Analyzing powers in the 12C( \vec d ,p)13C reaction at the energy T d = 270 MeV

The preliminary results on the tensor T₂₀ analyzing power for the ¹²C(,p)¹³C* reaction with the excitation of ¹³C levels and the d(,p)X reaction at the energies T _d = 140, 200 and 270 MeV at the emission angle Θ _cm = 0° are presented. The data on the tensor A _yy and vector A _y analyzing powers for the ¹²C(,p)¹³C* reaction at the energy T _d = 270 MeV in the angular range from 4° to 18° in the laboratory are also obtained.     

Divergence of the bulk resistance at criticality in disordered media

Consider the electrical resistancer _n (p) of a hypercubic bond lattice [O,n] ^d inZ ^d , where the bonds have resistance 1 with probabilityp or with probability 1-p. Letp _n (p)=n ^2-d r _n (p) andp(p)=lim_np_n(p). It is well known thatp(p)< ifp>p _c andp(p)= ifp<p _c , wherep _c is the percolation threshold. Here we show thatp(p _c )=, and .     

Status of the investigation of the spin structure of d, 3H, and 3He at VBLHE using polarized and unpolarized deuteron beam

The investigation of the spin structure of d, ³H, and ³He has been performed at the RIKEN acceleration research facility and VBLHE. Vector A _y and tensor A _yy , A _xx , A _xz analyzing powers for d → ³Hen and d → ³Hp are presented at 270 MeV. Themirror channels (³Hen and ³Hp) are comparedto each other in order to find possible manifestation of charge-symmetry breaking. The preliminary results on the polarization observables for d → ³Hp at 200MeV are also presented. The obtained data are compared with one-nucleon-exchange calculations.As a byproduct, d → pX and ¹²C → pX breakup reactions are investigated at 140, 200, and 270MeV. The experimental data on p elastic scattering were obtained at 270, 880, and 2000 MeV at the Nuclotron. The polarization of the deuteron beam was measured at 270 MeV at the internal target station. The preliminary data on the vector A _y and tensor A _yy , A _xx analyzing powers for the p elastic scattering at 880 MeV are presented. The calculations on A _y , A _yy , and A _xx analyzing powers for the p elastic scattering at 880 MeV were performed in the framework of the multiple-scattering model. The text was submitted by the authors in English.     

Stiffness exponents for lattice spin glasses in dimensions $\mathsf{d = 3,\ldots,6}$

The stiffness exponents in the glass phase for lattice spin glasses in dimensions are determined. To this end, we consider bond-diluted lattices near the T = 0 glass transition point p^*. This transition for discrete bond distributions occurs just above the bond percolation point p_c in each dimension. Numerics suggests that both points, p_c and p^*, seem to share the same 1/d-expansion, at least for several leading orders, each starting with 1/(2d). Hence, these lattice graphs have average connectivities of near p^* and exact graph-reduction methods become very effective in eliminating recursively all spins of connectivity , allowing the treatment of lattices of lengths up to L = 30 and with up to 10⁵-10⁶ spins. Using finite-size scaling, data for the defect energy width over a range of p > p^* in each dimension can be combined to reach scaling regimes of about one decade in the scaling variable . Accordingly, unprecedented accuracy is obtained for the stiffness exponents compared to undiluted lattices (p = 1), where scaling is far more limited. Surprisingly, scaling corrections typically are more benign for diluted lattices. We find in for the stiffness exponents y₃ = 0.24(1), y₄ = 0.61(2), y₅ = 0.88(5), and y₆ = 1.1(1).Received: 29 October 2003, Published online: 20 April 2004PACS: 05.50. + q Lattice theory and statistics (Ising, Potts, etc.) - 64.60.Cn Order-disorder transformations; statistical mechanics of model systems - 75.10.Nr Spin-glass and other random models - 02.60.Pn Numerical optimization     

Rate processes on fractals: Theory,simulations, and experiments

Heterogeneous kinetics are shown to differ drastically from homogeneous kinetics. For the elementary reaction A + A products we show that the diffusion-limited reaction rate is proportional tot ^– h[A]² or to [A]^x, whereh=1- d _s/2, X=1+2/d _s =(h-2)(h-1), andd _s is the effective spectral dimension. We note that ford = d _s =1, h =1/2 andX = 3, for percolating clustersd _s = 4/3,h = 1/3 andX = 5/2, while for dust ds <1, 1 >h > 1/2 and >X > 3. Scaling arguments, supercomputer simulations and experiments give a consistent picture. The interplay of energetic and geometric heterogeneity results in fractal-like kinetics and is relevant to excitation fusion experiments in porous membranes, films, and polymeric glasses. However, in isotopic mixed crystals, the geometric fractal nature (percolation clusters) dominates.     

