混沌介质光学常数测量

对基于漫射理论并应用CCD相机测量混沌介质的光学常数进行了实验研究.提出采用漫射中心环带约束法来提高逆向求解光学常数的精确性,以及采用在通过光的入射点和漫射中心的直线上截取一维原始数据的方法来提高算法的计算效率.以Intralipid脂肪乳剂作为混沌介质,对方法进行了实验验证.结果表明,本文提出的方法是可行的.     

Correlation characteristics of optical coherence tomography images of turbid media with statistically inhomogeneous optical parameters

Noisy structure of optical coherence tomography (OCT) images of turbid medium contains information about spatial variations of its optical parameters. We propose analytical model of statistical characteristics of OCT signal fluctuations from turbid medium with spatially inhomogeneous coefficients of absorption and backscattering. Analytically predicted correlation characteristics of OCT signal from spatially inhomogeneous medium are in good agreement with the results of correlation analysis of OCT images of different biological tissues. The proposed model can be efficiently applied for quantitative evaluation of statistical properties of absorption and backscattering fluctuations basing on correlation characteristics of OCT images.     

On the determination of molecular parameters for NO

All available high precision measurements on the ground state of NO have been used simultaneously in a weighted least squares procedure to determine the molecular parameters. In the present work the theoretical values were computed according to a model referred to as Hund's case (c_α), since this model seems to combine simplicity and high accuracy. The agreement between theoretical and observed frequencies is excellent and better than in previous investigations, even with a lower number of molecular parameters. Term values for NO are also computed, and they should be useful for predicting unobserved transitions.     

光电子材料光学参数的无损检测

利用消光式椭圆偏振光谱法 ,在室温下可见光区对光电子材料镓铟磷的光学参数进行了测量 ,得到该材料的折射率和吸收系数随光子能量的变化关系曲线 ,并对结果进行了分析和讨论 ,给出了镓铟磷带隙的位置     

Layer-number determination of two-dimensional materials by optical characterization

Initiated by graphene, two-dimensional(2D) layered materials have attracted much attention owing to their novel layer-number-dependent physical and chemical properties. To fully utilize those properties, a fast and accurate determination of their layer number is the priority. Compared with conventional structural characterization tools, including atomic force microscopy, scanning electron microscopy, and transmission electron microscopy, the optical characterization methods such as optical contrast, Raman spectroscopy, photoluminescence, multiphoton imaging, and hyperspectral imaging have the distinctive advantages of a high-throughput and nondestructive examination. Here, taking the most studied 2D materials like graphene, MoS_2, and black phosphorus as examples, we summarize the principles and applications of those optical characterization methods. The comparison of those methods may help us to select proper ones in a cost-effective way.     

Noncontact optical tomography of turbid media

Optical tomography of turbid media has so far been limited by systems that require fixed geometries or measurements employing fibers. We present a system that records noncontact optical measurements from diffuse media of arbitrary shapes and retrieves the three-dimensional surface information of the diffuse medium. We further present a novel method of combining this composite data set and obtain accurate fluorescence reconstructions. This approach offers significant experimental simplicity and yields high-information-content datasets. The performance of this novel tomographic approach is demonstrated with experimental reconstructions of phantoms.     

Sensitive solid-state optical sensible materials for photothermal determination of trace metals

Methods of photothermal (thermal-lens) determination of iron and mercury on the basis of solid polymer matrices with immobilized reagents are developed. These methods combine selective and efficient preconcentration of trace elements to be analyzed on a transparent polymer matrix, the sensitivity of determination with the reliable and traceable photometric procedures and highly sensitive thermal-lens detection (enhanced in polymers compared to solutions). The advantage of this approach is in the use of sensitive organic reagents previously developed for spectrophotometry. In this study, transparent polymethacrylate matrices modified with copper dithizonate and 1,10-phenanthroline were applied to the determination of mercury(II) and iron(II), respectively.     

Harmonic oscillator model and determination of optical parameters

The Lorentz dispersion theory and the Kramers-Kronig transformation were widely used to determine optical constants and oscillator parameters from reflectivity spectrum. Each range of data correspond to a different oscillation. Since the experimental data is in the limited range, this technique can be used to subtract information from unmeasured range. The inter-band optical properties in UV region have been investigated. Hydrogenated amorphous silicon nitride thin film was used as an example. The reflectivity spectrum of a-SiN_x:H was used to obtain the energy band gap in both standard and this technique. The measurement is in the UV-visible range. The optical energy gap value was found to be about for the sample illustrated, and these values are consistent for both techniques.     

Bifocal optical coherenc refractometry of turbid media

We propose and demonstrate a novel technique, which we term bifocal optical coherence refractometry, for the rapid determination of the refractive index of a turbid medium. The technique is based on the simultaneous creation of two closely spaced confocal gates in a sample. The optical path-length difference between the gates is measured by means of low-coherence interferometry and used to determine the refractive index. We present experimental results for the refractive indices of milk solutions and of human skin in vivo. As the axial scan rate determines the acquisition time, which is potentially of the order of tens of milliseconds, the technique has potential for in vivo refractive-index measurements of turbid biological media under dynamic conditions.     

