum well

We point out a novel manifestation of many-body correlations in the linear optical response of electrons confined in a quantum well. Namely, we demonstrate that along with the conventional absorption peak at a frequency omega close to the intersubband energy delta, there exists an additional peak at frequency h omega approximately = 2delta. This new peak is solely due to electron-electron interactions, and can be understood as excitation of two electrons by a single photon. The actual peak line shape is comprised of a sharp feature, due to excitation of pairs of intersubband plasmons, on top of a broader band due to absorption by two single-particle excitations. The two-plasmon contribution allows us to infer intersubband plasmon dispersion from linear absorption experiments.     

Plasmons in a free-standing nanorod with a two-dimensional parabolic quantum well caused by surface states

The collective charge density excitations in a free-standing nanorod with a two-dimensional parabolic quantum well are investigated within the framework of Bohm-Pine’s random-phase approximation in the two-subband model.The new simplified analytical expressions of the Coulomb interaction matrix elements and dielectric functions are derived and numerically discussed.In addition,the electron density and temperature dependences of dispersion features are also investigated.We find that in the two-dimensional parabolic quantum well,the intrasubband upper branch is coupled with the intersubband mode,which is quite different from other quasi-one-dimensional systems like a cylindrical quantum wire with an infinite rectangular potential.In addition,we also find that higher temperature results in the intersubband mode(with an energy of 12 meV(～ 3 THz)) becoming totally damped,which agrees well with the experimental results of Raman scattering in the literature.These interesting properties may provide useful references to the design of free-standing nanorod based devices.     

Plasmon modes of a superlattice — Classical vs quantum limits

The collective plasmon excitations of a superlattice are investigated in both the classical and quantum limits. Using a model that is applicable to superlattices whose constituent layers are either semiconductor- semiconductor, semiconductor-metal, or metal-metal, we show that the surface plasmon interface modes of each layer (slab) couple via the long range Coulomb interaction into two bands of plasmons with dispersion along the superlattice axis. Results for plasmon dispersion are presented for the classical limit (de Broglie wavelength less than the layer width) where the response is treated via a solution of Maxwell's equations using the bulk 3-D dielectric constant to describe each intervening layer. These results are compared to the plasmon dispersion in the quantum regime where the wave-vector frequency dependent dielectric constant of the superlattice is calculated taking into account quantization effects (subband structure). The relationship between the modes in both limits is derived.     

Femtosecond mid-infrared spectroscopy of low-energy excitations in solids

Recent progress in the generation and spectroscopic application of femtosecond pulses in the wavelength range between 3 and 25 m has led to new insight into low-energy excitations of solids, in particular semiconductors, semiconductor nanostructures, and high-T_C superconductors. The ultrafast nonequilibrium dynamics of such excitations has been observed in real-time and the underlying microscopic interactions have been analyzed. This article gives a brief overview of this exciting field of ultrafast science with the main emphasis on pulse generation and applications in semiconductor research where femtosecond intersubband Rabi flopping in quantum wells and quantum coherent electron transport in quantum cascade devices have been observed. PACS 78.67.De; 73.21.Fg; 07.57.Hm; 42.65.Re     

半导体超晶格子带间跃迁光吸收理论研究

从理论上研究了半导体超晶格子带间跃迁的光吸收性质,以GaAs/AlxGa1－xAs超晶格为例进行数值计算,分析了该材料的吸收系数随入射光光子能量、光场强度和超晶格结构参量（阱宽,垒宽,势垒高）的变化关系计算表明：随着入射光光子能量的变化,出现非对称的吸收峰;光强只改变吸收系数大小;超晶格结构参量会改变吸收谱的谱宽和吸收峰所对应的入射光频率随着超晶格阱宽（垒宽）的增大,吸收谱由宽变窄,吸收峰红移;随着超晶格Al组分变大,吸收谱变窄.     

Elementary excitations in multiple quantum wire structures

We calculate the plasmon dispersion of electrons in multiple quantum wire structures. Wave function overlapping effects between different wires are neglected. The Coulomb interaction potential is calculated for a model with circular wire area. Analytical results for the excitation spectrum of electron multiple quantum wire structures are obtained within an one-subband model. Landau damping of intrasubband plasmons is discussed. Results for an electron superlattice within a two-subband model are presented and the coupling of intersubband plasmons with intrasubband plasmons is calculated. We compare the theoretical results with recent Raman measurements of intrasubband plasmons in Al _x Ga_1–x As/GaAs wire superlattices. The plasmon dispersion for boson multiple quantum wire structures also is calculated.     

Ultrafast dynamic control of spin and charge density oscillations in a GaAs quantum well

We use subpicosecond laser pulses to generate and monitor in real time collective oscillations of electrons in a modulation-doped GaAs quantum well. The observed frequencies match those of intersubband spin- and charge-density excitations. Light couples to coherent density fluctuations through resonant stimulated Raman scattering. Because the spin- and charge-related modes obey different selection rules and resonant behavior, the amplitudes of the corresponding oscillations can be independently controlled by using shaped pulses of the proper polarization.     

Intersubband transitions in band gap engineered parabolic potential wells

Intersubband transitions in spike-inserted wide parabolic quantum wells are investigated. A thin potential barrier within the pure parabola devides the electron system in two well separated but strongly coupled layers, which in turn drastically changes the collective excitations scheme. In contrast to a pure parabolic quantum well where according to the generalised Kohn's Theorem only one fixed resonance is observed, the collective intersubband transitions recover the complex coupling and splitting scheme of the single particle states of a strongly coupled system. We interpret our experimental findings in terms of resonant tunnel processes and discuss them using simple model calculations.     

Intersubband lifetimes in InAs/GaSb superlattices using saturated absorption spectroscopy

We investigate intersubband relaxation rates above the optical phonon energy in a InAs/GaSb superlattice using saturation spectroscopy. A high-intensity free-electron laser tuned to the intersubband transition energy is used to saturate the absorption process revealing picosecond relaxation rates. The effects of the parallel magnetic field and laser energy on the relaxation processes are explored.     

Strong correlation of electronic and lattice excitations in GaAs/AlGaAs semiconductor quantum wells revealed by two-dimensional terahertz spectroscopy

Coulomb-mediated interactions between intersubband excitations of electrons in GaAs/AlGaAs double quantum wells and longitudinal optical phonons are studied by two-dimensional spectroscopy in the terahertz frequency range. The multitude of diagonal and off-diagonal peaks in the 2D spectrum gives evidence of strong polaronic signatures in the nonlinear response. A quantitative theoretical analysis reveals a dipole coupling of electrons to the polar lattice that is much stronger than in bulk GaAs, due to a dynamic localization of the electron wave function by scattering processes.