Electron spin polarization in a rotating triplet

The triplet model of electron spin polarization in fluid media is evaluated. The model consists of an initial singlet molecule rotating in a static, externally applied magnetic field. Intersystem crossing into different zero-field states is represented by a rate matrix diagonal in the molecular frame, and this matrix is expressed as an effective spin operator. The triplet rotates, and the motion affects the polarization in the laboratory frame, and also causes spin relaxation in the triplet manifold. The triplet is chemically quenched, and the polarization appears in the doublet fragments. The model is treated in a density matrix formalism and on the basis of anisotropic rotational diffusion of the triplet molecule. Explicit expressions are obtained in terms of the molecular parameters, the various rate constants, and the rotational correlation time.     

Investigation of ultrafast nuclear spin polarization induced by short laser pulses

We theoretically investigate the dynamics of nuclear spin induced by short laser pulses and show that ultrafast nuclear spin polarization can take place. Combined use of the hyperfine interaction together with the static electric field is the key for that. Specifically we apply the idea to unstable isotopes, (27)Mg and (37)Ca, with nuclear spin of 1/2 and 3/2, respectively, and show that 88% and 62% of nuclear spin polarization can be achieved within a few to tens of ns, which is 2-3 orders of magnitude shorter than the time needed for any known optical methods. Because of its ultrafast nature, our scheme would be very effective not only for stable nuclei but also unstable nuclei with a lifetime as short as mus.     

磁性硅烯超晶格中电场调制的谷极化和自旋极化

研究了基于硅烯的静电势超晶格、铁磁超晶格、反铁磁超晶格中谷极化、自旋极化以及赝自旋极化的输运性质,分析了铁磁交换场、反铁磁交换场以及化学势对输运性质的影响,讨论了电场对谷极化、自旋极化以及赝自旋极化的调控作用.结果表明:当3种超晶格的晶格数达到10以上时,在硅烯超晶格中很容易实现100%的谷极化、自旋极化和赝自旋极化,而且通过调节超晶格上的外加电场可以使极化方向发生翻转,从而在硅烯超晶格中实现外电场对谷自由度、自旋自由度以及赝自旋自由度的操控.     

Splitting of spin excitations in nanometric rings induced by a magnetic field

We present a Brillouin light scattering investigation of the eigenmode spectrum of nanometric permalloy rings as a function of the applied magnetic field. In particular, different splitting effects induced by the applied magnetic field on the radial and azimuthal excitations have been observed and explained in terms of either mode localization or symmetry. The dynamical matrix approach has been used to calculate the whole set of eigenvectors and eigenvalues of the system, in both the vortex and saturated states.     

Ferroelectric polarization flop in a frustrated magnet MnWO4 induced by a magnetic field

The relationship between magnetic order and ferroelectric properties has been investigated for MnWO4 with a long-wavelength magnetic structure. Spontaneous electric polarization is observed in an elliptical spiral spin phase. The magnetic-field dependence of electric polarization indicates that the noncollinear spin configuration plays a key role for the appearance of the ferroelectric phase. An electric polarization flop from the b direction to the a direction has been observed when a magnetic field above 10 T is applied along the b axis. This result demonstrates that an electric polarization flop can be induced by a magnetic field in a simple system without rare-earth 4f moments.     

Controlling Luttinger liquid physics in spin ladders under a magnetic field

We present a 14N nuclear magnetic resonance study of a single crystal of CuBr4(C5H12N)2 (BPCB) consisting of weakly coupled spin-1/2 Heisenberg antiferromagnetic ladders. Treating ladders in the gapless phase as Luttinger liquids, we are able to fully account for (i) the magnetic field dependence of the nuclear spin-lattice relaxation rate T1(-1) at 250 mK and for (ii) the phase transition to a 3D ordered phase occurring below 110 mK due to weak interladder exchange coupling. BPCB is thus an excellent model system where the possibility to control Luttinger liquid parameters in a continuous manner is demonstrated and the Luttinger liquid model tested in detail over the whole fermion band.     

Electric field induced nuclear spin resonance mediated by oscillating electron spin domains in GaAs-based semiconductors

We demonstrate an alternative nuclear spin resonance using a radio frequency (rf) electric field [nuclear electric resonance (NER)] instead of a magnetic field. The NER is based on the electronic control of electron spins forming a domain structure. The rf electric field applied to a gate excites spatial oscillations of the domain walls and thus temporal oscillations of the hyperfine field to nuclear spins. The rf power and burst duration dependence of the NER spectrum provides insight into the interplay between nuclear spins and the oscillating domain walls.     

Enhanced magnetoresistance induced by spin transfer torque in granular films with a magnetic field

Spin-transfer torques (STT) provide a mechanism to alter the magnetic configurations of magnetic heterostructures, a result previously only achieved by an external magnetic field. In granular solids, we demonstrate a new form of STT effect that can be exploited to induce a large spin disorder when combined with a large magnetic field. We have obtained a very large magnetoresistance effect in excess of 400% at 4.2 K in a large magnetic field, the largest ever reported in any metallic systems. The STT characteristics of granular solids differ significantly from those of multilayers, showing no STT effect at low magnetic fields but prominent STT effects at high fields.     

