Experimental characterization of non-premixed turbulent jet propane flames

This paper reports an experimental study conducted on turbulent jet propane flames aiming at further understanding of turbulent structure in non-premixed slow-chemistry combustion systems. Measurements of mean and fluctuating velocity and temperature fields, mean concentration of major chemical species, correlation between velocity and temperature fluctuations, and dissipation of temperature fluctuations are reported in a turbulent round jet non-premixed propane flame, Re=20 400 and 37 600, issuing vertically in still air. The experimental conditions were designed to provide a complete definition of the upstream boundary conditions in the measurement domain for the purpose of validating computational models. The measured data depicts useful flow field information for describing turbulent non-premixed slow-chemistry flames. Velocity–temperature correlation measurements show turbulent heat fluxes tended to be restricted to the mixing layer where large temperature gradients occurred. Observations of non-gradient diffusion of heat at x/D=10 were verified. Temperature fluctuation dissipation, χ, showed the highest values in the shear layer, where the variance of temperature fluctuations was maximum and combustion occurred. The isotropy between the temperature dissipation in the radial and tangential directions was confirmed. By contrast, the observed anisotropy between axial and radial directions of dissipation suggests the influence of large structures in the entrainment shear layer on the production of temperature fluctuations in the flame region. The value of the normalized scalar dissipation at the stoichiometric mixture fraction surface, χ_st, was calculated, and ranges between 2 and 4 s⁻¹. The measured data were used to estimate the budgets in the balance equations for turbulent kinetic energy, Reynolds shear stresses, turbulent heat flux and temperature variance, quantifying the mechanisms involved in the generation of turbulence as well as in the transport of the temperature.     

Flow Structure of Swirling Turbulent Propane Flames

Flow structure of premixed propane–air swirling jet flames at various combustion regimes was studied experimentally by stereo PIV, CH* chemiluminescence imaging, and pressure probe. For the non-swirling conditions, a nonlinear feedback mechanism of the flame front interaction with ring-like vortices, developing in the jet shear layer, was found to play important role in the stabilisation of the premixed lifted flame. For the studied swirl rates (S = 0.41, 0.7, and 1.0) the determined domain of stable combustion can be divided into three main groups of flame types: attached flames, quasi-tubular flames, and lifted flames. These regimes were studied in details for the case of S = 1.0, and the difference in the flow structure of the vortex breakdown is described. For the quasi-tubular flames an increase of flow precessing above the recirculation zone was observed when increased the stoichiometric coefficient from 0.7 to 1.4. This precessing motion was supposed to be responsible for the observed increase of acoustic noise generation and could drive the transition from the quasi-tubular to the lifted flame regime.     

Temperature Imaging in an Unsteady Propane-Air Counterflow Diffusion Flame Subjected to Low Frequency Oscillations

Current emphasis in non-premixed turbulent combustion research is focused on the effects of hydrodynamic unsteadiness and transient effects in these flames. To address these effects, measurements of the temperature field in unsteady propane-air flames were made using planar laser-induced fluorescence of the hydroxyl radical to ascertain the effect of fluctuating hydrodynamics on flame temperature. Planar temperature measurements were made at four temporal locations within the 25 Hz velocity fluctuation as a function of initial steady strain rate and forcing amplitude. Results show that temperature in the propane flame is rather insensitive to initial strain rate for these weakly strained flames due to the balance between decreased heat release rate and reduced radiative losses resulting from diminished soot production as the strain rate is increased. The temperature is significantly influenced by the imposed velocity oscillation, however, which causes large fluctuations in the instantaneous strain rate. A decoupling of peak flame temperature and maximum PAH and excited CH concentration indicates significant transient effects resulting from the unsteady flow field even at these low oscillation frequencies. This revised version was published online in July 2006 with corrections to the Cover Date.     

