Optical whispering‐gallery mode (WGM) microcavities featuring ultrahigh Q factors and small mode volumes enhance significantly the interaction between light and matter, becoming an excellent platform for achieving ultralow‐threshold microlasers. However, the emission of traditional WGMs is isotropic due to the rotational symmetry of cavity geometries, which hinders the potential photonics applications. In this review, the progress in WGM microcavities towards unidirectional laser emission is summarized. When a subwavelength scatterer is placed on the boundary of the microcavity, the unidirectional emission occurs due to the collimation effect of the microcavity‐enhanced scattering field. Furthermore, microcavities deformed from the circular shapes can not only produce the chaos‐assisted unidirectional emission, but also maintain high Q factors by special design and fabrication processes. Finally, gratings along the circumference of the WGM microdisk or microring can scatter the WGMs in the vertical direction. The review also lists several important applications of these types of microcavities, such as wide‐band laser illumination source, free‐space coupling, evanescent‐field enhancement, optical energy storage, and sensing.
This work takes inspiration from chemistry where the spectral characteristics of the molecules are determined by hybridization of electronic states evolving from the individual atomic orbitals. Based on analogy between quantum mechanics and the classical electrodynamics, we sorted dielectric microspheres with almost identical positions of their whispering gallery mode (WGM) resonances. Using these microspheres as classical photonic atoms, we assembled them in a wide range of structures including linear chains and planar photonic molecules. We studied WGM hybridization effects in such structures using side coupling by tapered microfibers as well as finite difference time domain modeling. We demonstrated that the patterns of WGM spectral splitting are representative of the symmetry, number of constituting atoms and topology of the photonic molecules which in principle can be viewed as “spectral signatures” of various molecules. We also show new ways of controlling WGM coupling constants in such molecules. Excellent agreement was found between measured transmission spectra and spectral signatures of photonic molecules predicted by simulation.
A necessary condition for generation of bright soliton Kerr frequency combs in microresonators is to achieve anomalous group velocity dispersion (GVD) for the resonator modes. This condition is hard to implement in the visible as well as ultraviolet since the majority of optical materials are characterized with large normal GVD in these wavelength regions. We overcome this challenge by borrowing ideas from strongly dispersive coupled systems in solid state physics and optics. We show that photonic compound ring resonators can possess large anomalous GVD at any desirable wavelength, even if each individual resonator is characterized with normal GVD. Based on this concept, we design a mode‐locked frequency comb with thin‐film silicon nitride compound ring resonators in the vicinity of the rubidium D1 line (794.6 nm) and propose to use this optical comb as a flywheel for chip‐scale optical clocks.
Monocrystalline titanium dioxide (TiO2) micro‐spheres support two orthogonal magnetic dipole modes at terahertz (THz) frequencies due to strong dielectric anisotropy. For the first time, we experimentally detected the splitting of the first Mie mode in spheres of radii m through near‐field time‐domain THz spectroscopy. By fitting the Fano lineshape model to the experimentally obtained spectra of the electric field detected by the sub‐wavelength aperture probe, we found that the magnetic dipole resonances in TiO2 spheres have narrow linewidths of only tens of gigahertz. Anisotropic TiO2 micro‐resonators can be used to enhance the interplay of magnetic and electric dipole resonances in the emerging THz all‐dielectric metamaterial technology.
We present a general theory of circular dichroism in planar chiral nanostructures with rotational symmetry. It is demonstrated, analytically, that the handedness of the incident field's polarization can control whether a nanostructure induces either absorption or scattering losses, even when the total optical loss (extinction) is polarization‐independent. We show that this effect is a consequence of modal interference so that strong circular dichroism in absorption and scattering can be engineered by combining Fano resonances with planar chiral nanoparticle clusters.
Stimulated emission depletion (STED) microscopy has become a powerful imaging and localized excitation method, breaking the diffraction barrier for improved spatial resolution in cellular imaging, lithography, etc. Because of specimen‐induced aberrations and scattering distortion, it is a great challenge for STED to maintain consistent lateral resolution deep inside specimens. Here we report on deep imaging STED microscopy using a Gaussian beam for excitation and a hollow Bessel beam for depletion (GB‐STED). The proposed scheme shows an improved imaging depth of up to about 155 μm in a solid agarose sample, 115 μm in polydimethylsiloxane, and 100 μm in a phantom of gray matter in brain tissue with consistent super resolution, while standard STED microscopy shows a significantly reduced lateral resolution at the same imaging depth. The results indicate the excellent imaging penetration capability of GB‐STED, paving the way for deep tissue super‐resolution imaging and three‐dimensional precise laser fabrication.
