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1.
I. V. Kedyk P. Mathey G. Gadret A. A. Grabar K. V. Fedyo I. M. Stoika I. P. Prits Y. M. Vysochanskii 《Applied physics. B, Lasers and optics》2008,92(4):549-554
In this work we report results on electro-physical, optical and photorefractive investigations for Sb-doped Sn2P2S6 crystals. The crystals are obtained by two methods: the vapour-transport technique and the Bridgman technique using stoichiometric
Sn2P2S6 composition with different amounts of antimony in the initial compound. The good optical quality of the crystals obtained
with the Bridgman technique is underlined. The dependences of the photorefractive two-beam coupling coefficient and the grating
build-up time are investigated at the wavelength of 633 nm. It is found that the sample doped with 1.5% of Sb is characterized
by an optimal combination of the main photorefractive parameters exhibiting a fairly high two-beam coupling coefficient (up
to 20 cm−1) and a short response time (1.3 ms) that is the shortest among all the previously studied Sn2P2S6 crystals in the red spectral region. 相似文献
2.
Tingyin Ning Cong Chen Yueliang Zhou Heng Lu Dongxiang Zhang Hai Ming Guozhen Yang 《Applied Physics A: Materials Science & Processing》2009,94(3):567-570
CaCu3Ti4O12 (CCTO) thin films were successfully prepared on LaAlO3 substrates by pulsed laser deposition technique. We measured the nonlinear optical susceptibility of the thin films using
Z-scan method at a wavelength of 532 nm with pulse durations of 25 ps and 7 ns. The large values of the third-order nonlinear
optical susceptibility, χ
(3), of the CCTO film were obtained to be 2.79×10−8 esu and 3.30×10−6 esu in picosecond and nanosecond time regimes, respectively, which are among the best results of some representative nonlinear
optical materials. The origin of optical nonlinearity of CCTO films was discussed. The results indicate that the CCTO films
on LaAlO3 substrates are promising candidate materials for applications in nonlinear optical devices. 相似文献
3.
The absorption spectra, fluorescence spectrum and fluorescence decay curve of Nd3+ ions in CaNb2O6 crystal were measured at room temperature. The peak absorption cross section was calculated to be 6.202×10−20 cm2 with a broad FWHM of 7 nm at 808 nm for E//a light polarization. The spectroscopic parameters of Nd3+ ions in CaNb2O6 crystal have been investigated based on Judd-Ofelt theory. The parameters of the line strengths Ω
t
are Ω
2=5.321×10−20 cm2,Ω
4=1.734×10−20 cm2,Ω
6=2.889×10−20 cm2. The radiative lifetime, the fluorescence lifetime and the quantum efficiency are 167 μs, 152 μs and 91%, respectively. The fluorescence branch ratios are calculated to be β
1=36.03%,β
2=52.29%,β
3=11.15%,β
4=0.533%. The emission cross section at 1062 nm is 9.87×10−20 cm2. 相似文献
4.
L. Kovács M. Mazzera E. Beregi R. Capelletti 《Applied physics. B, Lasers and optics》2009,94(2):273-277
Several weak absorption bands have been observed in the optical absorption spectra of pure and rare-earth-doped YAl3(BO3)4 single crystals in the 3350– 3650 cm−1 wave number region. Two of them, peaking at about 3377 cm−1 and 3580 cm−1 in the 8 K spectra, appear in most of the samples. They are tentatively attributed to the stretching mode of OH− ions incorporated in the crystal during the growth. An additional absorption band at about 5250 cm−1 at 8 K has also been detected in almost all samples. The temperature and polarization dependences of these bands, and their
possible origin, are discussed. 相似文献
5.
E. Ambite D. Balboa J. L. Plaza L. Arizmendi 《Applied physics. B, Lasers and optics》2009,95(3):447-452
We have investigated the properties of thermally fixed holograms in LiNbO3 crystals doped with the optical damage inhibitor Zn as well as the photorefractive Fe dopants. Time decays of fixed holograms
at different temperatures showed a single thermally activated process with an activation energy of ∼1.08 eV. We have also
studied the effect of an external electric field on the diffraction efficiency of these holograms. Results analysis has provided
a new method to determine the photovoltaic field of the samples as well as the effective concentration of photorefractive
traps. 相似文献
6.
