The generation of terahertz radiation via optical rectification in the self-induced transparency regime

The possibility of efficient terahertz generation via optical rectification in electro-optic crystal doped with the two-level resonant impurities is demonstrated. Under conditions of the self-induced transparency regime the laser pulses slows down to achieve the phase matching condition. The terahertz generation is accompanied by periodic modulation and spectral deformation of the laser pulse. The most efficient generation occurs under condition of small negative detuning from the resonant frequency of the two-level system.     

Generation of terahertz radiation by optical rectification in presence of resonance impurities

We demonstrate the possibility of an efficient generation of terahertz radiation under optical rectification in a uniaxial crystal containing impurities with resonance two-level quantum transitions. The group velocity of an optical pulse entering the regime of self-induced transparency decreases to the value of phase velocity of the terahertz radiation, which results in phase matching of long- and short-wavelength waves. The terahertz generation is accompanied by strong self-modulation of the optical pulse. Two-component soliton-like structures can be formed at long distances accompanied by spectral red shift of the optical component.     

ZnTe晶体中光学整流产生的THz辐射及其电光探测研究

借助抽运-探测技术研究了ZnTe晶体中光学整流产生的太赫兹(THz)辐射，利用ZnTe晶体的线性电光效应探测THz辐射场分布，观察到了较窄(约为0.2 ps)的THz场分布及相应较宽(响应超过4 THz，半峰宽约为2.4 THz)的THz频谱，并运用琼斯矩阵对实验结果进行了理论拟合. 研究了飞秒激光脉冲波长(750—850 nm)、脉冲宽度(56—225 fs)和晶体旋转与THz辐射产生的关系. 同时改变探测光偏振方向进行偏振调制，并从理论上分析了偏振调制对THz辐射探测的影响. 关键词： THz辐射 光学整流 电光探测 ZnTe     

Generation of sub-mJ terahertz pulses by optical rectification

Recent theoretical calculations predicted an order-of-magnitude increase in the efficiency of terahertz pulse generation by optical rectification in lithium niobate when 500 fs long pump pulses are used, rather than the commonly used ~100 fs pulses. Even by using longer than optimal pump pulses of 1.3 ps duration, 2.5× higher THz pulse energy (125 μJ) was measured with 2.5× higher pump-to-THz energy conversion efficiency (0.25%) than reported previously with shorter pulses. These results verify the advantage of longer pump pulses and support the expectation that mJ-level THz pulses will be available by cooling the crystal and using large pumped area.     

Generating terahertz radiation by means of optical rectification

Various means of raising the efficiency of generating wideband terahertz radiation on the basis of optical rectification are analyzed.     

Generation of nanosecond terahertz pulses by the optical rectification method

The possibility of the generation of quasi-cw terahertz radiation by the optical rectification method for broad-band Fourier unlimited nanosecond laser pulses has been experimentally demonstrated. The broadband radiation of a LiF dye-center laser is used as a pump source of a nonlinear optical oscillator. The energy efficiency of terahertz optical frequency conversion in a periodically polarized lithium niobate crystal is 4 × 10⁻⁹ at a pump power density of 7 MW/cm².     

Generation of radially polarized terahertz pulses via velocity-mismatched optical rectification

We demonstrate the generation of radially polarized terahertz pulses via optical rectification in a Cherenkov geometry exploiting velocity mismatch, contrary to the traditional approach for generating linearly polarized terahertz beams. A compact system is implemented using 001-cut ZnTe pumped by an ultrafast Yb-doped fiber amplifier.     

Generation of phase-locked and tunable continuous-wave radiation in the terahertz regime

Broadly tunable phase-stable single-frequency terahertz radiation is generated with an optical heterodyne photomixer. The photomixer is excited by two near-infrared CW diode lasers that are phase locked to the stabilized optical frequency comb of a femtosecond titanium:sapphire laser. The terahertz radiation emitted by the photomixer is downconverted into RF frequencies with a waveguide harmonic mixer and measurement-limited linewidths at the Hertz level are demonstrated.     

Study of terahertz radiation generated by optical rectification on thin gold films

Emission of terahertz (THz) radiation as a result of optical rectification of intense femtosecond laser pulses on thin gold films has been studied by time-domain THz spectroscopy. The THz amplitude was measured as a function of film thickness and incidence angle. The experiments reveal that the emitted THz field is suppressed for a thickness below 100 nm, which gives evidence of the nonlocal character of the response. The variation of incidence angle allows us to estimate the components of susceptibility tensor chi2ijk. For thicker films and near grazing incidence, the emitted THz field attains a peak value of 4 kV/cm.     

Generation of terahertz radiation upon the optical breakdown of a gas

Terahertz radiation of plasma oscillations excited upon the optical (axicon) breakdown of a gas in the presence of external fields of other frequency ranges has been analyzed. It has been shown that the spectra and intensity of oscillations and radiation generated by them depend strongly on the character of the spatiotemporal evolution of the formed plasma. The intensity is maximal upon the rapid formation of the plasma with a sharp boundary and decreases to very low values for objects with a smooth density profile. New schemes and regimes of break-down have been proposed, which make possible, according to preliminary estimates, an emitted energy of about 10 mJ with moderate intensities of ionizing laser radiation.     

