Thermodynamic properties of CeCu6-xAux: Fermi-liquid vs. non-Fermi-liquid behaviour

We report on a detailed comparison of the thermodynamic properties of the heavy-fermion system CeCu₆ which can be described as a Fermi liquid at low temperatures T < 0.1 K, and CeCu_5.9Au_0.1 where strong deviations from the Fermi-liquid behaviour were found previously in the T dependence of the specific heat C, magnetization M and electrical resistivity p. The specific heat, magnetization and elastic constants are investigated in a large range of magnetic fields, corroborating the idea that the non-Fermi-liquid behaviour arises from low-lying spin excitations. For the elastic constants, a striking linear T dependence is found for CeCu_5.9Au_0.1 in contrast to the T² Fermi-liquid behaviour of CeCu₆.     

Instability of the non-Fermi-liquid state in a metal with d or f impurities

It is shown that the non-Fermi-liquid state is unstable with respect to scattering of multiparticle excitations with different quantum numbers by one another. As a result of the scattering, a multiparticle Fermi-liquid resonance forms at the Fermi level. An anomalous increase in the conductivity occurs as a result of a transition between the non-Fermi-liquid and Fermi-liquid states. Pis’ma Zh. éksp. Teor. Fiz. 69, No. 10, 721–726 (25 May 1999)     

Role of dipole-dipole interactions in half-field quantum transitions in magnetic nanoparticles

In order to better understand the origin of “forbidden” quantum transitions observed in superparamagnetic nanoparticles at low magnetic fields, electron magnetic resonance (EMR) studies have been performed at room temperature on iron oxide nanoparticles assembled inside parallel nanosized channels penetrating the anodic alumina membrane. The positions of both the main resonance and “forbidden” (2Q) transitions observed at the half-field demonstrate the characteristic angular dependence with the line shifts proportional to 3cos²θ−1, where θ is the angle between the channel axis and external magnetic field B. This result can be attributed to the inter-particle dipole-dipole interactions within elongated aggregates inside the channels. The angular dependence of the 2Q intensity is found to be proportional to sin²θcos²θ, that is consistent with the predictions of quantum-mechanical calculations with the account for the mixing of states by non-secular inter-particle dipole-dipole interactions. Good agreement is obtained between different kinds of measurements (magnetization curves, line shifts and 2Q intensity), pointing to possibility of the quantum approach to the magnetization dynamics of superparamagnetic objects.     

Quasi-one-dimensional quantum spin liquid in the Cu(C<Subscript>4</Subscript>H<Subscript>4</Subscript>N<Subscript>2</Subscript>)(NO<Subscript>3</Subscript>)<Subscript>2</Subscript> insulator

We analyze measurements of the magnetization, differential susceptibility and specific heat of quasi-onedimensional insulator Cu(C₄H₄N₂)(NO₃)₂ (CuPzN) subjected to magnetic fields. We show that the thermodynamic properties are defined by quantum spin liquid formed with spinons, with the magnetic field tuning the insulator CuPzN towards quantum critical point related to fermion condensation quantum phase transition (FCQPT) at which the spinon effective mass diverges kinematically. We show that the FCQPT concept permits to reveal and explain the scaling behavior of thermodynamic characteristics. For the first time, we construct the schematic T–H (temperature-magnetic field) phase diagram of CuPzN that contains Landau–Fermi-liquid, crossover and non-Fermi liquid parts, thus resembling that of heavy-fermion compounds.     

Studying the regime of complete decoupling of the bond between the electron and nuclear moments at the <Emphasis Type="Italic">D</Emphasis><Subscript>1</Subscript>-line of the <Superscript>39</Superscript>K potassium isotope using a spectroscopic microcell

