Baseline studies of radon/thoron concentration levels in and around the Lambapur and Peddagattu areas in Nalgonda district, Andhra Pradesh, India

Studies conducted by Atomic Minerals Directorate of Exploration and Research (AMD) of Hyderabad, India had established the presence of higher concentrations of uranium in Lambapur and Peddagattu areas of Nalgonda district, AP, India and it was estimated that it could be a viable source for commercial extraction. The envisaged extraction process involves dispersion of radioactive particulate matter into atmosphere. Environmental radioactive studies in and around proposed mining areas at this point of time will be extremely useful for establishing base line data before a large scale uranium extraction process comes into existence. To this end, Solid State Nuclear Track Detectors were installed to evaluate indoor radon and thoron concentration levels in the dwellings of the area. The geometric means of radon and thoron concentration levels were found to be (7.1±0.2)×10¹ and (6.7±0.3)×10¹ Bq/m³, respectively. Simultaneously, natural background radiation measurements were also made and these levels are found to vary from 770 to 3995 μGy/y in the spatial distribution.     

Spatial and temporal variations of radon concentration in soil air

The spatial and temporal variability of the soil gas radon concentration in typical soils is studied. The results obtained will be further used to predict indoor radon levels. To this end, 50 measuring points along geologic sections with known physicogeological parameters of soils were chosen. The soil gas radon concentration was measured with SSNTDs (Type III-b) at a depth of 70 cm from June to October, 2000. The radon exposure time was 72–96 h. The average radon concentration in the soil pore air for an urban area was 11 kBqm⁻³ (1.7–24 kBqm⁻³). Small-scale spatial variations in the concentration were found to lie within a narrower range. The effect of meteorological conditions on the soil gas radon concentration was investigated by performing 8 series of measurements at 5 closely spaced points in September–October, 2000. A significant correlation was found between the soil radon concentration and atmospheric pressure (K=−0.86), ambient temperature (K=0.75), and soil temperature (K=0.75).     

The effect of soil particle size on soil radon concentration

It has been suggested in the literature that the radon concentration in the soil gas is related to the particle size distribution of the soil. This paper examines this relation. Radon concentration was measured in the soil on the Carboniferous limestone south of Buxton in Derbyshire, England, using the can technique. At each site, a sample of soil was taken at the bottom of the hole in which the dosimeter was placed to determine the particle size distribution.

The correlations between the raw values of radon concentration, soil particle size fractions and elevation were weak. Nevertheless, the kriged maps of radon, silt, clay and elevation showed some spatial relation to one another. The kriged estimates showed stronger correlations among these properties, especially between radon and elevation.     

An experimental method for measuring the radon-222 emanation factor in rocks

An experimental method, based on a 21-day accumulation technique, is proposed for measuring the radon-222 emanation factor in undisturbed consolidated materials. The leakage rate is determined from the form of the radon growth curve in the measurement chamber. It was comparable to the radon decay. In order to obtain the “true” radon emanation factor, the thickness of the sample must be less than the radon diffusion length in the porous material. The method was used to measure the radon emanation factor in water-saturated claystones (argillites). The radon emanation factor, determined from experiments on a rock sample with a thickness of 5 mm, was 15%, a value typical for this kind of material.     

Measurements of radon concentration in soil gas by CR-39 detectors

A miniature diffusion chamber with a 25 × 4 × 0.5 mm CR-39 track etch detector (Pershore Moulding Ltd.), mounted on the 1.1 m long pole has been developed for radon gas measurements at 1 meter depth in the soil. For chemically etched CR-39 (7h, 70°C NaOH) and automatic track analysis the lowest detection limit of the chamber was found to be 0.5 MBq h m⁻³ and the useful exposure range from 2 to 20 MBq h m⁻³. The typical exposure time in the soil is between 2 to 14 days. The chamber was tested against the active AlphaGUARD PQ-2000 (Genitron Instruments GmbH) probe. The test yielded consistent results for soils with typical values of permeability and which are not miniature with water. The pilot measurements of radon gas in soil conducted with the miniature diffusion chambers around 48 buildings in Kraków and Silesia regions yielded an average radon concentration of 13 kBq m⁻³. The chambers are to be applied to measure radon concentration in soil before constructing new houses in order to avoid high radon risk areas.     

