铯原子nP_(3/2)(n=70—94)里德伯态的紫外单光子激发及量子亏损测量

基于成熟的光纤激光器、光纤放大器及高效激光频率转换技术,我们在实验中研制了一套瓦级输出的窄线宽连续波单频可调谐318.6 nm紫外激光系统,并在室温铯原子气室中实现了6S_(1/2)—nP_(3/2)(n=70—94)单光子跃迁里德伯激发.借助由铯原子6S_(1/2)(F=4)基态、6P_(3/2)(F′=5)激发态和nP_(3/2)(n=70—94)里德伯态构成的V型三能级系统,通过频率锁定于铯原子6S_(1/2)(F=4)—6P_(3/2)(F′=5)超精细跃迁的852.3 nm探测光束的吸收减弱信号获得了里德伯态的信息,并利用高精度波长计测量了铯原子nP_(3/2)(n=70—94)里德伯态的量子亏损值.经过与理论计算值的变化趋势进行对比,我们认为由于原子气室的里德伯屏蔽效应并不能完全屏蔽外部直流电场,铯原子气室内存在残余的直流电场,影响了对里德伯态的量子亏损值的实验测量.利用残余直流电场的Stark效应理论模型及其与有效主量子数n*的依赖关系,对铯原子里德伯态的量子亏损实验测量值进行了修正.修正后的铯原子nP_(3/2)(n=70—94)态量子亏损测量值为3.5591±0.0007,与理论计算值相吻合.     

Ratiometric comparison of intense field ionization of atoms and diatomic molecules

Intense-laser ionization rates for rare gas atoms and diatomic molecules have been precisely compared by making simultaneous measurements of ionization yield vs laser intensity for mixed atomic and molecular targets. At a given laser intensity, the N (2) and F (2) ionization yields are slightly greater than that of Ar. Conversely, comparison of O (2) and S (2) with Xe indicates significant ionization suppression in these molecules. Recent molecular ionization models that successfully describe ionization suppression in O (2) and its absence in N (2) fail to explain our observations in F (2) and S (2).     

Features of plasma plume evolution and material removal efficiency during femtosecond laser ablation of nickel in high vacuum

We present an experimental characterization describing the characteristics features of the plasma plume dynamics and material removal efficiency during ultrashort, visible (527 nm, ≈300 fs) laser ablation of nickel in high vacuum. The spatio-temporal structure and expansion dynamics of the laser ablation plasma plume are investigated by using both time-gated fast imaging and optical emission spectroscopy. The spatio-temporal evolution of the ablation plume exhibits a layered structure which changes with the laser pulse fluence F. At low laser fluences (F<0.5 J/cm²) the plume consists of two main populations: fast Ni atoms and slower Ni nanoparticles, with average velocities of ≈10⁴ m/s for the atomic state and ≈10² m/s for the condensed state. At larger fluences (F>0.5 J/cm²), a third component of much faster atoms is observed to precede the main atomic plume component. These atoms can be ascribed to the recombination of faster ions with electrons in the early stages of the plume evolution. A particularly interesting feature of our analysis is that the study of the ablation efficiency as a function of the laser fluence indicates the existence of an optimal fluence range (a maximum) for nanoparticles generation, and an increase of atomization at larger fluences. PACS 52.50.-b; 52.38.Mf; 79.20.Ds; 81.07.-b     

Laser action of C,N, O,F, Cl,and Br in hollow cathode discharges

C, N, O, F, Cl, and Br red and infrared laser emission was investigated using hollow cathode discharges in gas mixtures of helium and molecules containing the corresponding atoms. A total of 33 laser lines with wavelengths from 0.7 to 2.0m was observed. Three laser lines of atomic C, five laser lines of atomic N, two laser lines of atomic Cl and five laser lines of atomic Br were observed for the first time. Dissociation charge transfer and dissociative excitation transfer are suggested as being responsible for populating the upper laser levels.     

