The systematics of (n, α) reaction cross-sections at 14.5 MeV neutron energy

A comprehensive review of the experimental data for 14.5 MeV neutron induced reaction crosssections for (n, α) reaction has been made for the isotopes having Z up to 82. Two different parameter groups have been considered by the classification of nuclei into odd-mass and even-even nuclei. The empirical formulae with two parameters for the evaluation of (n, α) reaction cross-sections are discussed in the present study. The odd-even effects have been observed as the cross-sections of odd-mass nuclei are higher as compared to their neighboring even-even nuclei. The shell effects have also been established at magic nucleon numbers for these reaction cross-sections.     

偶-偶超重核基态性质的理论研究

在形变的相对论平均场模型下采用NL Z2,TMA两套参数对一些偶 偶核基态性质进行了系统的计算,并将理论计算的结合能、α衰变能与已知的实验数据进行了对比分析.结果发现两方面的数据能够比较好地吻合,从而验证了相对论平均场模型对超重核研究是可行的.同时在计算中给出了未知核素基态性质的计算结果,可供以后在理论或实验上研究超重核时参考. The ground state properties of the even even nuclei with proton number Z=94-104 have been systematically calculated in the deformed relativistic mean field (RMF) theory with two sets of force parameters, TMA and NL Z2. Comparing the calculated binding energies and alpha decay energys with the experimental ones, it is found that theoretical results are in good agreement with experimental data. The reliability of the RMF model for even even superheavy nuclei has been tested by this comparison...     

Theoretical Study on N = 126 Shell Evolution

The nuclei around magic number N = 126 are investigated in the deformed relativistic mean field (RMF) model with effective interactions TMA. We focus investigations on the N = 126 isotonic chain. The N = 126 shell evolution is studied by analyzing the variations of two-neutron (proton) separation energies, quadruple deformations, single particle levels etc. The good agreement of two-neutron separation energies between experimental data and calculated values is reached. The RMF theory predicts that the sizes of N = 126 shell become smaller and smaller with the increasing of proton number Z. However, the N = 126 shell exists in our calculated region all along. According to the calculated two-proton separation energies, the RMF theory suggests ²²⁰Pu is a two-proton drip-line nucleus in the N = 126 isotonic chain.     

New narrow nucleon N* (1685)

We argue that the existence of a new narrow (Γ ≤ 25 MeV) nucleon resonance N* (1685) is strongly supported by recent data on the η photoproduction off the nucleon. The resonance has a much stronger photocoupling to the neutron than to the proton. This nucleon resonance is a good candidate for the nonstrange member of the exotic antidecouplet of baryons—the partner of the pentaquark Θ⁺. All of the properties of new N* (1685) known to date are summarized. The text was submitted by the authors in English.     

相对论平均场模型对奇-偶超重核基态性质的系统研究

在形变的相对论平均场模型下,采用NL-Z2,TMA两套参数对质子数为103—109的奇–偶核基态性质进行了系统的计算,并将理论计算的结合能、α衰变能与已知的实验数据进行对比,发现两者符合得很好,肯定了相对论平均场模型对超重核研究的可靠性,同时对未知核素基态性质的计算结果可供未来的超重核理论和实验研究参考.     

Inelastic interactions of 9.38 GeV/c deuteron in emulsion

Characteristics of the inelastic interactions of 9.38 GeV/c deuterons with nuclear emulsion nuclei have been studied. These have been compared with nucleon-nucleus interactions at a corresponding momentum. The probability of nucleon stripping in deuteron-nucleus interactions has been observed to be 0.5. The charged particle multiplicity in deuteron-nucleus interactions exhibitA-dependence of the typeA ^α with α=0.08. The experimental data disagree with KNO scaling.     

Level inversion of N=9 isotones in the relativistic mean-field theory

We have studied the ground state properties of N=8 and N=9 isotones in the framework of the nonlinear relativistic mean-field (RMF) theory using force parameters NL-SH. Calculations show that the RMF theory can describe experimental data of binding energies and radii for these nuclei. The RMF theory can also reproduce the level inversion of N=9 isotones well if the ρ tensor coupling is included. One-neutron halos in ¹⁵C and ¹⁴B are predicted.     

High-frequency (94.9 GHz) EPR spectroscopy of paramagnetic centers in a neutron-irradiated sapphire single-crystal fiber

Initial results are reported of an EPR study, conducted at 94.9 GHz, of a thermally annealed, neutron-irradiated white sapphire (α-Al₂O₃) single-crystal fiber. The optical centers produced in sapphire by neutron irradiation and thermal annealing are of interest for optical technologies involving the phenomenon of spectral hole-burning. While these centers have been modeled as consisting of electrons localized at anion vacancies, experimental tests of this model have been very limited. EPR spectroscopy — a choice technique for elucidating structural details of such color centers — reveals signals from numerous paramagnetic centers in this material. The predominant signals, with amplitudes a hundredfold greater than any other signals, derive from three closely related, highspin-multiplicity centers. These centers do not, however, derive from radiation-induced lattice defects: they are readily identified as Cr³⁺ (S = 3/2) and a pair of crystallographically equivalent Fe³⁺ (S=5/2) impurity ions. The advantages of high-frequency-EPR instrumentation in facilitating this identification are presented and discussed in detail. These advantages include enhanced sensitivity for this volume-limited, fiber sample. Moreover, the analysis of the spectra — entailing spectral assignments, evaluation of the spin-Hamiltonian parameters, and spin-counting — is greatly facilitated when the Zeeman interaction is dominant.     

