Temporal evolution and instability in a viscoelastic dielectric elastomer

Dielectric elastomer transducers are being developed for applications in stretchable electronics, tunable optics, biomedical devices, and soft machines. These transducers exhibit highly nonlinear electromechanical behavior: a dielectric membrane under voltage can form wrinkles, undergo snap-through instability, and suffer electrical breakdown. We investigate temporal evolution and instability by conducting a large set of experiments under various prestretches and loading rates, and by developing a model that allows viscoelastic instability. We use the model to classify types of instability, and map the experimental observations according to prestretches and loading rates. The model describes the entire set of experimental observations. A new type of instability is discovered, which we call wrinkle-to-wrinkle transition. A flat membrane at a critical voltage forms wrinkles and then, at a second critical voltage, snaps into another state of winkles of a shorter wavelength. This study demonstrates that viscoelasticity is essential to the understanding of temporal evolution and instability of dielectric elastomers.     

On the dynamic electromechanical loading of dielectric elastomer membranes

Dielectric elastomer actuators (DEAs) have received considerable attention recently due to large voltage-induced strains, which can be over 100%. Previously, a large deformation quasi-static model that describes the out-of-plane deformations of clamped diaphragms was derived. The numerical model results compare well with quasi-static experimental results for the same configuration. With relevance to dynamic applications, the time-varying response of initially planar dielectric elastomer membranes configured for out-of-plane deformations has not been reported until now. In this paper, an experimental investigation and analysis of the dynamic response of a dielectric elastomer membrane is reported. The experiments were conducted with prestretched DEAs fabricated from 0.5 mm thick polyacrylate films and carbon grease electrodes. The experiments covered the electromechanical spectrum by investigating membrane response due to (i) a time-varying voltage input and (ii) a time-varying pressure input, resulting in a combined electromechanical loading state in both cases. For the time-varying voltage experiments, the membrane had a prestretch of three and was passively inflated to various predetermined states, and then actuated. The pole strains incurred during the inflation were as high as 25.6%, corresponding to slightly less than a hemispherical state. On actuation, the membrane would inflate further, causing a maximum additional strain of 9.5%. For the time-varying pressure experiments, the prestretched membrane was inflated and deflated mechanically while a constant voltage was applied. The membrane was cycled between various predetermined inflation states, the largest of which was nearly hemispherical, which with an applied constant voltage of 3 kV corresponded to a maximum polar strain of 28%. The results from these experiments reveal that the response of the membrane is a departure from the classical dynamic response of continuum membrane structures. The dynamic response of the membrane is that of a damped system with specific deformation shapes reminiscent of the classical membrane mode shapes but without same-phase oscillation, that is to say all parts of the system do not pass through the equilibrium configuration at the same time. Of particular interest is the ability to excite these deformations through a varying electrical load at constant mechanical pressure.     

Electric field-induced surface transformations and experimental dynamic characteristics of dielectric elastomer membranes

Acute and tunable surface transformations of a monolithic structure by application of an electric field have immediate significance for adaptive structures, morphing concepts and optical applications. Dielectric elastomer (DE) membranes are electric field-responsive materials typically employed as large strain electrostatic actuators. In this paper, it is demonstrated that an electric field will generate several symmetric surface shapes analogous to the mode shapes in the classical drumhead or stretched membrane problem. In a previous experimental study, a single surface transformation creating ripples or waves on an initially smooth surface was observed for an electrically excited DE membrane. The unexpected result led to the development of an experimental setup that would facilitate extensive characterization of the dynamic surface transformations of dielectric elastomer membranes. The new results clearly show that the electric field can be used to tune the patterns of the DE surface. Furthermore, the membrane will go through resonance when a periodic electric field is applied if the system conditions are favorable, which has not been observed before now. This presents a unique opportunity to increase the output displacement of DE membranes without electrically overloading the membrane. The experiments show that increasing the size of the chamber onto which the membrane is clamped will increase the peak deformation as well as cause the membrane's resonance peaks to shift and change in number. For DE membranes driven at 1.5 kV, at the smallest chamber volume, the maximum actuation displacement is 81 μm; while at the largest chamber volume, the maximum actuation displacement is 1431 μm. This corresponds to a 1767% increase in maximum pole displacement. The dependence on chamber volume suggests that under dynamic conditions a systems level analysis is needed for DE actuators. The effect of voltage offset as a means of modulating the dynamic deformation response is also reported in this study.     