Relativistic and nonrelativistic oscillator strengths in the Na isoelectronic sequence

We report the general trend of the nonrelativistic Hartree-Fock relativistic Hartree-Fock, nonrelativistic configuration-interaction, and relativistic configuration-interaction length form of the oscillator strengths for the resonance excitation 1s ²2s ²2p⁶3s ² S _J ^e 1s ²2s ²2p ⁵3s ^{2 2} P _J ^o . transition, which leads to autoionization (Auger transition), in Na, Mg¹⁺, Al²⁺, Si³⁺, P⁴⁺, S⁵⁺, Cl⁶⁺, Ar⁷⁺, K⁸⁺, Ca⁹⁺, Sc¹⁰⁺, Ti¹¹⁺, Fe¹⁵⁺, Cu¹⁸⁺, Zn¹⁹⁺, Br²⁴⁺, and Kr²⁵⁺ ions of the sodium isoelectronic sequence.     

Resonance-enhanced multiple-photon ionisation spectroscopy of excited sulphur atoms

Sulfur atoms are produced in the excited 3s ²3p ^{4 1} D ₂ and 3s ²3p ^{4 1} S ₀ levels by two-photon photodissociation of CS₂ in the gas phase in the region 285–305 nm. These excited atoms are detected by three-photon (two to resonance) ionisation at selected laser wavelengths. Many new transitions have been observed which have not been reported previously. The new dark states that have been accessed by two-photon absorption have been characterised and the energy levels with respect to the ground ³ P ₂ state have been determined. Configuration interaction between 6p ³ P ₁, 6p ⁵ P ₁, and 4p¹ P ₁ states, and also between 6p ³ P ₂, 6p ⁵ P ₂, and 4p¹ D ₂ states has been observed. It is found that intermediate states reached from the ¹ S ₀ level through two-photon absorption lie above the first ionisation potential of S⁺(⁴ S ⁰). It is proposed that autoionisation into the ⁴ S ⁰+e^– continuum is a dominant mechanism in the decay of these levels, although ionisation by a further photon absorption is not ruled out.     

Time constants of radiative transitions from the 5<Emphasis Type="Italic">d</Emphasis>[3/2]<Subscript>1</Subscript> level of a xenon atom

Integral yields of spontaneous emission at wavelengths of 1.73, 2.03, and 2.65 μm have been measured upon excitation of pure xenon by a pulsed electron beam. These yields have been analyzed and experimental data have been obtained on time constants of radiative transitions 5d[3/2]₁ → 6p[5/2]₂, 5d[3/2]₁ → 6p[3/2]₁, and 5d[3/2]₁ → 6p[1/2]₀ of XeI, which appeared to be equal to (2300 ± 400) × 10^?9, (300 ± 40) × 10^?9, and (1300 ± 200) × 10^?9 s, respectively. It is shown that the experimental data are in a qualitative agreement with the results of computational and theoretical investigations. The results of averaging the experimental and calculated data are proposed for use as recommended values of the corresponding constants.     

Evidence for incipient O dimerization and absence of Cu+3 in temperature-dependent XPS of highT c superconducting oxides

From temperature-dependent X-ray photoemission (XPS) spectra between 300 and 10 K of Sr doped La₂CuO₄ and 123 compounds (YBa₂Cu₃O_7–) we deduce the absence of the Cu3d ⁸(Cu³⁺) configuration in the ground state of these Mott insulators. The metallic character of these samples and involving those Cu atoms which are relevant for the superconducting properties arises from (d ⁹ p ⁶)+(d ¹⁰ p ⁵) valence fluctuations, while the superconducting transition is indicated to be closely related to an incipient oxygen dimerization which is best detected upon cooling far belowT _c .     

On the phase transition to sheet percolation in random Cantor sets

Thed-dimensional random Cantor set is a generalization of the classical middle-thirds Cantor set. Starting with the unit cube [0, 1] ^d , at every stage of the construction we divide each cube remaining intoM ^d equal subcubes, and select each of these at random with probabilityp. The resulting limit set is a random fractal, which may be crossed by paths or (d–1)-dimensional sheets. We examine the critical probabilityp _s(M, d) marking the existence of these sheet crossings, and show that p_s(M,d)1–p_c(M ^d) asM, where p_c(M ^d) is the critical probability of site percolation on the lattice (M ^d) obtained by adding the diagonal edges to the hypercubic lattice ^d. This result is then used to show that, at least for sufficiently large values ofM, the phases corresponding to the existence of path and sheet crossings are distinct.     

