NO（D^2∑）共振增强的多光子离化谱

利用皮秒Nd：YAG激光器泵浦的光学参量发生傲大器作激发源，获得了NO分子在460～570nm波长范围内的多光子离化谱，测量了离化信号随激光强度的关系，其近五次方关系表明在460～570nm波长范围内NO分子吸收5个光子而离化。通过对谱线的归属，确认在此波长范围内，NO分子的离化过程是通过高激发态D^2∑的共振增强的多光子离化过程。用最小二乘法拟合，获得了D^2∑态的基振动频率和相互作用的力常数。     

Tm:YVO4晶体的光谱参数计算

由测量的Tm :YVO4晶体的吸收光谱 ,考虑到单轴晶体在各个方向上的吸收不同和折射率随波长的变化 ,根据Judd Ofelt理论计算了Tm3 +在YVO4中的强度参数、各个能级的振子强度、自发辐射几率、荧光分支比、积分发射截面等参数。强度参数为Ω2 =1 9416× 10 - 2 0 (cm2 ) ,Ω4=0 15 6 8× 10 - 2 0 (cm2 ) ,Ω6=0 396 3× 10 - 2 0 (cm2 )。计算结果表明 ,1 D2 → 3 F4的跃迁几率远大于1 D2 向其他各个能级的跃迁几率     

Cyclotron-resonance harmonics in the ac response of a 2D electron gas with smooth disorder

The frequency-dependent conductivity sigma(xx)(omega) of 2D electrons subjected to a transverse magnetic field and smooth disorder is calculated. The interplay of Landau quantization and disorder scattering gives rise to an oscillatory structure that survives in the high-temperature limit. The relation to recent experiments on photoconductivity by Zudov et al. and Mani et al. is discussed.     

Observation of out-of-phase bilayer plasmons in YBa(2)Cu(3)O(7-delta)

The temperature dependence of the c-axis optical conductivity sigma(omega) of optimally and overdoped YBa2Cu3Ox ( x = 6.93 and 7) is reported in the far- (FIR) and midinfrared (MIR) range. Below T(c) we observe a transfer of spectral weight from the FIR not only to the condensate at omega = 0, but also to a new peak in the MIR. This peak is naturally explained as a transverse out-of-phase bilayer plasmon by a model for sigma(omega) which takes the layered crystal structure into account. With decreasing doping the plasmon shifts to lower frequencies and can be identified with the surprising and so far not understood FIR feature reported in underdoped bilayer cuprates.     

Magneto-oscillations due to electron-electron interactions in the ac conductivity of a two-dimensional electron gas

Electron-electron interactions give rise to the correction, deltasigma(int)(omega), to the ac magnetoconductivity, sigma(omega), of a clean 2D electron gas that is periodic in omega_(c)(-1), where omega_(c) is the cyclotron frequency. Unlike conventional harmonics of the cyclotron resonance, which are periodic with omega, this correction is periodic with omega(3/2). Oscillations in deltasigma(int)(omega) develop at low magnetic fields, omega_(c)相似文献   

Qualitative modification of the high energy atomic photoionization cross section

It is demonstrated that the nonrelativistic high energy omega-->infinity behavior of the photoionization cross section of an nl atomic subshell, sigma(nl)(omega), for l>0 is independent of l and is given by sigma(nl)(omega) approximately 1/omega(9/2), rather than the previously generally accepted sigma(nl)(omega) approximately 1/omega(l+7/2). Furthermore, for l = 1, although the exponent does not change, the coefficient is significantly altered. This modification of sigma(nl)(omega) is due to the interchannel interaction between ns photoionization channels and l not equal0 channels in the atom. As a result, for the photoionization of l not equal0 electrons, the single-particle approximation is never correct in the omega-->infinity limit. This has important consequences for sum rule calculations.     

Theory of inelastic scattering from magnetic impurities

We use the numerical renormalization group method to calculate the single-particle matrix elements T of the many-body T matrix of the conduction electrons scattered by a magnetic impurity at T=0 temperature. Since T determines both the total and the elastic, spin-diagonal scattering cross sections, we are able to compute the full energy, spin, and magnetic field dependence of the inelastic scattering cross section sigma(inel)(omega). We find an almost linear frequency dependence of sigma(inel)(omega) below the Kondo temperature T(K), which crosses over to a omega(2) behavior only at extremely low energies. Our method can be generalized to other quantum impurity models.     

