Decay schemes and total decay energies of89Br and90Br

Spectroscopical investigations of⁸⁹Br and⁹⁰Br have been performed, utilizing the formation of the molecular ion AlBr⁺ in the ion-source of an isotope separator on-line a reactor. Detailed level schemes have been constructed for⁸⁹Kr and⁹⁰Kr, and theβ-strength function of⁸⁹Br and⁹⁰Br below the neutron binding energy is presented. The total decay energy of^89,90Br, as well as of⁸⁹Kr, have been measured by means ofβ γ-coincidences, and the population of excited states in⁸⁹Kr via⁹⁰Br delayed neutrons has been deduced.     

The energy dependence of Delbrück scattering investigated at Z = 73, 82 and 92

Using neutron capture γ-rays from a ¹⁴⁰CeO₂ source installed in the Grenoble high-flux reactor, differential cross sections for the elastic scattering of photons by Ta, Pb and U through θ = 120° have been measured for E = 4.291 and 4.767 MeV. These data have been supplemented by measuring elastic differential cross sections for U, θ = 120° and energies ranging from 0.279 to 1.332 MeV, using radioactive sources. The experimental differential cross sections below 1 MeV confirm the predicted Rayleigh amplitudes based on the second-order S-matrix within 3%. An excellent agreement between experiment and lowest-order Delbrück theory is observed between 1.0 and 1.4 MeV, showing that Coulomb corrections are small close to the threshold for pair production. At 4.291 and 4.767 MeV experiment and lowest-order Delbrück theory agree within ~12%     

Level structure of 147Nd2 (iii). The 146Nd(n,e?) reaction

The conversion electrons following thermal neutron capture in ¹⁴⁶Nd have been studied in the energy range 30 < E_e < 125 keV, with a conversion electron spectrometer installed at the Grenoble high-flux reactor. Precise values of the multipole mixing ratio M1/E2 have been obtained for transitions up to 100 keV. Furthermore, the spin and parity for the 215 keV level is verified. The states of ¹⁴⁷Nd are compared with the two other N = 87 isotones; the properties of these nuclei can be understood in the framework of the spherical shell model.     

Level structure of 42K from the 41(n, γ) and 41K(d,p) reactions

The γ-ray spectrum emitted after thermal neutron capture in ⁴¹K has been measured with pair and Ge(Li) spectrometers at the ILL high-flux reactor. About 630 transitions have been assigned to the decay of 133 excited states in ⁴²K. The level energies have been determined with a precison of 20 ppm; the neutron binding energy was determined to be E_B = 7533.82(15) keV. On the basis of the many transitions to known states, several spin-parity assignments have been made. In addition, high-resolution proton spectra of the reaction ⁴¹K(d,p) have been taken at 20MeV deuteron energy with the München Q3D spectrometer. These data have been essential in establishing the newly-found levels and in differentiating between primary and secondary transitions in the (n, γ) work. A statistical analysis of the level density and relative strengths of primary transitions is given.     

Thermal neutron capture in isotopes of nickel

The gamma-ray spectra associated with thermal neutron capture in targets of⁵⁸Ni,⁶⁰Ni,⁶²Ni, and⁶⁴Ni have been observed with a high-sensitivity pair-spectrometer. Level schemes for the four product nuclei are discussed, correlation of widths with neutron single-particle states examined, and estimates forM1 andE2γ-ray strength functions obtained.     

Gamma ray energies and 36Cl level scheme from the reaction 35Cl(n, γ)

The γ-ray spectrum emitted after thermal neutron capture in ³⁵Cl has been studied by use of the crystal and pair spectrometers installed at the ILL high flux reactor. We identified about 400 transitions in this reaction 326 of which were placed into the ³⁶C1 level scheme; several new states were found. The level energies up to 3.5 MeV were measured with a precision of 5–20 eV relative to the 412 keV ¹⁹⁸Au standard, those above 3.5 MeV with a precision of ¹⁰ppm. The neutron binding energy was determined to be E_B = 8579.68(9) keV.     

