Excitation of K X-Rays by bombardment of thick solid targets with 150 MeV Xe ions

The yield of K X-radiation arising from the interaction of ¹³⁶₅₄Xe ions with ₄₁Nb, ₄₂Mo, ₄₅Rh, ₄₆Pd, ₄₇Ag, ₄₈Cd, ₄₉In, ₅₀Sn, ₅₇La, ₆₄Gd, ₆₅Tb, ₇₀Yb, ₇₁Lu, ₇₃Ta, ₇₇Ir, ₇₈Pt, ₇₉Au and ₈₃Bi targets was measured using Si(Li) and Ge(Li) detectors. The dependence of the yield on the atomic number of the target material is discussed on the basis of the molecular orbital model.     

Production of neutrons in thick targets by high-energy protons and nuclei

This article is dedicated to the physics of spallation neutron production by high-energy particles and applications thereof. This field of research is related to the rapidly developing branch of nuclear physics that is high-energy neutron physics. The central part of this article is a review of experimental results obtained in different laboratories of the world during the last more than a quarter of a century. Analysis of the characteristics of multiple neutron production in targets induced by protons and nuclei with energies higher than several hundreds of mega-electronvolts per nucleon is performed. The results of measurements that were carried out at the Joint Institute for Nuclear Research with beams of protons, deuterons, and light nuclei are discussed. Natural and artificial sources of spallation neutrons and their role in up-to-date studies are considered.     

(Ti,Al,Si,C)N nanocomposite coatings synthesized by plasma-enhanced magnetron sputtering

Materials’ surface service property could be enhanced by transition metal nitride hard coatings due to their high hardness, wear and high temperature oxidation resistance, but the higher friction coefficient (0.4-0.9) of which aroused terrible abrasion. In this work, quinternary (Ti,Al,Si,C)N hard coating 3-4 μm was synthesized at 300 °C using plasma enhanced magnetron sputtering system. It was found that the coating's columnar crystals structure was restrained obviously with the increase of C content and a non-columnar crystals growth mode was indicated at the C content of 33.5 at.%. Both the XRD and TEM showed that the (Ti,Al,Si,C)N hard coatings had unique nanocomposite structures composed of nanocrystalline and amorphous nc-(Ti,Al)(C,N)/nc-AlN/a-Si₃N₄/a-Si/a-C. However, the coatings were still super hard with the highest hardness of 41 GPa in spite of the carbon incorporation. That a-C could facilitate the graphitization process during the friction process which could improve the coating's tribological performance. Therefore, that nanocomposite (Ti,Al,Si,C)N coatings with higher hardness (>36 GPa) and a lower friction coefficient (<0.2) could be synthesized and enhance the tribological performance and surface properties profoundly.     

Quasimolecular K X-ray excitation by bombardment of Ge atoms with Ge ions

By bombardment of Ge targets with ⁷⁴₃₂Ge⁵⁺ of 81 MeV, a continuous X-ray intensity distribution has been obtained, which ranges up to the K X-ray energies of ₆₄Gd. The shape of the spectra, corrected for the detector efficiency, confirms the assumption that this continuum is caused by K X-rays of Z = 64 quasimolecules, which are transiently formed during the adiabatic heavy-ion collision. The yield of quasimolecular radiation was determined to be about 4 x 10⁻⁵ X-rays per beam K-vacancy.     

Soft X-ray amplification by Li-like Al10+ and Si11+ ions in recombining plasmas

Experimental studies of soft X-ray lasers were carried out on the six-beam laser facility and the LF 12 laser facility of SIOM. Using a home-made one-dimensional spatially resolved grazing incidence grating spectrograph, XUV amplification has been observed in Li-like aluminum and silicon ions, by irradiation of slab targets with a line-focused laser. Based on time-integrated measurement, gain coefficients are 3.1 cm^–1 for the 105.7 Å 5f–3d transition in Li-like Al ions, and 1.5 cm^–1 and 1.4 cm^–1 for the 88.9 Å 5f–3d and the 87.3 Å 5d–3p transitions in Li-like Si ions, respectively. The maximum gain × length products (GL) are about 2.5.     

Energy and angular distributions of backscattered electrons from collisions of 5 keV electrons with thick Al,Ti, Ag,W and Pt targets

The energy and angular distributions of backscattered electrons produced under the impact of 5 keV electrons with thick Al, Ti, Ag, W and Pt targets are measured. The energy range of backscattered electrons is considered between E _B = 50 eV and 5000 eV. The angle of incidence α and take-off angle θ are chosen to have values α = 0 and 10 and θ = 100, 110 and 120 respectively. The measured energy spectra are compared with the available theoretical models for α = 0 and 10. The elastic peak intensity of backscattered electrons is found to be a function of angle of incidence, take-off angle and atomic number of the target material. The considered theories are reasonably in good agreement with experiment for the energy spectra of the backscattered electrons having their reduced energies ∈ (= E _B/E ₀) in the range of 0.20 to 1.00.      

