Measurement of fission anisotropy for 16O+181Ta

Anisotropies in fission fragment angular distributions measured for the system ¹⁶O + ¹⁸¹Ta over a range of bombarding energies from 83 MeV to 120 MeV have been analysed. It is shown that statistical transition state model (TSM) with pre-scission neutron correction described adequately the measured anisotropy data. Strong friction parameter is found to be necessary to estimate the pre-saddle to pre-scission neutron ratio.     

Langevin study of neutron emission in the reactions 16O+181Ta and 19F+178Hf

The pre-scission neutrons measured in the reactions 16O+181Ta and 19F+178Hf are studied via a Langevin equation coupled with a statistical decay model.We find that because of the mass asymmetry of different entrance channels,the spin distributions of compound nuclei would be different,consequently,the measured neutrons in these two reactions would also different.This means that the entrance channel will affect the particle emission in the fission process of hot nuclei.     

Fission fragment angular momentum in ODD-Z fissioning systems

Independent isomeric yield ratios of ¹²⁸Sb, ¹³⁰Sb, ¹³², ¹³¹Te, ¹³³Te, ¹³²I, ¹³⁴I, ¹³⁶I, ¹³⁵Xe and ¹³⁸Cs have been determined in the fast neutron induced fission of ²³⁷Np and ²⁴¹Am using radiochemical and gamma spectrometric technique. From the independent isomeric yield ratios, fragment angular momenta (J_rms) have been deduced using spin-dependent statistical model analysis. Comparison of these data with the literature data for even-Z fissioning systems shows the following important features: (i) Angular momenta for fragments with spherical 82n shell and even-Z products are lower compared to the fragments with out the 82n shell and odd-Z products indicating the effect of nuclear structure. (ii) Angular momentum of even-Z products in all the fissioning systems are comparable where as for odd-Z products it is slightly higher in the odd-Z fissioning systems than in the adjacent even-Z fissioning systems. This indicates the role of single particle on fragment angular momentum in odd-Z fissioning systems. Received: 26 March 1999 / Revised version: 16 October 1999     

Time-dependent perturbed angular correlation study of181Ta in Mg

The quadrupole interaction of¹⁸¹Ta in Mg metal has been investigated at room temperature by time differential perturbed angular correlation method yieldingv _Q=127±7 MHz. The observed EFG is calculated to be 20.8×10¹⁶ V/cm².     

Fission and emission of H and He in the reactions of 215 MeV16O with181Ta,208Pb and238U

The reactions of 215 MeV¹⁶O with¹²C,¹⁸¹Ta,²⁰⁸Pb and²³⁸U have been studied. Inclusive measurements for⁴He emission are given from each target, and for fission and^1,2,3H from Ta, Pb and U. For H/He a high-energy, forward-peaked component is observed with characteristics similar to those reported by others. At backward angles a low-energy, nearly-isotropic component is also observed for⁴He that cannot be accounted for by emission from fully accelerated fission products. The spectral shapes for this evaporative component are compared with statistical model calculations, and information is obtained concerning the effective barriers to emission. For the reactions of¹⁶O with¹²C, complete fusion seems to be overwhelmed by incomplete fusion. Fission angular distributions and cross sections are also presented and discussed.     

Fusion-fission angular distributions: A new probe of fast fission fractionation in nucleus-nucleus collisions

Fragment angular distributions in heavy ion-induced fission reactions have been analysed in terms of a two component model—fission following compound nucleus formation and fast fission events. It is seen that, contrary to the general assumption, fast fission competes with compound nucleus fission even when the composite system is formed with a spin less than the rotating liquid drop model limit for vanishing fission barrier.     

Fission fragment angular distribution in alpha-particle-induced fission of actinide elements

Using Lexan polycarbonate plastic as the fission fragment track detectors, the fragment angular distributions have been measured in the cases of fission of²³²Th and²³⁸U induced by alpha particles of various energies ranging from 40 to 70MeV obtained from the 88″ variable energy cyclotron at Calcutta. The center-of-mass angular distributions have been calculated and fitted by a series of Legendre polynomials. TheW(10°)/W(90°) ratios (defined as anisotropy) were measured at several energies for both the targets. These data are utilized in calculation of the energy dependence ofK ₀ ² , the standard deviation of the distribution in the angular momentum projection on the nuclear symmetry axis at the saddle point. Values of Γ _f /Γ _η , i.e. the ratio of the fission width to neutron emission width have been determined for²³²Th and²³⁸U nuclei. The integral cross-section for alpha induced fission in each target was determined by numerical integration of the respective center-of-mass angular differential cross-sections. The results were compared with similar data available in the literature which served to resolve some of the discrepancies observed in earlier measurements. The results were also compared with theoretical cross-sections.     

Sub-barrier fission fragment angular distributions for the system19F+232Th

The measurements of fission fragment angular distributions for the system¹⁹F+²³²Th have been extended to the sub-barrier energies of 89.3, 91.5 and 93.6 MeV. The measured anisotropies, within errors are nearly the same over this energy region. However, the deviation of the experimental values of anisotropies from that of standard statistical model predictions increases as the bombarding energy is lowered.     

