Investigations on the presence and distribution of radon in the Cacica salt mine,Romania

An important parameter for evaluating the possibilities of use of enclosed spaces (mines, caves, spas, etc.) for therapeutic purposes is the concentration of radon in different conditions of ventilation. The aim of this paper is to present the results of continuous radon gas measurement that were performed for ten days, at 20 min time intervals in different locations from Cacica salt mine (Romania) using a portable radon monitor. The average radon concentration was found to be between 96.5 ± 4.76 Bq/m³ and 20.5 ± 1.30 Bq/m³. These values are suitable for therapeutic applications and are useful for future experiments regarding the development of the radon therapy and speleotherapy in this salt mine.     

Radon levels assessment in some Northern Romanian salt mines

Due to their low radioactivity background, underground salt mines spaces offer a unique possibility for speleotherapy use. The knowledge of radon concentration levels in such underground environments is essential for therapeutic purposes of different respiratory and rheumatic diseases. In order to develop speleotherapy in Romania, this paper presents the results of an indoor radon concentration levels survey in some salt mines in Romania. The survey was carried out using radon monitor Pylon AB-5 system methodology validated by a CIS-P5M system. In order to investigate whether differences in depth and microclimate parameters translate into significant differences in salt mine indoor radon concentrations, have been chosen three salts mine test sites placed in the Northern part of Romania (Turda, Cacica and Ocna Dej) in stable areas of the mining field at 32?C120?m depth. Environmental microclimate conditions (mean values of air temperature 10?C14.5?°C, air humidity 65?C80%, air velocity 0.2?m/s saline aerosols and low microbial factors) have anti-bacterial, anti-microbial, and anti-inflammatory properties and recognized therapeutically effects on human body??s health. Air temperature is one of the most important factors which need to be considered when carrying out a survey of indoor radon concentrations in salt mines because temperature largely determines close spaces ventilation rates, and ventilation habits are known to have significant effects on indoor radon concentrations. The analyzed environmental conditions and recorded low levels of indoor mean radon concentration (6.9?±?0.39 and 96.5?±?4.76?Bq/m³) demonstrated the best suitability of the investigated three salt mines in Romania for speleotherapeutic applications.     

Exposure to underground radon in and around Kolkata Municipal Corporation area: an exhaustive study

Air radon survey was carried out at different underground locations at Kolkata using radon monitor. Average radon concentration for basements was found to be 22.70 ± 1.12 Bq/m³ with maximum 59.00 ± 7.18 Bq/m³ and minimum 8.50 ± 3.14 Bq/m³. Average level for sub-ways was 23.05 ± 2.59 Bq/m³ fluctuating between maximum 39.00 ± 1.24 Bq/m³ and minimum 13.50 ± 1.78 Bq/m³. In comparison, open air background at basement entrance was 19.44 ± 1.06 Bq/m³ and subway entrance was 18.58 ± 1.14 Bq/m³. Annual effective dose was calculated to assess probable health risk. Radon concentration level and annual effective dose were found well below safe levels recommended by International Agencies WHO and UNSCEAR.

     

Ground based radon (222Rn) observations in Bucharest, Romania and their application to geophysics

Atmospheric radon concentration was continuously monitored in Bucharest-Magurele area both near the ground at 1 m height as well as at 10 m height. This paper presents the results of radon in air near the ground concentrations obtained during the 1 July 2010 to 1 February 2012 period by use of solid state nuclear track detectors SSNTD CR-39. The mean atmospheric radon concentration near the ground at 1 m height was found to be 360.91 ± 66.49 Bq/m³, which was about more than an order of magnitude lower than average radon concentration in range of 44.92 ± 9.94 Bq/m³ recorded for period 1 August 2011 to 20 December 2011 at 10 m height by AlphaGUARD Radon monitor. The meteorological effects on the variation of atmospheric radon concentration were discussed. The analysis of spatio-temporal variations in time series radon concentration in air near the ground is a useful tool to study geo-dynamical processes associated with seismic activity in active Vrancea zone in Romania. Taking off the variations induced by external variables, such as temperature, barometric pressure, rainfall, and other meteorological parameters, can be assessed radon anomalies due to possible tectonic movements and also can be surveyed radioactivity background in relation with nuclear emergencies.     