Secondary ion emission under the bombardment of Si by multiply charged Si q+ ions

The spectra of secondary ion emission under the bombardment of a B-doped Si target by multiply charged Si ^q+ ions (q = 1?C5) have been studied in the energy range of 1 to 10 keV per unit of charge. A multifold increase in the yield of secondary cluster Sk _n ⁺ ions, multiply charged Si ^q/+ ion (q = 1?C3), and H⁺, C⁺, B⁺, Si₂N⁺, Si₂O⁺ is observed as the charge of the multiply charged ions increases. The increase in the yield of secondary ions with increasing charge of the multiply charged-ion charge is most significant for ions with relatively high ionization potentials.     

The Kα and Kβ X-ray spectra of Al,Ti, Cr,Fe and Ni induced by 84 MeV nitrogen ions

The K X-rays from the target elements due to N-ion bombardment are measured with a crystal spectrometer. Some aspects owing to high incident energy are discussed. The Kα satellite, Kα hypersatellite and Kβ satellite peak spacings are obtained.     

Secondary fusion reactions in the bombardment of light-element targets with low-energy heavy ions

Neutron emission was observed experimentally at the DC-60 cyclotron at the Institute of Nuclear Physics (Astana, Kazakhstan). The neutron yields were measured in the bombardment of light-element (Be, C, Al, Al₂O₃, and LiF) targets with heavy ions (Ar, Kr, and Xe) with energies below the Coulomb barrier. The angular distributions of neutrons from the targets were also measured. It was found that the observed neutrons were produced in secondary nuclear reactions between the resting target nuclei and recoil nuclei that acquire energy in the process of elastic scattering. The experimental results were compared with calculations based on the abovementioned secondary-reaction mechanism. The calculations allow one to estimate the yields of secondary reactions to within a coefficient of 2.     

Characteristic and non-characteristic X-ray yields produced from thick Ti element by sub-relativistic electrons

Measurements are performed to study the electron impact energy dependence of doubly differential bremsstrahlung yields (DDBY) and of characteristic Ti K_α line yields produced from sub-relativistic electrons (10–25 keV) colliding with a thick Ti (Z = 22) target. The emitted radiation is detected by a Si-PIN photo-diode detector with energy resolution (FWHM) of 180 eV at 5.9 keV. The measured data of DDBY are compared with the results predicted by Monte-Carlo (MC) simulations using the general purpose PENELOPE code. A reasonable agreement is found between experimental and simulation results within the experimental uncertainty of measurements of 12%. Characteristic Ti K_α yields are obtained for the considered impact energy range and they are compared with the existing theoretical results. A good agreement is found between the present measurements and the theoretical calculations. Furthermore, data are presented for impact energy dependence of the ratio K_α/(K_α+ K_β) of a thick Ti target under impact of 10–25 keV electrons. The ratio shows a very weak dependence on impact energy in the studied range. The average value of the ratio is found to be 0.881 ± 0.003.     

Neutron yields upon irradiation of thick targets by ions with energies below 1.75 MeV/Nucleon

The yields of neutrons produced in thick LiF, Be, C, Al, Al₂O₃, and Cu targets irradiated by Li, C, and N ions with energies below 1.75 MeV/nucleon are measured on the DC-60 cyclotron at the Institute of Nuclear Physics, Astana Branch, Kazakhstan. The experimental angular distributions of the neutron yields from the targets are measured and an empirical equation to describe the distributions is proposed. The measured neutron yields are compared with the figures calculated by the LISE++ program. The measured and predicted neutron yields in the reactions coincide to within a factor of 2.     

高电荷态离子Arq+与不同金属靶作用产生的X射线

研究了高电荷态离子Arq+(q=16,17,18)入射金属Be,Al,Ni,Mo,Au靶表面产生的X射线谱.实验结果表明,Ar的Kα-X射线是离子在与固体表面相互作用过程中固体表面之下形成空心原子发射的.电子组态1s2的高电荷态Ar16+离子在金属表面中性化过程中,存在的多电子激发过程使Ar16+的K壳层电子激发产生空穴,级联退激发射Ar的Kα特征X射线.Ar17+离子在金属表面作用过程中产生的X射线谱形与靶材料没有明显的关联,入射离子的Kα-X射线产额与其最初的电子组态有关,靶原子的X射线产额与入射离子的动能有关.     