The ferroelectric domain structures of periodically poled KTiOPO4 and two‐dimensional short range ordered poled LiNbO3 crystals are determined non‐invasively by interferometric measurements of the electro‐optically induced phase retardation. Owing to the sign reversal of the electro‐optical coefficients upon domain inversion, a π phase shift is observed for the inverted domains. The microscopic setup provides diffraction‐limited spatial resolution allowing us to reveal the nonlinear and electro‐optical modulation patterns in ferroelectric crystals in a non‐destructive manner and to determine the poling period, duty cycle and short‐range order as well as detect local defects in the domain structure. Conversely, knowing the ferroelectric domain structure, one can use electro‐optical microscopy so as to infer the distribution of the electric field therein.
This work proves the feasibility of a novel concept of differential absorption lidar based on the Scheimpflug principle. The range‐resolved atmospheric backscattering signal of a laser beam is retrieved by employing a tilted linear sensor with a Newtonian telescope, satisfying the Scheimpflug condition. Infinite focus depth is achieved despite employing a large optical aperture. The concept is demonstrated by measuring the range‐resolved atmospheric oxygen concentration with a tunable continuous‐wave narrow‐band laser diode emitting around 761 nm over a path of one kilometer during night time. Laser power requirements for daytime operation are also investigated and validated with single‐band atmospheric aerosol measurements by employing a broad‐band 3.2‐W laser diode. The results presented in this work show the potential of employing the continuous‐wave differential absorption lidar (CW‐DIAL) technique for remote profiling of atmospheric gases in daytime if high‐power narrow‐band continuous‐wave light sources were to be employed.
The design of micro‐optical resonator arrays are introduced and tailored towards refractive index sensing applications, building on the previously unexplored benefits of open dielectric stacks. The resonant coupling of identical hollow cavities present strong and narrow spectral resonance bands beyond that available with a single Fabry Perot interferometer. Femtosecond laser irradiation with selective chemical etching is applied to precisely fabricate stacked and waveguide‐coupled open resonators into fused silica, taking advantage of small 12 nm rms surface roughness made available by the self‐alignment of nanograting planes. Refractive index sensing of methanol‐water solutions confirm a very attractive sensing resolution of 6.5 × 10−5 RIU. Such high finesse optical elements open a new realm of optofluidic sensing and integrated optical circuit concepts for detecting minute changes in sample properties against a control solution that may find importance in chemical and biological sensors, telecom sensing networks, biomedical probes, and low‐cost health care products.
Teleportation describes the transmission of information without transport of neither matter nor energy. For many years, however, it has been implicitly assumed that this scheme is of inherently nonlocal nature, and therefore exclusive to quantum systems. Here, we experimentally demonstrate that the concept of teleportation can be readily generalized beyond the quantum realm. We present an optical implementation of the teleportation protocol solely based on classical entanglement between spatial and modal degrees of freedom, entirely independent of nonlocality. Our findings could enable novel methods for distributing information between different transmission channels and may provide the means to leverage the advantages of both quantum and classical systems to create a robust hybrid communication infrastructure.
A semiconductor optical amplifier at 2.0‐µm wavelength is reported. This device is heterogeneously integrated by directly bonding an InP‐based active region to a silicon substrate. It is therefore compatible with low‐cost and high‐volume fabrication infrastructures, and can be efficiently coupled to other active and passive devices in a photonic integrated circuit. On‐chip gain larger than 13 dB is demonstrated at 20 °C, with a 3‐dB bandwidth of ∼75 nm centered at 2.01 µm. No saturation of the gain is observed for an on‐chip input power up to 0 dBm, and on‐chip gain is observed for temperatures up to at least 50 °C. This technology paves the way to chip‐level applications for optical communication, industrial or medical monitoring, and non‐linear optics.
All‐optical signal processing on nonlinear photonic chips is a burgeoning field. These processes include light generation, optical regeneration and pulse metrology. Nonlinear photonic chips offer the benefits of small footprints, significantly larger nonlinear parameters and flexibility in generating dispersion. The nonlinear compression of optical pulses relies on a delicate balance of a material's nonlinearity and optical dispersion. Recent developments in dispersion engineering on a chip are proving to be key enablers of high‐efficiency integrated optical pulse compression. We review the recent advances made in optical pulse compression based on nonlinear photonic chips, as well as the future outlook and challenges that remain to be solved.
A novel approach to facilitate excitation and readout processes of isolated negatively charged nitrogen‐vacancy (NV) centers is proposed. The approach is based on the concept of all‐dielectric nanoantennas. It is shown that the all‐dielectric nanoantenna can significantly enhance both the emission rate and emission extraction efficiency of a photoluminescence signal from a single NV center in a diamond nanoparticle on a dielectric substrate. The proposed approach provides high directivity, large Purcell factor, and efficient beam steering, thus allowing an efficient far‐field initialization and readout of several NV centers separated by subwavelength distances.