Atomic transitions of the ³⁹K potassium isotope in strong (up to 1 kG) longitudinal and transverse magnetic fields have been studied with a high spectral resolution. It has been shown that crossover resonances are almost absent in the saturated absorption spectrum of potassium vapors in a 30-μm-thick microcell. This, together with the small spectral width of atomic transitions (~30 MHz), allows one to use the saturated absorption spectrum for determining frequencies and probabilities of individual transitions. Among the alkali metals, potassium atoms have the smallest magnitude of the hyperfine splitting of the lower level. This allows one to observe the break of the coupling between the electronic and nuclear angular momentums at comparatively low magnetic fields B > 500 G, i.e., to implement the hyperfine Paschen–Back regime (HPB). In the HPB regime, four equidistantly positioned transitions with the same amplitude are detected in circularly polarized light (σ⁺). In linearly polarized light (π) at the transverse orientation of the magnetic field, the spectrum consists of eight lines which are grouped in two groups each of which consists of four lines. Each group has a special distinguished G-transition and the transition that is forbidden in the zero magnetic field. In the HPB regime, the probabilities of transitions in a group and derivatives of their frequency shifts with respect to the magnetic field asymptotically tend to magnitudes that are typical for the aforesaid distinguished G-transition. Some practical applications for the used microcell are mentioned.     

Fine Structure of the Optical Spectrum and Multiparticle Excitations in Rb2MnCl4

Results of experimental investigations into the optical absorption spectrum of Rb₂Mn_xCd_1–x Cl₄ solid solutions corresponding to ⁶ A _1g ⁴ A _1g ⁴ E _g transitions in manganese ions are presented. The spectra were measured at variable temperatures, magnetic fields, and concentrations x. The magnetic phase transitions accompanying variations of these parameters cause considerable changes in the spectrum. The exciton and exciton-magnon bands, their cold and hot magnon analogs, and the phonon satellite bands have been detected. The specific features of the optical absorption spectrum caused by the low-dimensional magnetic order are elucidated.     

Coulomb screening of impurity charge and anomalous tunneling transparency

This paper analyzes the effect of the screened Coulomb interaction between metallic electrons in the sidewalls, on the one hand, and a localized electron in an impurity level, on the other, on the tunneling in doped quantum structures with an intrinsic two-dimensional continuum. We show that Mahan’s non-Fermi-liquid singularity at the Fermi level is unstable against additional scattering due to tunneling. As a result, the current-voltage characteristic changes radically when the Fermi level in the sidewalls is approached by the edge of the two-dimensional band. Specifically, the peak due to the non-Fermi-liquid singularity with a section of negative differential resistance is replaced with a step-like or a two-step feature, which corresponds to a single or split Fermi-liquid resonance near the edge of the 2D band involved in the tunneling process. Zh. éksp. Teor. Fiz. 115, 1843–1859 (May 1999)     

The quantum compass chain in a transverse magnetic field

We study the magnetic behaviors of a spin-1/2 quantum compass chain (QCC) in a transverse magnetic field, by means of the analytical spinless fermion approach and numerical Lanczos method. In the absence of the magnetic field, the phase diagram is divided into four gapped regions. To determine what happens by applying a transverse magnetic field, using the spinless fermion approach, critical fields are obtained as a function of exchanges. Our analytical results show, the field-induced effects depend on in which one of the four regions the system is. In two regions of the phase diagram, the Ising-type phase transition happens in a finite field. In another region, we have identified two quantum phase transitions (QPT)s in the ground state magnetic phase diagram. These quantum phase transitions belong to the universality class of the commensurate-incommensurate phase transition. We also present a detailed numerical analysis of the low energy spectrum and the ground state magnetic phase diagram. In particular, we show that the intermediate state (h _c1 < h < h _c2) is gapful, describing the spin-flop phase.     

Metals near a magnetic instability

Zero-temperature magnetic phase transitions exhibit an abundance of nearly critical magnetic fluctuations that allow to probe the traditional concepts of the metallic state. For the prototypical heavy-fermion compound, CeCu_6−x Au _x , a breakdown of the Fermi-liquid properties may be tuned by Au concentration, hydrostatic pressure, or magnetic field. The d-electron weak itinerant ferromagnet ZrZn₂, on the other hand, was recently found to display superconductivity in coexistence with ferromagnetism.     

