Change of optimum conditions of second harmonic generation of spatial limited laser beams in nonlinear crystals

Frequency doubling of spatially limited laser beams in nonlinear crystals is investigated theoretically. It was shown that the major factor, which reduces the second harmonic generation (SHG) efficiency in this case, is a diaphragm aperture effect, caused by influence of extraordinary polarized laser beams. In that case a spatial shift of mutually orthogonally polarized beams of the incident waves relative to each other in perpendicular direction of wave transmission at the entry to crystals lead to increase the efficiency of SHG of limited beams.     

飞秒激光在晶体中传输的级联非线性过程

系统地回顾了有关级联过程导致的各种非线性效应的工作,指出了级联效应可导致不同光谱成分间出现能量转移现象,且二阶级联过程中产生的白光还能够提供种子光进而得到基于参量放大过程的宽带锥形辐射。在此基础上,进一步研究了入射的基频波长对于超连续白光能量转移效果及产生倍频效率的影响以及二阶级联过程引起的偏振调制现象,指出当入射波长越靠近相位匹配波长时倍频效率越高,发现二阶级联效应还可以引起显著的基频光偏振调制。     

Blue laser light generation by intracavity frequency doubling of Cesium vapor laser

Blue laser light with a wavelength 447 nm was generated by intracavity frequency doubling of a Cs laser in PPKTP crystal. A continuous wave power of 600 mW was obtained at an optical-to-optical efficiency of 4%. In the pulsed operation, when thermal effects were reduced, the efficiency obtained was 14% and the peak blue power was 2.1 W.     

Quasi phase matching in two-dimensional nonlinear photonic crystals

We analyze quasi-phase-matched (QPM) conversion efficiency of the five possible types of periodic two-dimensional nonlinear structures: Hexagonal, square, rectangular, centered-rectangular, and oblique. The frequency conversion efficiency, as a function of the two-dimensional quasi-phase-matching order, is determined for the general case. Furthermore, it is demonstrated for two basic feasible motifs, a circular motif and a rectangular motif. This enables to determine the optimal motif dimensions for achieving the highest conversion efficiency. We find that a rectangular motif is more efficient than a circular motif for quasi-phase-matched processes that rely on a single reciprocal lattice vector (RLV), and that under optimal choice of motif dimensions, it converges into a one-dimensional periodic structure. In addition, in a few specific cases we found that higher order QPM can be significantly more efficient than lower order QPM.     

Second-harmonic generation by elliptic Bessel light beams in periodically polarized nonlinear crystals

The features of the frequency doubling of elliptic Bessel light beams under quasi-synchronous interaction in periodically polarized nonlinear crystals have been investigated. The overlap integrals describing the efficiency of second-harmonic generation by elliptic Bessel light beams have been investigated numerically. Reported at the Vth International Scientific-Technical Conference on Quantum Electronics, November 22–25, 2004, Minsk, Belarus. __________ Translated from Zhurnal Prikladnoi Spektroskopii, Vol. 72, No. 6, pp. 752–755, November–December, 2005.     

飞秒激光非线性频率转换的自适应优化过程

使用闭环控制的自适应控制光学系统对飞秒激光的波前进行调控,可以有效改善激光与物质相互作用中由于相位畸变或光路偏差导致的效率下降。利用可编程纯相位的液晶空间光调制器结合模拟退火算法设计的自适应优化系统,在BBO晶体的飞秒倍频过程中实现了对相位畸变和光路偏差导致倍频效率下降的自动补偿,从而实现飞秒倍频效率的最优化。     

Efficient collinear frequency tripling of femtosecond laser with compensation of group velocity delay

This paper demonstrates an approach that negative uniaxial crystal has a relative anomalous dispersion effect which can compensate group velocity delay, and applies this approach to nonlinear frequency conversion of an ultrafast laser field. High efficiency of the third harmonic generation is experimentally fulfilled by adopting a collinear configuration of doubing-compensation-tripling system. Through finely adjusting the incident angle and optical axis direction of the compensation plate, it obtains ultraviolet (UV) output energy of 0.32~mJ centered at 270~nm with spectral bandwidth of 2~nm when input beam at 800~nm was 70~fs pulse duration and 6~mJ pulse energy which was extracted from Ti:sapphire laser system by a diaphragm, corresponding to an 800-to-270~nm conversion efficiency of 5.3% and a factor-of-1.6 improvement in the third harmonic generation of UV band in comparison with a general conventional configuration. Furthermore, when the full energy of 18~mJ from a Ti:sapphire laser system was used and optimized, the UV emission could reach 0.83~mJ.     