Electro-mechanical coupling bifurcation and bulging propagation in a cylindrical dielectric elastomer tube

This paper explores the critical and post-bulging bifurcation of a cylindrical dielectric elastomer (DE) tube undergoing finite deformation under electro-mechanical coupling loading. Explicit expressions for the critical conditions of electro-mechanical bifurcation are derived by using a simplified mathematical method. The post-bifurcation path is comprehensively investigated by specifying the material model as ideal dielectric elastomer. In the post-bifurcation analysis, we analytically establish conditions for the phase coexistence of steady propagation and analyze the physical implications. We demonstrate a global instability under force or voltage control and a localized instability under volume or charge control. Cylindrical tube experiments have been carried out under electro-mechanical coupling loading to verify the theoretical predictions. Good agreements on the critical conditions as well as the post-bifurcation path are obtained. This work characterizes the bifurcation mechanism of rubber-like materials under complex coupling loading.     

Experimental slowing of flexural waves in dielectric elastomer films by voltage

Shape and physical properties of dielectric elastomers are changeable by voltage. Theoretical works show that these changes can be harnessed to tune the propagation of superposed elastic waves. We experimentally demonstrate this concept by manipulating waves in a dielectric elastomer film, focusing on the flexural mode at low frequencies. To this end, we design an experimental apparatus to pre-stretch, actuate, excite waves at low frequencies in a VHB™ 4910 film, and measure the velocity of the fundamental flexural mode. Our results show that the excited wave velocity is slowed down by the applied voltage, and provide experimental proof of concept for the application of deformable dielectrics as tunable waveguides.     

Mechanics of physisorption on elastomer surface

Mechanical aspects of physisorption on elastomeric substrates are studied via a continuum model in combination with the Lennard-Jones potential. In light of the incompressibility of elastomers, it is shown that the presence of a zero-dimensional adsorbate gives rise to a distributed force on the surface of the substrate. The induced surface deformation is determined, and the adsorption force and energy which depend on the substrate stiffness are derived. The results are then used to examine mutual interaction between two like adsorbates with small spacing, showing complicated attraction and repulsion arising from elastic deformation of the substrate. The dipole and quadruple moments of an adsorbate are also calculated, and the multipole approximation is adopted to quantify the interaction when the two adsorbates are separated remotely.     

Constitutive relation of viscoelastic dielectric elastomer

In this paper, we present a modified model describing the constitutive relation of viscoelastic dielectric elastomer (DE). The uniform uniaxial tension-recovery experiment was carried out at different stretching rates. Based on Yeoh hyper-elastic model, model-fitting approach is put forward to obtain the relationship between parameters of Yeoh model and stretching rate, thus the modified model was obtained. From the approximate relationship between harmonic motion and uniform reciprocating motion, the stress–strain curve in the recovery process was also identified through the hysteresis between stress and strain. The modified model, with concise form and evident physical concept, can describe the strong nonlinear behavior between deformation and mechanical stress of the material in a common stretching rate range (from 0.01s^?1 to 0.8s^?1 at least). The accuracy and reliability of the modified model was examined.     

The electro-mechanical response of elastomer membranes coated with ultra-thin metal electrodes

This paper presents experimental and theoretical analyses of the electro-mechanical response of metal/elastomer multilayers. A novel test has been devised to determine the relationship between the mechanical response of clamped elastomer membranes, coated on both sides with metal electrodes, and an applied electric field. The load-deflection response of the multilayers subjected to different voltages was measured using an instrumented spherical indenter having dimensions comparable to the freestanding span. The measurements are used with closed-form solutions for membrane deflection to determine the effective plane-strain modulus of cracked multilayers and electrically induced in-plane strains. The experiments demonstrate that: (i) electrically induced strains vary with the square of the electric field, as expected from electrostatic models of parallel plate capacitors, (ii) the transverse stiffness of membranes can be controlled using applied electric fields, (iii) analytical models accurately predict the relationship between electrode crack spacing, layer properties and effective moduli. Finally, we estimate the toughness of the sub-micron metal electrodes, using cracking models that relate crack spacing, imposed strain and the energy release rate governing channel crack formation.     

A nonlinear field theory of deformable dielectrics

Two difficulties have long troubled the field theory of dielectric solids. First, when two electric charges are placed inside a dielectric solid, the force between them is not a measurable quantity. Second, when a dielectric solid deforms, the true electric field and true electric displacement are not work conjugates. These difficulties are circumvented in a new formulation of the theory in this paper. Imagine that each material particle in a dielectric is attached with a weight and a battery, and prescribe a field of virtual displacement and a field of virtual voltage. Associated with the virtual work done by the weights and inertia, define the nominal stress as the conjugate to the gradient of the virtual displacement. Associated with the virtual work done by the batteries, define the nominal electric displacement as the conjugate to the gradient of virtual voltage. The approach does not start with Newton's laws of mechanics and Maxwell-Faraday theory of electrostatics, but produces them as consequences. The definitions lead to familiar and decoupled field equations. Electromechanical coupling enters the theory through material laws. In the limiting case of a fluid dielectric, the theory recovers the Maxwell stress. The approach is developed for finite deformation, and is applicable to both elastic and inelastic dielectrics. As applications of the theory, we discuss material laws for elastic dielectrics, and study infinitesimal fields superimposed upon a given field, including phenomena such as vibration, wave propagation, and bifurcation.     

