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1.
In this article simultaneous effects of external electric field and spin-orbit interaction on the linear and the nonlinear optical properties of a cubic quantum dot are studied. Based on the non- degenerate perturbation method, energy eigenvalues and eigenfunctions of the system under the influence of spin-orbit interaction are calculated. Furthermore, the linear and the nonlinear optical absorption coefficients and refractive index changes are obtained using the compact density matrix approach and iterative method. Our results show that, due to the spin-orbit interaction, resonant peak values of the optical absorption coefficients and refractive index changes decrease and occur at lower values of the incident photon energy. The variation of these optical parameters depend on the spin-orbit interaction strength, dot dimensions and external electric field.  相似文献   

2.
In this paper, the effect of hydrostatic pressure on both the intersubband optical absorption coefficients and the refractive index changes is studied for typical GaAs/Al x  Ga1?x As cubic quantum dot. We use analytical expressions for the linear and third-order nonlinear intersubband absorption coefficients and refractive index changes obtained by the compact-density matrix formalism. The linear, third-order nonlinear, and total intersubband absorption coefficients and refractive index changes are calculated at different pressures as a function of the photon energy with known values of box length (L), the incident optical intensity (I), and Al concentration (x). According to the results obtained from the present work, we have found that the pressure plays an important role in the intersubband optical absorption coefficient and refractive index changes in a cubic quantum dot.  相似文献   

3.
In this work electronic structure, the linear and the third-order nonlinear refractive index changes as well as optical absorption coefficients of a two-dimensional hexagonal quantum dot are investigated. Energy eigenvalues and eigenfunctions of the system are calculated by the matrix diagonalization technique, and optical properties are also obtained using the compact density matrix approach. As our results indicate, both the dot size and the confinement potential have a great influence on the intersubband energy intervals, the transition probability and consequently, the linear and the third-order nonlinear refractive index changes and optical absorption coefficients.  相似文献   

4.
Optical absorption coefficients and refractive index changes associated with intersubband transition in a parabolic cylinder quantum dot are theoretically investigated. In this regard, the electronic structure of the dot is studied using the one band effective mass theory, and by means of the compact-density matrix approach the linear and nonlinear optical absorption coefficients and refractive index changes are calculated. The effects of the size of the dot, optical intensity and electromagnetic field polarization on the optical absorption coefficient and refractive index changes are investigated. It is found that absorption and refractive index changes are strongly affected not only by the size of the dot but also by optical intensity and the electromagnetic field polarization.  相似文献   

5.
An investigation of the optical properties of a hydrogenic donor in sphericalparabolic quantum dots has been performed by using the matrix diagonalization method. The optical absorption coefficient between the ground (L=0) and the first excited state (L=1) have been examined based on the computed energies and wave functions. The results are presented as a function of the incident photon energy for the different values of the confinement strength. These results show the effects of the quantum size and the impurity on the optical absorption coefficient of a donor impurity quantum dot.  相似文献   

6.
The present work investigates the nonlinear optical properties of a GaN quantum dot in the disk limit via the exciton and biexciton states using the compact density matrix formalism. Based on this model, we calculate the ground state energy of the exciton and biexciton states by the variation method, within envelope function and effective mass approximations. Linear and nonlinear optical absorption (α (1), α (3)) and oscillator strengths attributed to the optical transitions are obtained. The details of the behaviour of α (1) and α (3) around the resonance frequencies and for different quantum dot geometries are presented. It is found that the size of quantum dot and the optical intensity have a remarkable effect on the optical absorption, and the biexcitonic two-photon absorption coefficient(K 2) has also been calculated in this system. The results show that this parameter is strongly affected by the size of the quantum dot.  相似文献   

7.
Wenfang Xie 《Physics letters. A》2008,372(33):5498-5500
A investigation of the nonlinear optical properties of a hydrogenic donor in a disc-like parabolic quantum dot has been performed by using the matrix diagonalization method. The optical absorption coefficient between the ground (L=0) and the first excited state (L=1) have been examined based on the computed energies and wave functions. The results are presented as a function of the incident photon energy for the different values of the incident optical intensity and the confinement strength. We found the total optical absorption coefficient is strongly affected by the incident optical intensity and the confinement strength.  相似文献   