Towards an Extension of TFC Model of Premixed Turbulent Combustion

In order to determine the mean rate of product creation within the framework of the Turbulent Flame Closure (TFC) model of premixed combustion, the model is combined with a simple closure of turbulent scalar flux developed recently by the present authors based on the flamelet concept of turbulent burning. The model combination is assessed by numerically simulating statistically planar, one-dimensional, developing premixed flames that propagate in frozen turbulence. The mean rate of product creation yielded by the combined model decreases too slowly at the trailing edges of the studied flames, with the effect being more pronounced at longer flame-development times and larger ratios of rms turbulent velocity u′ to laminar flame speed S _L . To resolve the problem, the above closure of turbulent scalar flux is modified and the combination of the modified closure and TFC model yields reasonable behaviour of the studied rate. In particular, simulations indicate an increase in the mean combustion progress variable associated with the maximum rate by u′/S _L , in line with available DNS data. Finally, the modified closure of turbulent scalar flux is validated by computing conditioned velocities and turbulent scalar fluxes in six impinging-jet flames. The use of the TFC model for simulating such flames is advocated.     

Effect of turbulence on flame radiative emission

A collection of radiative emissions by several flames is analyzed. Such flames have been obtained in a number of burners, either premixed or not, fed with different fuels, while radiative emission is collected by means of a photo-diode, whose sampled signal is able to carry a large quantity of information about chemistry of flames and its interaction with turbulence. All the spectra computed show a decaying trend towards high frequencies with a slope of −5/3, that is known to be the inertial scaling of kinetic energy for homogeneous, isotropic, nonreacting turbulent flows. The aim of this work is to propose a physical model for the interpretation of the radiant energy scaling law coming from this simple instrument. To this purpose radiative emission of the flame has been splitted into two contributions, and its dynamics analyzed. The first contribution is the chemiluminescence effect, whereas the other is to be accounted for thermal emission of a gray/black body, ruled by Planck radiative equation. The time fluctuation of radiative emission is proposed to be linked to a thin reacting surface fluctuating in time and space under the constraint of turbulent fluid dynamic field. The thin reacting surface should be considered as the local flame front in premixed combustion, and as the local stoichiometric mixture fraction front in nonpremixed case. Taking into account such emission mechanisms, a physical interpretation of the −5/3 slope is proposed.     

Effects of Turbulence on Self-sustained Combustion in Premixed Flame Kernels: A Direct Numerical Simulation (DNS) Study

The effects of mean flame radius and turbulence on self-sustained combustion of turbulent premixed spherical flames in decaying turbulence have been investigated using three-dimensional direct numerical simulations (DNS) with single step Arrhenius chemistry. Several flame kernels with different initial radius or initial turbulent field have been studied for identical conditions of thermo-chemistry. It has been found that for very small kernel radius the mean displacement speed may become negative leading ultimately to extinction of the flame kernel. A mean negative displacement speed is shown to signify a physical situation where heat transfer from the kernel overcomes the heat release due to combustion. This mechanism is further enhanced by turbulent transport and, based on simulations with different initial turbulent velocity fields, it has been found that self-sustained combustion is adversely affected by higher turbulent velocity fluctuation magnitude and integral length scale. A scaling analysis is performed to estimate the critical radius for self-sustained combustion in premixed flame kernels in a turbulent environment. The scaling analysis is found to be in good agreement with the results of the simulations.     

A Comparison of the Blow-Off Behaviour of Swirl-Stabilized Premixed, Non-Premixed and Spray Flames

Confined short turbulent swirling premixed and non-premixed methane and heptane spray flames stabilized on an axisymmetric bluff body in a square enclosure have been examined close to the blow-off limit and during the extinction transient with OH* chemiluminescence and OH-PLIF operated at 5 kHz. The comparison of flames of different canonical types in the same basic aerodynamic field allows insights on the relative blow-off behaviour. The flame structure has been examined for conditions increasingly closer to blow-off. The premixed flame was seen to change from a cylindrical shape at stable burning condtions, with the flame brush closing across the flow at conditions close to blow-off. The PLIF images show that for the gaseous non-premixed flame, holes appear along the flame sheet with increasing frequency as the blow-off condition is approached, while the trend is less obvious for the spray flame. Non-premixed and spray flames showed randomly-occurring lift-off, which is further evidence of localised extinction. The mean lift-off height increased with increasing fuel jet velocity and decreased with increasing air velocity and approaches zero (i.e. the flame is virtually attached) just before the blow-off condition, despite the fact that more holes were evident in the flame sheet as extinction was approached. It was found that the average duration of the blow-off event, when normalised with the characteristic flow time d/U _b (d being the bluff-body diameter and U _b the bulk velocity) was in the range 9–38 with the spray flame extinction lasting a shorter time than the gaseous flames. Finally, it was found that correlations based on a Damköhler number collapse the blow-off velocity data for all flames with reasonable accuracy. The results can help the development of advanced turbulent combustion models.     

