Motion of domain walls under the action of spin-polarized current in a magnetic junction

The effect of spin-polarized current on a domain structure in a magnetic junction consisting of two ferromagnetic metallic layers separated by an ultrathin nonmagnetic layer is studied within a phenomenological theory. The magnetization of one ferromagnetic layer (layer 1) is assumed to be fixed, while that of the other ferromagnetic layer (layer 2) can be freely oriented both parallel and antiparallel to the magnetization of layer 1. Layer 2 can be split into domains. Charge transfer from layer 1 to layer 2 is not attended with spin scattering by the interface but results in spin injection. Due to s-d exchange interaction, injected spins tend to orient the magnetization in the domains parallel to layer 1. This causes the domain walls to move and “favorable” domains to grow. The average magnetization current injected into layer 2 and its contribution to the s-d exchange energy are found by solving the continuity equation for carriers with spins pointing up and down. From the minimum condition for the total magnetic energy of the junction, the parameters of the periodic domain structure in layer 2 are determined as functions of current through the junction and magnetic field. It is shown that the spin-polarized current can magnetize layer 2 up to saturation even in the absence of an external magnetic field. The associated current densities are on the order of 10⁵ A/cm². In the presence of the field, its effect can be compensated by such a high current. Current-induced magnetization reversal in the layer is also possible.     

Anomalous magnetic behaviour of zinc and chromium ferrites without any hyperfine splitting

Two groups of ferrite namely zinc ferrite and chromium ferrite were synthesized by citrate precursor route in the size range of 8 to 35 nm. We have studied the structural and magnetic behaviour of these ferrites using X-ray diffraction (XRD), vibrating sample magnetometer (VSM) and Mössbauer spectroscopic techniques. Our studies show that the nanocrystalline ferrites interact with the hand magnet strongly and give large magnetization in the VSM measurement. The maximum magnetization in the samples sensitively depends on the particle size of synthesized ferrites. We observed as large as 28 Am²/kg of magnetization in the zinc ferrite nanoparticles while that in chromium ferrite is around 11 Am²/kg. In spite of the large magnetization in the zinc ferrite nanoparticles we did not observe any hyperfine splitting even down to 12 K of temperature. Similar behaviour is also observed for chromium ferrite down to 16 K.     

The magnetic barkhausen effect

When the magnetization of a ferromagnet (in this paper “ferromagnet” will often include “fernmagnet”) is changed under the influence of an applied magnetic field, the magnetization, particularly in the vicinity of the coercive force, is not smooth function of the field but rather shows a structure composed of many individual steps. This structure is evidence of irreversible changes in magnetization and is known as the barkhausen effect. The effect was named after its discoverer who, in 1919, connected a coil surrounding a ferromagnet to a newly invented amplifier and listened to the output of the amplifier with earphones.¹     

Preparation and characterization of magnetic nanoparticles with controlled magnetization

The effect of molar ratio of two hydrated iron salts used as precursors into a (co)precipitation-based synthesis method, on the composition, size and specific saturation magnetization of mixed iron oxides and oxyhydroxides magnetic nanoparticles as reaction products, was studied. The preparation procedure is based on a salt-assisted solid-state chemical reaction. The obtained products are magnetic multiphase components with the mean size ranging from 3 to 10 nm and specific saturation magnetization between 25 and 95.5 emu/g. The specific saturation magnetization modifies in a non-linear manner as the molar ratio of the iron salts varies. Excepting one sample, for which Fe²⁺/Fe³⁺ molar ratio was zero, all magnetic nanoparticles show a ferrofluid-like behaviour in the colloidal form. The small size, ferrofluid-like behaviour, and controlled specific saturation magnetization allow the use of new synthesized nanoparticles in specific biomedical or industrial applications.     

Behavior of the magnetic subsystems in Nd2BaNiO5

The temperature dependences of the heat capacity, the magnetic susceptibility, and the splitting of the ground Kramers doublet of the Nd³⁺ ion in the chain magnet Nd₂BaNiO₅ are studied. An antiferromagnetic phase transition manifests itself as anomalies in all these dependences. The parameters of the Nd-Ni and Nd-Nd interactions are estimated. The field dependence of the magnetization has two anomalies. A strong magnetic anisotropy prevents the magnetic moments of the Nd³⁺ ion from deviating from axis c in the crystal even in an external magnetic field. The processes of magnetization and the internal specific features of a chain of spins S = 1 are discussed.     