Influence of pre-fission neutron emission on fission fragment angular distribution for the system209Bi +16O

The data of fission fragment anisotropies measured for the system¹⁶O +²⁰⁹Bi in the centre of mass energy region of 73 to 95 MeV have been compared with the saddle point statistical model calculations. The corrections to the nuclear temperature and the spin distribution arising due to pre-fission neutron emission have been made. While the resultant calculations reproduce very well the data in the near- and sub-barrier energy regions, they deviate from the data at higher energies. This observation is similar to what was already reported for¹⁶O +²⁰⁸Pb system.     

Electric quadrupole interaction at181Ta in tetragonal C16 intermetallic compounds

The TDPAC technique was employed for studies of the hyperfine interaction of¹⁸¹Ta in the Hf₂Ni and Zr₂Ni compounds with Al₂Cu-type structure. A linear temperature dependence of the quadrupole frequencies was measured in the temperature region 300–1100 K.     

Rotational bands in 181Ta

High-spin states in ¹⁸¹Ta have been studied via the ¹⁷⁶Yb(¹¹B,α2n) reaction at 52 MeV using the PEX array and at 57 MeV using the NORDBALL array, with α-particle detection. The previously known, K^π=(7/2)⁺ ground state band and K^π=(9/2)⁻ band have been extended to spins (29/2)⁺ and (31/2)⁻, respectively. Two new one-quasiparticle bands, the K^π=(5/2)⁺ band built on the known (5/2)⁺ isomer and a K^π=((1/2)⁻) band have been observed. Two other rotational bands with three-quasiparticle structure, K^π=(15/2)⁻ and ((19/2)⁺ with π(7/2)[404]ν²(1/2)[510](9/2)[624] and π(9/2)[514]ν²(1/2)[510](9/2)[624] configurations, respectively, have been newly observed. The half-life of the K^π=((19/2)⁺) bandhead which decays to the head of the (15/2)⁻ band has been measured to be 140(36) ns. However, transitions from the ((19/2)⁺) state to the (15/2)⁻ band have not been observed. Received: 26 August 1998     

Fission fragment angular distributions for neutron fission of 232Th and their interpretation with a triple-humped fission barrier

The fission fragment angular distributions have been measured for the neutron fission of ²³²Th at a number of energies near the neutron threshold. An exhaustive search has been made for a set of transition states and barrier parameters that would simultaneously fit the angular distributions and reproduce quantitatively the structure seen in the neutron fission cross section. No satisfactory fit to both types of data could be obtained with a double-humped fission barrier. However, use of a triple-humped fission barrier does provide a reasonable fit to all the experimental data.     

Fission product energies and anisotropies following complete fusion of16O+238U

Radioactive recoil techniques have been developed for measuring angular distributions and range distributions of individual fission products following heavy ion induced fission. From these measurements, values can be extracted for the recoil velocity of the fissioning nucleus, the velocity imparted by fission, and the fission anisotropy. These techniques were applied to reactions of 101 MeV¹⁶O on²³⁸U, and confirmed that the reaction mechanism is essentially entirely complete fusion-fission. Accepting this, the data determine the kinetic energy release in forming the various products to a precision of 1%; while the overall magnitude of the energy is in good agreement with previous results, the data suggest a systematic correlation between kinetic energy and the position of a product on the nuclear charge dispersion curve, not previously reported, which is similar to but significantly larger in magnitude than the effect expected from simple Coulomb repulsion. Significant variations in anisotropy are also observed between products, which appear to be partially correlated with the variations in kinetic energy.     

Fission fragment damage in zircon

Abstract

X-ray diffraction, electron microscope and optical studies have been : ade on zircons damaged by fission fragments derived from the action of neutrons on uranium impurities in the zircon lattice. A dosage of about 10¹⁴ fission events · cm^?3 was required to produce diffuse x-ray scattering, observable by conventional photographic methods, and a dosage of about 10¹⁶ fission events · cm^?3 appears to be required to render a zircon amorphous. An optical absorption band, generated apparently by γ-rays, was observed near 270 nm in undoped zircon. The valence state of the uranium impurities was unchanged by irradiation with 10¹⁴ fission events · cm^?3, 2 × 10¹⁸ nvt of fast neutrons, or ～10¹⁰ R of γ-rays. A fission event in zircon was deduced to produce ～10⁴ times more displacement damage than an α-recoil atom. Individual fission tracks were observed directly by electron microscopy after dosage of 10¹⁰-10¹³ fission events - cm^?3, the tracks being similar in appearance to those found by other workers in other materials. With increasing dosage, fission fragment uradiation appears to produce a progressive disordering of the lattice, as was previously deduced for the case of α-recoil irradiation, rather than the formation of new crystallographic phases.     