Study of a Filtered Flamelet Formulation for Large Eddy Simulation of Premixed Turbulent Flames

Despite significant advances in the understanding and modelling of turbulent combustion, no general model has been proposed for simulating flames in industrial combustion devices. Recently, the increase in computational possibilities has raised the hope of directly solving the large turbulent scales using large eddy simulation (LES) and capturing the important time-dependant phenomena. However, the chemical reactions involved in combustion occur at very small scales and the modelling of turbulent combustion processes is still required within the LES framework. In the present paper, a recently presented model for the LES of turbulent premixed flames is presented, analysed and discussed. The flamelet hypothesis is used to derive a filtered source term for the filtered progress variable equation. The model ensures proper flame propagation. The effect of subgrid scale (SGS) turbulence on the flame is modelled through the flame-wrinkling factor. The present modelling of the source term is successfully tested against filtered direct numerical simulation (DNS) data of a V-shape flame. Further, a premixed turbulent flame, stabilised behind an expansion, is simulated. The predictions agree well with the available experimental data, showing the capabilities of the model for performing accurate simulations of unsteady premixed flames.     

Reynolds stress, mean velocity, and dynamic static pressure measurement by a four-hole pressure probe

An improved version of the four-hole directional pressure probe, or Cobra probe, is described, in which the frequency response has been extended to 1.5 kHz. The probe measures all three orthogonal mean and turbulent velocity components at a point in the flow field. The probe also resolves the local mean and turbulent components of static pressure, allowing moments between the fluctuating velocity components and pressure to be determined. The techniques developed to allow the improved frequency response and the use of the probe in turbulent, developed pipe flow (a calibration flow) are described. Also given are the turbulent pressure-velocity correlations, which show a high degree of anticorrelation for one velocity component.     

Radiative heat flux characteristics of methane flames in oxy-fuel atmospheres

Oxy-fuel combustion is a promising alternative for power generation with CO₂ capture, where the fuel is burned in an atmosphere enriched with oxygen and CO₂ is used as a diluent. This type of combustion is characterised by uncommon characteristics in terms of thermal heat transfer budget as compared to air supported systems. The study presents experimental results of radiative heat flux along the flame axis and radiant fractions of non-premixed jet methane flames developing in oxy-fuel environments with oxygen concentrations ranging from 35% to 70%, as well as in air. The flames investigated have inlet Reynolds numbers from 468 to 2340. The data collected have highlighted the effects of the flame structure and thermo-chemical properties of oxy-fuel combustion on the heat flux radiated by the flames. It was first observed that peak heat flux increases considerably with oxygen concentration. More generally the radiant fraction increases with both increasing Reynolds number in the laminar regime and oxygen concentration. It was found that despite a difference in flame temperature, the radiative characteristics of the flames (heat flux distributions and radiant fraction) in air were similar to those with 35% O₂ in CO₂. The radiative properties of flames in oxy-fuel atmosphere with CO₂ as diluents appear to be dominated by the flame temperature.     

Assessing the Predictive Capabilities of Combustion LES as Applied to the Sydney Flame Series

Large Eddy Simulation (LES) and flamelet-based combustion models were applied to four bluff-body stabilized nonpremixed and partially premixed flames selected from the Sydney flame series, based on Masri’s bluff-body test rig (University of Sydney). Three related non-reacting flow cases were also investigated to assess the performance of the LES solver. Both un-swirled and swirled cases were studied exhibiting different flow features, such as recirculation, jet precessing and vortex breakdown. Due to various fuel compositions, flow rates and swirl numbers, the combustion characteristics of the flames varied greatly. On six meshes with different blocking structure and mesh sizes, good prediction of flow and scalar fields using LES/flamelet approaches and known fuel and oxidizer mass fluxes was achieved. The accuracy of predictions was strongly influenced by the combustion model used. All flames were calculated using at least two modeling strategies. Starting with calculations of isothermal flow cases, simple single flamelet based calculations were carried out for the corresponding reacting cases. The combustion models were then adjusted to fit the requirements of each flame. For all flame calculations good agreement of the main flow features with the measured data was achieved. For purely nonpremixed flames burning attached to the bluff-body’s outer edge, flamelet modeling including strain rate effects provided good results for the flow field and for most scalars. The prediction of a partially premixed swirl flame could only be achieved by applying a flamelet-based progress variable approach.     

