Theory of plasmon-assisted transmission of entangled photons

The recent surface plasmon entanglement experiment [Nature (London) 418, 304 (2002)]] is theoretically analyzed. The entanglement preservation upon transmission in the nonfocused case is found to provide information about the interaction of the biphoton and the metallic film. The entanglement degradation in the focused case is explained in the framework of a fully multimode model. This phenomenon is a consequence of the polarization-selective filtering behavior of the metallic nanostructured film. It is shown that the "which-way" labels that degrade entanglement are not located in the degrees of freedom of the metallic film but rather in the spatial degrees of freedom of the photon field.     

Broadband perfect polarization conversion metasurfaces

We propose a broadband perfect polarization conversion metasurface composed of copper sheet-backed asymmetric double spilt ring resonator(DSRR).The broadband perfect polarization convertibility results from metallic ground and multiple plasmon resonances of the DSRR.Physics of plasmon resonances are governed by the electric and magnetic resonances.Both the simulation and measured results show that the polarization conversion ratio(PCR)is higher than 99%for both x-and y-polarized normally incident EM waves and the fractional bandwidth is about 34.5%.The metasurface possesses the merits of high PCR and broad bandwidth,and thus has great application values in novel polarization-control devices.     

Surface plasmon photodetectors and their applications

Surface plasmon photodetectors are of vigorous current interest. Such detectors typically combine a metallic structure that supports surface plasmons with a photodetection structure based on internal photoemission or electron‐hole pair creation. Detector architectures are highly varied, involving surface plasmons on planar metal waveguides, on metal gratings, on nano‐particles, ‐islands, or ‐antennas, or involving plasmon‐mediated transmission through one or many sub‐wavelength holes in a metal film. Properties inherent to surface plasmons, such as sub‐wavelength confinement and their ability to resonate on tiny metallic structures, are exploited to convey useful characteristics to detectors in addressing applications such as low‐noise high‐speed detection, single‐plasmon detection, near‐ and mid‐infrared imaging, photovoltaic solar energy conversion, and (bio)chemical sensing. The operating principles behind surface plasmon detectors are reviewed, the literature on the topic is surveyed, and avenues that appear promising are highlighted.     

Dual-broadband and near-perfect polarization converter based on anisotropic metasurface

A novel dual-broadband and near-perfect reflective polarization converter based on anisotropic metasurface is presented and analyzed in this paper. The unit cell of the proposed converter is composed of a double-cut slotted metallic split-ring and a metallic ground sheet separated by an F4B-2 substrate. Both numerical analysis and measured results demonstrate that the proposed converter has five plasmon resonance frequencies, and can near-completely convert the x- or y-polarized incident wave to its orthogonal counterpart in two frequency bands (9.5–12.9 GHz, 16.1–20.2 GHz). The corresponding polarization conversion ratio is more than 98.3% in the first frequency band and 99.7% in the second one. In addition, the bandwidths and central frequencies of the two frequency bands can be effectively tuned over a wide range by adjusting the geometrical dimensions of the metasurface, while the high conversion efficiency is preserved. The proposed polarization converter may have great potentials in electromagnetic polarization control applications.     

Ultra-broadband and high-efficiency polarization conversion metasurface with multiple plasmon resonance modes

In this paper, we present a novel metasurface design that achieves a high-efficiency ultra-broadband cross polarization conversion. The metasurface is composed of an array of unit resonators, each of which combines an H-shaped structure and two rectangular metallic patches. Different plasmon resonance modes are excited in unit resonators and allow the polarization states to be manipulated. The bandwidth of the cross polarization converter is 82% of the central frequency,covering the range from 15.7 GHz to 37.5 GHz. The conversion efficiency of the innovative new design is higher than 90%.At 14.43 GHz and 40.95 GHz, the linearly polarized incident wave is converted into a circularly polarized wave.     

Fano resonances in dipole-quadrupole plasmon coupling nanorod dimers

We theoretically investigate the plasmon coupling in metallic nanorod dimers. A pronounced dip is found in the extinction spectrum due to plasmonic Fano resonance, which is induced by destructive interference between the bright dipole plasmon of a short nanorod and the dark quadrupole plasmon of a long nanorod. This Fano interference can also be explained as the coupling between the bright and dark modes both supported by the whole dimer. The Fano resonance can be tuned by adjusting the spatial or spectral separation between two nanorods in the dimer.     

Sidebands in the light absorption of driven metallic nanoparticles

The dynamics of the surface plasmon in laser-driven metallic nanoparticles is described by means of a master-equation formalism. Within the Markov approximation, the dynamics is studied for different regimes ranging from weak excitation in photoabsorption experiments to strong excitation in pump-probe spectroscopy. It is shown that two collective levels are sufficient to describe the dynamics of the surface plasmon. On this basis, we predict the appearance of sidebands in the absorption spectrum of the probe laser field in pump-probe experiments.     

