Intense laser-cluster interaction in the strong coupling regime

The interaction of noble gas clusters with moderately intense laser radiation at 100 and 800 nm is investigated via molecular dynamics simulations. It is shown that the laser-cluster interaction creates a strongly coupled plasma, which is characterized by a dominance of collisional processes. This has led to several findings. (1) A new heating mechanism is identified that explains the observation of unusually high-charge states in recent experiments with 100 nm radiation at DESY. We find that energy absorption takes place in the following cycle: many-body collisions resulting in an enhanced recombination of free electrons to exited states, and subsequent reionization. (2) Cluster interaction with 800 nm radiation is a promising system for investigating the transition from weakly coupled plasmas, where collective processes dominate, to strongly coupled plasmas. We achieve this transition by varying a single parameter: the laser intensity. The experimental and theoretical accessibility of laser-cluster interaction, thus, allows a systematic combined study of the interplay between collective and collisional processes.     

Deep strong coupling regime of the Jaynes-Cummings model

We study the quantum dynamics of a two-level system interacting with a quantized harmonic oscillator in the deep strong coupling regime (DSC) of the Jaynes-Cummings model, that is, when the coupling strength g is comparable or larger than the oscillator frequency ω (g/ω?1). In this case, the rotating-wave approximation cannot be applied or treated perturbatively in general. We propose an intuitive and predictive physical frame to describe the DSC regime where photon number wave packets bounce back and forth along parity chains of the Hilbert space, while producing collapse and revivals of the initial population. We exemplify our physical frame with numerical and analytical considerations in the qubit population, photon statistics, and Wigner phase space.     

Nonlinear emission of semiconductor microcavities in the strong coupling regime

We report on the nonlinear laserlike emission from semiconductor microcavities in the strong coupling regime. Under resonant continuous wave excitation we observe a highly emissive state. The energy, dispersion, and spatial extent of this state is measured and is found to be dispersionless and spatially localized. This state coexists with luminescence that follows the usual cavity-polariton dispersion. It is attributed to the amplification of luminescence by a parametric gain due to cavity-polariton scattering. Despite the resonant excitation at 1.6 K, we observe no sign of Bose-Einstein condensation nor Boser action.     

Potentialities of GaN-based microcavities in strong coupling regime at room temperature

In a recent publication [N. Antoine-Vincent, F. Natali, D. Byrne, A. Vasson, P. Disseix, J. Leymarie, M. Leroux, F. Semond, J. Massies, Phys. Rev. B 68 (2003) 153313], we have highlighted for the first time the exciton–photon strong coupling in a GaN-based microcavity and obtained a Rabi splitting of 31 meV persistent at 77 K. Our aim is now to study the feasibility of GaN-based microcavities for which the strong coupling regime would be maintained at room temperature. A complex heterostructure containing GaN/AlGaN quantum wells (QWs) is investigated by photoreflectivity and reflectivity at 5 K. The QW thickness is 3 nm and the Al composition and thickness of the barriers are respectively 0.11 and 10 nm. From the modeling of the experimental spectra, the values of the oscillator strength, the energy and the broadening parameter of the QW fundamental transition are determined; the broadening is found to be relatively weak (15 meV). Simulations of microcavities containing QWs have then been performed including this set of parameters: a theoretical Rabi splitting of 34 meV is obtained at 5 K. Considering an additional broadening induced by the increase of the temperature (23 meV), the strong coupling regime could be maintained theoretically at room temperature in such a structure. This is due to the low value of the inhomogeneous broadening related to the QW transition which is lower than in bulk GaN. The influence of the QW number and the nature of the Bragg mirror on the Rabi splitting is then discussed in realistic structures.     

Nonequilibrium steady state transport of collective-qubit system in strong coupling regime

We investigate the steady state photon transport in a nonequilibrium collective-qubit model. By adopting the noninteracting blip approximation, which is applicable in the strong photon–qubit coupling regime, we describe the essential contribution of indirect qubit–qubit interaction to the population distribution, mediated by the photonic baths. The linear relations of both the optimal flux and noise power with the qubits system size are obtained. Moreover, the inversed power-law style for the finite-size scaling of the optimal photon–qubit coupling strength is exhibited, which is proposed to be universal.     