Quantum limit in a parallel magnetic field in layered conductors

We show that electron wave functions in a quasi-two-dimensional conductor in a parallel magnetic field are always localized on conducting layers. In particular, wave functions and the electron spectrum in a quantum limit, where the sizes of quasiclassical electron orbits are of the order of nanoscale distances between the layers, are determined. ac infrared measurements to investigate Fermi surfaces and to test Fermi-liquid theory in quasi-two-dimensional organic and high-Tc materials in high magnetic fields, H approximately equal 10-45 T, are suggested.     

Paramagnetic intrinsic Meissner effect in a bulk

We calculate the free energy of a quasi-two-dimensional (Q2D) superconductor with ξ_⊥ < d in a parallel magnetic field, where ξ_⊥ is a perpendicular to the conducting layer coherence length and d is the interlayer distance. It is shown to be different from that in the famous Lawrence-Doniach model. In particular, at high enough magnetic fields, the Meissner currents are found to create an unexpected paramagnetic moment due to the shrinking of the Cooper pairs “sizes” in a direction perpendicular to the conducting layers. We suggest measuring this paramagnetic intrinsic Meissner effect in Q2D superconductors and superconducting superlattices. The text was submitted by the author in English.     

Non-Fermi-liquid effects in tunneling

Non-Fermi-liquid tunneling mechanisms in a quantum structure with its own two-dimensional continuum doped with transition metal impurities are considered. New physical realizations of the two-channel Kondo orbital model with mechanisms different from those previously described in literature occur in such quantum structures. The tunneling transparency is anomalously high owing to new channels generated by multiparticle Fermi-liquid resonances near the edge of the two-dimensional energy band in the process of tunneling. The widths of new edge resonances can be much smaller than the width of the “bare” non-Fermi-liquid resonance at the Fermi level in the banks. The additional scattering due to tunneling induces a transition from the non-Fermi-liquid to the Fermi-liquid state as the separation between the Fermi level in the banks and the two-dimensional band edge in the quantum well varies. Zh. éksp. Teor. Fiz. 114, 1466–1486 (October 1998)     

Possible observation of the quadrupolar Kondo effect in dilute quadrupolar system Pr(x)La(1-x)Pb3 for x <or= 0.05

We have studied non-Fermi-liquid (NFL) behavior in Pr(x)La(1-x)Pb3 with Gamma3 quadrupolar moments in the crystalline-electric-field ground state. The specific heat C/T shows NFL behavior in the very dilute region for x 相似文献   

Photon-drag effect in a two-dimensional electron gas in high magnetic fields

We present the first measurements concerning the photon drag effect in a two-dimensional electron gas based on intersubband transitions in high magnetic fields. It is shown that the excitation mechanism of the drag voltage in a magnetic field differs obviously from the case of zero magnetic field. The longitudinal as well as the Hall drag voltage show strong oscillations around zero when the magnetic field is swept. Both consist of a B-symmetrical and an antisymmetrical part with the same periodicity in B as the magnetoresistanceR_xx. The drag voltage oscillations are strongly correlated to the relative position of Fermi energy and Landau levels and are independent of the photon energy in the range of usable laser lines.     

Spin Excitations in the Field-Induced Phase of the Quasi-One-Dimensional S = 1 Heisenberg Antiferromagnet NDMAP

The S = 1 quasi-one-dimensional Heisenberg antiferromagnet [Ni(C₅H₁₄N₂)₂N₃](PF₆), abbreviated as NDMAP, has been studied by electron spin resonance in a magnetic field above the critical field (H _c). We studied angular and frequency dependences of spin excitations. The angular dependence of the spin excitations in the vicinity of H _c is explained well by a phenomenological field theory, but the agreement between the experiment and the calculation is not satisfactory above 10 T. In high magnetic fields above 15 T, we obtained some characteristic spin excitations which are well explained by conventional antiferromagnetic resonance modes. These results suggest that the spin excitations change from a quantum state to a classical one due to the suppression of quantum fluctuations by high magnetic fields.     