8.
由于微制造技术的不断发展,如液相外延(LPE),气相外延(VPE),金属有机化学气相沉积(MOCVD)以及分子束外延技术(MBE)等先进的材料生长技术方法也日趋完善,从而使得各种低维半导体量子器件(如半导体、超晶格、量子阱、量子线和量子点等)制造日趋成熟。由于这些低维半导体量子器件具有很强的非线性光效应,而且随着材料、外形、尺寸等的不同,非线性光效应也有很大的差别,更由于其可能存在的广泛的应用前景,所以近年来,一直是人们研究的重点。近来,由于人们相信,利用GaAs/AlGaAs量子阱有可能制造出一些新型的光学仪器,如光开关、光限幅器、光调制器等,所以,对不同势形的GaAs/AlGaAs量子阱的非线性光学特性一直吸引着人们进行理论和实验的研究。而在最近几年,对双量子阱的研究也成为了人们的研究重点。通过密度矩阵和迭代的方法,得到双量子阱中的第一、第三阶子带光吸收表达式,我们将用一个典型的GaAs/AlGaAs双量子阱代入其中进行数值计算,并进行讨论。我们的计算结果显示,阱的光吸收峰不但与中间的势垒宽度有关,更与入射光强有关。  相似文献   

9.
Simultaneous effects of an on-center hydrogenic impurity and band edge non-parabolicity on intersubband optical absorption coefficients and refractive index changes of a typical GaAs/Al x Ga 1 x As spherical quantum dot are theoretically investigated,using the Luttinger-Kohn effective mass equation.So,electronic structure and optical properties of the system are studied by means of the matrix diagonalization technique and compact density matrix approach,respectively.Finally,effects of an impurity,band edge non-parabolicity,incident light intensity and the dot size on the linear,the third-order nonlinear and the total optical absorption coefficients and refractive index changes are investigated.Our results indicate that,the magnitudes of these optical quantities increase and their peaks shift to higher energies as the influences of the impurity and the band edge non-parabolicity are considered.Moreover,incident light intensity and the dot size have considerable effects on the optical absorption coefficients and refractive index changes.  相似文献   

10.
Based on the Schr ¨odinger equation for envelope function in the effective mass approximation, linear and nonlinear optical absorption coefficients in a multi-subband lens quantum dot are investigated. The effects of quantum dot size on the interband and intraband transitions energy are also analyzed. The finite element method is used to calculate the eigenvalues and eigenfunctions. Strain and In-mole-fraction effects are also studied, and the results reveal that with the decrease of the In-mole fraction, the amplitudes of linear and nonlinear absorption coefficients increase. The present computed results show that the absorption coefficients of transitions between the first excited states are stronger than those of the ground states. In addition, it has been found that the quantum dot size affects the amplitudes and peak positions of linear and nonlinear absorption coefficients while the incident optical intensity strongly affects the nonlinear absorption coefficients.  相似文献   

11.
A investigation of the linear and nonlinear optical properties of an exciton in a spherical parabolic quantum dot has been performed by using the matrix diagonalization method. The optical absorption coefficients between the ground state (L=0,π=+1) and the first excited state (L=1,π=-1) have been examined based on the computed energies and wave functions. The results are presented as a function of the incident photon energy for the different values of the incident optical intensity and the confinement strength. We found the optical absorption coefficient is strongly affected by the incident optical intensity and the confinement strength.  相似文献   

12.
Semi oblate and semi prolate are among the most probable self-organized nanostructures shapes. The optoelectronic properties of such nanostructures are not just manipulated with the height and lateral size but also with the wetting layer element. The practical interest of derivatives of germanium and silicon has a great important role in optoelectronic devices. This study is a contribution to the analysis of linear and nonlinear optical properties of Si0.7Ge0.3/Si. In the framework of the effective mass approximation, we solve numerically the Schrödinger equation relative to one particle confined in Si0.7Ge0.3/Si semi prolate and semi oblate quantum dots by using the finite element method and by taking into consideration the effect of the wetting layer. The energy spectrum of the lowest states and the dipolar matrix for the fourth allowed transitions are determined and discussed. We also calculate the detailed optical properties, including absorption coefficients, refractive index changes, second and third harmonic generation as a function of the quantum dot sizes. We found that with the change in the size of prolate and oblate quantum dots, there is a shift in the resonance peaks for the absorption coefficient and refractive index. It is due to the modification in the energy levels with changing size. The study proves a redshift in the second harmonic generation and third harmonic generation coefficients with an increase in the height/radius of the oblate/prolate quantum dot, respectively. We also demonstrated the variation of wavefunction inside the quantum dot with the change in wetting layer thickness.  相似文献   

13.
The coupling effects on the optical absorption spectrum of semiconductor quantum dots arestudied by using the standard model with valence and conduction band levels coupled todispersive quantum phonons of infinite modes. By deducing the analytical expression of theoptical absorption coefficient, the relationship between the measurable quantities and theintrinsic properties of the semiconductor quantum dot is established. By this expression,the peak position, the line shape, the linewidth, and the energy shift of the absorptionspectrum of semiconductor quantum dot can be calculated precisely for a wide range ofparameters. The role of coupling strength as a mechanism of absorption line asymmetry isinvestigated, and the calculation results clearly show the coupling-induced asymmetry inthe absorption line. This analytical approach is applied to GaAs quantum dot, and theresults are consistent with those of experiment observations.  相似文献   