High-speed adaptive interferometer for optical coherence-domain reflectometry through turbid media

Two-wave mixing in a dynamic holographic film acts as the adaptive beam combiner in a short-coherence interferometer that performs optical coherence-domain reflectometry (OCDR) through turbid media. This approach combines the high spatial resolution and sensitivity of coherence-domain reflectometry with photorefractive quantum-well-based adaptive homodyne detection. A depth resolution of 28 microm and penetration through 16 mean free paths in a turbid medium have been obtained in this adaptive OCDR application.     

Determination of the depth-resolved Stokes parameters of light backscattered from turbid media by use of polarization-sensitive optical coherence tomography

Polarization-sensitive optical coherence tomography (PS-OCT) was used to characterize completely the polarization state of light backscattered from turbid media. Using a low-coherence light source, one can determine the Stokes parameters of backscattered light as a function of optical path in turbid media. To demonstrate the application of this technique we determined the birefringence and the optical axis in fibrous tissue (rodent muscle) and in vivo rodent skin. PS-OCT has potentially useful applications in biomedical optics by imaging simultaneously the structural properties of turbid biological materials and their effects on the polarization state of backscattered light. This method may also find applications in material science for investigation of polarization properties (e.g., birefringence) in opaque media such as ceramics and crystals.     

On the determination of the rigidity parameters of nanoobjects

The aim of this work is to develop theoretical grounds for experimental determination of the rigidity parameters of nanoobjects. An efficient way of determining elastic moduli used in macromechanics consists in measuring the eigenfrequencies of an object under testing. Details of applying this approach to nanoobjects are discussed. A method of experimental determination of the rigidity parameters is suggested that is based on dynamic damping of vibrations (antiresonance). This method provides the possibility of separating out the eigenfrequencies of the nanoobject from the frequency spectrum of a system composed of a nanoobject and the cantilever of an atomic force microscope.     

High-precision frequency-domain measurements of the optical properties of turbid media

We report high-precision measurements of the absorption and the reduced scattering coefficients for turbid media. Using a frequency-domain measurement technique for a point-source infinite-medium geometry, we find that the standard deviations of multiple measurements of the absorption coefficient mu(a) and the reduced scattering coefficient mu(s)(?) are less than 0.6%, and three independently derived values for mu(a) and mu(s)(?) agree to better than 1%. Measurements of mu(a) agree with measurements of a nonscattering medium to within 1.2%. To obtain high precision requires attention to proper conditions for the spherical photon-density wave model, the detection linearity, and the ratio of the absorption rate to the source modulation rate. Frequency-domain amplitude and phase measurements deviate from fitted curves by 0.1% and 0.06 degrees rms, respectively.     

Frequency-domain immersion technique for accurate optical property measurements of turbid media

We demonstrate that absorption coefficient micro(a) and reduced scattering coefficient micro(s)(?) of a small turbid object can be measured to high accuracy with a frequency-domain immersion technique. For this technique the sample is immersed in a calibrated scattering medium and the optical properties are obtained from a differential measurement. Compared with conventional approaches, the immersion technique improves accuracy, minimizes variations owing to probe coupling and motion, reduces the effects of boundary conditions, and offers simple and rapid measurement once the immersion medium is calibrated. Accuracy tests of immersion-based measurements of micro(a) and micro(s)(?) agree with reference values to within 3.6% and 2.6%, respectively. These tests are limited by the accuracy of the reference samples rather than by the accuracy of the immersion medium or the precision of the immersion approach. We demonstrate the in vivo capabilities of the technique through time-resolved measurements of micro(a) and micro(s)(?) for a human hand during cuff occlusion on the upper arm.     

Theory of optical analysis of inhomogeneous turbid textures

A trial theory of optical diagnosis of inhomogeneous and turbid materials is firstly proposed, considering mutual photon exchanges due to scattering among conglomerate textures. Including scattering and redistribution of photons between neighboring segments, a collective model of photon flow behaviors is analytically constructed. Employing simple inhomogeneous parameters, a set of equations is formulated to express quasi three-dimensional photon redistribution between segments. The important feature of the theory is a simple framework regarding the complex photon flow to be solved by linear algebra. For qualitative and quantitative analyses of respective components, the simultaneous equations can be solved with their characteristic optical coefficients. Each of the ingredients can be analytically identified and evaluated separately. Some of the calculations are exemplified, to show differences from conventional homogeneous theory. Advantageous applications in medical diagnosis are suggested.     

Determination of optical parameters of partially transparent materials by the invariant embedding method

Optics and Spectroscopy - A method of invariant immersion to solve the inverse problem of identification of the indicators of the absorption and scattering of heat-resistant quartz ceramics by the...