Vibrational Population of Hydrogen Molecules Excited by an RF Discharge in an Expanding Thermal Arc Plasma as Determined by Emission Spectroscopy

This work is devoted to the determination of the vibrational population of hydrogen molecules in the ground and excited electronic states from the analysis of visible spectra of the H₂ molecules excited by an RF discharge in an expanding thermal arc plasma. Comparison of the experimental results on relative electron-impact excitation cross sections for the transition H₂(X¹Σ, υ⁰ = 0)→ H₂(d³II_u, υ′) with other experiments, and with calculations based on the Franck-Condon principle, shows good agreement. This means, that for plasma under investigation: 1) in the ground electronic state H₂(d³II_u,υ′), only the lowest vibrational level with υ⁰ = 0 is significantly populated, and 2) direct electron exictation of H₂(d³II_u, υ′, υ′) state from the ground state H₂(X¹Σ, υ⁰ = 0) dominates.     

Optical properties of CdIn2Se4 thin films

The optical constants (the refractive index n, the absorption index k, and the absorption coefficient ) of CdIn₂Se₄ thin films were determined in the spectral range of 500–2000 nm. Graphical representation of log() as a function of log(1/) shows two distinct, linear parts indicating the existance of both direct and indirect optical transitions. The corresponding forbidden energy gaps E _g ^d and E _g ^Emphasis>d were determined. The effect of both annealing temperature as well as the substrate temperature on the optical constants of CdIn₂Se₄ thin films was also investigated.     

Fractal chemical kinetics: Reacting random walkers

Computer simulations on binary reactions of random walkers (A + A A) on fractal spaces bear out a recent conjecture: ( ^–1 – ₀ ^–1) t ^f , where is the instantaneous walker density and ₀ the initial one, andf=d _s /2, whered _s is the spectral dimension. For the Sierpinski gaskets:d=2, 2f=1.38 (d _s =1.365);d=3, 2f=1.56 (d _s =1.547); biased initial random distributions are compared to unbiased ones. For site percolation:d= 2,p=0.60, 2f= 1.35 (d _s =1.35); d=3,p=0.32, 2f=1.37 (d _s =1.4); fractal-to-Euclidean crossovers are also observed. For energetically disordered lattices, the effective 2f (from reacting walkers) andd _s (from single walkers) are in good agreement, in both two and three dimensions.Supported by NSF Grant No. DMR 8303919.     

Local electronic structure of Cu2O,CuO and YBa2Cu3O7−δ

Cu 3d and O 2p electronic states of Cu₂O, CuO, and the highT _c compound YBa₂Cu₃O_7– have been probed by means of high resolution x-ray emission spectroscopy (XES). The CuL and OK XES bands are compared in detail with recently reported x-ray photoelectron and ultraviolet photoelectron spectroscopy (XPS and UPS) measurements and densities of states obtained by local density functional (LDF) theory. The XES data show that the hybridization between Cu 3d and O 2p states is completely modified in CuO and YBa₂Cu₃O_7–, whered-d correlation energy is large, as compared to LDF predictions. Such is not the case for Cu₂O where agreement between theory and experiment is good.The Cu 3d states are found to be highly localized in YBa₂Cu₃O_7– (though less so than in CuO). The O 2p states lie at lower binding energies than in the simpler oxides and are mainly situated above the Cu 3d states. The respective positions of the centre of gravity of the OK emission bands on an x-ray energy scale indicate that the oxygen sites are less well screened by the O 2p states in the highT _c compound. This provides indirect evidence for the presence ofd-like states at the oxygen sites.     

Laser- and gamma-ray induced crystallization of IR-transmitting calcium gallate glass

Ar⁺-laser (=488 nm) irradiation of calcium gallate (CG) glass with the composition of 60CaO·39Ga₂O₃·Fe₂O₃ resulted in a distinct decrease in the IR transmittance (T) due to the formation of crystalline CaGa₂O₄ and CaGa₄O₉ phases. The Mössbauer spectrum of non-irradiated glass comprised a broad doublet due to distorted Fe³⁺(T_d) with, , and of 0.20, 1.33, and 1.00 mm s^–1, respectively. An additional doublet due to Fe³⁺(T_d) was observed in the Ar⁺-irradiated glass and, , and were 0.17, 1.32, and 0.75 mm s^–1, respectively. A decrease inT was also observed after the⁶⁰Co -ray irradiation with doses 10⁵Gy, and the precipitation of CaO, Ga₂O₃, and CaGa₄O₇ phases was confirmed by X-ray diffraction.     