Predicting failure modes and ductility of dual phase steels using plastic strain localization

Ductile failure of metals is often treated as the result of void nucleation, growth and coalescence. Various criteria have been proposed to capture this failure mechanism for various materials. In this study, ductile failure of dual phase steels is predicted in the form of plastic strain localization resulting from the incompatible deformation between the harder martensite phase and the softer ferrite matrix. Microstructure-level inhomogeneity serves as the initial imperfection triggering the instability in the form of plastic strain localization during the deformation process. Failure modes and ultimate ductility of two dual phase steels are analyzed using finite element analyses based on the actual steel microstructures. The plastic work hardening properties for the constituent phases are determined by the in-situ synchrotron-based high-energy X-ray diffraction technique. Under different loading conditions, different failure modes and ultimate ductility are predicted in the form of plastic strain localization. It is found that the local failure mode and ultimate ductility of dual phase steels are closely related to the stress state in the material. Under plane stress condition with free lateral boundary, one dominant shear band develops and leads to final failure of the material. However, if the lateral boundary is constrained, splitting failure perpendicular to the loading direction is predicted with much reduced ductility. On the other hand, under plane strain loading condition, commonly observed necking phenomenon is predicted which leads to the final failure of the material. These predictions are in reasonably good agreement with experimental observations.     

Dynamic response of dielectric elastomers

Dielectric elastomers have received a great deal of attention recently for effectively transforming electrical energy to mechanical work. Their large strains and conformability make them enticing materials for many new types of actuators. Unfortunately, their non-linear material behavior and large deformations make actual devices difficult to model. However, the reason for this difficulty can also be used to design actuators that utilize these material and geometric non-linearities to obtain multiple stable equilibria. In this work, we investigate one of the simplest possible configurations, a spherical membrane, using a model that incorporates both mechanical and electrostatic pressure as well as inertial effects that become important when transitioning from one equilibrium to another.     

Nonlinear dynamic analysis of dielectric elastomer membrane with electrostriction

The dielectric elastomer (DE) is an important intelligent soft material widely used in soft actuators, and the dynamic response of the DE is highly nonlinear due to the material properties. In the DE, electrostriction denotes the deformation-dependent permittivity. In the present study, we formulate the nonlinear dynamic governing equations of the DE membrane considering the electrostriction effect. The free vibration and parametric excitation of the DE membrane with different geometric sizes are calculated. The free vibration bifurcations induced by the initial location and the voltage are both discussed according to an energy-based approach. The amplitude-frequency characteristics and bifurcation diagrams of parametric excitation are also given. The results show that electrostriction decreases the free vibration amplitude and increases the frequency, but it has less influence on the parametric excitation oscillation frequency and decreases the parametric excitation amplitude except when the membrane resonates. The initial location and the applied voltage can induce the snap-through instability of the free vibration. A large geometric size will lead to a much lower resonance frequency. The resonance amplitudes increase while the resonance frequencies decrease with the increase in the applied voltage. The critical voltage of snap-through instability for the parametric excitation is larger than that for the free vibration one.

     

Cohesive fracture simulation and failure modes of FRP–concrete bonded interfaces

A work-of-fracture method using three-point bend beam (3PBB) specimen, commonly employed to determine the fracture energy of concrete, is adapted to evaluate the mode-I cohesive fracture of fiber reinforced plastic (FRP) composite–concrete adhesively bonded interfaces. In this study, a bilinear damage cohesive zone model (CZM) is used to simulate cohesive fracture of FRP–concrete bonded interfaces. The interface cohesive process damage model is proposed to simulate the adhesive–concrete interface debonding; while a tensile plastic damage model is used to account for the cohesive cracking of concrete near the bond line. The influences of the important interface parameters, such as the interface cohesive strength, concrete tensile strength, critical interface energy, and concrete fracture energy, on the interface failure modes and load-carrying capacity are discussed in detail through a numerical finite element parametric study. The results of numerical simulations indicate that there is a transition of the failure modes controlling the interface fracture process. Three failure modes in the mode-I fracture of FRP–concrete interface bond are identified: (1) complete adhesive–concrete interface debonding (a weak bond), (2) complete concrete cohesive cracking near the bond line (a strong bond), and (3) a combined failure of interface debonding and concrete cohesive cracking. With the change of interface parameters, the transition of failure modes from interface debonding to concrete cohesive cracking is captured, and such a transition cannot be revealed by using a conventional fracture mechanics-based approach, in which only an energy criterion for fracture is employed. The proposed cohesive damage models for the interface and concrete combined with the numerical finite element simulation can be used to analyze the interface fracture process, predict the load-carrying capacity and ductility, and optimize the interface design, and they can further shed new light on the interface failure modes and transition mechanism which emulate the practical application.     