The angular distributions of elastic scattering of 12,13C+Zr

To obtain the neutron spectroscopic amplitudes for \begin{document}${}^{90-96}$\end{document}Zr overlaps, experimental data of elastic scattering with small experimental errors and precise optical potentials were analyzed. In this study, the elastic scattering angular distributions of \begin{document}${}^{12,13}$\end{document}C + \begin{document}${}^{A} {\rm{Zr}}$\end{document} (A = 90, 91, 92, 94, 96) were measured using the high-precision Q3D magnetic spectrometer in the Tandem accelerator. The S?o Paulo potential was used for the optical potential. The optical model and coupled channel calculations were compared with the experimental data. The theoretical results were found to be very close to the experimental data. In addition, the possible effects of the couplings to the inelastic channels of the \begin{document}${}^A {\rm{Zr}}$\end{document} targets and \begin{document}${}^{12, 13}$\end{document}C projectiles on the elastic scattering were studied. It was observed that the couplings to the inelastic channels of the \begin{document}${}^{12,13}$\end{document}C projectiles could improve the agreement with the experimental data, while the inelastic couplings to the target states are of minor importance. The effect of the one-neutron stripping in the \begin{document}${}^{13}$\end{document}C+\begin{document}${}^A {\rm{Zr}}$\end{document} elastic scattering was also studied. The one-neutron stripping channel in \begin{document}${}^{13}$\end{document}C + \begin{document}${}^A {\rm{Zr}}$\end{document} was found to be not relevant and did not affect the elastic scattering angular distributions. Our results also show that in the reactions with the considered zirconium isotopes, the presence of the extra neutron in \begin{document}${}^{13}$\end{document}C does not influence the reaction mechanism, which is governed by the collective excitation of the \begin{document}${}^{12}$\end{document}C core.     

Electric field gradients at 181Ta probe in ZrNi: Results from perturbed angular correlation and first-principles calculations

Results of temperature dependent perturbed angular correlation (PAC) measurements in the equiatomic ZrNi alloy have been reported for the first time using ¹⁸¹Hf probe. At room temperature, values of quadrupole frequency and asymmetry parameter for the major component (~80%) are found to be ω_Q=26.8(4) Mrad/s, and η=0.413(7). The resulting electric field gradient comes out to be V_zz=2.99 ×10¹⁷ V/cm² and this corresponds to the probe nuclei occupying the regular substitutional Zr sites. In ZrNi system, no magnetic interaction is observed down to 77 K indicating absence of any magnetism in this material. X-ray diffraction (XRD) and X-ray photoelectron spectroscopy (XPS) studies on an inactive but similarly prepared sample confirm the dominant presence of the orthorhombic ZrNi phase in the sample. A complementary density functional theory (DFT) calculation results in V_zz=−2.35×10¹⁷ V/cm², η=0.46 at the ¹⁸¹Ta probe impurity site and zero magnetic moment on each atomic site, in close agreement with the experimental results. Furthermore, it is found that electric field gradient for the regular component follows a T^3/2 temperature dependence between 77 and 353 K, beyond which it varies linearly with temperature.     

Positron spectra from internal pair conversion observed in 238U + 181Ta collisions

We present new results from measurements and simulations of positron spectra, originating from ²³⁸U + ¹⁸¹Ta collisions at beam energies close to the Coulomb barrier. The measurements were performed using an improved experimental setup at the double-Orange spectrometer of GSI. Particular emphasis is put on the signature of positrons from Internal-Pair-Conversion (IPC) processes in the measured e⁺-energy spectra, following the de-excitation of electromagnetic transitions in the moving Ta-like nucleus. It is shown by Monte Carlo simulations that, for the chosen current sweeping procedure used in the present experiments, positron emission from discrete IPC transitions can lead to rather narrow line structures in the measured energy spectra. The measured positron spectra do not show evidence for line structures within the statistical accuracy achieved, although expected from the intensities of the observed γ-transitions ( E _γ∼ 1250-1600 keV) and theoretical conversion coefficients. This is due to the reduced detection efficiency for IPC positrons, caused by the limited spatial and momentum acceptance of the spectrometer. A comparison with previous results, in which lines have been observed, is presented and the implications are discussed. Received: 27 April 2000 / Accepted: 14 September 2000     

Angular momentum dependence of 200Pb fission studied by comparison of 19F on 181Ta with 16O on 184W

The time development of fission in highly excited Pb nuclei has been studied by the crystal blocking technique. Thin Ta crystals were bombarded with ¹⁹F ions in the energy range 90–120 MeV and the yield of fission fragments was measured for emission directions close to a strong axis. The experimental blocking dips are compared with calculated dips containing a superposition of two components, corresponding to short- and long-lived compound nuclei. The information extracted is the energy dependence of the relative amount of fission which comes from compound nuclei with lifetimes of τ≳3 × 10⁻¹⁷s. The total fission cross section and angular distribution of fission fragments were also measured for ¹⁹F bombardment of ¹⁸¹Ta in the energy range 84.3–114.7 MeV and for ¹⁶O bombardment of ¹⁸⁴W in the energy range 83.4–107.9 MeV. The results of the three types of measurements have been interpreted through comparison with statistical model calculations that follow the spin and energy distribution of compound nuclei through the neutron evaporation cascade. The ¹⁹F + ¹⁸¹Ta measurements, when compared with the present ¹⁶O + ¹⁸⁴W cross section and angular distribution measurements and earlier lifetime measurements for ¹⁶O + W, yield information on the spin distribution for the compound nucleus and its influence on the fission process.