Microstructures and characteristics of Ti/Al interface with segregated Si element

We present a systematic first principles study for evaluating the potential impact of Si on adhesion of α-Ti (0 0 2)/Al (1 1 1) interface at the atomic level. The results show that Si atom tends to segregate to the interface by following the replacement rather than the interstitial path. The favorite replacement site is observed in Ti layer. Segregated Si contributes to form the covalent bonding between Si and other Al and Ti atoms, and enhances the strength of the whole interface area. This is in accordance with the experimental outcomes.     

Emission of alpha particles in the interaction of 10–85 MeV protons with48,50Ti

The excitation functions of twenty nuclear reactions induced by protons of up to 85 MeV incident upon⁴⁸Ti and⁵⁰Ti targets have been measured. Most of these involve the emission of one to three alpha particles. The Exciton model has been used to calculate these excitation functions. An expanded and more precise treatment of nucleon-alpha scattering has been incorporated into the model. It is presented and the implications of its predictions discussed. The agreement of experiment and calculation is very good lending support to the approach to alpha particle interactions introduced in this work.     

CalciumK X-ray spectra produced by oxygen,alpha-particle,and proton bombardment

Kα andKβ X-rays of calcium were produced by bombarding a thick calcium wafer with oxygen, helium and hydrogen ions. These reactions produce a substantial amount of inner shell ionization. TheK X-ray spectra contain X-ray lines from calcium which emanate from initial states with a varying degree ofK orL shell vacancies. The initial configurations were assigned on the basis of Hartree-Fock-Slater calculated energies. Related intensity ratio of1s→2p (Kα) transitions and of1s→3p (Kβ) transitions of H plus Ca, He plus Ca and O plus Ca were obtained. In addition to observing many new transitions due to multipleK and/or multipleL shell vacancies, energy shifts relative to the H plus Ca spectrum were observed in the O plus Ca spectrum due toM shell vacancies.     

Measurements of neutron yields and spatial distributions in U/Pb, Pb and Hg thick targets bombarded by 0.5 and 1.0 GeV protons

Measurements have been carried out on neutron yields and spatial distributions in U/Pb, Pb and Hg thick targets and the surrounding paraffin moderators bombarded by 0.533 and 1.0 GeV protons. CR-39 detectors were deployed on the surfaces of targets and moderators to record the neutrons produced in the targets. The measurements show that:

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磁控溅射(Ti,N)/Al纳米复合薄膜的微结构和力学性能

采用Al和TiN靶通过磁控共溅射方法, 制备了一系列Ti:N≈1的不同(Ti, N) 含量的铝基纳米复合薄膜, 利用X射线能量分散谱仪、X射线衍射仪、透射电子显微镜和纳米力学探针表征了薄膜的成分、 微结构和力学性能, 研究了(Ti, N)含量对复合薄膜微结构和力学性能的影响. 结果表明: Ti, N原子的共同加入使复合薄膜形成了同时具有置换固溶和间隙固溶特征的"双超过饱和固溶体", 薄膜的晶粒随着溶质含量的增加逐步纳米化, 并进一步形成非晶结构, 晶界区域形成溶质原子的富集区. 相应地, 复合薄膜的硬度在含1.8 at.%(Ti, N) 时就可迅速提高到3.9 GPa; 随着TiN含量的增加, 薄膜的硬度进一步提高到含17.1 at.%(Ti, N)时的8.8 GPa. 以上结果显示出Ti和N"双超过饱和固溶"对Al薄膜极其显著的强化效果.     

Dissociation of 14N2+ ions induced by slow electrons

The cross sections and thermal rate coefficients for the dissociative recombination (DR) of the molecular nitrogen ions initially in the first four vibrational levels of the ground electronic state have been computed in the framework of the multichannel quantum defect theory. An energy range of 0.001–1 eV has been considered. The contribution of the indirect DR mechanism involving Rydberg states associated with the first excited ion core has also been investigated.     

Recoil properties of spallation products from bombardment of Z = 13–29 targets with 150,300 and 600 MeV protons

A semi-empirical relation developed using the classical model of high-energy nuclear reactions has been applied to spallation data obtained from thick-target — thick-collector recoil experiments. The ²⁴Na, ⁴²K, ⁴³K, ^44mSc, ⁴⁶Sc, ⁴⁷Sc ranges produced in Al, Sc, Ti, V, Fe, Co, Cu targets by 150, 300 and 600 MeV protons were determined. The excitation energies of the residual nuclei, deduced from the ranges, have been compared with theoretical calculations. The analysis shows that if the mass difference of the target and product nucleus is ΔA ? 10 the cascade plays a privileged role. If ΔA>10 an averaging effect is observed. In this case the number of prompt nucleons is about one-third of the total number and the excitation energy per evaporated nucleon is about 11 MeV.