Untersuchung der Anregungen von186Re nach der (n, γ)-Reaktion

Prompt and delayedγ-γ-coincidences were measured after slow neutron capture in¹⁸⁵Re by use of Ge(Li)-detectors. New isomers were found at 99.4 keV (T_1/2=27±7ns) and at ≈330keV (T_1/2=17.4±0.7 ns). The evaluation of coincidence data established 10 rotational bands with band heads below 700 keV. The level scheme is discussed in detail: Nilsson assignments are proposed for the band configurations, and calculations of Coriolis mixing andγ-transition probabilities are presented which reproduce the experimental level energies and transition intensities very satisfactorily.     

Properties of isomeric states and the πd 3/2-vi 13/2 multiplet in194Au

The level structure of¹⁹⁴Au has been studied by observing prompt and delayedγ-rays following¹⁹⁴Pt(p,n) and¹⁹⁵Pt(p,2n) reactions. The conversion electron andγ-ray spectra from the decay of the 0.42s (10^?) and 0.60s (5⁺) isomers at 476 keV and 107.4 keV, respectively, have been measured using the He-jet method. The half-lives of the 6⁺ (278.2 keV, 1.1±0.4 ns), 7⁺ (224.6 keV, 2.6±0.2 ns) and 8⁺ (406.8 keV, 2.9±0.4 ns) members of theπd _3/2-vi _13/2 multiplet have been obtained from the time distributions between cyclotron beam pulses andγ-rays depopulating these levels. A calculation made assuming a pure two-particle configuration for the multiplet predicts very well theB(E2) values for the transitions between the levels of this multiplet but the calculatedB(M1) values are not in agreement with experimental results.     

Properties of the πh 9/2 ⊗ νi 13/2 band in odd-odd 188Au

A new rotational band has been identified and assigned to ¹⁸⁸Au for the first time using the ¹⁷³Yb(¹⁹F,4nγ) reaction at the beam energies of 86 and 90 MeV. This band is proposed to be built on the πh _9/2 ⊗ νi _13/2 configuration by comparing the band properties with known bands in neighboring nuclei. The prolate-to-oblate shape transition through triaxial shape has been proposed to occur around ¹⁸⁸Au for the ηh _9/2 ⊗ νi _13/2 bands in odd-odd Au isotopes on the basis of total Routhian surface (TRS) calculations.

     

Nuclear structure studies of the neutron deficientN=50 nucleus96Pd

The neutron deficient nucleus⁹⁶Pd, four proton holes below the doubly magic¹⁰⁰Sn, has been studied in the reaction⁶⁴Zn (³⁶Ar, 2p 2n). Innγ andγγ coincidences levels up to 7 MeV excitation energy were established, and a new neutron core-excited isomer with T_1/2=35(4)ns and g=0.83 (5) was identified. A detailed shell model study yields excellent agreement for states within the π(p_1/2,g_9/2) configuration space but fails to reproduce the isomerism andg-factor for the core-excited state.     

Decay of 161m1,m2Dy isomers under conditions of a resonance environment (Mössbauer Screen)

The half-lives of the isomers ^161m1Dy and ^161m2Dy (E = 25.6 keV and T _1/2 ～ 30 ns for the former and E = 74.6 keV and T _1/2 ～ 3 ns for the latter) placed in a ¹⁶⁰Gd₂O₃ crystal lattice at T = 300 K and surrounded by stable ¹⁶¹Dy nuclei in the composition of ¹⁶¹Dy₂O₃ were measured by the method of (β-γ) coincidences in the beta-decay process ¹⁶¹Tb → ¹⁶¹Dy. Nuclei of ^161m1,m2Dy were obtained according to the chain ¹⁶⁰Gd(n, γ)¹⁶¹Gd → ¹⁶¹Tb → ¹⁶¹Dy from ¹⁶⁰Dy₂O₃ weighted portions irradiated at the PWR-M reactor of the Petersburg Nuclear Physics Institute (PNPI, Gatchina, Russia). The T _1/2 value observed for the isomer ^161m1Dy was found to be correlated with the number of surrounding ¹⁶¹Dy nuclei. The presence of this correlation in ^161m1Dy can be explained by the multiple resonance scattering of photons from isomer decay within the sample used. No such correlation was observed for ^161m2Dy. The half-lives measured for the isomers ^161m1Dy and ^161m2Dy in the absence of the above environment are 29.2(1) and 3.50(1) ns, respectively.     