Indoor radon concentration levels in Mexican caves, using nuclear track methodology, and the relationship with living habits of the bats

This work presents the results of a study of the radon levels in four caves in Mexico: Los Riscos Cave and El Judío Cave in the State of Querétaro, and Coyozochico Cave and Karmidas Cave in the State of Puebla. The measurements were made using the passive closed-end cup system, with CR-39 (Lantrack^®) as detection material, and following protocols established for the measurement of indoor radon, developed at the Dosimetry Applications Project of the Physics Institute of the Universidad Nacional Autónoma de México. The radon concentration at one location with Karmidas Cave reached more than 60,000 Bq/m³, while concentrations in the other three caves varied from 83.1–1216.0 Bq/m³, was found. During the study was observed an interesting coincidence between the radon concentration distribution inside the caves, and the bat colonies location. In general, the bat colonies are located at the medium or low radon concentration levels zones.     

Annual average radon concentration in the show caves of Hungary

Radon can accumulate in underground areas such as show caves. Repairmen and tourist guides working in such caves may thus be exposed to significant radiation doses. Therefore, it is necessary to measure the radon concentration to estimate the exact radiation dose caused by radon. Considering that the radon concentration in caves usually shows significant seasonal fluctuations, the monthly change of radon concentration was studied for 1 year in nine show caves opened to the public in Hungary. Despite the fact that all of the caves were formed in karst rocks, the annual average radon concentration levels were rather different between each other (541–8287 Bq m⁻³). The significant monthly fluctuation of the radon concentration indicates that the annual average radon concentration in caves can only be accurately obtained by year-long measurements.     

Assessment of radon concentration and external gamma radiation level in the environs of Narwapahar uranium mine,India and its radiological significance

In the environs of uranium mining, milling and processing facilities and in the uranium mineralized terrain, a little higher ambient radon concentration and gamma radiation level may be expected in comparison with natural background. The present study gives a brief account of atmospheric radon concentration, gamma absorbed dose rate and radiation dose received by the members of public in the vicinity of Narwapahar uranium mine. The ambient radon concentration in the air in the study area was found to vary from 5 to 107 Bq m⁻³ with geometric mean of 24 Bq m⁻³ and geometric standard deviation of 1.74 Bq m⁻³. The measured gamma absorbed dose rate in air at 1 m above the ground ranged from 87 to 220 nGy h⁻¹ with an overall arithmetic mean of 128 ± 18.5 nGy h⁻¹. The mean annual effective dose received by the members of public from inhalation of radon and its progeny and external gamma exposure was estimated to be 0.32 mSv year⁻¹, which is comparable to other reported values elsewhere.     

Radon survey in office room and effective dose estimation for staff

This study aims to: (1) Acquire the radon level in closed office rooms, providing radon exposure data for preliminary health risk assessment of office-working population. (2) Pre-analyze the relationship between radon concentration and indoor temperature, relative humidity. (3) Estimate seasonal, annual and total radon effective dose for ordinary office-working population. The results show that the 24-h or 8-h average radon concentrations in closed office rooms were about 32.0 Bq/m³ and 29.5 Bq/m³ during detection period, and the estimated effective doses in office rooms calculated by using 24-h and 8-h average radon concentrations were all far below that in residential environment.

     

Calibration technique for a CR-39 detector for soil and water radon exhalation rate measurements

The calibration factor of 0.029 ± 0.0002 track cm^?2 per Bq d m^?3 for radon concentration measurements was determined using CR-39 and RAD7 detectors. The ²²²Rn concentration varied from 2,225 to 9,950 and 12 to 1,002 Bq m^?3 in soil and water, respectively. The highest radon exhalation and gamma dose rates were found in Acid and undifferentiated granitic rocks and Miscellaneous soils.     