Enhanced circular dichroism of plasmonic system in the strong coupling regime

The circular dichroism(CD) signal of a molecule is usually weak,however,a strong CD signal in optical spectrum is desirable because of its wide range of applications in biosensing,chiral photo detection,and chiral catalysis.In this work,we show that a strong chiral response can be obtained in a hybridized system consisting of an artificial chiral molecule and a nanorod in the strong coupling regime.The artificial chiral molecule is composed of six quantum dots in a helix assembly,and its CD signal arises from internal Coulomb interactions between quantum dots.The CD signal of the hybridized system is highly dependent on the Coulomb interactions and the strong coupling progress through the electromagnetic interactions.We use the coupled oscillator model to analyze strong coupling phenomenon and address that the strong coupling progress can amplify the CD signal.This work provides a scenario for designing new plasmonic nanostructures with a strong chiral optical response.     

Coherent response of a semiconductor microcavity in the strong coupling regime

We have studied the coherent dynamics of a semiconductor microcavity by means of interferometric correlation measurements with subpicosecond time resolution in a backscattering geometry. Evidence is brought of the resolution of a homogeneous polariton line in an inhomogeneously broadened exciton system. Surprisingly, photon-like polaritons exhibit an inhomogeneous dephasing. Moreover, we observe an unexpected stationary coherence up to 8 ps for the lower polariton branch close to resonance. All these experimental results are well reproduced within the framework of a linear dispersion theory assuming a coherent superposition of the reflectivity and resonant Rayleigh scattering signals with a well-defined relative phase.     

Optical spectra of organic quantum dots in the strong coupling regime

We analyze the emission spectrum of a single organic quantum dot coupled to a microcavity in the strong coupling regime. We take into account non-linearities arising from both exciton–exciton interactions and the Pauli exclusion principle. We apply the recently developed Pade approximation for regular truncation of Green functions to calculate the emission spectrum. We show that as the number of excitations in the quantum dot increases the Rabi doublet evolves into a more complicated triplet structure.     

Solvable model of dissipative dynamics in the deep strong coupling regime

We describe the dynamics of a qubit interacting with a bosonic mode coupled to a zero-temperature bath in the deep strong coupling (DSC) regime. We provide an analytical solution for this open system dynamics in the off-resonance case of the qubit-mode interaction. Collapses and revivals of parity chain populations and the oscillatory behavior of the mean photon number are predicted. At the same time, photon number wave packets, propagating back and forth along parity chains, become incoherently mixed. Finally, we investigate numerically the effect of detuning on the validity of the analytical solution.     

Dispersion of incoherent spectral features in systems with strong electron-phonon coupling

We study (inverse) photoemission from systems with strong coupling of doped carriers to phonons. Using an adiabatic approximation, we develop a method for calculating spectra. This method is particularly simple for systems where the electron-phonon coupling can be neglected in the initial state, e.g., the undoped t-J model. The theory then naturally explains why the electron-phonon coupling just leads to a broadening of spectra calculated without electron-phonon coupling, without changing the dispersion. This is in agreement with recent angle-resolved photoemission spectroscopy (ARPES) on undoped cuprates, and it supports the interpretation in terms of strong electron-phonon interaction. The theory also shows that for systems with strong electron-phonon coupling in the initial state, the result cannot in general be related to the spectrum obtained without electron-phonon coupling.     

Emission spectrum of a qubit in Rabi model in strong coupling regime

The analytical eigenenergies and eigenstates of the Rabi model are obtained approximately based on a unitary transformation and a generalized rotating-wave approximation (GRWA). Using these analytical expressions without the rotating wave approximation (RWA), we generalize the definition of the physical emission spectrum valid with the RWA in order to meet without the RWA with some modifications. Taking into account the counter-rotating wave terms and the intercrossing of energy level in the strong coupling regime, the physical emission spectrum of qubit is investigated. Different from the case with RWA, the multi-peak vacuum Rabi splitting, even when the qubit initially in its ground state and the bosonic field initially in vacuum, can emerge. These new features of physical emission spectrum originate from the effect of counter-rotating wave terms. Moreover, the intercrossing of energy level can also be observed in the strong coupling regime.     

