丙三醇溶液声致发光中的黑体辐射谱

利用U型管圆锥泡声致发光装置,测量到了丙三醇溶液中圆锥泡声致发光的光谱和光脉冲。结果表明,测量得到的发光光谱为光滑的连续谱,且与理论模拟得到的黑体辐射谱相吻合,拟合温度分布于2 600～3 500 K范围内。文章从空间和时间两方面分析了圆锥泡空化发光中存在黑体辐射的原因：较大的气泡体积(气泡塌缩半径为1.4 cm)与较长的发光时间(几十微秒)。另外,实验研究表明随着发光波长的增长,光脉冲宽度变宽,从而进一步证明了圆锥泡声致发光中的黑体辐射机制。最后,利用测量得到的发光光谱和脉冲计算得到了发光光强为0.18 J,远远高于其他方式得到的声致发光光强。     

乙二醇溶液中圆锥泡声致发光的发光特性

利用一种改进后的U形管圆锥泡声致发光装置，研究了乙二醇溶液中圆锥泡声致发光的发光特性.实验结果表明，利用乙二醇溶液可以得到超强的单个发光脉冲，其脉冲宽度可以达到150 μs，其值远远高于其他方式产生的声致发光的脉冲宽度.测量得到的光谱为一从紫外到可见光波长范围的连续谱，在589 nm附近叠加有钠的3P-3S原子发射谱线.在钠的原子发射谱线两侧测量得到了Na-Ar分子激发态跃迁形成的蓝卫星带，并在声致发光实验中测得了Na-Ar的红卫星带以及钠的3S-4S原子发射谱线. 关键词： 圆锥泡声致发光 光脉冲 光谱 卫星带     

圆锥气泡发光的光谱性质

在改进的U型管装置中观察到一种圆锥气泡声致发光现象。声致发光产生的单个光脉冲的能量可达到约1.4 毫焦. 脉冲宽度约100 毫秒。发光光谱由连续光谱上叠加C2,CN,和CH的激发态光谱构成。这种圆锥气泡声致发光为单泡声致发光和多泡声致发光提供了一种联系。     

声致发光的流体动力学实验方法

介绍两种使用流体动力学实现声致发光的方法:刹管法和U管圆锥泡法.这两种方法的设备简单,操作方便,容易在普通物理实验中进行,所得结果和传统单泡声致发光有所不同.U管圆锥泡法创造了发光功率和单脉冲能量的新记录,并首次用条纹相机得到了时间分辨发射光谱.     

乙二醇溶液中直管圆锥泡声致发光光脉冲和光谱

在U型管声致发光装置的基础上建立了一套新型的声致发光装置—直管圆锥泡声致发光装置,详细地介绍了此装置的结构和实验操作步骤,利用此装置得到了超强的发光脉冲。测量得到了乙二醇溶液中圆锥泡声致发光的发光脉冲,结果显示脉冲半宽度大约为80 μs左右,远远高于其他声致发光形式所产生的脉冲宽度,这主要是由于圆锥泡可以获得远远高于超声声致发光中气泡所能得到的能量。发光光谱为一从紫外光至可见光波长范围的连续谱,上面叠加C₂有d3Π_g→d3Π_u的跃迁形成的五个序列谱带,分别对应于Δν＝-2,Δν＝-1,Δν＝0,Δν＝1和Δν＝2;同时叠加有CN的B2Σ+→X 2Σ+跃迁形成的3个序列谱带和CH的A2Δ→X 2Π 跃迁谱带。特别是实验中测量得到了斯旺带光谱序列谱带清晰的振动结构。最后,通过与理论模拟得到的斯旺带光谱相对强度的比较,估算得到了C₂分子的振动温度大约为(4 200±200) K。     

GaP:N光致发光的脉冲测量

本文介绍了由脉冲式溴代铜激光器和Boxcar平均器等组成的光致发光测量装置.测量了液相外延片GaP:N在不同温度(80～300K)下和不同厚度处的光致发光谱.根据谱图,分析了绿色发光机理.     

发光光弹性涂层折射率测量方法

涂层的折射率是发光光弹性涂层方法采用斜射法应变分离时不可缺少的参数之一. 通过对发光光弹性涂层受斜入射光波激发时, 发射光波沿入射光波原路径返回振幅变化的理论分析, 提出一种基于发光涂层光学菲涅耳响应的折射率在线测量方法. 实验测量了罗丹明B为发光染料的发光光弹性涂层在入射角为60°、波长为465 nm光波激发下的涂层折射率. 测量结果表明: 新的折射率测量方法是可行的, 对于其他用途的发光涂层折射率测量同样适用. 关键词： 折射率 光学测量 光学涂层 光致发光     

激光脉冲宽度对远距离尾流气泡后向检测的影响

为了分析激光脉冲宽度对远距离尾流气泡后向检测的影响,基于Fournier Forand体积散射函数,通过Monte Carlo方法建立了水中激光脉冲后向散射信号时域特征的分析模型.利用该模型研究了初始激光脉冲宽度不同时,水中远距离舰船尾流气泡的激光脉冲后向散射信号变化情况.结果表明:随着初始激光脉冲宽度的增加,后向散射...     

激光脉冲宽度对远距离尾流气泡后向检测的影响

为了分析激光脉冲宽度对远距离尾流气泡后向检测的影响,基于Fournier Forand体积散射函数,通过Monte Carlo方法建立了水中激光脉冲后向散射信号时域特征的分析模型.利用该模型研究了初始激光脉冲宽度不同时,水中远距离舰船尾流气泡的激光脉冲后向散射信号变化情况.结果表明:随着初始激光脉冲宽度的增加,后向散射信号中水体散射信号与尾流气泡回波信号的轮廓变得模糊|当脉冲宽度增大到一定程度时,无法从后向散射信号中辨别出回波信号|并且,随着尾流区气泡散射强度的减小以及气泡区与检测器之间距离的减短,这种变化趋势变得更加明显.基于仿真结果,提出一种基于逆卷积运算的尾流气泡回波信号提取方法.     