Intense source of cold cesium atoms based on a two-dimensional magneto–optical trap with independent axial cooling and pushing

We report our studies on an intense source of cold cesium atoms based on a two-dimensional(2D) magneto–optical trap(MOT) with independent axial cooling and pushing.The new-designed source,proposed as 2D-HP MOT,uses hollow laser beams for axial cooling and a thin pushing laser beam to extract a cold atomic beam.With the independent pushing beam,the atomic flux can be substantially optimized.The total atomic flux maximum obtained in the 2D-HP MOT is4.02 × 1010atoms/s,increased by 60 percent compared to the traditional 2D+MOT in our experiment.Moreover,with the pushing power 10 μW and detuning 0Γ,the 2D-HP MOT can generate a rather intense atomic beam with the concomitant light shift suppressed by a factor of 20.The axial velocity distribution of the cold cesium beams centers at 6.8 m/s with an FMHW of about 2.8 m/s.The dependences of the atomic flux on the pushing power and detuning are studied in detail.The experimental results are in good agreement with the theoretical model.     

激光冷却气体原子研究的起步阶段

文章记述了开展激光冷却气体原子研究的起步阶段,描述了推动文章作者从原子钟研究走向激光冷却气体原子研究的动力.在研究初期阶段,文章作者着重思考了激光冷却气体原子物理机制,如:积分球红移漫反射激光冷却气体原子的设想和利用光频移效应(交流斯塔克效应)激光冷却气体原子的物理思想.文章还描述了作者所在实验室用于激光冷却原子研究的原子束实验装置,并展示了几个物理实验结果.最后,文章还总结了经验和教训,深感起步艰辛和今日可贵,期盼光辉的未来.     

Tuning the scattering length with an optically induced Feshbach resonance

We demonstrate optical tuning of the scattering length in a Bose-Einstein condensate as predicted by Fedichev et al. [Phys. Rev. Lett. 77, 2913 (1996)]. In our experiment, atoms in a 87Rb condensate are exposed to laser light which is tuned close to the transition frequency to an excited molecular state. By controlling the power and detuning of the laser beam we can change the atomic scattering length over a wide range. In view of laser-driven atomic losses, we use Bragg spectroscopy as a fast method to measure the scattering length of the atoms.     

全光学冷却与囚禁133Cs原子玻色-爱因斯坦凝聚的可能性

综述了近年来有关蒸发冷却¹³³Cs原子样品的实验进展,分析了磁囚禁¹³³Cs原子玻色爱因斯坦凝聚(BEC)的困难,并在此基础上提出了一个全光型冷却与囚禁¹³³Cs原子BEC的新方案.该方案主要由一个来自半导体激光(λ=0852μm)的倒金字塔形中空光束重力光学囚禁(pyramidal-hollow-beam gravito-optical trap,缩写为PHB GOT)和一个来自Ar⁺激光(λ=05013μm)的圆锥形中空光束重力光学囚禁(conical-hollow-beam gravito-optical trap,缩写为CHB GOT)组成.在PHB GOT中,冷原子经历了一个有效的中空光束感应的Sisyphus冷却(也即强度梯度冷却)和抽运光感应的几何冷却,原子温度将被从磁光囚禁(MOT)温度(约为60μK)冷却至几个光子反冲极限(约为2μK);而在Ar⁺中空光束囚禁(CHB GOT)中,冷原子将被Raman冷却或速度选择相干粒子数囚禁技术(velocity-selection coherent population trap,缩写为VSCPT)进一步冷却至光子反冲极限以下,并被激光频率高于原子共振频率的(也即蓝失谐的)covering光束压缩.我们就PHB冷却的动力学过程进行了Monte-Carlo模拟,并计算了Ar⁺中空光束囚禁¹³³Cs原子的光学势.研究结果表明,实现一个全光学冷却与囚禁的¹³³Cs原子BEC是可能的 关键词： 倒金字塔型中空光束重力光学囚禁 强度梯度冷却 氩离子中空光束囚禁 喇曼冷却 铯原子BEC     

Direct frequency comb measurements of absolute optical frequencies and population transfer dynamics

A phase-stabilized femtosecond laser comb is directly used for high-resolution spectroscopy and absolute optical frequency measurements of one- and two-photon transitions in laser-cooled 87Rb atoms. Absolute atomic transition frequencies, such as the 5S1/2 F=2-->7S1/2 F"=2 two-photon resonance measured at 788,794 768,921 (44) kHz, are determined without a priori knowledge about their values. Detailed dynamics of population transfer driven by a sequence of pulses are uncovered and taken into account for the measurement of the 5P states via resonantly enhanced two-photon transitions.     