Fast liquid chromatographic determination of radiochemical and chemical purity of [11C]methionine by UPLC technique

Salinity, water logging, high nitrate, fluoride and dissolved uranium concentration in drinking water of southwest Punjab has impacted the local population leading to health issues and additional burden on economy. Though it was known that both U and its daughter products especially Rn contribute to radiological dose to the population through drinking water, there were no correlation studies carried out between these radioactive elements in U impacted regions of southwest Punjab. In this study, an initiative has been taken to assess the doses due to dissolved radon in drinking water. In addition, the U–Rn couple is evaluated in detail along with other hydrochemical parameters. The radon concentration ranges from 360–1700 Bq/m³ for Faridkot and 140–1400 Bq/m³ for Muktsar for both seasons and the related average total dose due to radon for both season of Faridkot and Muktsar are 9.79 µS/year and 7.74 µS/year respectively. The total dissolved uranium is in range of 16–350 µg/L for Faridkot and 14–106 µg/L for Muktsar for both seasons. An inverse correlation was observed between Rn and U, which could be attributed to diverse geochemistry of U and Rn in groundwater.

     

Study of radon in ground water and physicochemical parameters in Khartoum state

This study was conducted primarily to measure and map radon activity concentration in wells within water supply network of Khartoum State. Ground water samples were collected before and after autumn and analysed using low level γ-spectrometry equipped with HPGe-detector. Radon activity concentration was found in the range of 1.58–345.10 Bq/L with an average value of 59.20 ± 6.60 Bq/L. Upon comparing the radon concentration values obtained with EPA it was found they were far below the maximum contaminant level of EPA with the exception five samples. Physicochemical water parameters were measured and no correlation was noted between radon concentration and these parameters. The overall annual effective dose for adults due to radon ingestion is less than WHO recommended reference dose level for most except 14 samples.     

Outdoor 222Radon concentrations monitoring in relation with particulate matter levels and possible health effects

Air quality monitoring could potentially improve exposure estimates for use in epidemiological studies. We investigated air quality by monitoring concentrations of ²²²Rn near the ground and particulate matter (PM) with an aerodynamic diameter less than or equal to 10 μm (PM10) and 2.5 μm (PM2.5) for Bucharest-Magurele periurban area. Atmospheric radon concentrations have been continuously monitored near the ground at 1 m height as well as at 10 m height. This paper presents time-series of radon concentrations monitoring in air near the ground measured during 1 January 2011–1 January 2012 by use of solid state nuclear track detectors SSNTD CR-39, exposed for 10 days periods. The daily average atmospheric radon concentration near the ground registered at 1 m height was found to be in range of 40.25 ± 7.53 Bq/m³, which was comparable with the daily average radon concentration of 44.92 ± 9.94 Bq/m³ recorded for period 1 August 2011–20 December 2011 at 10 m height by AlphaGUARD Radon monitor. Also, was done a comparative analysis of spatio-temporal variations in time series of outdoor radon concentration and PM in two size fractions (PM10 and PM2.5) in Bucharest Magurele area for 2011 year. The predominant recorded component in PM10 was PM2.5. Observational results show that recorded yearly average PM2.5 and PM10 concentrations were 35.96 μg/m³ and 40.91 μg/m³, respectively. The average ratio of PM2.5/PM10 was 87.9 % at this sampling site. However, in densely populated Bucharest urban and suburban areas the mean daily EC limit values for PM10, PM2.5 and attached ²²²Rn are frequently exceeded leading to serious public concern during the last years. The ambient air pollution measurements like as PM10 and PM2.5 levels are used as a proxy for personal exposure levels. Have been investigated also meteorological effects on the temporal patterns of atmospheric radon and particle matter.     