Observation of self-similar behavior of the 3D, nonlinear Rayleigh-Taylor instability

The Rayleigh-Taylor unstable growth of laser-seeded, 3D broadband perturbations was experimentally measured in the laser-accelerated, planar plastic foils. The first experimental observation showing the self-similar behavior of the bubble size and amplitude distributions under ablative conditions is presented. In the nonlinear regime, the modulation sigma(rms) grows as alpha(sigma)gt(2), where g is the foil acceleration, t is the time, and alpha(sigma) is constant. The number of bubbles evolves as N(t) alpha(omegat sq.rt(9) + C)(-4) and the average size evolves as (t) alpha omega(2)gt(2), where C is a constant and omega = 0.83 +/- 0.1 is the measured scaled bubble-merging rate.     

Characteristics of alternating current hopping conductivity in DNA sequences

This paper presents a model to describe alternating current (AC) conductivity of DNA sequences, in which DNA is considered as a one-dimensional (1D) disordered system, and electrons transport via hopping between localized states. It finds that AC conductivity in DNA sequences increases as the frequency of the external electric field rises, and it takes the form of σ_ac (ω)～ω ²\ln ²(1/ω). Also AC conductivity of DNA sequences increases with the increase of temperature, this phenomenon presents characteristics of weak temperature-dependence. Meanwhile, the AC conductivity in an off-diagonally correlated case is much larger than that in the uncorrelated case of the Anderson limit in low temperatures, which indicates that the off-diagonal correlations in DNA sequences have a great effect on the AC conductivity, while at high temperature the off-diagonal correlations no longer play a vital role in electric transport. In addition, the proportion of nucleotide pairs p also plays an important role in AC electron transport of DNA sequences. For p < 0.5, the conductivity of DNA sequence decreases with the increase of p, while for p ≥ 0.5, the conductivity increases with the increase of p.     

ab plane ac conductivity in the cuprates: pseudogap effects below Tc

Building on our understanding of the superfluid density rho(s)(T), we show how the pseudogap enters the in-plane optical conductivity sigma(omega,T) for temperatures T相似文献   

Correlation matrix of a completely polarized, statistically stationary electromagnetic field

It is shown that, for a 3 x 3 correlation matrix Wij(r, r, omega), (i, j = x, y, z) of the electric vector of a random, stationary electromagnetic field to represent a field that is completely polarized at a point r and frequency omega, each element of the matrix must factorize. More precisely, a necessary and sufficient condition for the correlation matrix to represent a fully polarized field at a point r is that the matrix has the form Wij(r, r, omega) = epsilon(i)*(r, omega)epsilon(j)(r, omega), where epsilon(i)(r, omega) (i = x, y, z) are deterministic functions, i.e., that all pairs of the Cartesian components of the electric field at a point r and frequency omega are completely correlated.     

Observation of the color-suppressed decay B( 0)-->D(0)pi(0)

We report the first observation of color-suppressed B( 0)-->D(0)pi(0), D(*0)pi(0), D0eta, and D0omega decays, and evidence for B( 0)-->D(*0)eta and D(*0)omega. The branching fractions are B(B( 0)-->D0pi(0)) = (3.1 +/- 0.4 +/- 0.5)x10(-4), B(B( 0) -->D(*0)pi(0)) = (2.7(+0.8+0.5)(-0.7-0.6))x10(-4), B(B( 0) --> D0eta) = (1.4(+0.5)(-0.4) +/- 0.3)x10(-4), B(B( 0) --> D0omega) = (1.8 +/- 0.5(+0.4)(-0.3))x10(-4), and we set 90% confidence level upper limits of B(B( 0) --> D(*0)eta)<4.6 x 10(-4) and B(B( 0)-->D(*0)omega)<7.9 x 10(-4). The analysis is based on a data sample of 21.3 fb(-1) collected at the Upsilon(4S) resonance by the Belle detector at the KEKB e(+)e(-) collider.     