有机溶液中圆锥泡声致发光

在U形管声致发光装置的基础上建立了一套新型的声致发光装置——直管圆锥泡声致发光装置. 利用此装置以有机溶液为液体介质得到了超强的发光脉冲并测量得到了其发光光谱. 结果表明发光光谱为一从紫外光至可见光波长范围的连续谱,上面叠加有C₂的d³Π_g→d³Π_u跃迁形成的五个序列谱带,分别对应于Δv=-2,Δv=-1,Δv=0,Δv< 关键词： 声致发光 光谱 斯旺带 振动温度     

Conical bubble photoluminescence from rhodamine 6G in 1, 2-propanediol

A modified U-tube conical bubble sonoluminescence device is used to study the conical bubble photoluminescence. The spectra of conical bubble sonoluminescence at different concentrations of rhodamine 6G (Rh6G) solution in 1,2-propanediol have been measured. Results show that the sonoluminescence from the conical bubbles can directly excite Rh6G, which in turn can fluoresce. The light emission of this kind is referred to as conical bubble photoluminescence. The maximum of fluorescence spectral line intensity in the conical bubble photoluminescence has a red shift in relative to that of the standard photo-excited fluorescence, which is due to the higher self-absorption of Rh6G, and the spectral line of conical bubble photoluminescence is broadened in width compared with that of photo-excited fluorescence.     

Influence of ultrasonic frequency on multibubble sonoluminescence

Computer simulations of bubble oscillations are performed under conditions of multibubble sonoluminescence (MBSL) in water for various ultrasonic frequencies. The range of the ambient bubble radius for sonoluminescing bubbles narrows as the ultrasonic frequency increases; at 20 kHz it is 0.1-100 microm while at 1 MHz it is 0.1-3 microm. At 1 MHz, any sonoluminescing bubble disintegrates into a mass of smaller bubbles in a few or a few tens of acoustic cycles, while at 20 kHz and 140 kHz some sonoluminescing bubbles are shape stable. The mechanism of the light emission also depends on the ultrasonic frequency. As the ultrasonic frequency increases, the amount of water vapor trapped inside bubbles at the collapse decreases. As a result, MBSL originates mainly in plasma emissions at 1 MHz while it originates in chemiluminescence of OH radicals and plasma emissions at 20 kHz.     

A unique circular path of moving single bubble sonoluminescence in water

Based on a quasi-adiabatic model,the parameters of the bubble interior for a moving single bubble sonoluminescence (m-SBSL) in water are calculated.By using a complete form of the hydrodynamic force,a unique circular path for the m-SBSL in water is obtained.The effect of the ambient pressure variation on the bubble trajectory is also investigated.It is concluded that as the ambient pressure increases,the bubble moves along a circular path with a larger radius and all bubble parameters,such as gas pressure,interior temperature and light intensity,increase.A comparison is made between the parameters of the moving bubble in water and those in N-methylformamide.With fluid viscosity increasing,the circular path changes into an elliptic form and the light intensity increases.     

光在水中吸附膜层气泡上的散射特性

光在水中大尺度气泡上散射特性的研究多是基于Davis模型.该模型没有考虑到吸附膜层对光在气泡上散射的影响,而海水中的大多数气泡都有膜层附着,这些膜层会影响到气泡的光散射特性.本文从几何光学的角度出发,建立了吸附膜层气泡的体积散射函数简化公式.在此理论基础上,模拟计算了尺度远大于入射光波长的大气泡散射光强分布曲线,得出光照射下气泡上散射光强的远场特性,讨论了影响气泡散射光强分布的主要因素.并与无膜气泡光散射分布曲线比较,讨论了油膜膜厚、折射率等参量对气泡的光散射特性影响.得出结论:吸附膜层气泡的光强分布曲线与无膜气泡相似,但吸附膜层会削弱前向散射光,增强后向散射光.     

Calculation of light emission in sonoluminescence

We modify a uniform model of single bubble sonoluminescence, in which heat diffusion, water vapor diffusion and chemical reactions are included to describe the bubble dynamics, and the processes of electron-atom bremsstrahlung, electron-ion bremsstrahlung and recombination radiation, radiative attachment of electrons to atoms and molecules, line emissions of OH radicals and Na atoms are taken into account to calculate the light emission. With this model, we compute the light pulse width, the photon number per flash, the continuum and line spectra and the gas species as the products of chemical reactions, and try to compare with all the experimental data available. We obtain good agreement with the observations of Ar and Xe bubbles in many cases, but fail to match the experimental data of the photon number per flash. We also find that for He bubble the computed photon number is always too small to interpret the observations. Supported by the National Natural Science Foundation of China (Grant Nos. 10674081 and 10434070)     

Analysis of high-frequency wind-driven ambient noise in shallow brackish water

Ambient noise spectra in a shallow brackish water environment were found to be steeper than expected at frequencies above 10 kHz. The high-frequency behavior of the spectra was resolved by modeling dispersion and noise in bubbly water. Bubble size distributions fitted to the brackish water spectra exhibit a distinctive maximum in the radius range 0.1-0.3 mm, and a substantial drop in bubble density below a radius of 0.1 mm. The brackish water distributions were tied to an oceanic spectrum with a spectral slope of 5.7 dB/octave obtained with a -3 / 2 power law dependence of bubble size density on radius.