B. Xu X. Li J. Sun L. Yi 《The European Physical Journal B - Condensed Matter and Complex Systems》2008,66(4):483-487
Using first-principles calculations based on density-functional theory in
its local-density approximation, we investigated the Electronic structure,
ferroelectricity and optical properties of CaBi2Ta2O9 (CBT)
for the first time. It is found that CBT compound has an indirect band gap
of 3.114 eV and the O 2s and 2p states are strongly hybridized with the 6s
states of Bi which belong to the (Bi2O2)2+ planes. The quite
strong Ta–O and Bi–O hybridization is the primary source for
ferroelectricity. Our results imply that the interaction between Bi and O is
highly covalent. The anisotropy occurs mainly above 4 eV in the optical
properties. The different optical properties have been discussed. 相似文献
7.
A. Shumelyuk M. Wesner M. Imlau S. Odoulov 《Applied physics. B, Lasers and optics》2009,95(3):497-503
The intensity dependence of the photorefractive response of Sn2P2S6 is studied for the Kr+-laser wavelength of 647 nm and pump-beam intensities of up to 10 W/cm2. A considerable enhancement of the two-beam coupling gain factor with increasing intensity at a grating spacing of ≃1 μm
is attributed to a light-induced increase of the effective trap density. The large gain reached at high intensities is applied
for the build up of a double phase conjugate mirror with a sub-millisecond switch-on time. 相似文献
8.
S. M. Kostritskii 《Applied physics. B, Lasers and optics》2009,95(3):421-428
Original results on investigation of the photorefractive effect in straight channels and integrated-optical circuits such
as a directional coupler, Y-splitter and Mach–Zehnder interferometer, exploiting titanium-indiffused and proton-exchanged
LiNbO3 waveguides, are presented. It has been found that the photorefractive damage is non-negligible for IR radiation with wavelengths
near 1.5 μm in all circuits studied. The new methods for accurate evaluation of small extents of photorefractive effect are
proposed. 相似文献
9.
A series of Zn:Fe:LiNbO3 crystals were prepared by the Czochralski technique with 0.015 wt. % Fe2O3 content and various concentrations of ZnO. The ultraviolet-visible absorption spectra and the infrared absorption spectra
of the Zn:Fe:LiNbO3 crystals were detected in order to investigate their defect structure. Their optical damage resistance was characterized
by the photoinduced birefringence change and transmission facula distortion method. The optical damage resistance of the Zn:Fe:LiNbO3 crystals increases remarkably when the concentration of ZnO is over its threshold concentration (more than 6.0 mol. %). The
effects of defects on the optical damage resistance of the Zn:Fe:LiNbO3 crystals are discussed in detail.
Received: 25 October 2002 / Revised version: 6 January 2003 / Published online: 22 May 2003
RID="*"
ID="*"Corresponding author. Fax: +86-451/2300-926, E-mail: zzxxhhdoctor@sina.com 相似文献
10.
A. Shumelyuk D. Barilov S. Odoulov E. Krätzig 《Applied physics. B, Lasers and optics》2003,76(4):417-421
We apply, for the first time to our knowledge, photorefractive grating spectroscopy to obtain not-yet-known data on the anisotropy
of the dielectric permittivity of Sn2P2S6. Two independent techniques are used, one based on measurements of the amplitude of the space-charge field grating as a function
of grating spacing and the other based on measurements of the grating decay time, also as a function of grating spacing. Both
techniques provide close values for the anisotropy, which appears to be well pronounced, a ratio εxx/εzz≈4 is revealed for two of the three independent components of the dielectric tensor. Our data also allow us to conclude that
the charge mobility is nearly isotropic in the same plane, μxx/μzz≈1.
Received: 2 December 2002 / Published online: 26 March 2003
RID="*"
ID="*"Corresponding author. Fax: +380-44/265-2359, E-mail: odoulov@iop.kiev.ua 相似文献
11.
S. A. Ahmed 《Applied Physics A: Materials Science & Processing》2008,92(3):565-570
Thermoelectric power and electrical resistivity measurements on polycrystalline samples of Bi2Se3 and stoichiometric ternary compound in the quasi-binary system SnSe–Bi2Se3 in the temperature range of 90–420 K are presented and explained assuming the existence of an impurity band. The variation
of the electron concentration with temperature above 300 K is explained in terms of the thermal activation of a shallow donor,
by using a single conduction band model. The density of states effective mass m
*=0.15m
0 of the electrons, the activation energy of the donors, their concentration, and the compensation ratio are estimated. The
temperature dependence of the electron mobility in conduction band is analyzed by taking into account the scattering of the
charge carriers by acoustic phonon, optical phonon, and polar optical phonon as well as by alloy and ionized impurity modes.