LES/CMC of Blow-off in a Liquid Fueled Swirl Burner

Large Eddy Simulations of two-phase flames with the Conditional Moment Closure combustion model have been performed for flow conditions corresponding to stable and blow-off regimes in a swirl n-heptane spray burner. In the case of stable flame (i.e. low air velocity), the predicted mean and r.m.s. velocities and the location and shape of the flame agree reasonably well with experiment. In particular, the presence of localised extinctions is captured in agreement with experiment. Using model constants previously calibrated against piloted jet methane flames (Sandia F) with localised extinction, we obtain that at the experimentally determined blow-off velocity of the swirling spray flame, the predicted flame also blows off, demonstrating that the LES-CMC approach can capture the global extinction point in a realistic configuration.     

Performance of a 12-sensor vorticity probe in the near field of a rectangular turbulent jet

The design and operational characteristics of a 12-sensor hot wire probe for three-dimensional velocity–vorticity measurements in turbulent flow fields is described and discussed. The performance of the probe is investigated in comparison with X-sensor probe measurements in the near field of a rectangular turbulent jet with aspect ratio 6. Measurements have been conducted at Reynolds number Re _D = 21,000 at nozzle distances of x/D = 1, 3, 6 and 11, where D is the width of the nozzle. The results obtained with the 12-sensor probe compare well to the results of the X-sensor probe. Distributions of mean and fluctuating velocity–vorticity fields are presented and discussed. Among the results the most prominent is the experimental confirmation of the high levels of fluctuating vorticity in the shear layers.     

A Lagrangian-based flame index for the transported probability density function method

We propose a new flame index for the transported probability density function(PDF) method. The flame index uses mixing flux projections of Lagrangian particles on mixture fraction and progress variable directions as the metrics to identify the combustion mode, with the Burke-Schumann solution as a reference. A priori validation of the flame index is conducted with a series of constructed turbulent partially premixed reactors. It indicates that the proposed flame index is able to identify the combustion mode based on the subgrid mixing information. The flame index is then applied the large eddy simulation/PDF datasets of turbulent partially premixed jet flames. Results show that the flame index separate different combustion modes and extinction correctly. The proposed flame index provides a promising tool to analyze and model the partially premixed flames adaptively.     

Analysis of Algebraic Closures of the Mean Scalar Dissipation Rate of the Progress Variable Applied to Stagnating Turbulent Flames

In the turbulent premixed reactive flows considered in this study, i.e. large Damköhler and Reynolds numbers, the flamelet regime of turbulent combustion applies and the scalar dissipation rate and mean reaction rate are inter related. In this situation various algebraic models for the mean chemical rate that are obtained from an equilibrium of the dominant terms of the transport equation for the scalar dissipation rate, are evaluated through their application to flames stabilized in a turbulent stagnating flow. An asymptotic analysis is first performed and results obtained through the resulting one-dimensional calculation are compared with the experimental data of Li et al. (Proc Combust Inst 25:1207–1214, 1994). Eventually, three-dimensional CFD calculations including suited algebraic closures to represent the turbulent transport terms are carried out. Results are satisfactorily compared to the experimental data of Cho et al. (Proc Combust Inst 22:739–745, 1988). As a first outcome, the analysis confirms the interest and the relevance of the corresponding algebraic closures to deal with turbulent premixed combustion in such conditions. In the search of a satisfactory representation of such premixed impinging flames, the computational results also clearly emphasize the strong intertwinment that exits between the mean reaction rate, i.e. scalar dissipation rate or micro-mixing taking place at the smallest scale of the reactive flowfield, and the Reynolds fluxes modelling, i.e. turbulent macro-mixing.     

Stability of a nanopowder boundary-layer flow on a concave plate

Using hot-wire probe measurements, the mean and fluctuating velocities in a boundary layer on a concave plate immersed in the flow of a nanosized silicon dioxide powder are studied. A region of destabilization of disturbances is detected.     

