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1.
采用大涡模拟和直接积分矩方法,数值模拟了在Reynolds数为8300的平面射流中,水蒸气(相对湿度φ=70%)和硫酸蒸气(质量分数为5×10-6)二元体系中纳米颗粒的成核与凝并,详细分析了颗粒数密度、体积密度和平均粒径的分布.计算结果表明.射流场混合动量厚度的增长和实验结果一致;射流场的拟序结构导致了涡核中心处硫酸蒸气浓度的明显减小,而纳米颗粒数密度则明显增加;拟序结构的出现导致颗粒碰撞概率增大,提高了颗粒凝并效率;在颗粒数密度较大的涡核中心,颗粒成核作用增强,从而加
关键词:
纳米颗粒
成核
凝并
平面射流 相似文献
2.
自由分子区布朗凝并作用下的颗粒尺寸分布变化 总被引:1,自引:0,他引:1
对于燃烧过程中生成的亚微米颗粒,其一次颗粒的长大过程主要是通过碰撞凝并实现的。本文通过对颗粒的初始分布作出一个合理的正态对数分布的假设,运用矩方法(Moment Method)研究了自由分子区的颗粒在布朗碰撞作用下的颗粒尺寸分布的变化情况。所得到的长时间碰撞凝并结果符合布朗碰撞凝并过程的自保持特性。数值结果还表明,颗粒初始的宽粒径分布会显著提高粒子云的在凝并初期的凝并速率和生成粒子的平均直径,且最终生成的粒子尺寸都是宽分布的。这说明在预报微细颗粒的迁移和长大过程中有必要考虑粒子的宽分布特性。 相似文献
3.
La Follett JR Williams KL Marston PL 《The Journal of the Acoustical Society of America》2011,130(2):669-672
Backscattering of sound by a solid aluminum cylinder was measured in the free field and with the cylinder near a flat surface. The target was suspended just below the surface of a water tank to simulate some aspects of backscattering when resting on the seabed. Measurements were compared with predictions made by an approximate hybrid approach based on multiple two-dimensional finite element calculations and the use of images. Many of the spectral features present in the tank data were present in the model. Comparing numerical model predictions with experimental data serves to build credibility for the modeling approach and can assist in developing insight into the underlying physical processes. 相似文献
4.
The Pontryagin equation was applied to calculating the average time for the random process escaping the assign interval: this gives the average delay time for waiting of particle ignition moment in a turbulent flow of gas. A direct numerical simulation method was developed for gas temperature fluctuations with assigned autocorrelation function and particle temperature fluctuations due to exothermal chemical reaction. The method was based on numerical solution of a system of stochastic differential equations. Results of direct simulation were validated through comparing with the analytical solution available for particles without exothermal reaction. Analytical calculations and results of direct numerical simulation for the delay time of particle ignition are in agreement. 相似文献
5.
The Reynolds averaged N-S equation and dynamic equation for nanoparticles are numerically solved in the two-phase flow around cylinders, and the distributions of the concentration M0 and geometric mean diameter dg of particles are given. Some of the results are validated by comparing with previous results. The effects of particle coagulation and breakage and the initial particle concentration m00 and size d0 on the particle distribution are analyzed. The results show that for the flow around a single cylinder, M0 is reduced along the flow direction. Placing a cylinder in a uniform flow will promote particle breakage. For the flow around multiple cylinders, the values of M0 behind the cylinders oscillate along the spanwise direction, and the wake region in the flow direction is shorter than that for the flow around a single cylinder. For the initial monodisperse particles, the values of dg increase along the flow direction and the effect of particle coagulation is larger than that of particle breakage. The values of dg fluctuate along the spanwise direction; the closer to the cylinders, the more frequent the fluctuations of dg values. For the initial polydisperse particles with d0 = 98 nm and geometric standard deviation σ = 1.65, the variations of dg values along the flow and spanwise directions show the same trend as for the initial monodisperse particles, although the differences are that the values of dg are almost the same for the cases with and without considering particle breakage, while the distribution of dg along the spanwise direction is flatter in the case with initial polydisperse particles. 相似文献
6.