High-spin states in106Cd

Levels of¹⁰⁶Cd, populated by¹⁰⁴Pd(α, 2nγ)¹⁰⁶Cd have been studied measuring direct and delayedγ-ray spectra,γ-γ coincidences andγ-ray angular distributions. A decay level scheme is proposed including states up to 4659.8 keV. IntenseE2 transition cascades have been observed. The half-life of an isomeric level located at 4659.8 keV has been measured:T _1/2= 62±6ns. Nuclear Reactions ¹⁰⁴Pd(α, 2nγ),E _α=31MeV; measuredE _γ,I _γ,γ-γ coinc, σ(θ)T _1/2.¹⁰⁶Cd deduced levels,J, π, Enriched targets. Ge(Li) detectors.     

High spin states in153Er

High spin states in¹⁵³Er have been populated in the¹⁴⁴Sm(¹²C, 3n)¹³³Er reaction. Excitation functions, lifetimes, angular distributions,γ-γ coincidences and internal conversion coefficients were measured. Three isomeric states at 2.75 MeV (T _1/2=400 ns), 2.95 MeV (T _1/2～10 ns) and 5.2 MeV (T _1/2=200 ns) have been observed. A fourth isomer seems to be weakly excited above 6.8 MeV. The level scheme proposed is discussed in term of the nuclear shell model.     

On-line Time Differential Perturbed Angular Correlation with Light Probe Nucleus 19F

An on-line time differential perturbed angular correlation technique has been developed with the light probe nucleus ¹⁹F. The first on-line TDPAC measurement was carried out to determine the field gradient in Cd and quadrupole moment of ¹⁹F (0.197 MeV: I ^π = 5/2⁺, T_1/2 = 89 ns). This revised version was published online in September 2006 with corrections to the Cover Date.     

Transition probabilities and the structure of some negative-parity states in 126,130Xe and 132Ba

The lifetimes of several negative-parity states in ^126,130Xe and ¹³²Ba have been determined by means of the generalized centroid-shift method. The reactions ^124,128Te(α, 2n) and ¹²²Sn(¹³C, 3n) have been used. Following results were obtained: T_1/2(2758 keV) = 1.3 ± 0.2 ns in ¹²⁶Xe, T_1/2 (2060 keV) = 0.20 ± 0.10 ns, T_1/2 (2104 keV) = 0.50 ± 0.10 ns, T_1/2 (2376 keV) = 0.30 ± 0.10 ns and T_1/2 (2973 keV) = 4.6 ± 0.4 ns in ¹³⁰Xe as well as T _1/2(2120 keV) = 0.40 _?0.10 ^+0.20 ns in ¹³²Ba. A systematics of the B(E2; 7 ₁ ^? ? 5 ₁ ^? ) values in the N = 76 nuclei is presented. Electric dipole and quadrupole transition rates are discussed in terms of octupole and quadrupole collectivity. The structure of the 5 ₁ ^? and 7 ₁ ^? states is considered. Nuclear reactions: ^124,128Te(α, 2n), E = 26 MeV, ¹²²Sn (¹³C, 3n), E = 53 MeV; measured E_{gg}, I_{gg}, γ-r.f. Deduced T_1/2, B(σL) in ^126,130Xe and ¹³²Ba. Ge detectors. Generalized centroid-shift analysis.     

New insight in the level structure of <Superscript>153</Superscript>Er

The high-spin level structure of the ¹⁵³Er nucleus has been reinvestigated by in-beam γ-ray and electron spectroscopy with (¹⁴N,pxn) reaction. Excitation energies, spin and parity assignments are unambiguously established for the two lowest isomers T _1/2≃ 380 ns and T_1/2\simeq 10 ns. The characteristics of the third one (T _1/2≃ 250 ns) at 5.2 MeV are still questionable but its main decay modes are better known. An extension of the level scheme is proposed up to 8.4 MeV.Experimental results have been discussed in terms of shell model multiplets and compared with the other structures observed in N=85 neighbouring nuclei. Received: 8 November 1999 / Revised version: 13 December 1999     

Isomeric transitions between shape coexisting states in iodine isotopes withA=115, 119 and 121

Applying delayed- r.f. coincidences and generalized centroid-shift analysis, nanosecond isomers in some odd-A iodine isotopes are studied in-beam. The reactions¹⁰⁶Cd(¹²C,p2n) and^116,118Sn(⁶Li,3n) have been used. The following half-lives were determined:T _1/2(565 keV)=0.50±0.10 ns andT _1/2(837 keV) =0.90±0.20 ns in¹¹⁵I,T _1/2(687 keV)=5.50±0.50 ns andT _1/2(2418 keV)=4.0±0.50 ns in¹¹⁹I as well asT _1/2(812 keV)=0.35±0.20 ns andT _1/2(445 keV)<0.10 ns=">¹²¹I. A systematics of the absolute probabilities for the transitions deexciting theg _9/2 9/2⁺ and _11/2 11/2 ₁ ^– band heads in^115–125I is presented and discussed.Partly supported by the Bulgarian National Research Foundation under contracts PH14, and PH31 and Kernforschungszentrum Karlsruhe, Stabsabteilung Internationale Beziehungen     

