Multipole mixing ratios of transitions in175Lu populated from the decay of175Hf

Electron capture decay of¹⁷⁵Hf(70 d) provides a possibility for unambiguous determination of the sign and magnitude of multipole mixing ratios for 89 keV and 114 keV transitions in¹⁷⁵Lu. This is because both gamma rays are in coincidence with the 230 keV transition which is of a pureE2 character. The results of theγ —γ directional correlation measurements, in terms ofE2/M1 mixing ratiosδ, areδ ₈₉ = 0.11±0.07 andδ ₁₁₄ = 0.465±0.005. In addition the directional correlation measurements of the 89γ- 343γ and 319γ-114γ cascades yieldδ ₃₄₃ = 0.08±0.07 andδ ₃₁₉ = ?0.152±0.015.Radioactivity ¹⁷⁵Hf from¹⁷⁴Hf(n, γ); measuredγ —γ(θ) deducedδ(E2/M1); Ge(Li) detectors.     

Multipole mixing ratios of transitions in Te

Gamma-gamma directional correlation measurements were made on nine transitions in ¹²⁴Te with a NaI(Tl)-Ge(Li) detector arrangement and multichannel analysis. The multipole mixing ratios obtained were δ(646) = 0.000±0.001, δ(714) = 1.5_−0.3^+0.6, δ(723) = −3.3±0.2, δ(1437) = 3.7_−2.0^+2.7, δ(1489) = −3.4_−1.5^+0.9, δ(968) = −0.03_−0.05^+0.06, δ(1368) = −0.045±0.090, δ(1045) = 0.041_−0.041^+0.047, δ(1691) = −0.02±0.01, and δ(2091) = 0.00_−0.03^+0.02. The first δ is M3/E2, the next three are E2/M1, and the last five are M2/E1. The retardation (a factor of approximately 50) of the crossover to cascade transitions from the 2039 keV, third 2⁺ level to the second and first 2⁺ levels is essentially the same for both the M1 and E2 components. In addition, spin and parity assignments of 2⁺ were made for the 2039 and 2092 keV levels.     

g-Faktoren und Multipol-Mischungsverhältnisse in156Gd

By integral perturbedγ-γ-angular correlation the gyromagnetic ratios of a 2-quasi-particle state at 1,513 keV and the 4⁺ state of the ground state rotational band in¹⁵⁶Gd were measured, using sources prepared by¹⁵⁹Tb(γ, 3n) and¹⁵⁶Gd(d, 2n) reactions:g _{1;513 keV} ⁴⁺ =0.78±0.05;g _R ⁴⁺ =0.37±0.05. In addition we obtain the multipole mixing ratiosδ _{535 keV}(M2/E1)=?0.09±0.01;δ _{1,225 keV}(E2/M1)=+1.83±0.10 for the 535 keV and 1,225 keVγ-rays. The classification of the 1,513 keV state is discussed. The internal field of Gd in Tb metal at 77 °K was found to beH=(?192±16)kOe.     

铝-镉-铜三元系富铜合金相图

铝-镉-铜三元系富铜合金相图的室温固相截面已用X-射线方法测定。合金含量最高达30％(重量)铝及30％镉。室温相截面由五个单相区α,γ₂,δ,ζ₂,η₂;十个两相区α+β,α+γ₂,β+γ₂,γ₂+δ,β+δ,δ+ζ₂,ζ₂+η,η₂+δ,η₂+β,η₂+θ及四个三相区α+β+γ₂,β+γ₂+δ,β+δ+η₂,δ+ζ₂+η₂所构成。没有发现新相。     