Anisotropic electromagnetic response of lightly doped La2-xSrxCuO4 within the CuO2 planes

Using infrared spectroscopy, we show that spin self-organization in untwinned La2-xSrxCuO4 (LSCO) crystals has profound consequences for the dynamical conductivity sigma(omega). The electronic response of CuO2 planes acquires significant anisotropy in the spin ordered state with enhancement of the conductivity along the direction of the diagonal spin stripes by up to a factor of 2. An examination of the anisotropic response indicates that the diagonal spin texture in weakly doped LSCO is also accompanied by the modulation of charge density. The electronic response of the charge stripes is found to be gapless consistent with the hypothesis of the metallic ground state. Our experiments directly show that the striped ordered systems reveal new degrees of freedom not present in ordinary one-dimensional conductors.     

Anisotropy in conductance of a quasi-one-dimensional metallic surface state measured by a square micro-four-point probe method

We have devised a "square micro-four-point probe method" using an independently driven ultrahigh-vacuum four-tip scanning tunneling microscope, and succeeded for the first time to directly measure anisotropic electrical conductance of a single-atomic layer on a solid surface. A quasi-one-dimensional metal of a single-domain Si(111)4 x 1-In had a surface-state conductance along the metallic atom chains (sigma(axially)) to be 7.2(+/-0.6) x 10(-4) S/square at room temperature, which was larger than that in the perpendicular direction (sigma(radially)) by approximately 60 times. The sigma(axially) was consistently interpreted by a Boltzmann equation with the anisotropic surface-state band dispersion, while the sigma(radially) was dominated by a surface-space-charge-layer conductance.     

On interference effects in the elastodynamic Green's functions G33(x, omega) of Si and GaAs

In this paper, we analyze interference effects present in the elastodynamic Green's functions G33(x,omega) of the cubic crystals Si and GaAs, which are associated with folded portions of the wave surface of the slow transverse (ST) acoustic mode. G33(x,omega) represents the three dimensional extension of the amplitude distribution imaged in the transmission acoustic microscopy of these crystals. The intensity contrast for oscillations of a particular wave vector k in the interference pattern is determined essentially by the 3D Fourier transform of G33(x,omega)G33*(x,omega). According to the Fourier autocorrelation theorem, that transform is equivalent to the autocorrelation function of the corresponding distribution G(33)(k,omega) in k-space. We show that due to the linear mapping between k-space and the slowness vector s-space, the interference phenomena discussed here are related to geometrical features of the slowness surface of the ST mode. We present calculations of these effects based on the angular spectrum technique.     

透明光学树脂中Eu3+辐射参数的理论和实验研究

报道了一种新合成的含三元稀土配合物的透明光学树脂材料的辐射特性的研究。基于J-O参数理论,利用含稀土配合物Eu(TTA)3phen-0.31wt%的光学树脂的发射荧光光谱,计算了Eu3 在光学树脂基质中的J-O参数Ω2=10.139 4×10-20cm2,Ω4=3.810 9×10-20cm2,Ω6=9.050 7×10-20cm2。利用得到的J-O参数可以计算光学树脂中Eu3 的跃迁振子强度fcal,5D0激发态的辐射跃迁概率A(456.6 s-1)、辐射寿命τ(2 190.1μs),还计算了光学树脂中Eu3 的跃迁5D0→7FJ′(其中J′=1,2,4,6)的发射截面σ、荧光分支比β。通过分析计算得到的J-O参数可知,光学树脂中Eu3 的5D0亚稳态的寿命较长,跃迁5D0→7F2的发射截面最大,说明含稀土配合物的光学树脂具有作光放大或激光材料的潜在性。     

核介质中强子性质的手征σ模型研究

采用手征σ模型描述核多体系统,考虑真空极化的影响,首先由核物质的饱和性质确定模型参数,进一步研究了强子性质在核介质中的变化。手征σ模型的研究结果给出,核子和ω介子的有效质量随核物质密度的增大而减小,但σ介子的有效质量随密度的增大而增大。这些结果与不满足手征对称性的Walecka模型结果进行了比较。计算中采用的重整化方法会对结果有一定的影响。The modification of hadron masses in nuclear medium is studied by using the chiral sigma model, which is extended to generate the omega meson mass by the sigma condensation in the vacuum in the same way as the nucleon mass. The chiral sigma model provides proper equilibrium properties of nuclear matter. It is shown that the effective masses of both nucleons and omega mesons decrease in nuclear medium, while the effective mass of sigma mesons increases at finite density in the chiral sigma model. The resuits obtained in the chiral sigma model are compared with those obtained in the Walecka model, which includes sigma and omega mesons in a non-chiral fashion.     