Peculiarities of the inverse Faraday effect induced in iron garnet films by femtosecond laser pulses

The inverse Faraday effect in iron garnet films subjected to femtosecond laser pulses is experimentally investigated. It is found that the magnitude of the observed effect depends nonlinearly on the energy of the optical pump pulses, which is in contradiction with the notion that the inverse Faraday effect is linear with respect to the pump energy. Thus, for pump pulses with a central wavelength of 650 nm and an energy density of 1 mJ/cm², the deviation from a linear dependence is as large as 50%. Analysis of the experimental data demonstrates that the observed behavior is explained by the fact that the optically induced normal component of the magnetization is determined, apart from the field resulting from the inverse Faraday effect, by a decrease in the magnitude of the precessing magnetization under the influence of the femtosecond electromagnetic field.     

Surface effects on saturation magnetization in nanoporous Ni

Nanoporous Ni specimens with ligament lengths of 10–210 nm and specific surface areas of 0.03–0.58 nm^?1 were fabricated by the dealloying of Ni_0.25Mn_0.75 alloy and annealing at 473–873 K, and saturation magnetization investigated in terms of their size dependence. Saturation magnetization decreased with decreasing ligament length or increasing specific surface area. This trend is the same as that for nanoparticle Ni. However, the saturation magnetization of nanoporous Ni tends to be lower than that of the nanoparticle Ni when their specific surface areas are the same. It is suggested, therefore, that the surface effect due to a noncollinear arrangement is enhanced by the surface defects in the nanoporous Ni.     

Mössbauer and magnetic studies of nanocrystalline zinc ferrites synthesized by microwave combustion method

Zinc ferrite nano-crystals were synthesized by a microwave assisted combustion route with varying the urea to metal nitrates (U/N) molar ratio The process takes only a few minutes to obtain Zinc ferrite powders. The Effect of U/N ratio on the obtained phases, particle size, magnetization and structural properties has been investigated. The specimens were characterized by XRD, Mössbauer and VSM techniques. The sample prepared with urea/metal nitrate ratio of 1/1 was a poorly crystalline phase with very small crystallite size. A second phase is also detected in the sample. The crystallite size increases while the second phase decrease with increasing the urea ratio. The saturation magnetization and coercivity of the as prepared nano-particles changed with the change of the U/N ratio. The powder with the highest U/N ratio showed the presence of an unusually high saturation magnetization of 16 emu/g at room temperature. The crystallinity of the as prepared powder was developed by annealing the samples at 700 ^°C and 900 ^°C. Both the saturation magnetization (Ms) and the remnant magnetization (Mr) were found to be highly dependent upon the annealing temperature. Mössbauer studies show magnetic ordering in the powder even at room temperature. The Mössbauer and the magnetic parameters of this fraction are different from the standard values for bulk zinc ferrite.     

Magnetic properties of CoFeRu alloys in the f.c.c. and h.c.p. phases

Measurements have been made of the magnetization, the Fe⁵⁷ Mössbauer effect, and the crystal structures of Co-rich CoFeRu alloys. The alloys with f.c.c. structure behave in a typical ferromagnetic way, while those with h.c.p. structure show non-saturation of the magnetization in magnetic fields as high as 80 kG, and they show relatively small magnetic moments per atom and a broad single Mössbauer absorption.     

Direction of magnetization and domain wall mobility in (Dy,Y)Fe2

Magnetization measurements in the (Dy _x Y_1−x )Fe₂ intermetallic compounds show evidence of blocking of domain wall motion. This effect is a function of concentrationx. The direction of magnetization is also dependent on the Dy concentration. We have used the Mossbauer spectroscopy of⁵⁷Fe to verify the direction of magnetization in the series as a function ofx and temperature. The results show that this change in easy direction occurs at higher temperatures than those where the blocking is detected through DC magnetization measurements. supported by RHAE/SCT.     