Multipole mixing ratios of electromagnetic transitions in Gd

Using γ-γ(θ), γ(θ) (nuclear orientation) and e_k-γ(θ) directional correlation techniques, we have determined the multipole character of some transitions connecting the quadrupole and octupole quasi-vibrational bands to the ground state quasi-rotational band in ¹⁵²Gd following the decay of ¹⁵²Tb. For the γ-γ directional correlation measurements a high-energy resolution system employing a Ge(Li) and a NaI(Tl) detector was used while for the e_k-γ correlation we used a NaI(Tl) and magnetic lens spectrometer system. The nuclear orientation measurements were carried out at low temperatures obtained with a ³He-⁴He dilution refrigerator. The results show that the 2⁺ → 2⁺ transition between the β-vibrational and the ground state bands contains ≈ 10% Ml admixture, δ = − 3.05 ± 0.14, and a large E0 contribution while the similar transition from the γ-vibrational band has δ = 4.3 ± 0.7. These results are compared with Kumar's predictions for similar transitions in ¹⁵²Sm. Three other mixing ratios were also determined.     

Nuclear orientation study of the excited states of 129I populated in the decay of 129gTe and 129mTe

From the angular distributions of γ-rays emitted by oriented ^129gTe and ^129mTe nuclei implanted in iron by isotope separator, unique spin assignments could be made for the excited states of ¹²⁹I at 487.4 keV $\text{(}\text{5}\text{2}{}^{\mathrm{+}}\text{)}$, 696.0 keV $\text{(}\text{11}\text{2}{}^{\mathrm{+}}\text{)}$, 729.6 keV $\text{(}\text{9}\text{2}{}^{\mathrm{+}}\text{)}$, 768.9 keV $\text{(}\text{7}\text{2}{}^{\mathrm{+}}\text{)}$, 1050.4 keV $\text{(}\text{7}\text{2}{}^{\mathrm{+}}\text{)}$ and 1111.8 keV $\text{(}\text{5}\text{2}{}^{\mathrm{+}}\text{)}$. In addition, E2/M1 amplitude ratios for the following ¹²⁹I γ-rays (energies are in keV) are derived: δ(459.6) = ?(0.076^+0.037_?0.148); δ(487.4) = 0.50^+0.17_?0.10 or δ^? = 0.35^+0.15_?0.09; δ(556.7) = 0.06±0.02 or δ^? = ?(0.10±0.02); δ(624.4) = 0.10±0.26 or δ^? > 0.4; the 696.0 keV γ-ray is pure E2; δ(729.6) = ?(0.34±0.06) or δ^?1 = 0.55±0.05; δ(741.1) = ?(0.27±0.10) or δ^?1 = ?(0.43±0.12); δ(817.2) = 0.46±0.04 or δ^?1 =0.20±0.03 if $\text{I}{}^{\mathrm{\pi }}\text{(845}\text{keV}\text{) =}\text{7}\text{2}{}^{\mathrm{+}}$; δ(1022.6) = ?(0.02 ±0.02) or δ^?1 = ?(0.23±0.02); $\text{δ(1084) = 0.56}{}^{\mathrm{+0.04}}{}_{\mathrm{?0.14}}$; δ(1111.8) = 0.06±0.05 or δ^?1 = ?(0.08±0.05). The anisotropy of the 531.8 keV γ-ray excludes $\text{1}\text{2}{}^{\mathrm{+}}$ as a possible spin assignment for the 559.6 keV level, so that no $\text{1}\text{2}{}^{\mathrm{+}}$ level is fed in the decay from ¹²⁹Te. Anisotropies for the 209, 250.7, 278.4 and 281.1 keV γ-rays are also measured. Comparison of the level scheme is made with theoretical predictions from both the pairing-plus-quadrupole model and the intermediate coupling unified model.     