Angular distributions in quasi-fission reactions: Evidence for incomplete relaxation of the tilting mode

The integral β^?-spectra of²³⁵U and²³⁹Pu fission products have been measured with a plastic scintillator telescope at an external neutron guide tube at the high flux reactor of the ILL in Grenoble. The highly enriched targets (150 – 800 γg/cm²) were placed in a fission chamber at a distance of approximately 110 m from the reactor core. From the measured beta-spectra absolute counting rates per MeV and fission have been calculated, which are compared with the results of earlier experiments of other authors and with recent theoretical calculations.     

The level structure of 114Cd from (n, γ) and (d,p) studies

Gamma rays and conversion electrons have been measured following thermal neutron capture in ¹¹³Cd using the crystal spectrometers GAMS and the β-spectrometer BILL at the High Flux Reactor of the ILL at Grenoble. Primary γ-rays following thermal and average resonance neutron capture at E_n = 2 keV and 24 keV were recorded at the High Flux Beam Reactor at the Brookhaven National Laboratory. The ¹¹³Cd(d, p)¹¹⁴Cd reaction was studied with the Q3D spectrograph at the Munich tandem accelerator. Combining all these experimental results an almost complete level scheme of ¹¹⁴Cd was constructed up to 3.3 MeV including 48 excited levels with spin and parity information. The level scheme is discussed in terms of particle-hole excitations across the Z = 50 closed shell coupled to collective states, as well as in an interacting boson configuration mixing scheme.     

Voltage calibration of low-energy accelerators

The¹²C(p, γ)¹³N reaction has been used as a method to determine the absolute proton beam energy in the region ofE _p =150–350 keV with a precision of the order of 0.4 keV. The method makes use of the resulting captureγ-ray transition, whose intensity varies smoothly with beam energy and whose varying energy can be determined to high accuracy by comparison with precisely known energies ofγ-rays from radioactive sources. The energy calibration atE _p =80–150 keV has been carried out with the use of the nonresonant capture reaction D(p, γ)³He. The results have been applied to determine the absolute energies of proton-induced resonances on several light target nuclei.     

Energy levels,decay scheme, γ-ray branching ratios and lifetimes in 55Fe from the 55Mn(p,nγ)55Fe reaction

The reaction ⁵⁵Mn(p, nγ)⁵⁵Fe has been studied at E_p = 4.0 and 6.0 MeV using a pulsed beam. From the experiments at 6.0 MeV, the energy levels of ⁵⁵Fe up to an excitation of 3810 keV, their decay scheme and the γ-ray branching ratios have been determined. Levels have been identified for the first time in the (p, nγ) reaction. The results have been compared with those available from the literature. From the 4.0 MeV experiment, the mean lifetime of the 1408 keV level has been determined to be 142.7 ± 6.6 ps by direct timing techniques.     

Analysis of average primary gamma-transition intensities and cross sections of the113Cd(n, γ) reaction

A combined analysis of the available data on the primaryγ-ray intensities from the¹¹³Cd(n, γ) reaction atE _n=1.9 and 24.3 keV neutron energies together with the data on¹¹³Cd neutron capture cross sections in theE _n=3–200 keV energy region was carried out. The neutron strength functions were determined asS _n0=(0.260±0.073) 10^?4 and S_n1=(5.06±0.67) 10^?4. No spin-orbit splitting of thep-wave neutron strength function was found. The energy dependence of theE 1 radiative strength function {ie147-01} was fitted by the Kadmenski-Furman model somewhat better than by a standard Lorentzian. TheM 1 giant resonance parameters were obtained as E _G ^{M 1} =8.8±1.6 MeV and Γ _G ^{M 1} = 4.7±2.6 MeV. The neutron capture cross section of¹¹³Cd from its isomeric state ({ie147-02}=11/2^?, E ₁ ^m =263.7 keV) was calculated.     