Magnetic property of pyrolytic carbon prepared on diamond powder in applied magnetic field

We have prepared pyrolytic carbon samples from triethylamine on diamond powder in applied magnetic field of 6 T and investigated their magnetic properties. A ferromagnetic sample was obtained from the pyrolysis products even at room temperature, with spontaneous magnetization of 6.4 A m²/kg at 300 K, which is twice as large as that of the sample prepared without diamond powder. Therefore, the diamond powder seems to promote the formation of a three-dimensional ferromagnetic structure in pyrolytic carbon.     

Dynamics of paramagnetic agents by off-resonance rotating frame technique in the presence of magnetization transfer effect

The simple method for measuring the rotational correlation time of paramagnetic ion chelates via off-resonance rotating frame technique is challenged in vivo by the magnetization transfer effect. A theoretical model for the spin relaxation of water protons in the presence of paramagnetic ion chelates and magnetization transfer effect is described. This model considers the competitive relaxations of water protons by the paramagnetic relaxation pathway and the magnetization transfer pathway. The influence of magnetization transfer on the total residual z-magnetization has been quantitatively evaluated in the context of the magnetization map and various difference magnetization profiles for the macromolecule conjugated Gd-DTPA in cross-linked protein gels. The numerical simulations and experimental validations confirm that the rotational correlation time for the paramagnetic ion chelates can be measured even in the presence of strong magnetization transfer. This spin relaxation model also provides novel approaches to enhance the detection sensitivity for paramagnetic labeling by suppressing the spin relaxations caused by the magnetization transfer. The inclusion of the magnetization transfer effect allows us to use the magnetization map as a simulation tool to design efficient paramagnetic labeling targeting at specific tissues, to design experiments running at low RF power depositions, and to optimize the sensitivity for detecting paramagnetic labeling. Thus, the presented method will be a very useful tool for the in vivo applications such as molecular imaging via paramagnetic labeling.     

Entanglement spectrum and magnetization plateaus in an S = 1 bond-alternative Heisenberg chain with single-ion anisotropy and magnetic field

Entanglement spectrum and quantum phase transitions (QPTs) in S = 1 bond-alternative antiferromagnetic Heisenberg chain with single-ion anisotropy and magnetic field are investigated by the infinite time-evolving block decimation (iTEBD) method. The combined effects of the single-ion anisotropy and magnetic field have been discussed, and a rich ground-state phase diagram is obtained. We find that the single-ion anisotropy is advantageous to the stability of the 1/2 magnetization plateau. Both entanglement entropy and entanglement spectrum, as two model-independent measures, are capable of describing all the QPTs. Especially, doubly degenerate entanglement spectrum on even bond is observed in the 1/2 plateau phase. Besides constant spontaneous magnetization, three magnetization plateaus (M ^z = 0, 1/2, and 1) are found to have constant entanglement entropy, entanglement spectrum, and nearest-neighbor correlation. In addition, all the QPTs in such a model have been determined to belong to the second-order category.     

Variation of the saturation magnetization through a neon implanted YIG film

The saturation magnetization of a YIG film implanted with 5*10¹⁴ neon ions/cm² at an energy of 450 keV was studied. By removing very thin layers from the ion implanted part of the film the magnetization was found to change. As a result of the analysis of these changes in the saturation magnetization it was possible to establish a profile for the magnetization as a function of depth through the ion implanted part of the film. The profile is asymmetric and shows a decrease in the magnetization of up to 35 % of the initial value at a depth coinciding with the depth of maximum strain.     

Photomagnetic effect in molecular magnets based on nitrosyl complexes of ruthenium and rare-earth ions

The magnetic properties of new bifunctional molecular magnets based on nitrosyl complexes of ruthenium and thiacalix[4]arenes of rare-earth ions (Gd³⁺, Dy³⁺) have been investigated. A photoinduced decrease in the magnetization of the molecular magnet with rare-earth ions Gd³⁺ and the absence of a photomagnetic effect in crystals with rare-earth ions Dy³⁺ have been revealed at a temperature of 2 K. It has been found that, in the sample containing Dy³⁺ ions, the magnetization deviates by 6% from the calculated value for noninteracting ions. A comparison of the results obtained for two groups of isostructural samples, which differ only in the type of rare-earth ions, has demonstrated that the observed deviation of the magnetization is caused by the interaction of the orbital moment of the Dy³⁺ ions with the crystal field.     