Multipole mixing ratios of γ-transltions in 182W

γ-γ directional correlation experiments were performed on 14 cascades in ¹⁸²W populated from the β^? decay of ¹⁸²Ta(115 d). Two Ge(Li) detectors were used in a coincidence arrangement, and the ¹⁸²Ta sources were dissolved in HF acid to minimize extranuclear perturbations. For the 1189keV, 2^? → 2⁺ transition, the measured directional correlation coefficients are consistent only with multipole mixing ratios $\text{δ}\text{(}\text{M}\text{2}\text{E}\text{1)}\text{= 0.45 ± 0.03}\text{and}\text{δ}\text{(E3}\text{E1)}\text{= ?0.67 ± 0.07}$. These mixing ratios are discussed and compared with the known conversion coefficients for the 1189keV transition. The E2/M1 multipole mixing ratios determined are (energy in keV): δ(66) = 0.15 ± 0.15, δ(85) = 0.31 ± 0.05, δ(114) = 0.31 ± 0.05, 0.56 ≦ δ(179) ≦ 1.36, δ(1121) = 12⁺²_?1, and δ(1231) = ?(32⁺¹⁴²_?15). The measured M2/E1 mixing ratios are: δ(68) = 0.03 ± 0.02, δ(152) = 0.014 ± 0.013 and δ(156) = ?0.13 ± 0.19.     

High-spin states in112Cd from the110Pd(α, 2n γ)-reaction

The decay scheme of¹¹²Cd has been studied by γ-ray spectroscopy with the¹¹⁰Pd(α, 2nγ) reaction. Spin and parity assignments were made on the basis of coincidence measurements, angular distributions and excitation functions. Twelve new energy levels were established. A vibrational-like positive-parity band up to spin 8⁺ and a negativeparity side band 5^?, (7^?), (9^?) were found. For the negative-parity states a (v_j, vh_11/2) configuration is suggested. Nuclear Reactions:¹¹⁰Pd(α,2nγ),E _α =15–22.5 MeV; measuredE _γ ,E _γ , (E,E _γ ),E _γ (θ),γ-γ- coincidence;¹¹²Cd deduced levels,J; enriched target.     

Structure of the mirror nuclei21Ne and21Na

Theγ-decay of levels in²¹Ne up to 10 MeV excitation energy has been investigated byn — γ coincidence measurements initiated with the¹⁸O(α, nγ) reaction at 12, 13, 14.5 and 15.4 MeV bombarding energies. Spin(-parity) assignments of excited states are obtained by combining then — γ angular correlation measurements performed atE _α=11, 11.82 and 13.6 MeV with a consideration of lifetimes, neutron penetrabilities of the unbound states, and information from the mirror nucleus²¹Na. The resulting values of E_x[keV]?J ^π are as follows: 4525-5⁺, 4686-3⁺, 5431-7⁺, 5549-3⁺, 5819-7^?, 6175-7⁺, 6268-9⁺, 6550-9, 6639-9, 7006-7⁺, 7041-9, 7356-7 or 9, 7422-11^(?), 7648-7⁺, 7981-11 or (7⁺), 8154-9, 8240-11, 8664-9^? or 11 or 13^?, 9401-13^?, 9867-13^? or 15⁺, 9941-13^? or 15 or 17⁺. The assignment of mirror levels in²¹Ne —²¹Na has been extended to the 6175 keV level of²¹Ne. Excitation energies, electromagnetic properties, Gamow?Teller matrix elements and spectroscopic factors of positive parity states are compared with the results of shell-model calculations which employ a unifieds—d shell Hamiltonian and the unrestricted configuration space of the 0d _5/2 —1s _1/2—0d_3/2 shell. Collective properties contained in shell model wave functions are explored up to the termination of bands atJ=17/2 or 19/2. The spectrum of intruder states in²¹Ne is observed to begin with a 5628 keV,J ^π=7/2⁺ state. The 7422, 8664 and 9401 keV levels are assigned as members of previously established negative-parity rotational bands.     

Band structures in73Se

Excited states of⁷³Se have been investigated up to spin, 21/2 using techniques of in-beamγ-ray spectroscopy in connection with the⁷⁰Ge(α, n) reaction. Mean lifetimes of 12 levels have been determined applying Doppler-shift andγ-RF-methods. Five different bands have been identified that reflect a variety of different excitation modes. The decoupled 9/2⁺ band is likely to correspond to an oblate deformation while the 5/2⁺ band is interpreted as a strongly coupled prolate band built on the Nilsson configuration [422] 5/2⁺. The 3/2^? band is a strongly coupled band built on the [301] 3/2^} configuration.Nuclear reactions:⁷⁰Ge(α,n),E=14, 16, 18, 19, 20MeV; measuredE _γ,I _γ,σ(E _γ,θ),γγ-coin, linear polarization, DSA,γ(t).⁷⁵Se deduced levels,I, π, τ, δ(E2/M1), B(σλ). Enriched targets, Ge detectors.     