Microscopic study of electromagnetic properties and band spectra of neutron deficient ~(133,135,137)Sm
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Rakesh K. Pandit R.K. Bhat Rani Devi S.K. Khosa G.H. Bhat J.A. Sheikh 《中国物理C(英文版)》2019,43(12):124108-124108-20
A microscopic high spin study of neutron deficient and normally deformed ~(133,135,137)Sm has been carried out in projected shell model framework.The theoretical results have been obtained for the spins,parities and energy values of yrast and excited bands.Besides this,the band spectra,band head energies,moment of inertia and electromagnetic transition strengths are also Predicted in these isotoPes.The calculations successfully give a deeper understanding of the mechanism of the formation of yrast and excited bands from the single and multi-quasi particle configurations.The results on moment of inertia predict an alignment of a pair of protons in the proton(1 h_(11/2))~2 orbitals in the yrast ground state bands of ~(133-137)Sm due to the crossing of one quasiparticle bands by multi-quasiparticle bands at higher spins.The discussion in the present work is based on the deformed single particle scheme.Any future experimental confirmation or refutation of our predictions will be a valuable information which can help to understand the deformed single particle structure in these odd mass neutron deficient ~(133-137)Sm. 相似文献
7.
Particle formation in opposed-flow diffusion flames of ethylene: An experimental and numerical study
Andrea D’Anna Mario Commodo Patrizia Minutolo 《Proceedings of the Combustion Institute》2009,32(1):793-801
An experimental and numerical study on particles inception and growth is performed in opposed-flow diffusion flames of ethylene and air characterized by different sooting tendencies. Spectrally resolved UV-visible laser induced fluorescence, laser induced incandescence and laser light scattering measurements are used to characterize different classes of combustion-generated compounds. A detailed kinetic model accounting for both gas-phase and particle formation is used. Comparison between experimental results and numerical predictions gives a qualitative view of the mechanism of particle formation in opposed-flow flames.Particle inception is the result of both chemical growth and coagulation of aromatic compounds. In the region close to the flame front where the temperature is relatively high and radicals are abundant, the particle inception is due to a chemical growth mechanism by which aromatic molecules add aromatic radicals leading to the formation of biphenyl-like structures. The growth process continues as high-molecular mass aromatics are moved away from the flame zone towards the stagnation plane by the addition of acetylene and other aromatics forming particles of increasing sizes. Graphitization of these particles and thermal annealing lead to the formation of soot particles. At relatively lower temperatures, found across the stagnation plane, particles growth still occurs and it is mainly due to a process of physical coagulation of PAHs.The experimental and numerical results obtained in this work demonstrate and explain the sensibility of inception and growth of particles to radical concentration and temperature in opposed-flow flame configurations. 相似文献
8.
Carlos A. Echavarria JoAnn Slama Lighty Andrea D’Anna 《Proceedings of the Combustion Institute》2009,32(1):705-711
This study demonstrates the major differences in the evolution of the particle size distributions (PSDs), both measured and modeled, of soot in premixed benzene and ethylene flat flames. In the experiments, soot concentration and PSDs were measured by using a scanning mobility particle sizer (SMPS, over the size range of 3-80 nm). The model employed calculations of gas phase species coupled with a discrete sectional approach for the gas-to-particle conversion. The model includes reaction pathways leading to the formation of nano-sized particles and their coagulation to larger soot particles. The particle size distribution, both experimental and modeled, evolved from a single particle mode (the nucleation mode) to a bimodal size distribution. An important distinction between the results for the ethylene and benzene flames is the behavior of the nucleation mode which persists at all heights above the burner (HAB) for ethylene whereas it was greatly suppressed at greater HAB for the benzene flames. The explanation for the decreased nucleation mode at higher elevations in the benzene flame is that the aromatics are consumed in the oxidation zone of the flame. Fair predictions of particle-phase concentrations and particle sizes in the two flames were obtained with no adjustments to the kinetic scheme. In agreement with experimental data, the model predicts a higher formation of particulate in the benzene flame as compared with the ethylene flame. 相似文献
9.