Study of uranium, radium and radon exhalation rate in soil samples from some areas of Kangra district, Himachal Pradesh, India using solid-state nuclear track detectors

LR-115 plastic track detectors have been used for the measurement of radon exhalation rate and radium concentration in soil samples collected from some villages of Kangra district, Himachal Pradesh, India. Uranium concentration has also been determined in these soil samples using fission track technique. Radium concentration in soil samples has been found to vary from 11.54 to 26.71 BqKg⁻¹, whereas uranium concentration varies from 0.75 to 2.06 ppm. The radon exhalation rate in these samples has been found to vary from 15.16 to 35.11 mBqKg⁻¹ h⁻¹ (502.12 to 1162.64 mBqm⁻² h⁻¹).     

Variation of radon concentrations in soil and groundwater and its correlation with radon exhalation rate from soil in Budhakedar, Garhwal Himalaya

Radon was measured in soil-gas and groundwater in the Budhakedar area of Tehri Garhwal, India in summer and winter to obtain the seasonal variation and its correlation with radon exhalation rate. The environmental surface gamma dose rate was also measured in the same area. The radon exhalation rate in the soil sample collected from different geological unit of Budhakedar area was measured using plastic track detector (LR-115 type II) technique. The variation in the radon concentration in soil-gas was found to vary from 1098 to 31,776 Bq.m⁻³ with an average of 7456 Bq.m⁻³ in summer season and 3501 to 42883 Bq.m⁻³ with an average of 17148 Bq.m⁻³ in winter season. In groundwater, it was found to vary from 8 to 3047 Bq.l⁻¹ with an average value 510 Bq.l⁻¹ in summer and 26 to 2311 Bq.l⁻¹ with an average value 433 Bq.L⁻¹ in winter. Surface gamma dose rate in the study area varied from 32.4 to 83.6 μR.h⁻¹ with an overall mean of 58.7 μ-R.h⁻¹ in summer and 34.6 to 79.3 μR.h⁻¹ with an average value 58.2 μR.h⁻¹ in winter. Radon exhalation rate from collected soil samples was found to vary from 0.1 × 10⁻⁵ to 5.7 × 10⁻⁵ Bq.kg⁻¹.h⁻¹ with an average of 1.5 × 10⁻⁵ Bq.kg⁻¹.h⁻¹ in summer season and 1.7 × 10⁻⁵ to 9.6 × 10⁻⁵ Bq.kg⁻¹.h⁻¹ with an average of 5.5 × 10⁻⁵ Bq.kg⁻¹.h⁻¹. A weak negative correlation was observed between radon exhalation rate from soil and radon concentration in the soil. Radon exhalation rate from the soil was also not found to be correlated with the gamma dose rate, while it shows a positive correlation with radon concentration in water in summer season. Inter-correlations among various parameters are discussed in detail.      

Measurement of indoor radon levels in Erbil capital by using solid state nuclear track detectors

Radon alpha activity concentration has been measured in 28 homes in the Erbil Capital-Iraqi Kurdistan region during the autumn season by using time-integrated passive radon dosimeters containing CR-39 solid state nuclear track detectors “SSNTDs”. The radon activity concentrations in these homes range from (10.33–90.34) with an average of . The average absorption effective dose equivalent for a person living in homes for which the investigation were done was found to be , obtained by using an equilibrium factor of 0.5 and an occupancy factor of 0.8. The average lung cancer cases per year per 10⁶ person was found to be 23±12.     

Correlations between radon in soil gas and the activity of seismogenic faults in the Tangshan area,North China

The spatial variation of soil gas radon values were correlated with the seismogenic faults and earthquakes in the Tangshan area (north China). Radon concentrations were measured at 756 sites in an area about 2500 km² from April to May 2010. The background and anomaly threshold values calculated were 4730.4 Bq/m³ and 8294.1 Bq/m³, respectively. Radon concentrations highlight a decreasing gradient from NE to SW in the area. Higher values mostly distributed in the NE sector of the Tangshan fault and the Luanxian fault where the Tangshan (Ms 7.8), and Luanxian (MS 7.1) earthquakes occurred in 1976 and 17 earthquakes with MS = 3.0 occurred in this area since 2005. Radon values illustrated a close relation with the shallow fault trace and earthquake activity in the area. The active fault zones and the associated fractures formed by the larger earthquakes, act as paths for radon migration.     