Studies of γ-ray transitions in171Yb

The decay of¹⁷¹ Lu(t_1/2=8.2 day) to the levels of¹⁷¹Yb has been studied using large volume high resolution Ge(Li), x-ray Ge(Li) and NaI(Tl) detectors.γ-γ coincidence and directional correlation experiments have been performed. Spin-parity of 5/2^?, 7/2⁺, 5/2^?, 9/2⁺, 7/2^?, 7/2^?, 11/2⁺, 9/2^?, 9/2^? and 5/2^? have been assigned to the 75.87, 95.26, 122.37, 167.62, 208.00, 230.61, 259.02, 835.21, 948.37 and 1024.87 keV levels respectively. Several new coincidence relations have been observed in the present work. Two newγ-transitions at 141.45 and 821.30 keV observed and two levels at 766 and 944 keV been proposed. Multipolarity assignments have been made for most of theγ-transitions from theK-shell internal conversion coefficients obtained using the presentγ-ray intensities and the published conversion electron intensities. A revised level scheme for¹⁷¹Yb has been proposed and compared with published data. Radioactivity¹⁷¹Lu; measuredT _1/2,E _γ ,I _γ ,γγ coin,γγ (θ), I.C.C.,¹⁷¹Yb deduced levels,J, γ-mixing,π. Enriched targets, Ge(Li) detectors.     

Gyromagnetic ratios of the 4+ and 6+ rotational states of184W

The nuclear Larmor precession has been observed for the 2⁺, 4⁺ and 6⁺ rotational states of¹⁸⁴W in the hyperfine field of WFe by application of the TDPAC and the IPAC techniques. A carrier free radioactive source of^184m Re alloyed with high purity iron was used for all three measurements. From the Larmor precession observed in the 2⁺ state by TDPACω _L = 944(15) MHz and the knowng-factor the hyperfine fieldB _{300 K} ^hf (WFe)=?69.6(27)T was derived. The deviation from the result of a spin echo experiment with¹⁸³WFe extrapolated to room temperature may be caused by the Bohr-Weisskopf effect (hyperfine anomaly). IPAC measurements with the same sample polarized in an external magnetic field of 1.6T gave for the 4⁺ and 6⁺ rotational states: ω _L τ(4⁺)=0.0609(22) andω _L τ(6⁺)=0.00735(102). By use of experimentalB(E2)-values theg _R -factors were derived asg _R (4⁺)=+0.276(26) andg _R (6⁺)=+0.281(45). The directional correlation of the 537?384 keVγ-γ cascade has been analysed in terms of anE1/M2/E3 mixture for theK-forbidden 537keV transition. We obtained the mixing ratiosδ(M2/E1)=±0.086(16),δ(E3/E1)=?0.028(5) with the sign convention of Krane and Steffen.     

Level structure of106Mo

The level scheme of the very neutron rich nucleus ₁₀₆ ⁴² Mo₆₄ has been studied for the first time through theβ decay of¹⁰⁶Nb. Six new excited states were observed inγ singles andγ-γ coincidence experiments in addition to the 2⁺, 4⁺ and 6⁺ members of the ground state band. The excitation energies and the deexcitation pattern suggest the interpretation of the levels at 710, 885 and 956 keV as the 2 ₂ ⁺ , 3 ₁ ⁺ and 0 ₂ ⁺ states, respectively. The data support the assumption of a non-axial deformation of¹⁰⁶Mo. A half-life of (1.02±0.05) s has been determined for theβ decay of¹⁰⁶Nb.     