On the geometric QCD meson spectrum in the strong coupling regime

By giving the explicit calculations in the first order of the strong coupling we extend this method to higher orders and show that there will always appear new excited mesons at higher order, independent of the approximation used. These states are analogous to be bound states of a confining potential, which has an infinite barrier at radiusr=a.     

Photon antibunching from a single quantum-dot-microcavity system in the strong coupling regime

We observe antibunching in the photons emitted from a strongly coupled single quantum dot and pillar microcavity in resonance. When the quantum dot was spectrally detuned from the cavity mode, the cavity emission remained antibunched, and also anticorrelated from the quantum dot emission. Resonant pumping of the selected quantum dot via an excited state enabled these observations by eliminating the background emitters that are usually coupled to the cavity. This device demonstrates an on-demand single-photon source operating in the strong coupling regime, with a Purcell factor of 61+/-7 and quantum efficiency of 97%.     

Auto-and cross-correlation functions of a one-atom laser in a regime of strong coupling

The spectral properties of an incoherently pumped one-atom laser operating in a regime of strong coupling are studied. The spectrum of the field outgoing from the cavity, the spectrum of resonance fluorescence of an atom, and the spectrum of the atom—field cross-correlation function are numerically calculated. Relations between the parameters of the system for which spectral lines corresponding to eigenstates of the Jaynes—Cummings Hamiltonian are resolved are found. A method for determining the widths of resonances from the spectrum of the atom—field cross-correlation function is proposed, and a procedure for measuring this function using spectroscopy of intensity fluctuations is described.     

Polariton thermalization in GaN microcavities in the strong light–matter coupling regime

We discuss the thermalization of the polariton population from a bulk GaN λ/2 microcavity at room temperature. Simultaneous optical measurements of reflectivity and photoluminescence (PL), as well as time resolved measurements, reveal strong light–matter coupling. Transfer matrix theory is used to calculate reflectivity, absorption, and transmission coefficients for the structure. The PL emission is found to be thermalized, despite its very short lifetime, suggesting the existence of very fast energy relaxation channels.     

Electron-phonon coupling and a polaron in the t-J model: from the weak to the strong coupling regime

We present numeric results for ground state and angle resolved photoemission spectra (ARPES) for a single hole in the t-J model coupled to optical phonons. The systematic-error-free diagrammatic Monte Carlo method is employed where the Feynman graphs for the Matsubara Green function in imaginary time are summed up completely with respect to phonon variables, while magnetic variables are subjected to the noncrossing approximation. We obtain that at electron-phonon coupling constants relevant for high T(c) cuprates the polaron undergoes a self-trapping crossover to the strong-coupling limit and theoretical ARPES demonstrate features observed in experiment: A broad peak in the bottom of the spectra has momentum dependence which coincides with that of a hole in the pure t-J model.     

Multivalued phase conjugate reflectivity in the reflection-type photorefractive four-wave mixing; strong coupling regime

Optical multistability based on the theory of four-wave mixing (FWM) is considered for the case of reflection geometry in photorefractive crystals. The resultant nonlinear algebraic equation obtained from the initial nonlinear coupled differential equations, is solved numerically by using a successive bisection method which can predict repeated zeros (roots) as well as discontinuities (jumps). We show that apart from the effects of photorefractive phase shift, the strong nonlinear coupling itself is sufficient to bring about multivalued branching behaviour of the phase conjugate reflectivity (PCR). As the coupling strength increases, the solutions become richer and more complex. We find that for certain values of pump and probe ratios and owing to the nature of strong nonlinear coupling the appearance of multiple solutions has a close connection with the phenomenon of bistability and self-oscillation.     

Modelling of strong coupling regime in bulk GaN microcavities using transfer matrix and quasiparticle formalisms

The evolution of the polaritonic Rabi splitting versus the excitonic broadenings is analyzed within two different formalisms: the transfer-matrix and the quasiparticle models. The splittings are deduced from angle-resolved reflectivity measurements performed at 5 K and 300 K on two GaN microcavities grown on silicon. Although the quasiparticle model allows a qualitative analysis when the quality factor of the cavity is high, the transfer-matrix formalism is more appropriate for the interpretation of the reflectivity spectra, whatever the configuration of the structure.