On the other hand, by considering the two-band model with electrons in both the conduction and impurity bands, the change
in the electrical resistivity with temperature between 420 and 90 K is explained. 相似文献
12.
H. J. Eichler R. Elschner G. Heppke R. Macdonald H. Schmid 《Applied physics. B, Lasers and optics》1995,61(1):59-62
Low-molar-mass liquid crystals consisting of a binary nematic mixture of two-naphthylester which exhibit an anisotropic glassy state at room temperature have recently proven to be a suitable material for erasable optical data-storage applications. Using the holographic-grating technique, it is shown that more than 1000 all-optical write, read and erase cycles can be realized without remarkable loss of reversibility. The recording intensities are of the order of 100 W/cm2 and optical erasure can be achieved with about twice that intensity. The times for recording and erasure of the optical gratings range on the millisecond scale and the stored gratings persist several months with a diffraction efficiency of typically 1 %. The spatial resolution has been proven down to 2 µm so far. The obtained results are compared with other reversible recording materials. 相似文献
13.
Mingfu Zhang Hengzhi Chen Bin Yang Wenwu Cao 《Applied Physics A: Materials Science & Processing》2009,97(4):741-744
Layered-perovskite ferroelectric Bi2.85La0.15TiNbO9 (LBTN) optical waveguiding thin films were grown on fused silica substrates by pulsed laser deposition (PLD). X-ray diffraction
(XRD) revealed that the film is highly (00l) textured. We observed sharp and distinct transverse electric (TE) and transverse magnetic (TM) multimodes and measured the
refractive indices of LBTN thin films at 632.8 nm. The ordinary and extraordinary refractive indices were calculated to be
n
TE=2.358 and n
TM=2.464, respectively. The film homogeneity and the film-substrate interface were analyzed using an improved version of the
inverse Wentzel–Kramer–Brillouin (iWKB) method. The refractive index of the film remains constant at n
0 within the waveguiding layer. The average transmittance of the film is 70% in the wavelength range of 400–1400 nm and the
optical waveguiding properties were evaluated by the optical prism coupling method. Our results showed that the LBTN films
are very good electro-optical active material. 相似文献
14.
The nonvolatile photorefractive characteristics of LiNbO3:Fe:Cu and In-doped LiNbO3:Fe:Cu crystals are investigated. The stronger nonvolatile blue photorefraction observed can be ascribed to its remarkable
characteristic of being in phase between the two gratings recorded in shallow and deep trap centers, which is one or two orders
of magnitude higher than those obtained in conventional two-color recordings under the same recording conditions. Furthermore,
it is interesting that, compared with LiNbO3:Fe:Cu, the recording properties, such as the saturation refractive index change, nonvolatile sensitivity and response time
at 488 nm wavelength are enhanced in LiNbO3:In:Fe:Cu crystals under the same recording conditions. The so-called damage-resistant dopants such as In3+ ions in red photorefraction are not damage resistant at 488 nm wavelength but they enhance the blue photorefraction.
PACS 42.40.Ht; 42.40.Lx; 42.70.Ln 相似文献
15.
Qiming Liu Xuan He Ting Hu Chang Gao Yanan Hou Xiujian Zhao 《Applied Physics A: Materials Science & Processing》2011,102(1):245-249
0.56GeS2-0.24Ga2S3-0.2KI (mol%) chalcohalide glass was prepared and second-harmonic generation was observed by the thermal poling process. Second-order
optical nonlinearity in the glass was also investigated by different poling temperature, voltage and time to optimize the
poling parameters to improve χ
(2). The maximum χ
(2) in our study as large as 3.74 pm/V was obtained under the optimized poling condition with 5.2 kV, 260°C and 120 minutes. 相似文献
16.
T. Rudolf Ch. Kant F. Mayr M. Schmidt V. Tsurkan J. Deisenhofer A. Loidl 《The European Physical Journal B - Condensed Matter and Complex Systems》2009,68(2):153-160
We studied the optical properties of antiferromagnetic ZnCr2Se4 by infrared spectroscopy up to 28,000 cm-1 and for temperatures from 5 to 295 K. At the magnetic phase transition at 21 K, one of the four phonon modes reveals a clear
splitting of 3 cm-1 as a result of spin-phonon coupling, the other three optical eigenmodes only show shifts of the eigenfrequencies. The antiferromagnetic
ordering and the concomitant splitting of the phonon mode can be suppressed in a magnetic field of 7 T. At higher energies
we observed a broad excitation band which is dominated by a two-peak-structure at about 18,000 cm-1 and 22,000 cm-1, respectively. These energies are in good agreement with the expected spin-allowed crystal-field transitions of the Cr3+ ions. The unexpected strength of these transitions with d-d character is attributed to a considerable hybridization of the
selenium p with the chromium d orbitals. 相似文献
17.