Stereodynamics study of reactions N(~2D)+HD→NH+D and ND+H

The product polarizations of the title reactions are investigated by employing the quasi-classical trajectory (QCT) method. The four generalized polarization-dependent differential cross-sections (PDDCSs) $({2\pi } / \sigma )(\d\sigma _{00} / \d\omega _t )$, $({2\pi } / \sigma )(\d\sigma _{20} / \d\omega _t )$, $({2\pi } / \sigma )(\d\sigma _{22 + } / \d\omega _t )$, and $({2\pi } / \sigma )(\d\sigma _{21 - } / \d\omega _t )$ are calculated in the centre-of-mass frame. The distribution of the angle between ${{\bm k}}$ and ${{\bm j^\prime }}$, $P(\theta _r )$, the distribution of the dihedral angle denoting ${{\bm k}}${--}$\bm k^\prime $--$\bm j^\prime $ correlation, $P(\phi _r )$, as well as the angular distribution of product rotational vectors in the form of polar plots $P(\theta _r ,\phi _r )$ are calculated. The isotope effect is also revealed and primarily attributed to the difference in mass factor between the two title reactions.     

Coherent control of photofragment separation in the dissociative ionization of IBr

We have investigated coherent control of the dissociative ionization of IBr using phase-controlled two-color omega+2omega laser pulses with an intensity of 1.0 x 10(12) W/cm and a pulse duration of 130 fs. The directional asymmetries of the photofragment angular distributions showed oscillation behavior dependent on the relative phase difference between the omega and 2omega pulses. The phase dependencies of the directional asymmetries observed for iodine ions and bromine ions were out of phase with each other. This result shows that a phase-controlled omega+2omega optical field can produce molecular orientation in which the optical field discriminates between parallel and antiparallel configuration of molecules that have a permanent dipole.     

On quantum analogue of dynamical stabilisation of inverted harmonic oscillator by time periodical uniform field

Quantum analogue of stabilised forced oscillations around an unstable equilibrium position is explored by solving the non-stationary Schrödinger equation (NSE) of the inverted harmonic oscillator (IHO) driven periodically by spatial uniform field of frequency \(\Omega \), amplitude \(F_{0}\) and phase \(\phi \), i.e. the system with the Hamiltonian of \(\hat{{H}}=(\hat{{p}}^{2}/2m)-(m\omega ^{2}x^{2}/2)-F_0 x\sin \) \(\left( {\Omega t+\phi } \right) \). The NSE has been solved both analytically and numerically by Maple 15 in dimensionless variables \(\xi = x\sqrt{m\omega /\hbar }\hbox {, }f_0 =F_0 /\omega \sqrt{\hbar m\omega }\) and \(\tau =\omega t\). The initial condition (IC) has been specified by the wave function (w.f.) of a generalised Gaussian type which suits well the corresponding quantum IC operator. The solution obtained demonstrates the non-monotonous behaviour of the coordinate spreading \(\sigma \left( \tau \right) \hbox { =}\sqrt{\big ( {\overline{\Delta \xi ^{2}\big ( \tau \big )} } \big )}\) which decreases first from quite macroscopic values of \(\sigma _{0} =2^{12,\ldots ,25}\) to minimal one of \(\sim \!(1/\sqrt{2})\) at times \(\tau <\tau _0 =0.125\ln \!\left( {16\sigma _0^4 +1} \right) \) and then grows back unlimitedly. For certain phases \(\phi \) depending on the \(\Omega /\omega \) ratio and \(n=\log _2\!\sigma _0 \), the mass centre of the packet \(\xi _{\mathrm {av}}( \tau )= \overline{\hat{{x}}(\tau )} \cdot \sqrt{m\omega /\hbar }\) delays approximately two natural ‘periods’ \(\sim \!(4\pi /\omega )\) in the area of the stationary point and then escapes to ‘\(+\)’ or ‘?’ infinity in a bifurcating way.  For ‘resonant’ \(\Omega =\omega \), the bifurcation phases \(\phi \) fit well with the regression formula of Fermi–Dirac type of argument n with their asymptotic \(\phi ( {\Omega ,n\rightarrow \infty } )\) obeying the classical formula \(\phi _{\mathrm {cl}} ( \Omega )=-\hbox {arctg} \, \Omega \) for initial energy \(E = 0\) in the wide range of \(\Omega =2^{-4},...,2^{7}\).