Energy levels of ions of silver and rhodium isoelectronic sequences with <Emphasis Type="Italic">Z</Emphasis> < 86

The method of extrapolation of the parameter of a model potential for states of one electron (4f, 5s, 5p, 5d, 5f) above the core 1s ²2s ²2p ⁶3s ²3p ⁶3d ¹⁰4s ²4p ⁶4d ¹⁰ and one vacancy (4d ⁹) in the same core is applied to calculate the energy levels in the silver and rhodium isoelectronic sequences with the maximum nuclear charge Z = 86. The energy levels of Ag-and Rh-like ions were used for the calculation of the energies of resonance transitions to the ground state ¹ S ₀ in Pd-like ions. Good agreement between the theoretical and calculated energies of the resonance transitions in Pd-like ions indicates the reliability of the results obtained.     

Detection of chlorinated hydrocarbons via Laser-atomization/Laser-induced fluorescence

Chlorinated hydrocarbons (CHC), photodissociated at 193 nm, are detected with high sensitivity by observing the atomic chlorine fragment via laser-induced fluorescence (LIF). Photofragment emission spectra from CH₃Cl, CH₂Cl₂, CHCl₃, CCl₄, C₂HCl₃, and C₂Cl₄ demonstrate that photofragment fluorescence and chemiluminescence are negligible in the region 700–800 nm where the 3p ⁴4p ⁴ S ⁰ 3p ⁴4s ⁴ P fluorescence from atomic chlorine is detected. There is also negligible interference for photodissociation in Ar, N₂, and air bath gases. Total CHC can be readily detected in air flows at mixing fractions less than 20 ppb and averaging times less than 1 minute. Techniques for considerable improvement in this detection limit are discussed.Supported by the NSF     

Dynamics of forest fire under rotational constraint

A rotationally constrained forest fire model is studied on square and triangular lattices of size 400×400. The critical probabilityp _c for onset of fire propagation is determined. The scaling relationsMt ^d _r, R_gt^v andMR _g ^d _f are analysed at fire propagation probabilityp=p _c whereM is the number of burnt trees,R _g the radius of gyration andd _f the fractal dimension of the cluster of burnt trees at timet. Numerical estimates ofd _t, v andd _f have been obtained.     

Finite-size dependence of the helicity modulus within the mean spherical model

The validity of the finite-size scaling prediction about the existence of logarithmic corrections in the helicity modulus of three-dimensional O(n)-symmetric order parameter systems in confined geometries is studied for the three-dimensional mean spherical model of geometryL ^3/s-d×^d, 0d<3. For a fully finite geometry the general case ofd _p0 periodic,d _a0 antiperiodic,d ₀0 free, andd ₁0 fixed (d _p+d_a+d₀+d₁=d, d=3) boundary conditions is considered, whereas for film (d=2) and cylinder (d=1) geometries only the case of antiperiodic and/or periodic boundary conditions is investigated. The corresponding expressions for the finite-size scaling function of the helicity modulus and its asymptotics in the vicinity, below, and above the bulk critical temperatureT _c and the shifted critical temperatureT _c,L are derived. The obtained results are not in agreement with the hypothesis of the existence of a log(L) correction term to the finite-size behavior of the helicity modulus in the finite-size critical region if d=3. In the case of film and cylinder geometries there are no logarithmic corrections. In the case of a fully finite geometry a universal logarithmic correction term –[(d ₀ –d ₁)/4–2^da–1/²] lnL/L is obtained only for (T _c-T) LlnL.     

Configuration interaction and radiative constants in spectra of argon-like Sc IV-Fe IX ions

The probabilities of the 3p ⁵3d, 3p ⁵4s?3p ⁶, 3p ⁵4p, 3s3p ⁶3d electric dipole transitions and radiative lifetimes of the 3p ⁵3d, 3p ⁵4p, 3p ⁵4s, and 3s3p ⁶3d levels are calculated for the Sc IV–Fe IX isoelectronic sequence.