S. Vatnik M. C. Pujol J. J. Carvajal X. Mateos M. Aguiló F. Díaz V. Petrov 《Applied physics. B, Lasers and optics》2009,95(4):653-656
The three thermo-optic coefficients of the biaxial laser host KLu(WO4)2 are measured at 633 nm by a deflection method. Their values at 300 K amount to ∂
n
g
/∂
T=−7.4×10−6 K−1; ∂
n
m
/∂
T=−1.6×10−6 K−1 and ∂
n
p
/∂
T=−10.8×10−6 K−1. Nearly athermal propagation directions are found for polarizations along the N
m
and N
p
dielectric axes. 相似文献
18.
N. Coluccelli G. Galzerano L. Bonelli A. Toncelli A. Di Lieto M. Tonelli P. Laporta 《Applied physics. B, Lasers and optics》2008,92(4):519-523
We present a comparative analysis on the growth, the spectroscopic features, and the cw laser action of room-temperature Yb(5%):LiYF4 (YLF) and Yb(10%):KYF4 (KYF) crystals. Optical slope efficiencies of 33% and 52% have been demonstrated for Yb:YLF and Yb:KYF crystals, respectively.
A remarkable wide wavelength tunability from 1.01 to 1.07 μm has been obtained for both laser crystals. 相似文献
19.
V. P.S. Awana A. Vajpayee M. Mudgel V. Ganesan A. M. Awasthi G. L. Bhalla H. Kishan 《The European Physical Journal B - Condensed Matter and Complex Systems》2008,62(3):281-294
We report synthesis, structure/micro-structure, resistivity under magnetic
field [ρ(T)H], Raman spectra, thermoelectric power S(T), thermal conductivity
κ(T), and magnetization of ambient pressure argon annealed
polycrystalline bulk samples of MgB2, processed under identical
conditions. The compound crystallizes in hexagonal structure with space
group P6/mmm. Transmission electron microscopy (TEM) reveals electron micrographs
showing various types of defect features along with the presence of 3–4 nm
thick amorphous layers forming the grain boundaries of otherwise crystalline
MgB2. Raman spectra of the compound at room temperature exhibited
characteristic phonon peak at 600 cm-1. Superconductivity is observed
at 37.2 K by magnetic susceptibility χ(T), resistivity ρ(T), thermoelectric power
S(T), and thermal conductivity κ(T) measurements. The power law fitting
of ρ(T) give rise to Debye temperature (ΘD) at 1400 K which is
found consistent with the theoretical fitting of S(T), exhibiting Θ
D of 1410 K and carrier density of 3.81 × 1028/m3. Thermal
conductivity κ(T) shows a jump at 38 K, i.e., at Tc, which was
missing in some earlier reports. Critical current density (Jc) of up to
105 A/cm2 in 1–2 T (Tesla) fields at temperatures (T) of up to 10 K
is seen from magnetization measurements. The irreversibility field, defined
as the field related to merging of M(H) loops is found to be 78, 68 and 42 kOe
at 4, 10 and 20 K respectively. The superconducting performance parameters
viz. irreversibility field (Hirr) and critical current density
Jc(H) of the studied MgB2 are improved profoundly with addition of
nano-SiC and nano-diamond. The physical property parameters measured for
polycrystalline MgB2 are compared with earlier reports and a
consolidated insight of various physical properties is presented. 相似文献
20.
Indium Tin Oxide (ITO) films prepared by reactive rf sputtering show excellent properties for optical recording applications in a very narrow range of oxygen partial pressure (around 4×10–5 Torr). This narrow range is at the edge of a plateau in the electrical conductivity of the films. A small increase in the oxygen partial pressure (P(O2)5×10–5 Torr) causes a large and abrupt change in the electrical conductivity as well as in the structural and optical properties of these films. In addition, irradiating films at the edge of the plateau (P(O2)4×10–5) with a low-power pulsed laser (25 mW) yields transparent films. These results suggest that the same mechanism may be responsible for the opaque to transparent transformations observed in these experiments. 相似文献