飞秒激光中脉冲内差频技术进展

中红外激光具有多种优势,可以广泛地用到生物、化学、物理等科学研究领域。通常采用直接激射和非线性频率转换这两种方式产生中红外激光,然而,为了实现中红外宽带超短脉冲的发射,非线性频率下转换是现今的唯一方法。脉冲内差频（IP-DFG）是一种简单的非线性频率转换方法,文中对红外IP-DFG的工作做了详细的回顾,从中红外激光晶体和基于IP-DFG产生具有超宽带的中红外超短脉冲的先进工作两个方面做了综述和评论,分别比较了非线性晶体类型、驱动脉冲源、产生超宽带中红外脉冲的光谱范围、转化效率等,并在最后讨论和阐明了IP-DFG领域面临的机遇和挑战。

     

Nonreciprocal frequency doubling of electromagnetic waves through double resonance and Bragg reflection in photonic crystals

A computational study of the uni-directional second-harmonic generation in a one-dimensional dual photonic crystal structure made of GaAs, AlAs and SiO₂ with quadratic optical nonlinearity and material dispersion is presented. The computational approach uses a shooting method to solve nonlinear wave equations for coupled fundamental and second-harmonic fields and the invariant imbedding method to obtain the linear transmittance and group index spectra. The dual structure consists of two substructures, the conversion structure creating a strongly enhanced second-harmonic signal and the filter structure blocking the fundamental frequency field by Bragg reflection while permitting the passage of the second-harmonic field. The conversion structure is built with an elementary cell consisting of four sublayers whose thicknesses are systematically varied. Doubly resonant second-harmonic generation with very high conversion efficiency is achieved for light incident from the conversion structure side by choosing the geometrical parameters of the elementary cell optimally and controlling the band structure. A new mechanism to enhance second-harmonic generation by controlling the energy flow between the fundamental frequency and second-harmonic fields has also been found.     

中远红外非线性光学晶体研究进展

3—5μm和8—12μm波段中远红外激光,在国防和民用领域均具有广泛的应用,作为全固态激光频率转换系统的核心部件,非线性光学晶体需要不断地优化和发展.本文从红外非线性光学晶体材料组成角度出发,总结了几种具有重大应用前景的磷族化合物(ZnGeP_2,CdSiP_2)、硫属化合物(CdSe, GaSe, LiInS_2系列,BaGa_4S_7系列)以及准位相匹配晶体(OP-GaAs, OP-GaP)等中远红外波段非线性光学晶体的研究进展.     

Light frequency conversion in photonic crystals

Light frequency conversion when light interacts with a shock wave propagating through a photonic crystal is investigated. Two new phenomena are found, the first is that frequency increases by integral multiple of a certain amount in the process of frequency conversion. The second phenomenon is frequency conversion that still occurs when the shock wave front is replaced by a vacuum area. Through FDTD simulations and analytical theory, photon-phonon interaction and surface decaying mode interpretations for the mechanism of frequency conversion are found.     

Eigenvalue spectrum analysis for temporal signals of Kerr optical frequency combs based on nonlinear Fourier transform

Based on the nonlinear Schr?dinger equation(NLSE) with damping, detuning, and driving terms describing the evolution of signals in a Kerr microresonator, we apply periodic nonlinear Fourier transform(NFT) to the study of signals during the generation of the Kerr optical frequency combs(OFCs). We find that the signals in different states, including the Turing pattern, the chaos, the single soliton state, and the multi-solitons state, can be distinguished according to different distributions of the eigenvalue spectrum. Specially, the eigenvalue spectrum of the single soliton pulse is composed of a pair of conjugate symmetric discrete eigenvalues and the quasi-continuous eigenvalue spectrum with eye-like structure.Moreover, we have successfully demonstrated that the number of discrete eigenvalue pairs in the eigenvalue spectrum corresponds to the number of solitons formed in a round-trip time inside the Kerr microresonator. This work shows that some characteristics of the time-domain signal can be well reflected in the nonlinear domain.     