Temperature effects on the dynamic response of viscoelastic dielectric elastomer

Viscoelasticity and temperature can significantly affect the performance of a dielectric elastomer. In the current study, we use a thermodynamic model to describe the effect of temperature and viscoelasticity on the electromechanical response undergoing a cyclic electric load by taking into account of the temperature dependent dielectric constant. Because of the significant viscoelasticity in the dielectric elastomer, the deformation and the nominal electric displacement can not keep in phase with the electric field at low frequencies. The results show that the magnitude of the cyclic electromechanical actuation strain increases with the decrease of the temperature and decreases with the increasing frequency, and viscoelasticity can result in significant hysteresis for dielectric elastomers under a relative low temperature and a low frequency.     

Impact of reinforcing filler on the dynamic moduli of elastomer compounds under shear deformation in relation to wet sliding friction

In pursuit of a better understanding of the relationship between wet sliding friction and bulk viscoelastic properties of elastomer compounds, especially the contribution from different reinforcing fillers, the linear thermorheological behavior, the nonlinear dynamic moduli under shear deformation (for strain up to about 140%), and the wet sliding friction have been characterized in detail for crosslinked compounds of low-cis polybutadiene filled with different reinforcing fillers including carbon black, graphitized carbon black, and precipitated silica. We examine the scenario of possible extra energy dissipation via higher harmonic excitation in rubber compounds coupled with dynamic deformation consisting of components at many frequencies during sliding of rubber on a rough surface. While no straightforward explanation is identified relating the observed difference in wet sliding friction arising from different fillers to the bulk viscoelastic properties, some unexpected viscoelastic features arising from the compounds are observed.     

An investigation into the effect of electric field on the performance of Dielectric Barrier Discharge plasma actuators

The influence of the inter-electrode electric field of a single Dielectric Barrier Discharge (DBD) actuator on the performance of the device was investigated. The electric field of the actuator was manipulated through the variation of the angle between the electrodes of the actuators. Response forces generated by the plasma actuators were used as performance indicators for these devices. These forces were measured directly utilizing a highly sensitive balance scale. It was verified that depending on the orientation of the variation of the angle between the electrodes, the performance of the actuator may be decreased or increased when compared to a DBD on a flat dielectric plate more commonly investigated in literature. The manner in which the ionic wind flows over the actuators was also explored in the effort to elucidate the influence of the variation of the angle between the electrodes on the response force generated by the device. Results demonstrated that the response forces generated by the actuators may be improved by up to 50% compared to the actuator configuration on a flat dielectric plate commonly investigated. These results indicate the potential available to advance plasma technology by physically manipulating these devices to increase the performances of the actuators.     

介电弹性作动器主动隔振模糊控制试验研究

采用模糊控制策略,开展介电弹性作动器的主动隔振性能试验研究。基于介电弹性材料的Maxwell应力模型建立了作动器的力电耦合模型,分析了作动器的非线性特性;针对隔振系统设计了Mamdani型模糊控制器,建立了控制电压信号与振动响应之间的关系;在此基础上,开展了介电弹性作动器主动隔振试验研究,并与加速度反馈控制进行了对比。试验结果表明,在相同驱动电压的情况下,基于模糊控制策略的主动隔振性能要优于加速度反馈控制,且能够显著降低由于非线性驱动力导致的倍频响应幅值,有助于提高隔振系统的稳定性。     

Electro-viscoelastic behaviors of circular dielectric elastomer membrane actuator containing concentric rigid inclusion

The time-dependent electro-viscoelastic performance of a circular dielectric elastomer (DE) membrane actuator containing an inclusion is investigated in the context of the nonlinear theory for viscoelastic dielectrics. The membrane, a key part of the actuator, is centrally attached to a rigid inclusion of the radius a, and then connected to a fixed rigid ring of the radius b. When subject to a pressure and a voltage, the membrane inflates into an out-of-plane shape and undergoes an inhomogeneous large deformation. The governing equations for the large deformation are derived by means of non-equilibrium thermodynamics, and viscoelasticity of the membrane is characterized by a rheological spring-dashpot model. In the simulation, effects of the pressure, the voltage, and design parameters on the electromechanical viscoelastic behaviors of the membrane are investigated. Evolutions of the considered variables and profiles of the deformed membrane are obtained numerically and illustrated graphically. The results show that electromechanical loadings and design parameters significantly influence the electro-viscoelastic behaviors of the membrane. The design parameters can be tailored to improve the performance of the membrane. The approach may provide guidelines in designing and optimizing such DE devices.