Terahertz plasmon and surface-plasmon modes in cylindrical metallic nanowires

We present a theoretical study on collective excitation modes associated with plasmon and surface-plasmon oscilla- tions in cylindrical metallic nanowires. Based on a two-subband model, the dynamical dielectric function matrix is derived under the random-phase approximation. An optic-like branch and an acoustic-like branch, which are free of Landau damp- ing, are observed for both plasmon and surface-plasmon modes. Interestingly, for surface-plasmon modes, we find that two branches of the dispersion relation curves converge at a wavevector qz = qrnax beyond which no surface-plasmon mode exists. Moreover, we examine the dependence of these excitation modes on sample parameters such as the radius of the nanowires. It is found that in metallic nanowires realized by state-of-the-art nanotechnology the intra- and inter-subband plasmon and surface-plasmon frequencies are in the terahertz bandwidth. The frequency of the optic-like modes decreases with increasing radius of the nanowires, whereas that of the acoustic-like modes is not sensitive to the variation of the radius. This study is pertinent to the application of metallic nanowires as frequency-tunable terahertz plasmonic devices.     

The nanoparticle shape's effect on the light scattering cross-section

In the framework of kinetic approach we develop a theory for light scattering by ellipsoidal metallic nanoparticles whose dimensions are less than those of a free electron path. In this case, the surface of the particle starts to play a dominant role in electron scattering. When the size of the particle decreases below the free electron path at least in one direction, the optical conductivity becomes a tensor quantity, and the diagonal components of this tensor define the half-widths of the plasmon resonances peaks. Thus, the effect of the particles' shape both on the frequencies of plasmon resonances and on their half-widths is considered. Additionally, the expression for a cross-section of the light scattering by a collection of chaotically oriented spheroidal nanoparticles is obtained and averaged over different directions of particles in the collection. Our results highlight the plasmonic properties of metallic nanospheroids, notably, the spectrum of the light scattering has two peaks at the frequencies of plasmon resonances even if there is no preferential direction in the collection of particles.     

A Kirchhoff solution to plasmon hybridization

Using Ohm’s law, a solution to plasmon hybridization via Kirchoff’s equations results in a simple and intuitive picture of a metal nanoparticle dimer as a capacitively coupled circuit. Calculated absorption spectra and surface charge densities show that dimers of different metallic composition support different super- and sub-radiant plasmons compared to homodimers. Strong screening of Coulomb interactions between nanoparticles of different metallic background prohibits the excitation of anti-bonding plasmons, while changes to the free electron conductivity upon a collective response result in coupled plasmon lifetimes which shift as a function of interparticle distance. Smaller separations then result in the longest lived plasmons.     

Controlling the optical spectra of gold nano-islands by changing the aspect ratio and the inter-island distance: theory and experiment

The extinction spectrum of a dielectric film with periodic array of metallic islands of different shapes and different mutual distances was studied both theoretically and experimentally. It is shown, analytically, numerically and experimentally, that the positions of the surface plasmon resonances depend on the nano-structural details. We propose two ways of controlling plasmon resonance frequency: changing the aspect ratio of the elliptical (or rectangular) islands and changing their mutual distances. A new analytical asymptotic approach for calculating the optical properties of such plasmonic systems is developed. The results of our analytical and numerical studies are in good qualitative agreement with experiment.     

基于厚金属狭缝阵列的表面等离子激元光刻

提出一种利用厚金属狭缝阵列耦合激发表面等离子激元制作非周期图形的纳米光刻模型.采用时域有限差分电磁场模拟仿真软件研究了厚金属狭缝阵列中表面等离子激元的激发、模式选择以及光刻胶中的光场分布.结果表明,通过优化厚金属狭缝阵列结构参量和匹配介质参量可有效抑制表面等离子激元在光栅狭缝出口处的发散,增加表面等离子激元的穿透深度,可获得高分辨率的较大曝光深度的周期和非周期纳米图形,可为纳米激光直写技术提供有益的借鉴.     

Efficient miniature circular polarization analyzer design using hybrid spiral plasmonic lens

The spin dependence of the focusing behavior of a spiral slot plasmonic lens can be utilized for a miniature circular polarization analyzer. However, the azimuthal polarization component of the incident circular polarization does not contribute to surface plasmon excitation and focusing because it is TE polarized with respect to the spiral slot. In this Letter, a hybrid metallic lens that consists of alternating spiral triangle array and spiral slot is designed to improve the plasmonic coupling efficiency. The spiral triangle array is responsible for coupling the azimuthal polarization component into surface plasmon. Numerical studies show that the field enhancement at the focus and power conversion efficiency can be increased by 39.53% and 94.69% compared to that of pure spiral slot plasmonic lens.     