A particle-size sorting system of lunar regolith using an electrostatic traveling wave is developed for In-Situ Resource Utilization on the Moon to extract indispensable resources from the regolith and realize long-term exploration. The regolith is sorted by utilizing a balance between the electrostatic and gravitational forces, which are determined depending on particle size, in vacuum conditions where the particles are not subjected to air drag. In this study, the effect of particle charge on the particle motion is confirmed by conducting model experiments and numerical calculations based on the distinct element method. In addition, it was experimentally demonstrated that particles less than approximately 20 μm in diameter were efficiently separated from the bulk of a lunar regolith simulant FJS-1 in a vacuum condition (∼1.5 × 10−2 Pa), and the performance of the size sorting system on the Moon was predicted by the numerical calculations. The system utilizes only the electrostatic force, and it does not require any gas, liquid, or mechanical moving parts. 相似文献
10.
Donato Bini Christian Cherubini Simonetta Filippi Andrea Geralico 《General Relativity and Gravitation》2009,41(12):2781-2795
An exact solution of Einstein’s equations representing the static gravitational field of a quasi-spherical source endowed
with both mass and mass quadrupole moment is considered. It belongs to the Weyl class of solutions and reduces to the Schwarzschild
solution when the quadrupole moment vanishes. The geometric properties of timelike circular orbits (including geodesics) in
this spacetime are investigated. Moreover, a comparison between geodesic motion in the spacetime of a quasi-spherical source
and non-geodesic motion of an extended body also endowed with both mass and mass quadrupole moment as described by Dixon’s
model in the gravitational field of a Schwarzschild black hole is discussed. Certain “reciprocity relations” between the source
and the particle parameters are obtained, providing a further argument in favor of the acceptability of Dixon’s model for
extended bodies in general relativity. 相似文献
11.
J.W. Labahn 《Combustion Theory and Modelling》2013,17(5):960-982
A turbulent combustion model, Conditional Source-term Estimation (CSE) is applied to a non-premixed turbulent jet methane flame. The conditional chemical source terms are determined on the basis of first order closure and the conditional averaged species concentrations are obtained by inverting an integral equation. The Tikhonov method is implemented for regularisation. Detailed chemistry is tabulated using the trajectory generated low-dimensional manifold method. Radiation due to the gaseous species is included. Reynolds Averaged Navier–Stokes calculations are performed using two different turbulence models. The objectives of the paper are (i) assessment of the impact of the main numerical parameters in CSE and (ii) comparison of the CSE numerical predictions with available experimental data and results from previous simulations for the selected flame. The number of CSE domains and the number of points in each CSE domain are shown to have a significant impact on the results if not selected appropriately. The present CSE calculations always converge to unique and stable predictions. The corrected k–ε model yields mixture fraction profiles in good agreement with the experimental data values for axial locations in the first half of the flame. Farther downstream, the RNG k–ε model performs better. Overall, the current predictions for the mixture fraction are in good agreement with the experimental data. The predicted temperatures using CSE and the k–ε turbulence model with a modified value of Cε1 = 1.47 are found to be in very good agreement with the experimental data. Further, the current CSE results are of comparable quality with previous simulations using the flamelet model and conditional moment closure. Future work may include further investigation on optimal determination of the regularisation parameter and alternative regularisation techniques, soot modelling within the CSE formulation, and improved formulation of radiation. 相似文献
12.
A. A. Pomeranskii I. B. Khriplovich 《Journal of Experimental and Theoretical Physics》1998,86(5):839-849
We consider the motion of a spinning relativistic particle in external electromagnetic and gravitational fields to first order
in the external field but to arbitrary order in the spin. The influence of the spin on the particle trajectory is properly
accounted for by describing the spin noncovariantly. Specific calculations are performed through second order in the spin.
A simple derivation is presented for the gravitational spin-orbit and spin-spin interactions of a relativistic particle. We
discuss the gravimagnetic moment (GM), a particular spin effect in general relativity. We show that for a Kerr black hole
the gravimagnetic ratio, i.e., the coefficient of the GM, equals unity (just as the gyromagnetic ratio equals 2 for a charged
Kerr hole). The equations of motion obtained for a spinning relativistic particle in an external gravitational field differ
substantially from the Papapetrou equations.
Zh. éksp. Teor. Fiz. 113, 1537–1557 (May 1998) 相似文献
13.
Nai‐Ning Wang 《Particle & Particle Systems Characterization》2001,18(1):26-32
Based on light scattering theory, an optical method is presented for measuring the concentration and particle size distribution of the dispersed phase in two‐phase flows. A prototype was also constructed. Comprehensive computer simulation and numerical calculations were carried out to calibrate the correctness of this method. An experimental study was also performed in gas–solid and gas–liquid two‐phase flows. The results of the measurements are given and discussed in detail. 相似文献
14.