Relativistic mean field and some recent applications

The essentials of the Relativistic Mean Field (RMF) theory and some of its recent applications are presented. The explicit calculations are carried out for a few selected isotopic, isotonic and isobaric chains of nuclei covering the entire periodic table. The calculated ground state properties are found to be in good agreement with the corresponding experiment: the binding energies are reproduced within 0.25%, on average, and the charge radii differ only in the second decimal place of fermi. The relativistic origin of the pseudo-spin symmetry is briefly discussed. The density distributions obtained, are found to be in good agreement with the experiment (where available). The peripheral factor, the ratio of neutron and proton densities on the nuclear periphery, extracted in the anti-proton annihilation experiments are well reproduced. The RMF densities are used to calculate the reaction (σ_R) and charge changing (σ_cc) cross sections in the Glauber model, as well as the α (cluster)-daughter interaction energy. The latter is then employed to estimate the decay half lives of Super-Heavy (trans-actinide) nuclei in the WKB approximation. The calculations are found to agree well with the experiment. This success of the RMF in accurately describing the nuclear properties with only a few fixed parameters is indeed remarkable. The text was submitted by the authors in English.     

Adjustment of Non-linear Interaction Parameters for Relativistic Mean Field Approach by Using Artificial Neural Networks

The relativistic mean field (RMF) model with a small number of adjusted parameters has been used successfully in the last thirty years for predictions of various ground-state nuclear properties of nuclei. In this model, Dirac and Klein–Gordon like equations obtained from application of variation principle on phenomenological Lagrangian density are solved iteratively for calculations of nuclear properties of nuclei. For this purpose, parameters such as masses of considered mesons, nucleon–meson coupling constants, and self-couplings of mesons are needed and they are fitted from experimental data. Some parameter sets for RMF model introduced to correct predictions of nuclear properties of nuclei cover nuclidic chart. Besides Artificial Neural Network (ANN) method is used successfully in many field of science as in nuclear physics. ANN is known as a very powerful tool that are used when standard techniques fail to estimate the correlation between the variables. In the present study, ANN method has been employed to check its understanding capability of relations between RMF model parameters and their predictions on the ground-state binding energies of some spherical nuclei. Understanding capability of ANN method for these relations of considered nuclei has been found well. Based on this success, new non-linear parameter set for RMF model called DEFNE by us have been produced by using ANN method. Furthermore, predictions of RMF model with DEFNE parameter set for ground-state binding energies and charge radii of nuclei cover nuclidic chart have been found as in agreement with the available experimental data.     

Ground State Properties of Z = 126 Isotopes within the Relativistic Mean Field Model

The ground state properties of Z = 126 isotopes with neutron numbers N = 174-244 are calculated by the relativistic mean field(RMF) theory with effective interactions NL-Z2. In order to make a comprehensive understanding of the possible proton magic number Z = 126, we also perform the calculations in the vicinity of Z = 126, such as Z = 114, 116, 118, 120, 122, 124, 128 and 130 isotopic chains. The calculated results show there exist evident magicity for proton number Z = 120 and relatively weak magicity for proton number Z = 126.     

Shape coexistence around the Z=82 closed shell probed by α-decay

Shape coexistence around the Z=82 closed proton shell, probed via the fine structure in the α-decay of even–even nuclei, is discussed. The power of α-decay studies is demonstrated by presenting the results from a number of decay experiments of Rn isotopes performed at ISOLDE. The total body of experimental evidence on α-decay of even–even nuclei in the Pb region is used to illuminate, through the α-decay reduced widths of the ground state to ground state transitions and through the hindrance factors of the fine structure, the role of multi-particle multi-hole proton excitations across the Z=82 shell. This revised version was published online in July 2006 with corrections to the Cover Date.     

Effect of the structure of neutron-rich <Superscript>8</Superscript>Li and <Superscript>9</Superscript>Li isotopes on the characteristics of proton elastic scattering

The differential cross sections of proton elastic scattering from ⁸Li and ⁹Li nuclei in inverse kinematics have been calculated. The cross sections were determined within the Glauber diffraction theory with the wave functions of nuclei in the three-particle α-t-n, α-t-2n, and ⁷Li-n-n models. Comparison with the existing experimental data for E = 700 and 60 MeV/nucleon made it possible to draw a conclusion about the quality of the wave functions and the adequacy of the potentials used for their calculations.     

