弱非线性复合体中的高阶非线性响应

利用谱表示理论和微扰展开法，从理论上给出了适合于一般微结构复合体系的有效非线性响 应的一般表示式，并结合有效媒质近似（EMA），在弱非线性条件下研究了由三阶非线性组 分（体积分数为p）和线性组分构成的非线性复合体系的有效非线性响应，讨论了复合 体系的有效介电常数ε～e=εe+χe|E0|2+ηe|E0| 4中的有效三次非线性响应χe和有效高次非线性响应ηe与体积分数p和 退极化因子L之间的关系，分析了非线性组分的介电常数为复数情形时体系的有效高阶非线 性响应，从理论上说明了组分的高次非线性响应对整个复合体系的有效介电常数的影响.  关键词： 非线性复合介质 有效非线性响应 谱表示理论     

Production of high-energy particles in laser and Coulomb fields and the e+e- antenna

A strong laser field and the Coulomb field of a nucleus can produce e(+) e(-) pairs. It is shown for the first time that there is a large probability that electrons and positrons created in this process collide after one or several oscillations of the laser field. These collisions can take place at high energy, resulting in several phenomena. The quasielastic collision e(+) e(-) --> e(+) e(-) allows acceleration of leptons in the laser field to higher energies. The inelastic collisions allow production of high-energy photons e(+) e(-) --> 2 gamma and muons e(+) e(-) --> micro(+) micro(-). The yield of high-energy photons and muons produced via this mechanism exceeds exponentially their production through conventional direct creation in laser and Coulomb fields. A relation of the phenomena considered with the antenna mechanism of multiphoton absorption in atoms is discussed.     

Investigations on analytic potential energy function,spectroscopic parameters and vibrational manifolds （d = 0） of the SD^＋（X^3∑^-） ion

This paper investigates the spectroscopic properties of the SD + (X 3 Σ ) ion by employing the coupled-cluster singles-doubles-approximate-triples [CCSD(T)] theory combining with the quintuple correlation-consistent basis set augmented with diffuse functions (aug-cc-pV5Z) of Dunning and co-workers. The accurate adiabatic potential energy function is obtained by the least-squares fitting method with the 100 ab initio points, which are calculated at the unrestricted CCSD(T)/aug-cc-pV5Z level of theory over the internuclear separation range from 0.09 to 2.46 nm. Using the potential, it accurately determines the spectroscopic parameters (D e , ω e χ e , α e and B e ). The present D e , R e , ω e , ω e χ e , α e and B e results are of 3.69119 eV, 0.13644 nm, 1834.949 cm 1 , 25.6208 cm 1 , 0.1068 cm 1 and 4.7778 cm 1 , respectively, which are in remarkably good agreement with the experimental findings. A total of 29 vibrational states has been predicted by numerically solving the radial Schro¨dinger equation of nuclear motion when the rotational quantum number J equals zero. The complete vibrational levels, classical turning points, inertial rotation and centrifugal distortion constants are reported when J = 0 for the first time, which are in good accord with the measurements wherever available.     

Computation of the electric and magnetic fields induced in a plasmacreated by ionization lasting a finite interval of time

S.C. Wilks et al. (1988) showed that when an infinite expanse of gas, carrying a linearly polarized electromagnetic wave, is instantly ionized, the initial wave is frequency upshifted. This phenomenon of frequency upconversion through flash ionization gives rise to steady-state transmitted and reflected electromagnetic waves and to a time-independent magnetic field. The case in which the final state of ionization is achieved not instantly but in a finite turn-on time, 0⩽t⩽t 0, which is followed by the steady state, is studied. It is shown that the electric field is obtained from the one-dimensional Helmholtz equation, d²F(t)/dt² +ω₀²g(t)F( t)=0, if electrons are born at rest when they are created during ionization. As a result, the instantaneous frequency of the upshifted radiation is ω(t)=√g(t). The electric field can be solved exactly for specific choices of g(t). It is solved using WKB approximations for arbitrary g(t). The magnetic field is then found by integrating Faraday's law. It is found that the steady-state electric field amplitude depends on the steady-state value o f g(t) but does not depend on the ionization time t₀. Conversely, the static magnetic field amplitude decreases with increasing turn-on time     

自旋极化电子原子散射的(e,eγ)符合实验研究

本文介绍了自旋极化电子原子散射的(e,eγ)符合实验的理论基础、实验装置和参数测量方法,描述了符合实验研究主要结果,说明了符合实验研究的物理意义。     

Charge-exchange processes in the quasi-elastic (e,e′p) and (e,e′n) reactions

Calculations of charge-exchange processes in the final state of the quasi-elastic (e, e′N) reaction have been performed employing the Lane formalism. The Lane equations were decoupled by means of a transformation to the isospin representation. It is found that charge exchange has a small effect on the (e, e′p) cross section, but may play an appreciable role in the (e, e′n) reaction.     

6Li(e,e′α) and (e,e′d) reactions

The correlation cross sections for the quasifree scattering in the ⁶Li(e,e′α) and (e,e′d) reactions are calculated in the microscopic model. The internal momentum distributions of clustering particles play an important role for explaining experimental data.     

