Field-free molecular orientation enhanced by tuning the intensity ratio of a three-color laser field

We theoretically study the field-free molecular orientation induced by a three-color laser field. The three-color laser field with a large asymmetric degree can effectively enhance the molecular orientation. In particular, when the intensity ratio of the three-color laser field is tuned to a proper value of I_3: I_2: I_1= 0.09 : 0.5 : 1, the molecular orientation can be improved by ～ 20% compared with that of the two-color laser field at intensity ratio I_2: I_1= 1 : 1 for the same total laser intensity of 2×10~(13)W/cm~2. Moreover, we investigate the effect of the carrier-envelope phase(CEP) on the molecular orientation and use the asymmetric degree of the laser field to explain the result. We also show the influences of the laser intensity, rotational temperature, and pulse duration on the molecular orientation. These results are meaningful for the theoretical and experimental studies on the molecular orientation.     

高功率全光纤啁啾脉冲放大激光系统

采用基于非线性偏振旋转原理的光纤被动锁模激光器作为主振荡器。输出信号脉冲的重复频率为30 MHz,脉冲半高全宽为265 fs。信号脉冲通过全光纤啁啾脉冲激光放大系统展宽至100 ps后,经过1级芯径10 m的光纤预放大器和1级芯径50 m的光纤功率放大器将脉冲平均功率放大至10 W,斜率效率41.5%。输出脉冲经光栅压缩器将脉宽压缩至594 fs。     

高功率全光纤啁啾脉冲放大激光系统

采用基于非线性偏振旋转原理的光纤被动锁模激光器作为主振荡器。输出信号脉冲的重复频率为30MHz,脉冲半高全宽为265fs。信号脉冲通过全光纤啁啾脉冲激光放大系统展宽至100ps后,经过1级芯径10μm的光纤预放大器和1级芯径50μm的光纤功率放大器将脉冲平均功率放大至10W,斜率效率41.5%。输出脉冲经光栅压缩器将脉宽压缩至594fs。     

Monotonically chirped pulse evolution in an ultrashort pulse thulium-doped fiber laser

We report on monotonically positively chirped pulse operation of a hybridly mode-locked thulium fiber laser. Dispersion management was realized with a small-core, high-NA fiber providing normal dispersion in the 2 μm wavelength region. The laser delivered pulses with 0.7 nJ energy at the 1927 nm center wavelength and sub-500-fs pulse duration after compression.     

A theoretical study about the chirped pulse amplification laser

Starting from the Maxwell‘s equation,and using the resonant-dipole equation together with the multilevel rate equations which take the effects of energy relaxation into consideration,we have derived a more realistic numerical model of the chirped pulse amplification for an ultra-broad band width laser amplifier.Numerical simulations of this model show that both the intensity profile and the energy fluence of the amplified chirped pulse are closely connected with the two relaxation effects:the relaxation of the thermalization among the components of the laser multiplets and the depletion of the lower laser level.The results are valuable for the design of ultra-broad bandwidth chirped pulse amplification lasers.     

Frequency-multiplexed gas sensing using chirped laser molecular spectroscopy

A method for frequency-multiplexed multi-sample gas sensing is presented. It enables measuring multiple samples placed simultaneously in the setup, without any optical or mechanical switching. Samples are measured using heterodyne detection and signal from each sensing path is encoded at different carrier frequency. Subsequently, a signal from particular sample is retrieved through heterodyne beatnote demodulation at unique frequency. This technique is particularly suitable for real-time calibration of the sensor through a sequential (or simultaneous) detection of three signals: from unknown sample, reference sample and baseline. Basic setup is demonstrated and proof-of-concept experiments are presented. Very good agreement with spectra measured using standard tunable diode absorption spectroscopy is obtained.     

Multiterawatt laser system based on optical parametric chirped pulse amplification

A compact multiterawatt laser system based on optical parametric chirped pulse amplification is demonstrated. Chirped pulses are amplified from 20 pJ to 900 mJ by two lithium triborate optical parametric preamplifiers and a final KDP optical parametric power amplifier with a pump energy of 5 J at 532 nm from Nd:YAG-Nd:glass hybrid amplifiers. After compression, we obtained a final output of 570-mJ-155-fs pulses with a peak power of 3.67 TW, which is the highest output power from an optical parametric chirped pulse amplification laser, to the best of our knowledge.     

Field-free molecular alignment and its application

Field-free molecular alignment can be achieved by nonadiabatic rotational excitation of molecules with strong femtosecond laser pulses. We experimentally and theoretically demonstrate that the degree of alignment can be improved with multi-pulse excitation. An approach is proposed to tune the frequency of few-cycle pulses using field-free alignment of molecules.     

利用Mach-Zehnder干涉仪提升啁啾脉冲信噪比

基于内置电光晶体的Mach-Zehnder干涉仪,利用Mach-Zehnder干涉仪双光束干涉原理和晶体的线性电光效应,提出了一种新的能有效提高啁啾脉冲信噪比的扫描滤波方法。定量分析了其扫描滤波谱特性,探讨了预脉冲噪声延时对信噪比提升效果的影响,并讨论了电光晶体的电压控制参数对信噪比提升效果的影响。研究结果表明：预脉冲噪声的延时和控制电压的变化会对滤波效果产生较大影响,利用该扫描滤波方法可将啁啾脉冲激光信噪比提升约2个量级,且信号光透过率高达95%以上。     