聚集速率是评估胶体体系特性及稳定性的关键参数, 静态光散射和动态光散射则是测量聚集速率的两个重要方法. 然而, 用静态光散射和动态光散射测量聚集速率时, 需要知道有关单粒子和双粒子聚集体光散射特性的数据. 为此, 通常需要把动、静两种方法结合, 才能消去这个数据. 以前各种近似理论曾用来解决这个问题, 但因粒子尺寸和形状的限制, 结果并不理想. 而T矩阵方法可以不受粒子大小和形状的限制计算其光散射特性. 本工作用T矩阵方法直接计算静态光散射和动态光散射所必须的粒子散射特性, 并将该法得到的聚集速率与动静态光散射结合法得到的聚集速率进行了比较, 两者结果很接近. 本工作为简化静态光散射和动态光散射测量聚集速率, 扩展其应用范围开辟了新途径.
关键词:
T矩阵')" href="#">T矩阵
光散射法
聚集速率 相似文献
15.
Diffusional coagulation of superparamagnetic particles in the presence of an external magnetic field
In this paper, we investigate the diffusional coagulation of colloidal superparamagnetic (SP) latex particles that are under the influence of an external magnetic field. The cluster size distributions (CSDs) that evolve with time were determined using an optical set-up that permits the direct visualization of particle clusters. Following the dynamic scaling analysis of van Dongen and Ernst (Phys. Rev. Lett. 54 (1985) 1396), we find that the CSDs all collapse onto a master curve when properly scaled. The bell-shape of this master curve indicates that large clusters preferentially scavenge small clusters in our system. From the time evolution of the average cluster size we infer that the reactivity between large clusters diminishes with increasing cluster size. These results are consistent with a simple mathematical formulation of the coagulation rate constant, or kernel, for the Brownian coagulation of magnetic particles. Moreover, our results support a growing body of evidence that the dynamic scaling theory developed by van Dongen and Ernst is a useful framework with which to study the microscale processes governing particle coagulation. 相似文献
16.
17.
Perihelion Precession in Gravitational Field of Center Mass with Electric Charge and Magnetic Moment
With a perfect mathematical method by us, we obtain some
expressions of the orbital effect for a test particle and some meaningful
results in the gravitational field of the center mass with electric charge
and magnetic moment. 相似文献
18.
Xi‐Qing Chen Metin Renksizbulut Xianguo Li 《Particle & Particle Systems Characterization》2001,18(3):120-133
A numerical analysis of polydispersed glass particles interacting with a confined turbulent bluff‐body flow was performed by combining the finite‐volume method for the gaseous flow with a mesh‐free Lagrangian approach for the particulate flow. Three turbulence‐closure models, namely the Reynolds‐stress, the standard k‐ϵ, and the nonlinear k‐ϵ models, were first comparatively studied for the single‐phase flow. The second‐moment Reynolds‐stress model was then selected for the prediction of the turbulent gaseous flow in a gas‐particle system, where an improved eddy‐interaction model was used to predict turbulence‐induced particle dispersion. The interaction between the two phases was accounted for through coupling source terms. Numerical predictions of two‐phase mean and fluctuating velocities for particle sizes ranging from 15 to 115 μm were compared with corresponding experimental data. Reasonably good agreement was achieved for the mean properties of both the gaseous and particulate flows. 相似文献
19.
20.
This paper presents our numerical and experimental results of the bifurcation found in Taylor-Couette system with a free surface.
The lengths of the two concentric cylinders are finite and their axes are parallel to the direction of the gravitational force.
When the end walls of the cylinders are fixed and stationary, numerical and experimental studies have shown that the flow
has multiple patterns depending on the cylinder lengths and the Reynolds numbers. Experimental studies on flows with free
surfaces also gave various flow modes. Our result shows that the measured and predicted time-dependent displacements of the
free surface are in favorable agreement. In case of the cylinder length comparable with the gap width between the cylinders,
gradual accelerations of the inner cylinder bring the normal mode flows with one, three and five toroidal vortices. The exchanges
of stabilities between these flow modes are summarized in a phase diagram. 相似文献