Atomic short-range order in CuMn alloys

The establishment of atomic short-range order (SRO) has been investigated in CuMn alloys (5, 8,13,16,20 at. % Mn) by measurement of the electrical resistivity during isochronal and isothermal annealing. An increasing degree of SRO is accompanied by a reduction of resistivity; this effect increases with Mn concentration. For 8,13 and 16 at. % Mn SRO kinetics turn out to deviate significantly from single exponential behavior with a maximum at 13 at. % Mn, whereas at 5 and 20 at. % Mn SRO is adjusted in a single exponential process. For data analysis three methods are used: a sum of two and three exponentials as well as a log-normal spectrum of relaxation times. The strong interaction between second-nearest-neighbor atoms in CuMn seems to be essential for SRO kinetics but of minor importance for the value of SRO-induced resistivity change.     

A mean field spin glass with short-range interactions

We formulate and study a spin glass model on the Bethe lattice. Appropriate boundary fields replace the traditional self-consistent methods; they give our model well-defined thermodynamic properties. We establish that there is a spin glass transition temperature above which the single-site magnetizations vanish, and below which the Edwards-Anderson order parameter is strictly positive. In a neighborhood below the transition temperature, we use bifurcation theory to establish the existence of a nontrivial distribution of single-site magnetizations. Two properties of this distribution are studied: the leading perturbative correction to the Gaussian scaling form at the transition, and the (nonperturbative) behavior of the tails.Research supported by the NSF under Grant No. DMR-8314625Research supported by the DOE under Grant No. DE-AC02-83ER13044Research supported by the NSF under Grant No. DMR-8503544Research supported by the NSF under Grant No. DMR-8319301     

Incommensurate spin-density wave order in electron-doped BaFe2 As2 superconductors

Neutron diffraction studies of Ba(Fe(1-x)Co(x))(2)As)(2) reveal that commensurate antiferromagnetic order gives way to incommensurate magnetic order for Co compositions between 0.056 < x < 0.06. The incommensurability has the form of a small transverse splitting (0, ± ε, 0) from the commensurate antiferromagnetic propagation vector Q(AFM) = (1,0,1) (in orthorhombic notation) where ε ≈ 0.02-0.03 and is composition dependent. The results are consistent with the formation of a spin-density wave driven by Fermi surface nesting of electron and hole pockets and confirm the itinerant nature of magnetism in the iron arsenide superconductors.     

The order parameter in a spin glass

Various possible precise definitions of an Edwards-Anderson type of order parameter for an Ising model spin glass are considered, using boundary conditions for a finite system, states of an infinite system, and a duplicate-system approach. Several of these definitions are shown to yield identical results.     

Short-range order in spin density wave antiferromagnets

The model of the short-range order state for itinerant antiferromagnets with SDW is developed. The thermodynamic transverse spin density fluctuation are shown to influence essentially on the formation of the long-range magnetic order. In the wide temperature range these occurs the shortprange, magnetic order regim. The properties of the low-frequency transverse excitations of the spin density are analized. The existence of a fully diffusive mode at small wave vectors is predicted.     

Atomic displacements and short-range order in the FeSi soft magnetic alloy: Experiment and ab initio calculations

In order to determine the mechanism responsible for the formation of short-range order in dilute FeSi solid solutions, the chemical bonding, atomic displacements near the metalloid, and the enthalpy of silicon dissolution in iron have been studied within density functional theory. It is found that the directed character of the Si-Fe chemical bond formed upon the p-d hybridization brings about an anisotropy in atomic displacements near silicon atoms. Calculations of the Si-Si effective pairwise interaction energy offer an explanation for the observed features in short-range order in FeSi and suggest that ferromagnetic bcc Fe does not have a tendency toward Si atom clusterization. The mechanism of formation of the anisotropy induced by application of an external load or a magnetic field is discussed.     

Atomic short-range order and its relation to the magnetic behavior of noble-metal based spin-glass alloys

We have investigated the spatial distribution of magnetic atoms (Mn or Fe) by determining the short range order parameters for the archetypal spin-glass alloys: $\text{Cu}$Mn, $\text{Au}$Mn, $\text{Au}$Fe and $\text{Pt}$Mn in the dilute limit. All four systems possess atomic short-range order (ASRO) such as to enhance local ferromagnetic regions. In the latter three systems the ASRO is relatively strong and initiates long-range structures which develop with increasing concentration and which eventually destroy the spin-glass state.     