Transport of subwavelength electromagnetic (EM) energy has been achieved through near‐field coupling of highly confined surface EM modes supported by plasmonic nanoparticles, in a configuration usually on a two‐dimensional (2D) substrate. Vertical transport of similar modes along the third dimension, on the other hand, can bring more flexibility in designs of functional photonic devices, but this phenomenon has not been observed in reality. In this paper, designer (or spoof) surface plasmon resonators (‘plasmonic meta‐atoms’) are stacked in the direction vertical to their individual planes in demonstrating vertical transport of subwavelength localized surface EM modes. The dispersion relation of this vertical transport is determined from coupled‐mode theory and is verified with a near‐field transmission spectrum and field mapping with a microwave near‐field scanning stage. This work extends the near‐field coupled resonator optical waveguide (CROW) theory into the vertical direction, and may find applications in novel three‐dimensional slow‐light structures, filters, and photonic circuits.
In this work, we report optomechanical coupling, resolved sidebands and phonon lasing in a solid‐core microbottle resonator fabricated on a single mode optical fiber. Mechanical modes with quality factors (Qm) as high as 1.57 × 104 and 1.45 × 104 were observed, respectively, at the mechanical frequencies and . The maximum Hz is close to the theoretical lower bound of 6 × 1012 Hz needed to overcome thermal decoherence for resolved‐sideband cooling of mechanical motion at room temperature, suggesting microbottle resonators as a possible platform for this endeavor. In addition to optomechanical effects, scatter‐induced mode splitting and ringing phenomena, which are typical for high‐quality optical resonances, were also observed in a microbottle resonator.
This article reviews the state of the art of ultrafast transient absorption microscopy, discusses current experimental concepts and highlights future challenges. The advantages of transient absorption microscopy over other micro‐spectroscopic techniques are its high optical resolution combined with high temporal resolution as well as its ability to study non‐fluorescent and weakly fluorescent molecular species and to probe excited‐state processes. In conventional transient absorption spectroscopy the spectroscopic information usually presents a spatial average over the focal spot of the typically weakly focused probe beam. Transient absorption microscopy, however, enables investigations of the excited state dynamics in individual microscopic areas of a sample. Hence, the technique does not only yield detailed morphological information based on a label‐free molecular contrast, but also gives insight into the ultrafast morphology‐dependent photoinduced processes in heterogeneous samples. Different variations of transient absorption microscopy have found a number of applications ranging from material sciences to biology, which are discussed in this review together with different setup modifications and approaches towards transient absorption spectroscopy with spatial resolution below the diffraction limit.
Conventional optics is diffraction limited due to the cutoff of spatial frequency components, and evanescent waves allow subdiffraction optics at the cost of complex near‐field manipulation. Recently, optical superoscillatory phenomena were employed to realize superresolution lenses in the far field, but suffering from very narrow working wavelength band due to the fragility of the superoscillatory light field. Here, an ultrabroadband superoscillatory lens (UBSOL) is proposed and realized by utilizing the metasurface‐assisted law of refraction and reflection in arrayed nanorectangular apertures with variant orientations. The ultrabroadband feature mainly arises from the nearly dispersionless phase profile of transmitted light through the UBSOL for opposite circulation polarization with respect to the incident light. It is demonstrated in experiments that subdiffraction light focusing behavior holds well with nearly unchanged focal patterns for wavelengths spanning across visible and near‐infrared light. This method is believed to find promising applications in superresolution microscopes or telescopes, high‐density optical data storage, etc.
Here we report on the hybrid nanostructures where a single ZnS nanobelt was half‐covered with an aluminum (Al) film, which is an ideal platform for studying the second‐harmonic generation (SHG) enhancement effects of the Al coating. It was fabricated by the lift‐off process and allowed for the accurate comparison of the SHG intensity between the Al‐covered and the same bare ZnS nanobelt under consistent test conditions. The results indicate that the Al coating in the hybrid nanostructures not only confines the pumping laser in the ZnS effectively, but also concentrates the emitted SHG signal greatly, increasing the signal collection efficiency. By the combination of these two effects, ∼60 times enhancement of the SHG intensity is achieved at the optimized geometry size (width and thickness) of the ZnS nanobelts. The Al‐based hybrid nanostructures open up new possibilities for low‐cost, highly efficient and directional coherent nanolight sources at short wavelengths.
Nanophotonic beamsplitters are fundamental building blocks in integrated optics, with applications ranging from high speed telecom receivers to biological sensors and quantum splitters. While high‐performance multiport beamsplitters have been demonstrated in several material platforms using multimode interference couplers, their operation bandwidth remains fundamentally limited. Here, we leverage the inherent anisotropy and dispersion of a sub‐wavelength structured photonic metamaterial to demonstrate ultra‐broadband integrated beamsplitting. Our device, which is three times more compact than its conventional counterpart, can achieve high‐performance operation over an unprecedented 500 nm design bandwidth exceeding all optical communication bands combined, and making it one of the most broadband silicon photonics components reported to date. Our demonstration paves the way toward nanophotonic waveguide components with ultra‐broadband operation for next generation integrated photonic systems.