Possible violation of the δS=δQ selection rule in leptonic decays of σ+-hyperons

We have found a possible example of the rare decayσ ⁺ →nΜ ⁺ Ν, which violatesδS=δQ. The positive decay track of theσ ⁺ comes to rest in the hydrogen bubble chamber and decays into ane ⁺. This track has all the characteristics of a stoppingΜ ⁺. The decay neutron fortuitously scatters twice, producing two recoil protons. The only other possible interpretation of the event isσ ⁺→nγ(π ⁺ →Μ ⁺ Ν), where theπ ⁺ →Μ ⁺ Ν decay produces no deflection (θ<0.1 rad) and no significant change in curvature. Using thep-wave radiative decay predictions ofBarshay et al. we calculate that the integrated branching ratio for such “accidental” events isγ(σ ⁺ →nγ(π ⁺ →Μ _stop ⁺ Ν))/γ(σ ⁺ →nπ ⁺)=1.6×10^?6. Most of the contribution to this “accidental” branching ratio comes from radiative decays where theπ ⁺ mesons have ranges less than 1 mm (p _π<20 MeV/c). If one excludes thoseΜ's with ranges less than 1.2 cm the above “accidental” branching ratio becomes 5.5×10^?7. With this figure we estimate that we should have seen 6.5×10^?2 events of this type thusfar in our experiment. The neutron momentum does not help in deciding between the two hypotheses. We therefore assign a confidence level of 7% for the radiative hypothesis. For the leptonic hypothesis we obtain an estimate of the branching ratio,γ(σ ⁺ →nΜ ⁺ Ν)/γ(σ ⁺ →nπ ⁺)=5×10^?5. If one further accepts theσ ⁺ →nπ ⁺ Ν event reported byBarbaro-Galtieri et al. and theσ ⁺ →ne ⁺ Ν event reported byNauenberg et al., one obtains theδS=?δQ leptonic branching ratio [γ(σ ⁺ →nΜ ⁺ Ν)+γ(σ ⁺ →ne ⁺ Ν)]/γ(σ ⁺ →nπ ⁺)=(4±3)×10^?5.     

Zirkulare Polarisation von Gamma-Strahlung nach Neutroneneinfang in23Na und31P

The circular polarization ofγ-rays following the capture of polarized thermal neutrons in a target of²³Na and³¹P was measured. The degree of polarization yielded the spinI=2⁺ for the 0.563 MeV level of²⁴Na. For the 6.53 MeVγ-transition from the compound state to the 0.563 MeV level the mixing ratioδ=0.26 _?0.10 ^0.14 between E2 andM1 radiation was deduced. The measurement is consistent with the spinvalueI=2⁺ of the 2.95 keV resonance for thermal neutron-capture of²⁴Na. For³²P we confirmed the earlier spin assignementI=1⁺ for the 1.149 MeV level. An upper limit 0<δ<0.15 for the mixing ratio of the 6.8 MeV capture-γ-transition was established.     

Measurements of γ-γ and γ-electron directional correlations in119Sb

The directional correlations ofγ-γ andγ-electron cascades in¹¹⁹Sb are measured, in the decay of^119mTe. Bothγ-γ andγ-electron directional correlation coefficients are determined for the cascades (energies in keV): 153.5-1212.7, 942.3-270.5, (976.2+979.3)-270.5, 1095.7-270.5 and 1136.8-270.5. For the cascades 912.6-1366.2, 2013.4-270.5 and 2089.9-270.5γ-γ directional correlations are measured. The mixing ratios evaluated are:δ(M2/E1, 153.5 keV)=0.0003±0.0023,δ(E2/M1, 270.5 keV)=-0.39±0.29,δ(E2/M1, 942.3 keV)= ?0.26±0.12,δ(E3/M2,1095.7 keV)=?0.01±0.07, andδ(M3/E2,1212.7 keV) =0.004±0.007. The result is compared with theoretical predictions.     