Field ionization of strongly magnetized rydberg positronium: A new physical mechanism for positron accumulation

Magnetized Rydberg positronium forms when an energetic positron ( e(+)) slows within a tungsten crystal and picks up an electron ( e(-)) as it emerges in a strong magnetic field. The signature is equal numbers of e(+) and e(-) when a weak electric field is applied, either of which can be accumulated and counted. The new e(+) accumulation technique is simple, robust, and much more efficient than any other demonstrated to be compatible with a cryogenic vacuum. Possible applications include the study of cold single component plasmas of e(+) and the formation of cold antihydrogen.     

Electroless deposition of Ag on Pd-activated TiN/p-Si(100) substrate

Nano-thick Ag films were electrolessly deposited on TiN/p-Si(100) substrates. The substrates were prepared by sputtering TiN on p-Si(100) wafers. An activation process of the substrates was performed by immersing the substrates in a solution of 0.0019 moLL^-1PdCl₂+0.45 moLL^-1HF+8.7 moLL^-1aceticacid+0.036 moLL^-1 HCl so as to obtain the Pd seed layer. The general composition of the electroless Ag bath was 0.0032 moLL^-1AgNO₃+2.24 moLL^-1NH₃+0.56 moLL^-1aceticacid+0.1 moLL^-1 NH₂NH₂ at pH 10.2. The morphologies of the Pd seed layer and the Ag films were characterized by atomic force microscopy (AFM). The effect of the Pd activation on electroless Ag deposition was tested by open circuit potential with time technology (OCP-t). For comparison, the morphology of the films deposited by electrochemical deposition on the substrates was also studied by AFM. PACS 82.45.Mp; 81.15.Pq; 81.10.Dn     

Search for flavor-changing neutral current and Lepton-flavor violating decays of D0-->l+l-

We report on a search for the flavor-changing neutral current decays D0-->e(+)e(-) and D0-->mu(+)mu(-), and the lepton-flavor violating decay D0-->e(+/-)mu(-/+). The measurement is based on 122 fb(-1) of data collected by the BABAR detector at the SLAC PEP-II asymmetric e(+)e(-) collider. No evidence is found for any of the decays. The upper limits on the branching fractions, at the 90% confidence level, are 1.2x10(-6) for D0-->e(+)e(-), 1.3x10(-6) for D0-->mu(+)mu(-), and 8.1x10(-7) for D0-->e(+/-)mu(-/+).     

On the relations between Markovian master equations and stochastic differential equations

We have investigated the relationship between Markovian master equations (m.e.) and the corresponding stochastic differential equations (s.d.e.) for closed systems, i.e., systems not subjected to external pumping. We show that the form of the fluctuations in the s.d.e., i.e., additive or multiplicative, depends upon the properties of the kernel of the m.e. and the range of the state space of the stochastic variable(s), i.e., bounded or unbounded. The knowledge of these two properties of the m.e. permits the determination of the way in which the fluctuations enter into the s.d.e. (i.e., additive or multiplicative) and the calculation of their statistics. Several examples are presented to illustrate the general theory.     

On the valence shell binding energy spectrum of carbonyl sulphide

The valence shell binding energy spectrum of carbonyl sulphide (10–45 eV) has been measured using both binary (e,2e) and dipole (e,2e) electron impact spectroscopy and calculated by the 2ph-TDA many body Green's function technique. The spectrum shows extensive structure above 20 eV, indicating a major breakdown of the quasi-particle picture for ionization of COS. The calculation is in good agreement with the present experimental and literature ESCA binding energy spectra. Binary (e,2e) spectra at two azimuthal angles support the theoretical prediction that this extensive final ion state structure arises primarily from ionization of the COS 6σ and 7σ inner valence electrons.     

Monte Carlo simulation of electron swarms in nitrogen in uniformE×B fields

The motion of electrons in nitrogen in uniform E× B fields is simulated using the Monte Carlo technique for 240⩽E/N⩽600 Td (1 Td=1×10^-17 V cm²) and 0⩽B/N⩽0.45×10^-17 T cm³ . The electron-molecule collision cross sections adopted are the same cross sections as those used previously for the numerical solution of the Boltzmann equation. The swarm parameters obtained from the Monte Carlo simulation are compared with the Boltzmann solution and with the experimental data available in the literature. In relation to E×B fields, it is concluded that the Monte Carlo approach provides an independent method of substantiating the validity of the equivalent electric-field approach     

在HT-7托卡马克上密度扫描实验中的边界湍流和输运

在HT-7托卡马克上密度扫描实验中使用一个快速扫描气动朗缪尔探针来研究边界湍流和输运。随着中心弦平均等离子体密度的增加，在等离子体边界观察到径向电场剪切增强，径向电场的增强能够解释边界输运的减小和全局粒子约束的改善。粒子约束时间的增加和垂直扩散系数的减小证明粒子输运降低了。在等离子体边界区域发现电离和辐射驱动湍流的特征，表明电离和辐射在湍流驱动过程中具有重要性。     

散射粒子的相互作用对He(e,3e)五重微分截面的贡献

计算了敲出电子等能分享几何安排下,入射能量分别为5 599 eV和1 099 eV时He(e,3e)反应五重微分截面,并比较在He(e,3e)过程中散射粒子的相互作用和它们之间的干涉效应对五重微分截面的贡献.结果表明,理论计算数据在误差范围内与实验数据基本吻合,并且散射粒子的相互作用以及干涉效应对五重微分截面的影响都是不容忽视的.     