The energy levels of79Br and81Br

The low-lying energy level and decay schemes of the stable bromine isotopes were studied by observing the γ-rays from the (n, n′γ) reactions in a natural bromine sample with the aid of a Ge (Li) detector. A pulsed neutron source and time-of-flight methods were used to reduce background due to neutron events in the detector. Most of the γ-rays observed could be assigned to transitions in either⁷⁹Br or⁸¹Br. In addition to those levels previously known from γ-decay or Coulomb excitation experiments, several new levels were excited in each isotope.     

Energy levels of80,82Br from (p,nγ) reactions

The levels of odd-odd^{80, 82}Br nuclei have been investigated via^{80, 82}Se(p, nγ)^{80, 82}Br reactions. Excitation functions and angular distributions were analysed with the Hauser-Feshbach compound nucleus theory. 27 and 29 levels have been identified. The transitions connecting the first 1⁺ and 2^?levels have been studied by the delayed coincidence method and their half-lives are 7.8±0.5 ns and 7.2±0.8 ns for⁸⁰Br and⁸²Br respectively. The experimental results are discussed in the framework of thej- j coupling.     

Untersuchungen zur Struktur des Kerns23Ne

Low-lying states of²³Ne up to about 3 MeV excitation energy have been investigated by studying the reactions²²Ne(d, p)²³Ne (E _d =4–6 MeV) and²³Na(n, p γ)²³Ne(E _n=8–9 MeV). From the (d, p) data,l-values and spectroscopic factors for the transferred neutron have been extracted by DWBA analyses. From the (n, p γ) data,γ-ray branchings and possible spin assignments have been derived. The results are used to discuss the applicability of the Nilsson model and the excited core model to the nucleus²³Ne.     

Triple differential cross section for angle,atomic number and energy (or angular momentum transfer) calculated for the 280MeV40Ar+58Ni (or 365MeV63Cu+197Au) system in a simple model

Highly excited levels of³³S populated by α-particle capture in²⁹Si have been investigated forE _α=1.962 MeV to 4.287 MeV. Excitation curves measured with Ge(Li) and BF₃ detectors are reported. More than fifty resonances can be identified with levels in³³S. (α, γ) angular distributions measured on five strong resonances have yieldedJ ^π values 1/2+, 3/2 +, 5/2?, 5/2?, 5/2? and 3/2+ respectively, for theE _x =10.054, 10.466, 10.523, 10.721, 10.758 and 10.776 MeV levels in³³S. Elastic scattering experiments have been performed and theJ ^π assignments are found to be consistent with thel-values inferred from the elastic scattering data. Decay schemes from the above³³S levels have been proposed. A new level at 9.245 MeV is also suggested and theJ ^π values for the 4.425 and 2.87 MeV states are shown to be consistent with 7/2+ and 3/2+ assignment, respectively. Nuclear Reactions²⁹Si(α, γ) and²⁹Si(α, α),E _α=1.962-4.287 MeV. Measured relative σ(E). DeducedJ ^π andE _γ of³³S levels. New³³S level atE _x =9.245 MeV. Enriched targets.     

Spectroscopy of excited states in212Po,210Pb,and213At employing18O induced few-nucleon transfer reactions

γ-ray spectroscopic techniques have been applied to measure properties of excited states (E ^*<2MeV) in²¹⁰Pb,²¹²Po, and²¹³At after populating these neutron rich (N=128) nuclei via¹⁸O induced few-nucleon transfer reactions on²⁰⁸Pb and²⁰⁹Bi targets. In²¹²Po an isomeric state is located atE ^*=1,477 keV with a halflife oft _1/2=14.7±0.3 ns. This state is interpreted to be the 8⁺ yrast level which decays to the ground state via the measured $$8^ + \left( {121.1 keV} \right)6^ + \left( {223.3 keV} \right)4^ + \left( {405.1 keV} \right)2^ + \left( {727.8 keV} \right)0^ + $$ γ-cascade.α-decay (E _α≈10.2 MeV) of the isomer is also observed. In²¹⁰Pb the time spectra for members of the 4⁺ (297.8keV) 2⁺ (799.4keV)0⁺ γ-cascade show a delayed component with a halflife oft _1/2=152±13 ns which is attributed to the known 8⁺ yrast state atE ^*=1.27 MeV. For²¹³At first results on theγ-decay of excited states are presented.     