Generating terahertz radiation via optical rectification in nonlinear crystals: Theory and experimental results

Key principles of terahertz radiation generation via laser pulse optical rectification are reviewed. The development of theoretical concepts is considered in connection with recent experimental results. The usability of resonant effects and metamaterials for the further development of this technique of generation is analyzed.     

Efficient generation of terahertz radiation by the method of optical rectification of terawatt laser pulses

Factors that lead to a decrease in the width and the mean frequency of the spectrum of terahertz (THz) radiation that were observed in recent experiments on optical rectification of powerful (∼0.5 TW) femtosecond laser pulses with a tilted amplitude front in a lithium niobate crystal are considered. A simple method is proposed that allows one to avoid the above transformation of the spectrum and to ensure a high efficiency of generation of THz radiation when laser pulses with a power of several TW are used.     

Generation of 30 microJ single-cycle terahertz pulses at 100 Hz repetition rate by optical rectification

We report the generation of 30 microJ single-cycle terahertz pulses at 100 Hz repetition rate by phase-matched optical rectification in lithium niobate using 28 mJ femtosecond laser pulses. The phase-matching condition is achieved by tilting the laser pulse intensity front. Temporal, spectral, and propagation properties of the generated terahertz pulses are presented. In addition, we discuss possibilities for further increasing the energy of single-cycle terahertz pulses obtained by optical rectification.     

Generation of terahertz radiation by the optical breakdown induced by a bichromatic laser pulse

Experimental results are presented on generation of terahertz radiation by the air breakdown induced by a high-intensity laser pulse having not only a fundamental component, but also a second-harmonic one. A theoretical explanation of the experimental data is proposed, based on a model of field ionization of a gas by a bichromatic laser.     

Generation of terahertz radiation in high-quality diamond samples

A method is proposed for generating terahertz radiation by producing a spectrally limited population inversion between light- and heavy-hole subbands in the valence band of semiconductors. This inversion is achieved by placing a sample in a static magnetic field and pumping it with an alternating electric field resonant with a cyclotron frequency of heavy holes. At a sufficiently low concentration of holes when the energy exchange between them is less effective than the exchange with the lattice, a considerable heating of heavy holes occurs with a nearly constant distribution function of light holes. However, the low hole concentration leads to a small terahertz field gain that can exceed the field loss only in high-quality diamond samples that are almost transparent in the terahertz range. An important advantage of this method for generating terahertz radiation over the previously proposed techniques is the possibility of implementing it at room temperature, which substantially increases its attractiveness, especially for use in biology and medicine.     

Generation of terahertz radiation in cubic non-centrosymmetric crystals

The conditions of parametric radiation generation on polaritons in cubic noncentrosymmetric crystals are studied. The possibility of such generation is theoretically justified. The polariton radiation frequencies are calculated for GaP, ZnSe, ZnTe, and GaAs crystals. The obtained generation frequencies are compared to the experimental results on Raman scattering on polaritons. The block diagram of the terahertz radiation generator operation using a GaP crystal and a pulsed laser with high peak power at low energy of laser pump pulses is presented. The lasing frequency shift is analyzed depending on the scattering geometry. The coefficient of exciting radiation conversion to the terahertz range is determined.     

Generation of subpicosecond electrical pulses by optical rectification

We describe the generation of subpicosecond electrical pulses by optical rectification of ultrashort optical pulses. The electrical pulses are generated by the second-order nonlinear response of a LiTaO(3) crystal bonded to a coplanar transmission line. A bipolar temporal waveform with a width of 875 fs was measured after a propagation distance of 175mum . This pulse width was limited by the response time of the photoconductive sampler. We observed both broadening and amplitude reduction in the temporal waveform owing to propagation.     

Percolation-enhanced generation of terahertz pulses by optical rectification on ultrathin gold films

Emission of pulses of electromagnetic radiation in the terahertz range is observed when ultrathin gold films on glass are illuminated with femtosecond near-IR laser pulses. A distinct maximum is observed in the emitted terahertz amplitude from films of average thickness just above the percolation threshold. Our measurements suggest that the emission is through a second-order nonlinear optical rectification process, enhanced by the excitation of localized surface plasmon hot spots on the percolated metal film.     

Transition from photocurrent surge to resonant optical rectification for terahertz generation in p-InAs

It has been demonstrated that the key to complete understanding of the mechanisms for terahertz (THz) generation from a p-type InAs wafer pumped by a subpicosecond Ti:sapphire amplifier lies in the dependences of the THz polarization on the azimuthal angle and polarization of the pump beam. At low enough pump intensities, photocurrent surge is the dominant mechanism for THz generation. However, the THz radiation originating from photocurrent surge is greatly reduced with increased pump intensity. Therefore, at sufficiently high pump intensities resonant optical rectification becomes the dominating mechanism for THz generation. The highest output power is measured to be 57 microW.