All-optical ion generation for ion trap loading

We have investigated the all-optical generation of ions by photo-ionisation of atoms generated by pulsed laser ablation. A direct comparison between a resistively heated oven source and pulsed laser ablation is reported. Pulsed laser ablation with 10 ns Nd:YAG laser pulses is shown to produce large calcium flux, corresponding to atomic beams produced with oven temperatures greater than 650 K. For an equivalent atomic flux, pulsed laser ablation is shown to produce a thermal load more than one order of magnitude smaller than the oven source. The atomic beam distributions obey Maxwell–Boltzmann statistics with most probable speeds corresponding to temperatures greater than 2200 K. Below a threshold pulse fluence between 280 mJ/cm² and 330 mJ/cm², the atomic beam is composed exclusively of ground-state atoms. For higher fluences ions and excited atoms are generated.     

磁光阱中单原子荧光信号的优化及单原子的高效装载

实验中首先通过增大四极磁场梯度、提高背景真空度、缩小冷却俘获激光光束直径的方法获得了磁光阱中单原子的装载.其次,通过减小冷却光失谐量、适当增加其光强、同时使用偏振光谱锁频技术抑制冷却光噪声的方法得到了磁光阱中高信号背景比的单原子荧光信号.此外,通过实时反馈控制磁光阱四极磁场梯度的方法,在实验中实现了单原子98%的装载概率.使用Hamburg Brown-Twiss方案测量了磁光阱中的单原子在连续光激发下所辐射荧光的光子统计特性,得到二阶关联度g(2)(τ=0)=0.09.     

Rb原子滤波器的实验研究

本文用热Rb原子进行了光学滤波的研究。将一束激光调谐到Rb原子D2线的F=1→F′=2共振吸收线上,使其泵浦Rb原子,实现原子布居极化(即将Rb原子制备到能级F=2上)。当一束信号光反向穿过该介质时,若信号光频率调谐到原子"吸收窗口"(D1线F=2→F′=2),该介质对信号光大量吸收,信号光透射率仅为0.14%;若信号光频率调谐到原子"透明窗口"(D1线F=1→F′=2),信号光透射率高于47.4%。这种极化的原子介质可以用来做光学滤波器。     

激光冷却获得高亮度的亚稳态惰性气体原子束和原子阱

高强度的亚稳态惰性原子束流在原子分子物理实验研究中具有广泛的应用.使用射频电离方法和激光横向冷却技术制备了高强度的亚稳态氪原子束流,并使用数值模拟方法对横向冷却激光场中的原子径迹进行了分析.通过激光诱导荧光光谱方法测量原子束的束流特性,结果显示,横向冷却后在束流源下游230 cm处的原子束流强度达1.6atoms/(s*sr),束流强度提高了两个量级.利用这种高强度原子束流,我们成功囚禁了1.3×10¹⁰个亚稳态⁸⁴Kr原子,同时冷原子装载速率达到了3.0×10¹¹atoms/s;并利用该装置成功地实现了高亮度的亚稳态氩原子束和原子阱. 关键词： 横向冷却 原子束 原子阱 惰性气体     

An Atomic Magnetometer with Spin-Projection Noise Proportional to (T_2)~(1/2)

There is a comm on sense view for atomic magnetometers that their spin-projection-noises(SPNs) are inversely proportional to (T_2)~(1/2), where (T_2)~(1/2) is the transverse relaxation time. We analyze the current atomic magnetometer types and give a counter-example of this common sense, which is the all-optical spin precession modulated threeaxis atomic magnetometer proposed by our group in 2015. Unlike the other atomic magnetometers, the SPN of this kind of atomic magnetometers is proportional to (T_2)~(1/2) due to the fact that the scale factor between P_x and B can be unrelated to the transverse relaxation time T_2. We demonstrate this irrelevance experimentally and analyze the SPN theoretically. Using short-pulse ultra-high power laser to fully polarize the atoms, the phenomenon that SPN decreases with T_2 may also be demonstrated experimentally and a new tool for researching SPN in atomic magnetometers may be realized.     