Investigation of theβ +-decay of105,106,109In and of100,102Ag

Isomers in the nuclei¹⁰⁰Ag (I=5⁺),¹⁰²Ag (I=5⁺),¹⁰⁵In (I=9/2⁺),¹⁰⁶In (I=6⁺),¹⁰⁸In (I=6⁺) were selectively populated by the reactions⁹⁰Zr(¹⁹F,xnγ),⁹²Mo(¹⁹F, 2pnγ),⁹²Mo(¹²C,pxnγ),⁹⁰Zr(¹⁹F,α3nγ) atE _lab=72 and 66MeV, and their (β ⁺+EC)-decay was studied with an Anticomptonγ-spectrometer. Spins of the beta-decaying isomers are determined. The results obtained for the beta strength functions are discussed as well as new information on the structure of the neutron-deficient even-even daughter nuclei nearZ=50.     

Reinvestigation of the decay scheme of the short-lived isomeric states in112In

The two short-lived isomeric states in¹¹²In have been reinvestigated by means of the¹¹²Cd(d, 2n) and¹⁰⁹Ag (α, n) reactions. Measurements of delayed X- andγ-ray, lifetime and TDPAD spectra have been performed. A 6.32(3) keVγ-ray has been identified in the isomeric decay and anM1 multipolarity has been assigned to it on the basis of the measured internal conversion coefficients:α _L =196(39) andα _tot=231(35). TheE1+M2(δ =+0.24(4)) andE2 multipolarities have been determined for the 263 and 188 keV transitions deexciting the 8^?(T _1/2=2.82(2) μs) and 7⁺ (T _1/2=0.93(2) μs) isomeric states, respectively. A revised isomeric decay scheme is presented.     

164Ta,identification of a new isotope

The new isotope¹⁶⁴Ta (T _1/2=13.6(2)s) was produced in the¹²⁷I(⁴⁰Ca, 3n) reaction and transported to a measuring station by helium jet. Decay properties were observed withα, γ, andγ-γ spectroscopy. TheZ assignment of the new isotope was based ongg-X-ray coincidence measurements. The mass assignment was deduced from measured excitation functions. The twoγ rays assigned to the new activity most likely originate from the 4⁺→2⁺→0⁺ decay sequence in¹⁶⁴Hf. A smallα branch, ≦0.016(5)%, with anα decay energy ofE _α=4,625(15) keV was found and assigned to the decay of¹⁶⁴Ta. The deduced upper limit of theα width for this branch,W _α≦0.6(2), is in accordance with those known for neighbouring nuclei.     

Fourier Transform Emission Spectroscopy of the FΣ-XΣ System of RuN

Emission spectra of RuN have been recorded at high resolution in the region 12 000-35 000 cm⁻¹ using a Fourier transform spectrometer. The molecules were excited in a ruthenium hollow cathode lamp in the presence of about 2.5 Torr of Ne and 5 m Torr of N₂. New bands with origins near 17 758.1, 18 866.4, 19 800.4 and 20 721.5 cm⁻¹ have been assigned as the 0-1, 0-0, 1-0, and 2-0 bands of a new ²Σ⁺-²Σ⁺ system with the lower state as the ground state. This transition has been labeled as F²Σ⁺-X²Σ⁺, with the F²Σ⁺ state arising from the 1σ²2σ²1π⁴1δ⁴4σ¹ configuration. A rotational analysis of these bands has been carried out and spectroscopic constants have been extracted. The principal equilibrium constants for the ground state of RuN are ΔG(1/2)″=1108.3235(22) cm⁻¹, B_e″=0.5545023(42) cm⁻¹, α_e″=0.0034468(57) cm⁻¹, r_e″=1.5714269(60) Å, while the equilibrium constants for the excited state are ω_e′=946.8471(40) cm⁻¹, ω_ex_e′=6.4229(14) cm⁻¹, B_e′=0.50085(21) cm⁻¹, α_e′=0.00375(10) cm⁻¹, r_e′=1.65345(34) Å. This transition is analogous to the E²Σ⁺-X²Σ⁺ system of RhC (W. J. Balfour et al., J. Mol. Spectrosc.198, 393 (1999)).