能量啁啾电子束自由电子激光放大啁啾脉冲

 提出采用具有能量啁啾电子束的自由电子激光放大器放大啁啾脉冲,分析说明了它的工作机理和滑移现象对其的影响。采用研制的1维非定态程序GOFEL-P,对能量啁啾自由电子激光放大器放大啁啾脉冲的过程进行了数值模拟和分析,计算了不同啁啾参数的脉冲被放大后的腔外压缩情况。结果表明：与单能电子束时相比,能量啁啾自由电子激光可以放大具有更大啁啾参数的啁啾脉冲,使压缩后的脉冲峰值功率增大至568 GW,脉冲宽度缩短至2.29 fs,大幅增强自由电子激光放大啁啾脉冲以及腔外压缩脉冲的效果。     

用于钕玻璃啁啾脉冲放大系统光谱整形的多层介质膜反射镜

在千焦拍瓦高功率啁啾脉冲放大系统设计中,为了尽量消除增益窄化和增益饱和效应的影响,同时尽可能提高高功率激光输出脉冲信噪比参数,激光脉冲时空和光谱的整形问题备受关注.提出一种光谱整形新方法,利用特定结构的多层介质膜反射镜,可实现对大能量高功率啁啾脉冲钕玻璃放大系统中啁啾脉冲的光谱整形.研究结果表明,只要合理选择多层介质膜系的结构参数,可有效地控制其反射率分布,且在保证反射相位基本不变的条件下其调制度可超过60%.针对钕玻璃1053nm波长设计而成的光谱整形反射镜,反射带宽可达到196nm,色分辨率约为0.1 关键词： 介质反射膜 光谱整形 千焦拍瓦 啁啾脉冲     

啁啾激光场中HF分子的经典解离

应用经典理论并采用辛算法，计算了HF分子在啁啾激光作用下的经典解离.讨论了激光场中HF分子的解离概率随时间的变化以及考虑振动-转动能级跃迁对分子解离概率的影响.计算结果与理论分析相符，说明运用经典理论并采用辛格式计算双原子分子在激光作用下的经典解离是有效和可行的. 关键词： 啁啾激光场 经典解离 辛算法     

Excitation of a two-level system by a chirped laser pulse

The excitation of a two-level system by a chirped laser pulse is analyzed using an analytical approach (in the perturbation-theory limit) that involves the modified rotating-wave approximation and the numerical solution to the Bloch equation. The dependence of the population of the upper energy level on the chirp is studied for various radiation intensities and pulse durations. An exact solution is compared with the result obtained using the modified rotating-wave approximation and the perturbation theory. It is demonstrated that, for a certain range of parameters, the excitation probability of a two-level system can be effectively controlled via a variation in the chirp.     

利用啁啾激光调制分子谐波信号

数值研究了啁啾激光驱动H_2~+辐射谐波的特点.结果表明,(1)在低强度和高强度激光驱动下,谐波光谱分别呈现红移和蓝移现象.引入正负向啁啾参数后,谐波频移和谐波辐射强度都可以得到调控.(2)谐波光谱在高强度激光驱动下呈现非奇次谐波.理论分析表明,非奇次谐波产生的原因是双H核频移不一致所导致的不对称相消干涉引起的.     

Diffraction characteristics of chirped femtosecond laser pulse by rectangle reflection grating

The spectral and temporal intensity distribution expression for the chirped femtosecond laser pulse diffracted by a rectangle reflection grating is derived. The effects of the chirped coefficient on the spatiotemporal and spectral characteristics are theoretically investigated in detail, and a criterion for judging whether or not the diffraction pulse is just split into two independent pulses in the temporal domain is obtained. The results show that the envelope curve of spectral intensity on the diffraction axis is more blue-shift, and its full width at e^? 1 maximum is wider for bigger chirped coefficient. The principal maximum on the temporal axis can split into two independent principal maximums for enough height from the upper and the nether reflection surface of the grating. Each principal maximum splits into two smooth pulses, namely one principal pulse and one secondary pulse, and the secondary pulse gradually increases with the increasing of the chirped coefficient; the duration of two principal pulses increases with the increasing of the height of the upper and the nether reflection surface of the grating.     

Generation of 7-fs laser pulse directly from a compact Ti:sapphire laser with chirped mirrors

A compact femtosecond Ti:sapphire laser resonator consisting of three chirped mirrors and one output coupler was designed. By accurately balancing the intra- cavity dispersions between Ti:sapphire crystal, air and chirped mirrors, we directly generated the laser pulse shorter than 7 fs at the average power of 340 mW with 3.1 W pump. The repetition rate of the laser oscillator is 173 MHz at the centre wavelength of 791 nm, and the ultrabroaden spectrum covers from 600 nm to 1000 nm. To the best of our knowledge, this is the simplest laser resonator capable of generating sub-10 fs laser pulse.     

Enhanced electron positron pair creation by the frequency chirped laser pulse

Based on the quantum Vlasov equation, the effect of frequency chirp on electron-positron pair production is investigated. The cycle parameter, which characterizes the laser field cycle degree within the pulse, is also considered. In both supercycle and subcycle laser pulses the frequency chirp can greatly enhance the momentum distribution function of created pairs and the pair number density. The pair number density created by a supercycle laser pulse is larger than that by a subcycle pulse under the same laser frequency and chirping. There exists an optimal cycle parameter corresponding to the maximum value of the created pair number density for different chirp rates. It is found that the pair number density is sensitive/insensitive to chirping rate when the cycle parameter lies below/above the optimal one.     

频率啁啾光脉冲在行波半导体激光放大器中的传播特性

本文就行波半导体激光放大器(TW-SLA)中载流子引起的群速度色散对激光脉冲传播特性的影响作了理论研究.由于载流子引起的群速度色散效应,使远离饱和区工作的TW-SLA会对有频率啁啾的光脉冲产生展宽或压缩.本文就TW-SLA参数、频率啁啾参数跟脉冲增宽因子的关系作了理论研究.结果表明,线性的TW-SLA具有对低能量光脉冲压缩的可能性.因此,在光学通信系统中,它可用作对光纤损耗及色散的补偿元件.