Quantum Statistical Behaviors of Interaction of an Atomic Bose-Einstein Condensate with Laser

We have investigated quantum statistical behaviors of photons and atoms in interaction of an atomic Bose-Einstein condensate with quantized laser field. When the quantized laser field is initially prepared in a superposition state which exhibits holes in its photon-number distribution, while the atomic field is initially in a Fock state, it is found that there is energy exchange between photons and atoms. For the input and output states, the photons and atoms may exhibit the sub-Poissonian distribution. The input and output laser fields may exhibit quadrature squeezing, but for the atomic field, only the output state exhibits quadrature squeezing. It is shown that there exists the violation of the Cauchy-Schwartz inequality, which means that the correlation between photons and atoms is nonclassical.     

铯原子7S1/2态磁偶极超精细常数的测量

在室温下的原子气室中, 基于铯原子6S_1/2-6P_3/2-7S_1/2(852.3 nm+1469.9 nm) 阶梯型能级系统, 利用电光调制器的主频和±1级边带分别产生的三套双共振吸收光谱, 当驱动电光调制器的信号源频率严格等于7S_1/2态超精细分裂的能级间隔时, 三套谱线中的一些超精细跃迁谱线重叠且线宽最窄, 利用这一现象很好地避免了激光器频率扫描时非线性效应的影响, 测量出了7S_1/2 态超精细分裂能级间隔: 2183.72 MHz±0.23 MHz, 并计算出该态的磁偶极超精细常数: A_hfs= 545.93 m MHz±0.06 MHz, 与文献中报道的测量结果一致.     

Quantum Statistical Behaviors of Interaction of an Atomic Bose-Einstein Condensate with Laser

We have investigated quantum statistical behaviors of photons and atoms in interaction of an atomic Bose Einstein condensate with quantized laser field. When the quantized laser field is initially prepared in a superposition state which exhibits holes in its photon-number distribution, while the atomic field is initially in a Fock state, it is found that there is energy exchange between photons and atoms. For the input and output states, the photons and atoms may exhibit the sub-Poissonian distribution. The input and output laser fields may exhibit quadrature squeezing, but for the atomic field, only the output state exhibits quadrature squeezing. It is shown that there exists the violation of the Cauchy-Schwartz inequality, which means that the correlation between photons and atoms is nonclassical.``     

Laser spectroscopy and optical pumping of alkali atoms in superfluid helium

In this paper, our recent works on the alkali atoms in superfluid helim (HeII) are reported. At first we mentions the laser-sputtering method for implantation, which is simple but is very efficient to produce various kinds of neutral atoms and molecules in HeII. Secondly, we report on the laser spectroscopy of alkali atoms in HeII. Optical excitation and emission spectra are found to be roughly explained by a spherical atomic bubble model, but the spectra corresponding to the D₂ lines indicate the quadrupole oscillation of the bubble shape. Optical pumping by a circularly polarized laser beam is found to produce perfect polarization, for both electron and nuclear spins. Using the rf-optical double resonance techniques, the magnetic and hyperfine resonances are observed. It is discussed also about the phenomena which have observed in the experiments done so far but have not been fully explained.     

Observation of lasing mediated by collective atomic recoil

We observe the buildup of a frequency-shifted reverse light field in a unidirectionally pumped high-Q optical ring cavity serving as a dipole trap for cold atoms. This effect is enhanced and a steady state is reached, if via an optical molasses an additional friction force is applied to the atoms. We observe the displacement of the atoms accelerated by momentum transfer in the backscattering process and interpret our observations in terms of the collective atomic recoil laser. Numerical simulations are in good agreement with the experimental results.     

采用四根单模光纤束实现消逝波原子(或分子)波导的理论分析

提出了一种利用四根亚微米单模光纤束实现冷原子(或冷分子)波导的新方案，计算了四光纤束内空心区域的消逝波光场及其光学囚禁势.研究表明这种蓝失谐的空心消逝波光场同样可用于实现冷原子(或冷分子)的激光波导，而且与传统的中空光纤原子波导方案相比，不仅简单方便，造价低廉，而且更容易实现冷原子物质波的高效单模波导. 关键词： 单模光纤 消逝波 原子(或分子)波导