Half-life measurements of intrinsic states in deformed odd-mass nuclei

The half-lives of the following intrinsic states in deformed odd-mass nuclei has been measured by delayed coincidences with a time-to-amplitude converter:

1. 5/2 5/2⁺[642] at 86.5 keV in¹⁵⁵Gd:T _1/2=6.7±0.3 ns, which results in the determination of theE1,ΔK=1 transition probability to the ground state 3/2 3/2^?[521] and first rotational state 5/2 3/2^?[521], yielding hindrance factors ofF _N ≈5.5 and ≈1.8 (F _W =3.1×10⁴ and 2.3×10⁴) respectively.
2. (3) 5/2 5/2^?[512] at 191.4 keV in¹⁶⁹Yb:T _1/2=3.35±0.15 ns and at 122.39 keV in¹⁷¹Yb:T _1/2=265±20 ns which results in the determination of the transition probabilities of theE1,ΔK=1 transitions to the ground states 7/2 7/2⁺[633], of theK-forbiddenM1 transitions to the 5/2 and 3/2 1/2^?[521] and of theE2 transitions to the 5/2, 3/2 and 1/2 1/2^?[521] states in both nuclei.

TheE1 transition probabilities are compared to the transitions between the same Nilsson states in¹⁷³Yb and¹⁷⁵Hf discussing the influence of the position of the Fermi surface — obtained from recent stripping and pick-up reactions — on these transition probabilities. Additional information on the decay scheme of¹⁷¹Lu→¹⁷¹Yb is obtained by delayed coincidence measurements. For testing the used time-to-amplitude converter the well known half-lives of the 482 keV level in¹⁸¹Ta (T _1/2=10.4±0.3 ns) and of the 279 keV level in²⁰³Tl (T _1/2=0.285 ±0.015 ns) were measured, in good agreement with other measurements.     

High-spin levels in137,139Ce and139,141Nd evidence for hole-core coupling

Excited states of the¹³⁷Ce,¹³⁹Ce,¹³⁹Nd and¹⁴¹Nd nuclei have been studied using the¹³⁸Ba(α, 5nγ)¹³⁷Ce,¹³⁸Ba(³He, 4nγ)¹³⁷Ce,¹³⁸Ba(α, 3nγ)¹³⁹Ce,¹⁴⁰Ce(α, 5nγ)¹³⁹Nd,¹⁴⁰Ce(³He,4nγ)¹³⁹Nd,¹⁴⁰Ce(α, 3nγ)¹⁴¹Nd and¹⁴²Ce(α, 5nγ)¹⁴¹Nd reactions. Singlesγ-ray spectra,γ —γ coincidence spectra, angular distributions and time distributions ofγ-rays with respect to beam pulses have been measured. Gamma transitions between excited states with spin values up to 21/2, 23/2 or 25/2 have been observed. Isomeric states with T_1/2=70 ns have been observed in¹³⁹Ce at 2631.5 keV (19/2) and in¹⁴¹Nd probably at 2952.0 keV (19/2). The level structure observed in the nuclei studied can be explained if the neutron-holes are coupled to the doubly even core excitations. The coupling of theh _11/2 neutron-hole with the 2⁺, 4⁺ and 3^? collective excitations are calculated in terms of the weak and intermediate coupling models. The intermediate coupling results seem to be in better agreement with the experimental data. The energies of theree-particle states, being the result of the coupling of theh _11/2 neutron-hole with the two-proton excitations in the core, are well reproduced in the calculations when empirical values of the two-body interaction matrix elements were used.     

Decay properties of the 19/2− isomers in113,117Sb

By means of the generalized centroid-shift method, the following half-lives were determined:T _1/2(3045 keV)=3.7±0.3 ns in¹¹³Sb using the reaction¹⁰⁴Pd(¹²C,p2n) as well asT _1/2 (1322.8 keV)=3.5±0.3 ns,T _1/2(2779.8 keV) =0.50±0.15ns,T _1/2(2874.9 keV)<0.2 ns andT _1/2(3072.9 keV)<0.1 ns in¹¹⁷Sb using the¹¹⁶In(α, 2n) reaction. Three-quasiparticle configurations of the type πd _5/2ν(h_11/2 d _3/2) in^113,117Sb are found to dominate in the wave functions of the 19/2^? states at 3045 and 2780 keV in¹¹³Sb and¹¹⁷Sb, respectively. TheB(E2, 19/2^? → 15/2^?) values in^113–119Sb are discussed.     