Levels in154Eu populated by thermal neutron capture

The level scheme of¹⁵⁴Eu has been investigated by means of thermal neutron captureγ-rays and conversion electrons. The high energyγ-ray spectrum from thermal neutron capture in enriched¹⁵³Eu has been studied in the energy range of 5700 to 6500 keV. Low energyγ radiation has been observed with Ge(Li) and Si(Li) detectors from 5 to 300 keV and conversion electrons have been measured from 15 to 300 keV. Low energy (n, γγ) coincidences and half lives of transitions have been measured. The data, combined with three very recent studies of the 8^? isomer decay in¹⁵⁴Eu has led to the construction of a level scheme with 12 excited levels. Nuclear Reaction¹⁵³Eu(n, γ),E _n =thermal, measuredE _γ ,I _γ ,E _ce ,I _ce ,γγ-coincidence, halflives,¹⁵⁴Eu deduced levels.     

New aspects of the rotational model in25Mg

Spin assignments have been made to the²⁵Mg levels in theE _x=5–6 MeV region fromγ-ray angular distributions measured in the²²Ne(α, n y) reaction atE _α=8.0 and 8.8 MeV and fromp-γ angular correlations measured in the²⁴Mg(d, p γ) reaction atE _d=6 MeV. Unique spin assignments ofJ=7/2, 5/2, 5/2, and 9/2 could be made to the levels atE _x=5005, 5511, 5851, and 5967 keV, respectively. Ambigious assignments have been made to the levels atE _x=5245, 5524, 5785, 6032 keV (J=11/2, 7/2), 5455 keVJ=13/2, 9/2), and 5738 keV (J=3/2, 5/2). The present data confirm previous assignments ofJ=1/2 to the levels atE _x=5108 and 5466 keV, respectively. Lifetime estimates have been obtained, using the Doppler-shift attenuation method, for the levels atE _x=5245 keV (τ=30–60 fs), 5785 keV (τ=50–100 fs), 5967 keV (τ=50–100 fs), and 5455 keV (τ>1ps). All other levels in theE _x=5–6 MeV region haveτ<60 fs. A breakdown of theK-selection rule has been observed in theγ-decay of some high spin states, indicating a deviation from the strong coupling model.     

Circular polarization and γ-γ angular correlation measurements in the 39K(n, γ)40K reaction

Circular polarization measurements of the γ-radiation from polarized neutron capture combined with γ-γ angular correlation measurements in the ³⁹K(n,γ)⁴⁰K reaction lead to J^π = 2^? assignments to the E_x = 0.80, 2.05 and 2.42 MeV states of ⁴⁰K, and to spin restrictions for the states at E_x = 2.10, 3.44 and 4.25 MeV. Multipole mixing ratios for the γ-rays which de-excite these levels have been determined.     

Radiative thermal neutron capture by natural sulfur

A high precision study of the gamma ray spectrum following neutron capture by a target of natural sulfur is reported. The energy precision obtained has permitted construction of decay schemes for³³S and³⁵S. In the case of the former isotope a total of 22 levels have been identified while for the latter and much weaker reaction 7 states have been observed. While some transitions attributable to capture by³³S are observed, their weakness prohibited detailed analysis. The neutron separation energies, based upon the¹⁴N(n, γ)¹⁵N standard are found to be 8,641.60 (3) keV and 6,985.84 (5) keV for³³S and³⁵S respectively.