Triangular antiferromagnets with a layered structure in a uniform field

We study the magnetic states and phase transitions in layered triangular antiferromagnets and show that in compounds of the VBr₂ (or VCl₂) type the quantum effects alter the structure of the ground state and initiate a series of transitions as the magnetic field strength is increased. We establish that planar structures with different spin configurations are realized when the magnetic field strength is far from the saturation value, while a nonplanar structure of the umbrella type is realized in fields close to the saturation value. Finally, we build the phase diagram of the ground state and indicate a finite range of field strengths where a collinear phase is possible, too. Zh. éksp. Teor. Fiz. 111, 627–643 (February 1997)     

Soliton wall superlattice charge-density-wave phase in a magnetic field

A model where phase transitions between the Peierls and periodic soliton wall superlattice (SWS) charge-density-wave phases occur in a magnetic field is proposed. The model accounts for the peculiarities of the electron spectrum in a quasi-one-dimensional conductor (Per)₂Pt(mnt)₂. Possible experimental investigations of the theoretically predicted phase transitions in (Per)₂Pt(mnt)₂ to discover a unique SWS phase are discussed. The text was submitted by the authors in English.     

Electron states in quantum-dot and antidot arrays placed in a strong magnetic field

Quantum electronic states in a dot (antidot) array in the presence of a dc magnetic field are studied. A new method of numerical calculation of the electron spectrum and wave functions in a two-dimensional periodic potential and perpendicular magnetic field is proposed. The magnetic-subband energies, density of electron states, and electron density |ψ(x,y)|², as well as the amplitude of the potential, and lattice period and degree of anisotropy for different magnetic fields have been found. The calculations were performed for quantum dots in the In_0.2Ga_0.8As-GaAs and GaAs-Al_0.3Ga_0,7As systems. The rearrangement of the spectrum with variation of magnetic field and with transition from the tight-binding to weak-binding approximation is studied (ω _c is the cyclotron frequency, and V ₀ is the periodic-potential amplitude). The calculations show that the two-dimensional lattices epitaxially grown presently on semiconductor surfaces permit observation of quantum effects associated with rearrangement of the spectrum (electron transport and optical absorption) in magnetic fields H⩽1 MG. Fiz. Tverd. Tela (St. Petersburg) 40, 1134–1139 (June 1998)     

Zeeman effect on the hyperfine structure of the D 1 line of a submicron layer of 87Rb vapor

An extremely thin cell with a wedge gap was developed that makes it possible to form a column of Rb atom vapor with thickness in the range from 100 to 600 nm. It is experimentally shown that the use of this cell, along with commercially available diode lasers, allows one to spectrally resolve individual transitions between the Zeeman sublevels of the hyperfine structure of the ⁸⁷Rb D ₁ line (transitions F _g =1, 2→F _e =1, 2) in the resonance fluorescence spectrum in the presence of an external magnetic field (B≈200 G). This makes it possible to realize systems consisting of nondegenerate atomic levels. For comparison, it is shown that transitions between the Zeeman sublevels in the fluorescence spectrum obtained with the aid of a conventional cell (1–10 cm long) in an external magnetic field with B～200 G remain completely masked by the Doppler-broadened profile. The results obtained can be used for the creation of a simple magnetometer based on an extremely thin cell with Rb vapor for the measurement of magnetic fields with a submicron local spatial resolution.     

Transition in a Luttinger liquid with two-level impurities to the fermi-liquid state

The mechanisms leading to instability of the non-Fermi-liquid state of a Luttinger liquid with two-level impurities are proposed. Since exchange scattering in 1D systems is two-channel scattering in a certain range of parameters, several types of non-Fermi-liquid excitations with different quantum numbers exist in the vicinity of the Fermi level. These excitations include, first, charge density fluctuations in the Luttinger liquid and, second, many-particle excitations due to two-channel exchange interaction, which are associated with band-type as well as impurity fermion states. It is shown that mutual scattering of many-particle excitations of various types leads to the emergence of an additional Fermi-liquid singularity in the vicinity of the Fermi level. The conditions under which the Fermi-liquid state with a new energy scale (which is much smaller than the Kondo temperature) is the ground state of the system are formulated.