Seasonal and diurnal variations of radon/thoron exhalation rate in Kanto-loam area in Japan

Radon and thoron concentration in the outdoor environment are affected by the magnitude of the exhalation rate that can vary diurnally and seasonally. This paper presents measurement results of radon and thoron exhalation rates and gamma-ray dose rate in different season at same location points in Gunma Prefecture Japan. Exhalation rates were measured by the MSZ instrument which is based on the accumulation method. Three measurement points Katashina Village, Midori City and Takasaki City were selected for measurement. Soil water saturation and soil temperature were measured to investigate their relationship with exhalation rate. The diurnal variation of exhalation rate may be correlated with soil temperature but no clear relationship was found between them. The gamma-ray dose rate do not vary significantly at the same places even in different season. The average radon exhalation rates were 11 ± 2, 2 ± 1, 5 ± 3 and 11 ± 4 mBq m⁻² s⁻¹ for spring, summer, autumn and winter, respectively. Those for thoron were 1,100 ± 100, 120 ± 30, 250 ± 80 and 860 ± 140 mBq m⁻² s⁻¹. Thus there was a variation of radon and thoron exhalation rate with different seasons. The radon and thoron exhalation rates in the summer and autumn surveys are higher than those in the spring and winter surveys which were affected by rainfall. It indicates that water saturation is an influential factor for radon and thoron exhalation rates.     

Determination of activity ratios of <Superscript>238,239+240,241</Superscript>Pu, <Superscript>241</Superscript>Am, <Superscript>134,137</Superscript>Cs,and <Superscript>90</Superscript>Sr in Bulgarian soils

The origins of different artificial radionuclides found in soils from Northern and Southern Bulgaria was determined by measurements of their actual concentrations and respective ratios. On the basis of the measured mobility and concentrations of the investigated radionuclides in soils, it was estimated that after the Chernobyl accident the mean depositions of fresh ¹³⁷Cs were 3.0 ± 2.5 kBq/m² for Northern Bulgaria and 15 ± 7 kBq/m² for Southern Bulgaria. As a result of global fallout following atmospheric nuclear weapon tests in the 1950s, mean depositions (corrected to 1965) were calculated for Northern and Southern Bulgaria as follows: for ⁹⁰Sr—1.0 ± 0.5 and 2.3 ± 1.3 kBq/m², ²³⁸Pu—1.3 ± 0.8 and 2.8 ± 1.6 Bq/m², ^239+240Pu—15 ± 14 and 47 ± 38 Bq/m², and ²⁴¹Pu—520 ± 200 and 760 ± 260 Bq/m².     

Radon measurements in groundwater

A device was developed for the collection, containment, and bubbling of radon from groundwater samples to facilitate concentration measurements in the field without the need for fragile glassware. Wellwater supplies were collected in high-potential areas of New York State in a comparison of the device with traditional methods (liquid scintillation and laboratory-based Lucas-cell counters). Waterborne radon levels to 4100 Bq L^–1 reveal the potential contribution to indoor air from everyday water use in a home, as levels of 1500 Bq L^–1 contribute about 150 Bq m^–3 (the EPA-recommended limit) to indoor-air radon levels. With a Geographic Information System (GIS), spatial coordinates from each site are used to correlate concentrations with bedrock geology.     

Radon concentration in air, hot spring water, and bottled mineral water in one hot spring area in Thailand

Hot springs are famous as spa resorts throughout the world. However, these areas usually have high natural radioactivity from radon gas. In this study radon concentrations in air, hot spring water, and bottled mineral water produced in a spa area of Suan Phueng district, Ratchaburi province, Thailand were measured. Radon concentrations in air were in the range of 10–17 and 11–147 Bq/m³ for outdoor and indoor, respectively. Committed effective dose from inhale of radon were assessed and found to be in the range of 0.004–0.025, 0.25–0.6, and 1.134 mSv/y for visitor, local people and resort workers, respectively. These doses were in the range of 1.2 mSv/y regulated by UNSCEAR for the general public. Radon in hot spring water ranged from 2–154 Bq/L. Radon in bottled mineral water produced from the hot spring water were in the range of 17–22 and 0.2–0.3 Bq/L for those that stored for 7 and 90 days, respectively, after production. Radon concentration levels were in the range of the US Environmental Protection Agency reference level for radon in air which is 148 Bq/m³ and alternative maximum concentration limit (AMCL) for raw water which is 150 Bq/L. However, when considering the USEPA (Maximum concentration limit), 11 Bq/L, for radon in drinking water, the mineral water should be stored for at least 8–9 days after bottling before selling to the market.     