级联亚波长平面介质栅偏振分束器研究

提出了一种纳米厚度金属层连接的级联亚波长平面介质光栅三明治结构,利用该结构中纳米金属连接层上下界面处的表面等离子共振的互作用形成多波长共振的特点设计了适用于光通信波段（1 300～1 600nm）高性能的宽带偏振器和宽带偏振分束器。利用严格耦合波理论分析发现偏振分束器带宽主要由金属连接层厚度控制,光栅厚度基本不影响偏振分束器带宽,只影响共振深度和共振波长。该结论为后续的制备提供了理论指导和借鉴作用。     

Negative role of surface plasmons in the transmission of metallic gratings with very narrow slits

It is generally admitted that the extraordinary transmission of metallic grating with very narrow slits is mainly due to the excitation of surface plasmons on the upper and lower interfaces of the grating. We show that the surface plasmon contribution is not the prime effect and that waveguide mode resonance and diffraction are responsible for the extraordinary transmission. Additionally and surprisingly, we reveal that the transmittance of subwavelength metallic gratings is always nearly zero for frequencies corresponding to surface plasmon excitation. This finding implies that surface plasmons play a negative role in the transmission.     

Enhanced transmission through periodic arrays of subwavelength holes: the role of localized waveguide resonances

By using the rigid full-vectorial three-dimensional finite-difference time-domain method, we show that the enhanced transmission through a metallic film with a periodic array of subwavelength holes results from two different resonances: (i) localized waveguide resonances where each air hole can be considered as a section of metallic waveguide with both ends open to free space, forming a low-quality-factor resonator, and (ii) well-recognized surface plasmon resonances due to the periodicity. These two different resonances can be characterized from electromagnetic band structures in the structured metal film. In addition, we show that the shape effect in the enhanced transmission through the Au film with subwavelength holes is attributed to the localized waveguide resonance.     

Enhanced light transmission through cascaded metal films perforated with periodic hole arrays

We report experimental results on enhanced light transmission through two periodically perforated metal films separated by a layer of dielectric. A perforated metal film (single metallic structure) exhibits extraordinary optical transmission, and when two such perforated metal films are spaced by a dielectric layer (cascaded metallic structure), the transmission is further increased. The maximum transmission of the cascaded metallic structure, which depends on the distance between the two metal films, can be more than 400% greater than that of a corresponding single metallic structure. It is proposed that the coupling of surface plasmon polaritons between the two metal films is involved in the process.     

Photoemission from multiply excited surface plasmons in Ag nanoparticles

Two-photon photoemission spectroscopy using femtosecond laser pulses is used to investigate the excitation and decay mechanisms of the surface plasmon resonance in Ag nanoparticles grown on graphite. The resonant excitation of this collective excitation leads to a two-orders-of-magnitude-enhanced two-photon photoemission yield from a graphite surface with Ag nanoparticles compared to the yield from pure graphite. From the shape of the photoemission spectra, the polarization dependence of the photoemission yield and the excitation probabilities for different excitation pathways we conclude that excitation with 400-nm femtosecond laser pulses leads to the coherent multiple excitation of the surface plasmon in the Ag nanoparticles. This multiply excited plasmon mode can decay via the coupling to a single-particle excitation leading to the emission of an electron if its final state is located in the continuum. The surface plasmon in metallic nanoparticles is a model system to investigate collective excitations in multiphoton processes. Received: 26 June 2000 / Accepted: 2 September 2000 / Published online: 12 October 2000     

A high figure of merit localized surface plasmon sensor based on a gold nanograting on the top of a gold planar film

We investigate the sensitivity and figure of merit （FOM） of a localized surface plasmon （LSP） sensor with gold nanograting on the top of planar metallic film. The sensitivity of the localized surface plasmon sensor is 317 nm/RIU, and the FOM is predicted to be above 8, which is very high for a localized surface plasmon sensor. By employing the rigorous coupled-wave analysis （RCWA） method, we analyze the distribution of the magnetic field and find that the sensing property of our proposed system is attributed to the interactions between the localized surface plasmon around the gold nanostrips and the surface plasmon polarition on the surface of the gold planar metallic film. These findings are important for developing high FOM localized surface plasmon sensors.     

金属表面等离体子振荡

深入浅出地分析了金属表面等离体子振荡形成的机理，利用拉普拉斯方程得到了半无限金属、金属薄膜和球状纳米金属颗粒的表面等离体子振荡频率。