Seasonal and location dependence of indoor and soil radon concentrations in two villages,Najran region,Saudi Arabia

Seasonal (winter-summer) indoor and soil radon comparison is made in two villages in Najran region, south west of Saudi Arabia, using CR-39 Dosimeter. Summer indoor radon concentrations were measured in the villages of Fara Al-Jabal and Hadadah. The respective winter-summer average values of 42 ± 4 Bq m⁻³ and 74 ± 5 Bq m⁻³ are measured in Fara Al-Jable village and the average values of 47 ± 4 Bq m⁻³ and 76 ± 5 Bq m⁻³ are measured in Hadadah village. The respective winter-summer soil values are 1.40 ± 0.21 kBq m⁻³ and 0.99 ± 0.04 kBq m⁻³ in Fara Al-Jabal village while those measured in Hadadah village are 2.90 ± 0.17 kBq m⁻³ and 1.40 ± 0.66 kBq m⁻³. Indoor radon levels are found to be seasonal dependent while that of soil are found seasonal and location dependent. Meteorological and geological factors are expected to have caused the measured significant differences in radon levels in dwellings and soil in the two villages.     

Determination of radon distribution patterns in the upper soil as a tool for the localization of subsurface NAPL contamination

A radon survey was carried out at an abandoned military airfield, heavily contaminated with non-aqueous phase-liquids (NAPLs). Geo-statistical analysis of the data was used to confirm the validity of the chosen soil gas sampling pattern. The survey revealed a non-uniform distribution of the soil gas radon concentration in the upper soil in spite of a virtually homogenous geological situation. The radon distribution pattern showed minimum zones with radon concentrations decreased by up to 90% with regard to the local background level. The determined radon minimum anomalies could be explicitly associated with the NAPL subsurface contamination. The observed effect is due to the strong partitioning of radon into NAPLs from soil gas or groundwater. Corresponding partitioning coefficients were determined in the laboratory for some NAPL. As result of the study, it was shown that naturally occurring soil gas radon has the potential to be used as an indicator for the localization of subsurface NAPL contamination. As possible options for survey equipment, the AlphaGUARD radon monitor and passive solid-state nuclear track detectors were successfully evaluated.     

An approach to discriminatively determine thoron and radon emanation rates for a granular material with a scintillation cell

A powder sandwich technique was applied to determine thoron (²²⁰Rn) and radon (²²²Rn) emanation rates for a granular material. The feature of this technique is the sample preparation, in which a granular material is put and fixed between two membrane filters. Airflow is directly given to this sandwich sample, will include thoron and radon emanated from the material, and then is transferred to the detector. This method makes sure that thoron and radon emanated are not retained in pore space within the sample volume, which is crucial for the appropriate emanation test. This technique was first introduced by Kanse et al. (2013) with the intention to measure the emanation of thoron - but not of radon - from materials having much higher ²²⁴Ra activity than ²²⁶Ra. In the present study, the methodology for the discriminative determination of thoron and radon emanation rates from a granular material has been examined using a flow-through scintillation cell and sandwich sample. The mathematical model was developed to differentiate total alpha counts into thoron- and radon-associated counts. With a sample of uranium ore, this model was experimentally validated by comparison between the scintillation cell and a reference detector that can discriminatively measure thoron and radon concentrations. Furthermore, the detection limits and uncertainties were evaluated to discuss the characteristics of this method. Key parameters for improving the determination of thoron and radon emanations were found to be the background radon concentration and the leakage of radon from the measurement system, respectively. It was concluded that the present method is advantageous to a sample that has much higher ²²⁶Ra activity than ²²⁴Ra.     