New isomers in83Br,85Rb,85Kr and86Kr

Using methods of in-beam spectroscopy in connection with 35 MeV⁷Li bombardment of⁸²Se targets four new isomers have been identified. They are observed in⁸³Br at 3070 keV (T_1/2=0.6±0.2 μs), in⁸⁵Rb at 2826 keV (T_1/2=12.5±0.6 ns), in⁸⁵Kr at 1991 keV (T_1/2=1.2+ _0.4 ^1.0 μs) and in⁸⁶Kr at 2250 keV (T_1/2=3.1±0.6 ns). Spin and parity 19/2^? have been assigned to the new isomer in⁸⁵Rb that is interpreted as the coupling of a p_3/2 proton to the g ₉ ^2/?2 two-neutron excitation of the N=48 neutron system. Using the TDPAD method an upper limit for the g-factor of ¦g¦≦0.17 has been estimated for this isomer. The same two-neutron excitation is also believed to be responsible for the new isomer in⁸³Br. The new isomers in⁸⁵Kr and⁸⁶Kr are interpreted as configurations containing the two-proton excitation (f ₅ ^2/?1 , p ₃ ^2/?1 ) where in the isomeric 17/2⁺ level of⁸⁵Kr an additional g_9/2 neutron hole is involved.     

Transition probabilities and hole-core coupled configurations in107In

The nucleus¹⁰⁷In was studied by in-beam spectroscopic methods in (HI, xn yp) reactions. Spin and parity values of some levels were determined by conversion electron andγ-ray measurements. Using the generalized centroid shift method, the half-lives T_1/2(19/2⁺, 2003.6 keV)=0.6±0.2 ns and T_1/2(17/2⁺, 1853.4 keV)=1.7±0.3 ns were measured. The systematics of the lowest members of the multipletπg ₉ ^2/?1 ×6 ₁ ⁺ in^111,109,107In is discussed     

In-beam study of high-spin states in199,200,201Po and systematical features of Z=84 polonium isotopes

Excited states in^199,200,201Po were populated in the reactions¹²C+¹⁹⁴Pt and¹²C+¹⁹⁵Pt. The subsequentγ-radiation was studied using conventional in-beam spectroscopic methods. States with spins up to (29/2), 18 and ≧35/2?, respectively, were populated in the three nuclides. Three isomeric states with the following half-lives were observed in²⁰⁰Po:T _1/2(8⁺)=90(15) ns,T _1/2(11^?)=120(20) ns andT _1/2(12⁺)=267(4) ns. The structure of the excited states was interpreted within the framework of the spherical shell model. The three isomers are suggested to be two-quasiparticle states with configurationsπ(h _{2 2})_8J, π(h₉i_13/2)₁₁- and v(i _{1 3/2 ?2})₁₂₊. A self-consistent Hartree-Fock calculation was performed to obtain ground-state deformations of the neighbouring Pb cores. From the results of the experiments and the calculations it was concluded that no appreciable deformations of the cores are manifested in the yrast states of these three Po nuclei.     

Investigation of theβ +-decay of105,106,109In and of100,102Ag

Isomers in the nuclei¹⁰⁰Ag (I=5⁺),¹⁰²Ag (I=5⁺),¹⁰⁵In (I=9/2⁺),¹⁰⁶In (I=6⁺),¹⁰⁸In (I=6⁺) were selectively populated by the reactions⁹⁰Zr(¹⁹F,xnγ),⁹²Mo(¹⁹F, 2pnγ),⁹²Mo(¹²C,pxnγ),⁹⁰Zr(¹⁹F,α3nγ) atE _lab=72 and 66MeV, and their (β ⁺+EC)-decay was studied with an Anticomptonγ-spectrometer. Spins of the beta-decaying isomers are determined. The results obtained for the beta strength functions are discussed as well as new information on the structure of the neutron-deficient even-even daughter nuclei nearZ=50.     

The g-factor of the Jπ=12+ isomeric state in188Hg

Using the reaction¹⁷⁵Lu(¹⁹F, 6n) theg-factor of the¹⁸⁸Hg isomeric state (J ^π=12⁺,T _1/2=135 ns) has been measured with the TDPAD method. The experimental value g=?0.168(10) supports the interpretation of an almost pure (vi13/2)^?2 configuration for this isomer.     

Study of Quasiparticles Bands in Odd-Odd 188Au

High-spin level structure of ¹⁸⁸Au has been studied via the ¹⁷³Yb(¹⁹F, 4nγ) reaction using techniques of in-beam γ-ray spectroscopy. Based on the experimental results, the level scheme of ¹⁸⁸Au has been revised significantly. The previously reported positive parity levels have been modified and a new 20⁺ level was proposed to feed the 18⁺ states via two low-energy transitions. The existence of the 20⁺ and the level structures above it are similar to those in the neighboring odd-odd ^190,192Au,therefore, the π h_{11/2}^{-1}\otimes \upnu i_{13/2}^{-2} h_{9/2}^{-1} configuration was assigned to the 20⁺ state.