Properties and structure of N=Z nuclei within relativistic mean field theory

The axially deformed relativistic mean field theory with the force NLSH has been performed in the blocked BCS approximation to investigate the properties and structure of N=Z nuclei from Z=20 to Z=48.Some ground state quantities such as binding energies, quadrupole deformations, one/two-nucleon separation energies, root-mean-square (rms) radii of charge and neutron, and shell gaps have been calculated.The results suggest that large deformations can be found in medium-heavy nuclei with N=Z=38-42.The charge and neutron rms radii increase rapidly beyond the magic number N=Z=28 until Z=42 with increasing nucleon number, which is similar to isotope shift, yet beyond Z=42, they decrease dramatically as the structure changes greatly from Z=42 to Z=43.The evolution of shell gaps with proton number Z can be clearly observed.Besides the appearance of possible new shell closures, some conventional shell closures have been found to disappear in some region.In addition, we found that the Coulomb interaction is not strong enough to breakdown the shell structure of protons in the current region.     

Direct experimental evidence for very long fission times of super-heavy elements

The blocking technique in single crystals has been applied to reaction time measurements for the ²³⁸U + Ge system at 6.1 MeV/nucleon. Backed up with a reaction mechanism analysis using the INDRA 4π detector, it provides a direct experimental evidence for Z = 124 compound nuclei living longer than 10^-18 s, indicating thus very high fission barriers for this element.     

K*0 and φ meson production in proton–nucleus interactions at ?s=41.6\textGeV\sqrt{s}=41.6\text{GeV}

The inclusive production cross sections of the strange vector mesons K^*0, K̄^*0, and φ have been measured in interactions of 920 GeV protons with C, Ti, and W targets with the HERA-B detector at the HERA storage ring. Differential cross sections as a function of rapidity and transverse momentum have been measured in the central rapidity region and for transverse momenta up to p_T = 3.5 GeV/c. The atomic number dependence is parametrised as σ_pA=σ_pN*A^α, where σ_pN is the proton–nucleon cross section. Within the phase space accessible, α(K^*0)=0.86±0.03, α(K̄^*0)=0.87±0.03, and α(φ)=0.96±0.02. The total proton–nucleon cross sections, determined by extrapolating the differential measurements to full phase space, are σ_pN→K*0=(5.06±0.54) mb, σ_pN→K̄*0=(4.02±0.45) mb, and σ_pN→φ=(1.17±0.11) mb. For all resonances the Cronin effect is observed; compared to the measurements of Cronin et al. for K^± mesons, the measured values of α for φ mesons coincide with those of K⁺ mesons for all transverse momenta, while the enhancement for K^*0/K̄^*0 mesons is smaller.     

Macroscopic-microscopic calculations of ground state properties of superheavy nuclei

We systematically calculate the ground state properties of superheavy even-even nuclei with proton number Z=94–118. The calculations are based on the liquid drop macroscopic model and the microscopic model with the modified single-particle oscillator potential. The calculated binding energies and α-decay energies agree well with the experimental data. The reliability of the macroscopic-microscopic(MM)model for superheavy nuclei is confirmed by the good agreement between calculated results and experimental ones. Detailed comparisons between our calculations and M?ller’s are made. It is found that the calculated results also agree with M?ller’s results and that the MM model is insensitive to the microscopic single-particle potential. Calculated results are also compared with results from relativistic mean-field (RMF) model and from Skyrme-Hatree-Fock(SHF) model. In addition, half-lives, deformations and shape coexistence are also investigated. The properties of some unknown nuclei are predicted and they will be useful for future experimental researches of superheavy nuclei.     

基于相对论平均场理论对超重核冷熔合反应截面的研究

在形变约束的相对论平均场理论框架下计算了合成Z=102—118元素的(可能)冷熔合反应中复合核及蒸发一或两个中子剩余核的位能曲面,得到了复合核和剩余核平衡点和鞍点的性质、静态裂变垒高度和冷熔合反应的最佳入射能;利用壳修正和对修正方法计算了平衡点和鞍点的壳修正能、对修正能和微观能.利用由此得到的壳结构信息,用简单的熔合蒸发唯象模型计算了相应反应的冷熔合截面.结果发现,TM1参数提供的结构性质给出了与实验接近的反应截面.     

Evaluation and use of the Pd | SrCe0.95Yb0.05O3| Pd electrochemical reactor for equilibrium-limited hydrogenation reactions

The current — overpotential characteristics of the H₂ - Pd - SCY interphase have been studied at atmospheric total pressure and temparatures between 400 – 550 °C in the single chamber reactor — cell: Pd | SCY | Pd. The results of I−η measurements indicate that the apparent anodic and cathodic charge tranfer coefficients are equal to: α_a=α_c=0.5. The present results are compared to those obtained with the single — chamber reactor cell: Ag | SCY | Ag. A solid state proton (H⁺) conducting reactor — cell with Pd electrodes was tested for the ammonia synthesis from its elements at atmospheric pressure. At 570 °C, over 75% of the ectrochemically supplied hydrogen was converted into NH₃. The thermodynamic requirement for a high pressure process was eliminated. Paper presented at the 5th Euroconference on Solid State Ionics, Benalmádena, Spain, Sept. 13–20, 1998.