Atomic fermi-bose mixtures in inhomogeneous and random lattices: from fermi glass to quantum spin glass and quantum percolation

We investigate strongly interacting atomic Fermi-Bose mixtures in inhomogeneous and random optical lattices. We derive an effective Hamiltonian for the system and discuss its low temperature physics. We demonstrate the possibility of controlling the interactions at local level in inhomogeneous but regular lattices. Such a control leads to the achievement of Fermi glass, quantum Fermi spin-glass, and quantum percolation regimes involving bare and/or composite fermions in random lattices.     

Stable mean-field solution of a short-range interacting SO(3) quantum Heisenberg spin glass

We present a mean-field solution for a quantum, short-range interacting, disordered, SO(3) Heisenberg spin model, in which the Gaussian distribution of couplings is centered in an antiferromagnetic (AF) coupling J[over ]>0, and which, for weak disorder, can be treated as a perturbation of the pure AF Heisenberg system. The phase diagram contains, apart from a Néel phase at T=0, spin-glass and paramagnetic phases whose thermodynamic stability is demonstrated by an analysis of the Hessian matrix of the free-energy. The magnetic susceptibilities exhibit the typical cusp of a spin-glass transition.     

Short-range order in spin density wave antiferromagnets with chemical dimerization

The spin density wave model in a quasi-one-dimensional itinerant antiferromagnet with staggered potential at finite temperature is studied. Only short-range ordering exists in this system above the Néel temperature. The local-band theory of spin fluctuations is developed to calculate the spin density wave amplitude and the effective exchange integral. The one-electron spectrum and magnon spectrum are obtained in the short-range ordering regime. Zh. éksp. Teor. Fiz. 114, 1346–1364 (October 1998) Published in English in the original Russian journal. Reproduced here with stylistic changes by the Translation Editor.     

Short-range magnetic order in a spin density wave in Cr-based multilayers

A mechanism of the formation of the short antiferromagnetic order with a spin density wave (SDW) in the vicinity of the interfaces in the Fe/Cr type multilayers is proposed. The main reason behind the emergence of magnetic ordering with SDWs is the redistribution of charge (and, hence, spin) density in the vicinity of Fe/Cr interfaces, which leads to the paramagnetic phase instability at a temperature considerably higher than the Néel temperature in chromium. The Ginzburg-Landau expansion for the free energy of the system is used for determining the inhomogeneous collinear structures of CDWs and for constructing the phase diagram (the dependence of the transition temperature on the thickness of the antiferromagnetic interlayer). The obtained results are used for discussing the experimental data on neutron scattering and tunnel microscopy.     

Structural and short-range order analysis of glassy system

To understand the effects of structural features and to locate their signatures in the As-Ag-Te glassy system, various properties were studied as a function of average coordination number, 〈r〉. The structure of the sample is analyzed by X-ray diffraction technique and is found to be crystalline. The d-spacing and the lattice parameters of the samples were calculated. The structural parameters were discussed on the basis of Ag (silver) effect on As-Ag-Te glassy system. Structural investigations on these compositions revealed the polycrystalline nature of compositions with the presence of hexagonal As-Ag-Te phases. Grain size increased with the Ag content and parameters of unit cell are determined. The variations in the mean atomic volume, V, and the glass transition temperature, T_g, for glass transition, with composition have been reported. The change in thermal parameters was measured using differential thermal analysis (DTA). The results of the program are in agreement with those of analytical method and realized by binding energy represented by the cohesive energy values. The generalized ‘8-n’ rule was used to estimate the average coordination number. Obtained results were treated in the frame of chemical bond approach. We estimated some of physical parameters viz. mean bond energy, glass transition temperature, cohesive energy, average single bond energy, density, compactness and molar volume of all bulk samples. Our experimental and theoretical results were discussed in light of the topological bonding structure, which involves a hierarchy of correlation ranges in short-range order.     

Twinning and short-range order in ordered titanium monoxide

Electron diffraction was used to study the annealed titanium monoxide TiO_1.087 containing the monoclinic ordered phase Ti₅O₅. The diffraction pattern of titanium monoxide in the (112)* _B1 plane of the reciprocal lattice of the parent B1 cubic structure contains not only structural, superstructural, and additional reflections but also a system of planar diffuse strips. It has been established that part of the additional reflections are twins of the superstructure reflections of the monoclinic ordered phase; the twinning plane is the ( $\overline 1 \overline 1 1$ ) plane of the reciprocal lattice of the parent cubic phase. The diffuse scattering contours cover finite plane areas in the reciprocal space characterized by the wave vectors K ₁₀₀ ～ ± (h + 0.07)k ₁₀₀, K ₀₁₀ ～ ±(k + 0.07)k ₀₁₀, and K ₀₀₁ ～ ±(l + 0.07)k ₀₀₁ in the B1 structure. The diffuse scattering is caused by short-range displacement order. Short-range substitution order and the corresponding diffuse scattering are absent.