Computing for second harmonic generation in one-dimensional nonlinear photonic crystals

A numerical study of second harmonic generation (SHG) in one-dimensional nonlinear photonic crystals based on full nonlinear system of equations, implemented by a combination of the method of finite elements and fixed-point iterations, is reported. This model is derived from a nonlinear system of Maxwell’s equations, which partly overcomes the known shortcoming of some existing models relied on the undepleted-pump approximation. We derive a general solution of SHG in one-dimensional nonlinear photonic crystals structures. The convergence of our method is fast. Numerical simulations also show the conversion efficiency of SHG can be significantly enhanced when the frequencies of the fundamental wave are located at the photonic band edges or are assigned to the designed defect states.     

超短脉冲谐波截止频率与载波相位关系的研究

采用Lewenstein模型计算了两个不同脉宽的超短脉冲高次谐波截止频率与包络载波相位的关系, 结果显示,其截止频率随载波包络相位的增加先减小后增加。随着脉冲宽度的减小,高次谐波截止频率变化的幅度增加。我们按准经典的三步模型解释所得结果,并讨论了量子辐射效应。     

A k-band broadband monolithic distributed frequency multiplier based on nonlinear transmission line

A fabrication technology of GaAs planar Schottky varactor diode (PSVD) is successfully developed and used to design and manufacture GaAs-based monolithic frequency multiplication based on 23-section nonlinear transmission lines (NLTLs) consisting of a coplanar waveguide transmission line and periodically distributed PSVDs. The throughout design and optimization procedure of 23-section monolithic NLTLs for frequency multiplication in the k-band range is based on a large signal equivalent model of PSVD extracted from small-signal S-parameter measurements. This paper reports that the distributed SPVD exhibits a capacitance ratio of 5.4, a normalized capacitance of 0.86 fF/μm2 and a breakdown voltage in excess of 22 V. The integrated 23-section NLTLs fed by 20-dBm input power demonstrates a 26-GHz peak second harmonic output power of 14-dBm with 25.3% conversion efficiency in the second harmonic output frequency range of 6 GHz-26 GHz.     

Optical bistability and temporal symmetry-breaking instability in nonlinear fiber resonators

In this work we analyze two different behaviors in a nonlinear passive fiber ring cavity with a synchronously pulsed pump iterating the infinite-dimensional Ikeda map. First, we show optical bistability with normal and anomalous dispersions. The obtained numerical results are compared with the cw pump case. Secondly, these cavities are subject to a temporal symmetry-breaking instability with anomalous dispersion. This instability is described and the range of parameters for its appearance is shown and discussed.     

新型硫族化合物在中红外非线性光学晶体方面研究进展

利用红外非线性光学晶体材料对已有的成熟的激光光源进行频率转换是获得3~5μm和8~12μm"大气窗口"红外激光的主要方法。传统的红外非线性光学晶体存在缺陷,不能满足应用要求,需要探索新型的红外材料。综述了以硫族化合物为研究对象,寻找新型中红外非线性光学晶体材料的研究进展。介绍了Li MQ2(M=Ga,In;Q=S,Se,Te),BaGa4S7,BaGa4Se7,BaGa2MQ6(M=Si,Ge;Q=S,Se)及Li2In2MQ6(M=Si,Ge;Q=S,Se)的研究进展。     

Subpicosecond pulse compression in nonlinear photonic crystal waveguides based on the formation of high-order optical solitons

We investigate by numerical simulation the compression of subpicosecond pulses in two-dimensional nonlinear photonic crystal (PC) waveguides. The compression originates from the generation of high-order optical solitons through the interplay of the huge group-velocity dispersion and the enhanced self-phase modulation in nonlinear PC waveguides.Both the formation of Bragg grating solitons and gap solitons can lead to efficient pulse compression. The compression factors under different excitation power densities and the optimum length for subpicosecond pulse compression have been determined. As a compressor, the total length of the nonlinear PC waveguide is only ten micrometres and therefore can be easily incorporated into PC integrated circuits.     

Generation of attosecond pulses in molecular nitrogen

We investigate the carrier-envelope phase dependence of the total ionization yield for single and double ionization of xenon. We compare our results to theoretical calculations and to the phase dependent asymmetry in photoelectron emission. We observe that the phase dependence of the photoion yields, regardless if single or double ionization, is at least 2-3 orders of magnitude below the photoelectron emission signal. We conclude that total photoionization yields are only very weakly dependent on the carrier envelope phase, and that they are not a useful means for measurement of the phase. It seems possible that the broad bandwidth of few-cycle pulses facilitates multiphoton ionization, which leads to a randomization of strong field ionization phase dependencies. Besides, we observe that the spatial asymmetry in photoelectron emission appears to be useful as an indicator for the laser pulse duration in the few cycle regime.