Assessment of FSD and SDR Closures for Turbulent Flames of Alternative Fuels

Detailed-chemistry DNS studies are becoming more common due to the advent of more powerful modern computer architectures, and as a result more realistic flames can be simulated. Such flames involve many alternative fuels such as syngas and blast furnace gas, which are usually composed of many species and of varying proportions. In this study, we evaluate whether some of the commonly used models for the scalar dissipation rate and flame surface density can be used to model such flames in the LES context. A priori assessments are conducted using DNS data of multi-component fuel turbulent premixed flames. These flames offer unique challenges because of their complex structure having many distinct consumption layers for the different fuel components unlike in a single-component fuel. Some of the models tested showed good agreement with the DNS data and thus they can be used for the multi-component fuel combustion.     

Performance of a probe for measuring turbulent energy and temperature dissipation rates

A probe consisting of four X-wires (a total of eight hot wires operated in constant temperature mode) and two pairs of parallel cold wires (operated in constant current mode) is in principle capable of providing simultaneous data for the instantaneous energy and temperature dissipation rates. To evaluate the performance of this probe, measurements have been made in decaying turbulence downstream of a grid/screen combination. The directly measured mean values of the energy and temperature dissipation rates are compared with those obtained from the streamwise decay rates of the mean turbulent energy and temperature variance. The probe also yields all three fluctuating vorticity components; after applying spatial resolution corrections, their spectra are in close agreement with isotropic calculations over nearly all wavenumbers. Both the vorticity variance and the mean energy dissipation rate exhibit the same power-law decay rate. Transport equations for the mean energy and temperature dissipation rates are satisfied to within ᆞ%.     

Experimental study of biogas combustion using a gas turbine configuration

The aim of the present work is to compare stability combustion domains, flame structures and dynamics between CH₄/air flames and a biogas/air flames (issued from waste methanisation) in a lean gas turbine premixed combustion conditions. Velocity profiles are obtained by Laser Doppler Anemometry measurements. CH* chemiluminescence measurements and temporal acquisition of chamber pressure are performed in order to describe flame structure and instabilities. Changes in flame structure and dynamics when fuel composition is varying are found to strongly depend on laminar flame speed. No clear correlation between the unstable flame and the reaction zone penetration in the corner recirculation can be found.     

Experimental Characterization of Gelled Jet A1 Spray Flames

Gelled propellants provide energetic performance similar to conventional liquid propellants and safety during storage and handling like a solid propellant. Experiments on unconfined gelled Jet A1 spray flames and the comparison with ungelled spray flames are reported for the first time in this paper in terms of the global features, burning regimes, stability limits, visible flame height, emission spectra, natural luminosity, and CH ^? chemiluminescence. Propellants were atomized by an internally impinging two-fluid atomizer, developed specifically for efficient atomization of non-Newtonian gels. Swirling and non-swirling spray flames were successfully stabilized on a burner incorporating bluff body and annular jet of combustion air over a wide range of operating parameters. Structural features of the atomizer impart high momentum to the (central) spray jet, such that the recirculation zone could be penetrated under all conditions. Long-exposure smoke and high-speed visualizations were employed to study cold flow structures and droplet-vortex interactions. Short-exposure direct and backlit imaging were used to observe global features of spray flames. Stability limits and visible flame heights were mapped for different thermal inputs, swirl numbers, and flow rates of atomizing and combustion air jets. Non-swirling stable anchored, partially blown off, and neck-blown off flames were observed. Lifted, and a transition regime, in which the flame could burn in stable and lifted mode repetitively, were observed for the swirling flames. Interactions between central and annular jets are important in these regimes, determining flame shape, symmetry, and flame height. Jet-like propagation zone determines the flame height through its dependence on momentum of spray jet. The length of this zone is affected by variations in thermal input, gas-liquid ratio, and air-fuel ratio. The gelled Jet A1 flames are remarkably shorter despite having a larger average droplet size than ungelled Jet A1. This experimental observation directly supports theoretical predictions reported in literature. These flames are more luminous than ungelled Jet A1, especially at the base and the neck regions. While, majority of the heat is released in the jet-like propagation zone for both the flames, significant heat is released in the neck zone of ungelled Jet A1 spray flame in comparison to ungelled Jet A1 spray flame due to intense turbulence and smaller droplet size.