Dynamics of nuclear polarization in InGaAs quantum dots in a transverse magnetic field

The time-resolved Hanle effect is examined for negatively charged InGaAs/GaAs quantum dots. Experimental data are analyzed by using an original approach to separate behavior of the longitudinal and transverse components of nuclear polarization. This made it possible to determine the rise and decay times of each component of nuclear polarization and their dependence on transverse magnetic field strength. The rise and decay times of the longitudinal component of nuclear polarization (parallel to the applied field) were found to be almost equal (approximately 5 ms). An analysis of the transverse component of nuclear polarization shows that the corresponding rise and decay times differ widely and strongly depend on magnetic field strength, increasing from a few to tens of milliseconds with an applied field between 20 and 100 mT. Current phenomenological models fail to explain the observed behavior of nuclear polarization. To find an explanation, an adequate theory of spin dynamics should be developed for the nuclear spin system of a quantum dot under conditions of strong quadrupole splitting.     

High-frequency dynamic nuclear polarization in the nuclear rotating frame

A proton dynamic nuclear polarization (DNP) NMR signal enhancement (epsilon) close to thermal equilibrium, epsilon = 0.89, has been obtained at high field (B(0) = 5 T, nu(epr) = 139.5 GHz) using 15 mM trityl radical in a 40:60 water/glycerol frozen solution at 11 K. The electron-nuclear polarization transfer is performed in the nuclear rotating frame with microwave irradiation during a nuclear spin-lock pulse. The growth of the signal enhancement is governed by the rotating frame nuclear spin-lattice relaxation time (T(1rho)), which is four orders of magnitude shorter than the nuclear spin-lattice relaxation time (T(1n)). Due to the rapid polarization transfer in the nuclear rotating frame the experiment can be recycled at a rate of 1/T(1rho) and is not limited by the much slower lab frame nuclear spin-lattice relaxation rate (1/T(1n)). The increased repetition rate allowed in the nuclear rotating frame provides an effective enhancement per unit time(1/2) of epsilon(t) = 197. The nuclear rotating frame-DNP experiment does not require high microwave power; significant signal enhancements were obtained with a low-power (20 mW) Gunn diode microwave source and no microwave resonant structure. The symmetric trityl radical used as the polarization source is water-soluble and has a narrow EPR linewidth of 10 G at 139.5 GHz making it an ideal polarization source for high-field DNP/NMR studies of biological systems.     

Consequences of the dynamical approach to the nuclear spin relaxation induced by molecular rotations in an external magnetic field

The evolution of two nuclear spins, interacting between themselves and with an external magnetic field, and situated on molecules of a fluid, is treated, under the assumption of the mixing property of molecular rotations, by the method of limit theorems for random differential equations. The limit diffusion behaviour of the system is derived and the results on relaxation times and (non-thermodynamical) equilibrium are obtained and discussed.     

Response of an isolated magnetic grain suspended in a liquid to a rotating field

We have studied the response of an isolated uniaxial magnetic grain suspended in a liquid to an applied fieldh rotating with frequencyω. In the presence of an applied static field (H?h), at low frequencies (i.e. for fast relaxation), the easy axis followsh, while at high frequencies the behavior is similar to that of a bulk sample. In zero static field, the response of a ferromagnetic grain is more complicated; there exists a critical frequencyω _e below which a steady state is reached, with the easy axis followingh. Forω>ω _e the mechanical behavior depends crucially on the initial conditions. Finally, a superparamagnetic grain has a (different) critical frequencyω _e, below which it reacts similarly to the ferromagnetic particle, while forω>ω _e it does not follow steadily the rotating field, but can only oscillate about its initial position.     

Electron spin polarization in field emission

The field emission microscope can be extended to determine the directionally weighted spin-dependent surface density of states of magnetic metals or to obtain information on the electronic structure of metal to magnetic-semiconductor interfaces. We describe the techniques of spin polarization measurements in field emission. The measurement of Kisker et al. on ferromagnetic EuS evaporated on W are discussed along with recent investigations on Ni.     

Dynamic nuclear polarization in electron spin echo

It is shown that under the action of a proper microwave pulse sequence the equilibrium polarization of the electron spin may be transferred dynamically to the longitudinal nuclear magnetization which will oscillate due to the nuclear spin precession around the effective fields relating to differnt electron quantum number manifolds. These oscillations may be measured directly in the radiofrequency band. Analytical formulae are obtained for the case when all the nuclei coupled to an unpaired electron have spins of 1/2.     

Dynamic nuclear polarization by electrical spin injection in ferromagnet-semiconductor heterostructures

Electrical spin injection from Fe into AlxGa1-xAs quantum well heterostructures is demonstrated in small (<500 Oe) in-plane magnetic fields. The measurement is sensitive only to the component of the spin that precesses about the internal magnetic field in the semiconductor. This field is much larger than the applied field and depends strongly on the injection current density. Details of the observed hysteresis in the spin injection signal are reproduced in a model that incorporates the magnetocrystalline anisotropy of the epitaxial Fe film, spin relaxation in the semiconductor, and the dynamic polarization of nuclei by the injected spins.     

Eddy-current loss in a rotating magnetic field

The eddy-current loss is calculated for nonferromagnetic disks in a rotating magnetic field. The power loss is found as a function of the magnetic field intensity, the field rotation velocity, and the disk dimensions. The eddy-current loss was measured experimentally in rotating fields in copper, aluminum, and zinc disks; a good agreement was found with the calculated values.Translated from Izvestiya Vysshikh Uchebnykh Zavedenii, Fizika, No. 1, pp. 38–42, January, 1971.