Ultralight sulfonated graphene aerogel for efficient adsorption of uranium from aqueous solutions

The radon activity concentration was measured in 67 rooms in kindergartens in Visegrad countries over a period of 1 year using the SSNTD method within the framework of the standard V4 project. In 7.5% of rooms radon activity concentration exceeded 300 Bq m^?3, the reference value recommended by the Council Directive 2013/59/EURATOM. The annual effective doses due to radon inhalation ranged from 0.5 to 13.3 mSv for children and from 0.3 to 8.3 mSv for staff.

     

Ground level ozone (O3) associated with radon (222Rn) and particulate matter (PM) concentrations in Bucharest metropolitan area and adverse health effects

The aim of this paper is to contribute with new information in the application of ground based radon (²²²Rn) observations to atmospheric research, namely its relation with air pollution due to ground-level ozone (O₃) and particle matter in two size fractions (PM10 and PM2.5) for Bucharest metropolitan area in Romania. During January 1–December 31, 2011, ground levels of radon, ozone and particulate matter (PM) have been continuously monitored in synergy with the main meteorological parameters (air temperature, humidity and pressure), and daily global air quality indices. A systematic analysis of surface ozone observations of ground level radon, ozone and PM is presented. Observational results indicate the following yearly daily mean ground level concentrations: 40.26 ± 7.54 Bq/m³ for radon, 90.51 μg/m³ for ozone, 35.96 μg/m³ for PM2.5, and 40.91 μg/m³ for PM10. The assessment of the results showed the influence of local and meteorological conditions on the daily mean radon, ozone and PM concentrations. However, in densely populated metropolitan area of Bucharest the mean daily values of ozone, PM2.5, PM10, and attached ²²²Rn are sometimes higher than European Community limit values leading to serious public concern during the last years. Due to the high risk of increased levels of O₃, PM2.5, PM10, and attached ²²²Rn on human health respiratory function (especially for children and older persons), and urban green, the results are very useful for atmospheric, radiological protection, epidemiological and environmental studies.     

Radon health hazards of some rocks of Iranian origin, frequently used as building stones

Radon exhalation rate from various types of stones, used inside the living buildings, is a major factor for evaluation of the environmental radon level. To verify the significance and lethal impacts of this unknown and obscure source of radiation upon the people around the world, the exhaled radon gas concentrations from the rocks, granodiorite, granite, limestone and aragonite, and the effect of their block sizes on the exhalation rate, have been studied. The block samples, collected from their ores, were transferred to plastic containers in which the CR-39 detectors could properly be placed and air tightened, for concentration measurements. The results show the radon concentration of 7.4 ± 0.8, 6.6 ± 0.6, 0.08 ± 0.02 and 0.09 ± 0.02 kBq m⁻³ for granodiorite, granite, limestone and aragonite, respectively. The corresponding annual dose values in a closed environment are: 186 ± 20, 166 ± 15, 2.5 ± 1 and 2 ± 1 mSv y⁻¹. These absorbed dose values indicate that granodiorite and granite when used inside the buildings could increase the risk of various cancers while aragonite and limestone have much lower risks and are recommended for use inside the buildings. The former ones when used in the closure areas remedial action should be implemented. The results do not show obvious dependence between the rock size of the samples and their radon exhalation rate.     

An unusual case of indoor air radon contamination: An unusual method for effective mitigation

In the course of routine surveillance for indoor radon in Austria, concentrations above 10,000 Bq/m³ were found in a house in the province of Carinthia, Austria. Multiple 3-day-measurements in all the rooms of the house were carried out for the next 21 months. All rooms of the house had elevated radon concentrations but radon levels decreased systematically from east to west within the house. Moreover, radon concentrations in one room of the building were found to be below 300 Bq/m³ in winter but above 12,000 Bq/m³ in summer. After installing a medium sized fan, operated only during the summer season, the semiannual summer radon levels dropped from approximately 8,000 Bq/m³ to 250 Bq/m³ at ground floor level. Note: The paper reflects the personal opinions of the authors.