Time‐resolved photoelectron spectroscopy using synchrotron radiation time structure

Synchrotron radiation time structure is becoming a common tool for studying dynamic properties of materials. The main limitation is often the wide time domain the user would like to access with pump–probe experiments. In order to perform photoelectron spectroscopy experiments over time scales from milliseconds to picoseconds it is mandatory to measure the time at which each measured photoelectron was created. For this reason the usual CCD camera‐based two‐dimensional detection of electron energy analyzers has been replaced by a new delay‐line detector adapted to the time structure of the SOLEIL synchrotron radiation source. The new two‐dimensional delay‐line detector has a time resolution of 5 ns and was installed on a Scienta SES 2002 electron energy analyzer. The first application has been to characterize the time of flight of the photoemitted electrons as a function of their kinetic energy and the selected pass energy. By repeating the experiment as a function of the available pass energy and of the kinetic energy, a complete characterization of the analyzer behaviour in the time domain has been obtained. Even for kinetic energies as low as 10 eV at 2 eV pass energy, the time spread of the detected electrons is lower than 140 ns. These results and the time structure of the SOLEIL filling modes assure the possibility of performing pump–probe photoelectron spectroscopy experiments with the time resolution given by the SOLEIL pulse width, the best performance of the beamline and of the experimental station.     

利用同步辐射光电子能谱技术测量ZnO/PbTe异质结的能带带阶

异质结结构界面的能带带阶是一个非常重要的参数,该参数的精确确定直接影响异质结的光电性质研究以及异质结在光电器件上的应用.利用同步辐射光电子能谱技术测量了ZnO/PbTe异质结结构的能带带阶.测量得到该异质结价带带阶为2.56 eV,导带带阶为0.49 eV,是一个典型的类型I的能带排列.利用变厚度扫描的测量方法发现,ZnO/PbTe界面存在两种键,分别是Pb—O键(低结合能)和Pb—Te键(高结合能).在ZnO/PbTe异质结界面的能带排列中导带带阶较小,而价带带阶较大,这一能带结构有利于PbTe中的激发电子输运到ZnO导电层中.该类结构在新型太阳电池、中红外探测器、激光器等器件中具有潜在的应用价值.     

北京同步辐射装置上的位相衬度成像

在北京同步辐射装置上首次用位相衬度成像方法对生物样品和复合材料进行研究,得到了非常清晰而精细的材料内部细观结构.其图像的清晰度和分辨率明显地优于吸收衬度成像 关键词： 位相衬度成像 相干光源 同步辐射硬X射线     

同步辐射软X射线显微成像

软X射线显微成像是同步辐射最主要的应用之一,本文简明介绍软X射线显微成像的衬度机制,光源,成像方法和一些应用结果。     

甲胺分子的同步辐射光电离解离质谱

在超声射流冷却条件下,利用同步辐射光源,结合飞行时间质谱对CH3NH2分子在60—140nm波长范围内的光电离解离进行了研究.主要动力学过程为母体离子的解离过程.CH2NH2+和CH3+由CH3NH2+在高能量时解离生成,而CH2NH2+的1,1脱H2过程则产生其他离子.CH3NH2分子的电离势(IP)为916±001eV,和分子轨道能量计算的理论值符合得非常好,并获得CH3NH2+和CH2NH2+的生成热分别为860±05kJmol和7541kJmol. 关键词： 同步辐射光电离 飞行时间质谱 电离势 生成热     

Physics design of SSRF synchrotron radiation security

High brightness of SSRF brings about synchrotron radiation security problems, which will be solved in physics design. The main radiations are generated from bending magnets and insertion devices. Since the fact that radiation power and radiating area are different in these two kinds of synchrotron radiation, the arrangements of photon absorbers, diaphragms and other vacuum components need to be treated distinctively. In addition, SSRF interlock protection threshold is defined and the beam orbit in the straight line is limited. Hence, beam orbit in the bending magnets and IDs are also restricted by the threshold. The orbit restriction is calculated and helps us to arrange the vacuum components. In this paper, beam orbit distortion restricted by interlock protection threshold, radiation power, radiation angle and illuminating area are calculated. From the calculation results, the physics designs in manufacture and installation vacuum components are put forward. By commissioning, it is shown that physics requirements are met rigidly in the engineering process.     