Seasonal variation on radon emission from soil and water

Radon is being measured continuously in spring water and soil-gas at Badshahi Thaul Campus, Tehri Garhwal in Himalayan region by using radon Emanometer since December 2002. An effort was made to correlate the variance of radon concentrations in spring water and soil-gas with meteorological parameters at the same location. The main meteorological parameters that affect the radon emanation from host material is surrounding temperature, barometric pressure, wind velocity, rain fall and water level of the spring. The correlation coefficient between radon concentration in spring water and different atmospheric parameters was computed. The correlation coefficient between radon concentration in spring water and the maximum atmospheric temperature was 0.3, while it was 0.4 for minimum atmospheric temperature at the monitoring site. The correlation coefficient for radon concentration in spring water with minimum and maximum relative humidity was 0.4. Spring water radon concentration was found positively correlated (0.6) with water discharge rate of the spring. A weak correlation (0.09) was observed between the radon concentration in spring water and rain fall during the measurement period. As temperature of near surface soil increases, the radon emanation coefficient from the soil surface also increases. The possible effects due to global warming and other climatic changes on environment radiation level were also discussed in detail.      

Variations of soil radon and thoron concentrations in a fault zone and prospective earthquakes in SW Taiwan

An automatic station for soil gas monitoring was set up on an active fault zone of SW Taiwan. After more than one year of continuous measurements, some spike-like anomalous high radon and thoron concentrations could be observed. A similar soil radon spectrum was also obtained from an independent monitoring station, which was only 100 m away. These anomalous peaks usually occurred a few days or weeks before the earthquakes (M_L4.5). This indicates that variations of both soil radon and thoron can serve as useful tools for earthquake surveillance, esp. at fault zones.     

A comparative study of indoor radon level measurements in the dwellings of Punjab and Himachal Pradesh, India

The LR-115 type-II plastic track detector has been used for measuring the indoor radon levels in the dwellings of some villages of Punjab and Himachal Pradesh. In Punjab, the villages surveyed are Rampura Phul, Lehra Mahabat and Pitho (villages in Bathinda district), and Amritsar city. The average indoor radon levels in these areas are found to vary from 64 to 152 Bq/m³, which are quite within the safe limits recommended by International Commission on Radiological Protection (Ann. ICRP 23(2)). The indoor radon levels have also been measured in the dwellings of Hamirpur district of Himachal Pradesh. The villages surveyed in this area are Nukhel, Badarn, Galore-Khas, Har-Upper, Tikker Brahamana and Awah-Lower where radon concentration has been found to vary from 261 to 724 Bq/m³. These values are higher than the recommended limit.     

Measuring radon exhalation rate by tracing the radon concentration of ventilation-type accumulation chamber

Radon exhalation rate is crucial in the estimation of radiation risk from various materials. RAD7 only focus on the count of the ²¹⁸Po in sniff mode, and is well suited to measure radon exhalation rates. This paper presents a fast method for measuring radon exhalation from medium surface with a ventilation-type accumulation chamber by the RAD7 while making the effects of leakage and back diffusion negligible. The radon exhalation rate can be obtained from the measured values before radioactive equilibrium between Radon and progeny occurs. This method is based on the principle for tracing radon concentration changes by deriving ²²²Rn concentrations through ²¹⁸Po measurements. Several radon exhalation rate measurements of medium surface have been performed in the Radon Laboratory of the University of South China. The radon exhalation rates obtained by verification experiments are within the accepted values for the reference value.     

Analysis of seasonal variation of indoor radon concentration in Tehri Garhwal, Northern India

The seasonal variation analysis of indoor radon has been carried out in the hilly region of Tehri Garhwal, Northern India by using LR-115 Type II, plastic track detector. In the analysis the winter/summer ratio radon values were found to vary from 0.63 to 1.64 and 1.02 to 1.22 for cemented houses and mud houses, respectively. Over all the average value of winter/summer ratio was found maximum in both cemented and mud houses respectively.      

A method for estimating the convective radon transport velocity in soils

A method for estimating the convective radon transport velocity in soils is developed. The approach under review is based on measurements of the radon concentration in soil air. Mathematical models for describing the convective radon transport velocity are discussed. Data on the convective radon transport velocity in commonly encountered soil types are presented. The results obtained from a 2-month experiment aimed at investigating the effect of the atmospheric condition on the convective radon transport velocity are reported. The soil gas radon concentration at 30–70 cm depth was measured by means of passive track detectors (Type III-b SSNTDs) with 72–96 h exposure time.