14.
利用紧致密度矩阵近似方法,研究了一个特殊量子点量子阱中的三阶非线性光学特性(三次谐波产生),得到了量子点量子阱系统的三次谐波产生系数的解析表达式,而且考虑了量子点量子阱系统中的两种电子束缚态-壳层阱内与阱外两种束缚态。对CdS/HgS构成的典型的量子点量子阱进行了数值计算,得到了10^-15(m/v)^2量级的三次谐波产生系数,并且绘出了三次谐波产生系数作为量子点量子阱的尺寸和泵浦光子能量的函数曲线,最后对曲线的特征及其形成的原因进行了解析。  相似文献   

15.
玻璃中CdSSe纳米晶体的光谱性能   总被引:4,自引:2,他引:2       下载免费PDF全文
对掺有镉、硒、硫的玻璃在650—800℃退火4?h,生长了不同尺寸的CdS0.13Se0.87纳米晶体,测量了纳米晶体的吸收光谱、光致发光(PL)谱和电调制光谱,确定了纳米晶体部分电子态的能量,讨论了CdSSe纳米晶体的光学性质与其尺寸之间的依赖关系.随着纳米晶体尺寸的增大,对应激子的吸收峰、PL峰及电吸收信号发生红移,表现出明显的量子尺寸效应.小尺寸纳米晶体的电吸收表现为量子受限的Stark效应,而大尺寸纳米晶体的电吸收线形与体材料的相似;随着纳米晶体尺寸的增大,电吸收信号增强.所有尺寸的纳米晶体都表现 关键词: CdSSe纳米晶体 吸收光谱 光致发光谱 电光响应  相似文献   

16.
An ultrafast all-optical modulator based on spherical quantum dot using electromagnetically induced transparency (EIT) technique in GaN/AlN structure, associated with inter-sublevel transitions, is proposed and analyzed. The aim of this paper is to modify and enhance the main parameters of an all-optical modulator such as, power consumption, modulation depth, maximum bit-rate and band-width. To realize these points, we have proposed a suitable quantum dot structure based on EIT in a strained GaN/AlN, with an internal barrier. Simulations show this barrier enhances the dot optical properties, such as dipole matrix element, linear susceptibility, and hence absorption coefficient, reducing the power consumption and increasing the modulation depth. Furthermore, using control signal in EIT process, carriers are driven from an upper state to a lower state from where they rapidly decay to the ground state increasing the modulation bit-rate and band-width.  相似文献   

17.
We consider the effects of quantum dot radius, confinement potential depth and controllable effective mass on the optical rectification coefficient (ORC) in spherical quantum dots, which is confined with Modified Kratzer–Coulomb Potential (MKCP). Using the Nikiforov–Uvarov method and compact density matrix theory, the ground state energy, ORC and wave function of electrons under the combined action of many factors are calculated. The results show that they affect the optical rectification response from different angles, including the position of peak and formant.  相似文献   

18.
We calculate the minimum Gibbs free energy of the InAs/InP quantum dot multilayer by combining the method of moving asymptotes and the finite element method. Based on the principle of the least energy, the transition between vertically aligned and anti-aligned quantum dot multilayers is studied. We investigate the influence of quantum dot base size and density on critical spacer thickness for the transition. The study results indicate that the critical thickness increases with the decrease in the density of quantum dots, while the base size of the quantum dot is linear to the critical thickness when the density is given.  相似文献   

19.
Analytical expressions of the optical absorption coefficient and the change in refractive index associated with intraband relaxation in a cylindrical quantum dot are obtained by using the density matrix formalism. Energy levels in conduction band were calculated with finite confining potential in the framework of the effective-mass envelope-function theory. Numerical calculations on a typical GaAs/AlβGa1−βAs QD are performed. It is found that the absorption and refraction index change sensitively depend not only on the incident optical wave but also on the dot size and the Al mole fraction β in the AlβGa1−βAs material.  相似文献   

20.
Pressure-induced binding energies of an exciton and a biexciton are studied taking into account the geometrical confinement effect in a CdTe/ZnTe quantum dot. Coulomb interaction energy is obtained using Hartree potential. The energy eigenvalue and wave functions of exciton and the biexciton are obtained using the self-consistent technique. The effective mass approximation and BenDaniel-Duke boundary conditions are used in the self-consistent calculations. The pressure-induced nonlinear optical absorption coefficients for the heavy hole exciton and the biexciton as a function of incident photon energy for CdTe/ZnTe quantum dot are investigated. The optical gain coefficient with the injection current density, in the presence of various hydrostatic pressure values, is studied in a CdTe/ZnTe spherical quantum dot. The pressure-induced threshold optical pump intensity with the dot radius is investigated. The results show that the pressure-induced electronic and optical properties strongly depend on the spatial confinement effect.  相似文献   

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