Kinetic studies of the reaction of phenacyl bromide derivatives with sulfur nucleophiles

The reaction of the substituted phenacyl bromides 1a–e and 2a–e with thioglycolic acid 3 and thiophenol 6 in methanol underwent nucleophilic substitution S_N2 mechanism to give the corresponding 2‐sulfanylacetic acid derivatives 4a–e, 5a–e and benzenethiol derivatives 9a–e, 10a–e. The reactants and products were identified by mass spectra, infrared and nuclear magnetic resonance. We measured the kinetics of these reactions conductometrically in methanol at a range of temperatures. The rates of the reactions were found to fit the Hammett equation and correlated with σ‐Hammett values. The ρ values for thioglycolic acid were 1.22–1.21 in the case of 4‐substituted phenacyl bromide 1a–e, while in the case of the nitro derivatives 2a–e they were 0.39–0.35. The ρ values for thiophenol were 0.97–0.83 in the case of 4‐substituted phenacyl bromide 1a–e, while in the case of the nitro derivatives 2a–e they were 0.79–0.74. The Brønsted‐type plot was linear with a α = ?0.41 ± 0.03. The kinetic data and structure‐reactivity relationships indicate that the reaction of 1a–e and 2a–e with thiol nucleophiles proceeds by a concerted mechanism. The plot of log k₄₅ versus log k₃₀, the plot log(k_x,3‐NO2/k_H) versus log(k_x/k_H), and the Brønsted‐type correlation indicate that the reactions of the thiol nucleophiles with the substituted phenacyl bromides 1a–e and 2a–e are attributed to the electronic nature of the substituents. Copyright © 2011 John Wiley & Sons, Ltd.     

Relativistic harmonic content of nonlinear electromagnetic waves inunderdense plasmas

The relativistic harmonic content of large-amplitude electromagnetic waves propagating in underdense plasmas is investigated. The steady-state harmonic content of nonlinear linearly polarized waves is calculated for both the very underdense (w_p/w ₀)≪1 and critical density (w_p/w₀)≃1 limits. For weak nonlinearities, eE₀/mcω₀<1, the nonlinear source term for the third harmonic is derived for arbitrary w_p/w₀. Arguments are given for extending these results for arbitrary wave amplitudes. It is also shown that the use of the variable x-ct and the quasi-static approximation leads to errors in both magnitude and sign when calculating the third harmonic. In the absence of damping or density gradients the third harmonic's amplitude is found to oscillate between zero and twice the steady-state value. Preliminary PIC simulation results are presented. The simulation results are in basic agreement with the uniform plasma predictions for the third-harmonic amplitude. However, the higher harmonics are orders of magnitude larger than expected and the presence of density ramps significantly modifies the results     

Improved limits on nu(e) emission from mu+ decay

We investigated mu(+) decays at rest produced at the ISIS beam stop target. Lepton flavor (LF) conservation has been tested by searching for nu(e) via the detection reaction p(nu(e),e(+))n. No nu(e) signal from LF violating mu(+) decays was identified. We extract upper limits of the branching ratio (BR) for the LF violating decay mu(+)-->e(+)+nu(e)+nu(-) compared to the standard model (SM) mu(+)-->e(+)+nu(e)+nu(mu) decay: BR<0.9(1.7) x 10(-3) (90% C.L.) depending on the spectral distribution of nu(e) characterized by the Michel parameter rho=0.75(0.0). These results improve earlier limits by one order of magnitude and restrict extensions of the SM in which nu(e) emission from mu(+) decay is allowed with considerable strength. The decay mu(+)-->e(+)+nu(e)+nu(mu) often proposed as a potential source for the nu(e) signal observed in the LSND experiment can be excluded.     

Direct measurement of the phi(1020) leptonic branching ratio

The process e(+)e(-)-->mu(+)mu(-) has been studied by the SND detector at the VEPP-2M e(+)e(-) collider in the phi(1020)-resonance energy region. The measured effective phi meson leptonic branching ratio B(phi-->l(+)l(-)) identical with square root of B(phi-->e(+)e(-))B(phi-->mu(+)mu(-))] = (2.89 +/- 0.10 +/- 0.06) x 10(-4) agrees well with the Particle Data Group value B(phi-->e(+)e(-)) = (2.91 +/- 0.07) x 10(-4), confirming mu-e universality. Without additional assumption of mu-e universality the branching ratio B(phi-->mu(+)mu(-)) = (2.87 +/- 0.20 +/- 0.14) x 10(-4) was obtained.