Photocontrol of magnetization in Al-substituted Fe3O4 thin films

Thin films of (111)-oriented spinel ferrite Al_0.5Fe_2.5O₄ have been prepared by a pulsed-laser deposition (PLD) technique on α-Al₂O₃ (0001) substrates. The films exhibit cluster-glass behaviors with a spin-freezing temperature, T_g, near or above room temperature. The magnetization was found to increase following light irradiation below T_g, which indicates the photoinduced melting of cluster-glass states. An analysis comparing the dynamic behavior of magnetic response to light irradiation between zero-field-cooled (ZFC) states and field-cooled (FC) states at 10 K under various light intensities, I, revealed that the direct photoexcitation of spins occurs when I≤0.78 mW/mm², while the thermal heating effect following the light absorption of the samples also contributes to the enhancement of magnetization when I≥1.22 mW/mm². The magnetization of the films could be controlled by light irradiation even at room temperature. This suggests the possibility of utilizing these films in the development of novel magneto-optical memory devices.     

Effect of conduction electrons on the law of approach to saturation of a metallic ferromagnet with surface pinning of the magnetic moment

The effect of conduction electrons on the magnetization curve of a metallic ferromagnet with surface pinning of the magnetic moment is investigated theoretically. The electronic contribution is due to the rearrangement of the discrete spectrum of charge carriers trapped by the nonuniform magnetic induction of such a ferromagnet, and it is a kind of diamagnetic effect that appreciably decreases the volume-averaged magnetization of the ferromagnet. A powerlaw dependence H ^−3/4 on the external magnetic field H is obtained according to the law of magnetization approach to saturation. This dependence is due to the contribution of the conduction electrons. Fiz. Tverd. Tela (St. Petersburg) 41, 647–653 (April 1999)     

Mössbauer and magnetization measurements on two ferromagnetic alloys containing 119Sn

¹¹⁹Sn Mössbauer effect and magnetization measurements have been performned at temperatures between 4.2 and 700°K on an invar alloy (35.8 at.% NiFe) and ordered FeCo containing tin. The Mössbauer results are shown to be consistent with a model in which interionic separation is important to the hyperfine interaction. The magnetization measurements on the invar alloy reflect its sensitive magnetic properties.     

Theoretical and experimental study of Fe/Cr nanometric quasiperiodic multilayers

An experimental and theoretical study of magnetization curves of Fe/Cr nanometric magnetic films grown with the structure of the quasiperiodic Fibonacci sequence is presented. Fe ferromagnetic films with interfilm exchange coupling provided by intervening Cr non-ferromagnetic layers were grown on MgO (100) by dc magnetron sputtering at 300 ^°C. The magnetization curves were investigated using the magneto-optical Kerr effect with the external field applied along the easy axis. The theoretical approach for this system is based on a realistic phenomenological model that includes the following contributions to free magnetic energy: Zeeman, cubic magneto-crystalline anisotropy, as well as bilinear and biquadratic exchange energies. Our numerical results are in very good agreement with the experimental data.     

相对论简并电子气体的磁化

中子星内部的致密电子是高度简并的相对论气体, 其输运性质与中子星磁或热的观测现象密切相关, 被认为是中子星磁场的主要载体. 外磁场中电子的朗道能级是分立的且高度简并的, 与无外场时的能量差决定 了系统的磁化程度, 用量子统计的方法可计算理想相对论电子气体的磁化率. 结果表明弱场条件下的磁化率在数量级上接近白矮星的10^-3. 强磁场下的磁化呈现出类似在某些低温金属中出现的de Haas-van Alphen 震荡效应, 高次谐频的震荡幅度有可能超出临界磁化时的磁化率. 表明中子星内部有可能存在非稳定的磁化过程, 发生类似气液转化的一级相变过程, 出现两种磁化共存的稳定态或过冷磁化的亚稳态(若不同磁化态间存在表面能). 从亚稳态向稳定态的突然转化可能与磁星的辐射有关, 可以解释在磁星巨闪过程中观测到的额外辐射问题.