同步辐射探测器的应用与发展

探测器是同步辐射实验的重要环节。探测器水平必须不断提高才能适应同步辐射发展的需求，最大限度地发挥先进光源为人类研究提供的强大支持作用。文章介绍了当前同步辐射实验中普遍使用的各种探测器的原理和特点，并就一些新型探测器的发展情况进行了阐述。     

同步辐射探测器的应用与发展

探测器是同步辐射实验的重要环节。探测器水平必须不断提高才能适应同步辐射发展的需求,最大限度地发挥先进光源为人类研究提供的强大支持作用。文章介绍了当前同步辐射实验中普遍使用的各种探测器的原理和特点,并就一些新型探测器的发展情况进行了阐述。     

上海光源同步辐射空间干涉仪研制

研制了上海光源同步辐射空间干涉仪,用于储存环束团横向截面尺寸及发射度的精确测量。对干涉仪工艺设计中的光路参数、关键设备选型、数据处理方法及数据采集处理软件结构进行了分析讨论。结合束流实验完成了系统调试及运行参数优化,结果表明,CCD增益系数与曝光时间设置对测量精度有显著影响,增益系数设为0 dB,曝光时间设为200 ms时,随机测量误差可控制在μm量级。对上海光源储存环横向束斑尺寸进行了精确测量,结果表明:空间相干度曲线近似为高斯分布,可以采用单一空间频率的相干度测量值进行快速束斑尺寸计算;水平束斑尺寸实测值为52.4 μm,与理论值预期值53.0 μm相比,差异小于2%;系统测量误差约为5.5%,主要误差来源为相干度随机测量误差。     

高压下的同步辐射能量色散粉末衍射

 同步辐射已经成为高压研究的一个非常理想的光源。在北京同步辐射装置（BSRF）上、结合金刚石对顶砧超高压实验技术建立起来的能量色散X射线粉末衍射系统,已用于物质状态方程和结构相变的研究。介绍了能量色散衍射方法,以及同步辐射原位测试过程。     

Physics design of SSRF synchrotron radiation security

High brightness of SSRF brings about synchrotron radiation security problems, which will be solved in physics design. The main radiations are generated from bending magnets and insertion devices. Since the fact that radiation power and radiating area are different in these two kinds of synchrotron radiation, the arrangements of photon absorbers, diaphragms and other vacuum components need to be treated distinctively. In addition, SSRF interlock protection threshold is defined and the beam orbit in the straight line is limited. Hence, beam orbit in the bending magnets and IDs are also restricted by the threshold. The orbit restriction is calculated and helps us to arrange the vacuum components. In this paper, beam orbit distortion restricted by interlock protection threshold, radiation power, radiation angle and illuminating area are calculated. From the calculation results, the physics designs in manufacture and installation vacuum components are put forward. By commissioning, it is shown that physics requirements are met rigidly in the engineering process.     

Ar?NO团簇的同步辐射光电离研究

利用国家同步辐射实验室合肥光源的真空紫外同步辐射，使NO分子和Ar原子混合物的超声分子束发生光电离，测量了Ar，NO和异类团簇Ar·NO的光电离效率谱. 在谱中，在与Ar原子的共振线对应的能量区域(11.5—12.0 eV)观察到一个强的类共振结构. 这个结果表明，在异类团簇Ar·NO的内部，稀有气体Ar原子的激发能转移到与它接触的分子NO上，使分子NO发生电离. 关键词： Ar·NO团簇 同步辐射 光电离 能量转移     

同步辐射的相对论推导

根据加速带电粒子在与其瞬时对静止的参考系中的辐射公式,通过场的相对论变换,直接导出同步辐射粒子的辐射公式。     

等离子体中相对论电子的同步曲率辐射特性研究

根据同步曲率辐射理论推导了在等离子体环境中,不同磁场条件下的相对论性电子的吸收系数和发射系数表达式，计算了电子的发射强度，并且在此基础上研究了同步曲率辐射机制的脉泽效应.研究了两种磁场位型，第一种是强度均匀但弯曲的磁场，第二种是偶极磁场，结果发现了一些偶极磁场下特有的辐射特性.考虑到在天体的环境下电子具有的不同的能谱分布，分别选用了三种典型的能谱分布(幂率分布，高斯分布，热分布)进行了研究，通过计算负吸收和脉泽放大效应在发射强度上的表现后， 发现在某些天体物理环境中，同步曲率辐射在等离子体中的确存在脉泽放大效应.这些研究结果对太阳系中行星外层辐射的研究和宇宙中的射电高亮温度等问题的研究可能提供有益的帮助. 关键词： 同步曲率辐射 负吸收 脉泽效应     

A system for low field imaging of laser-polarized noble gas

We describe a device for performing MRI with laser-polarized noble gas at low magnetic fields (<50 G). The system is robust, portable, inexpensive, and provides gas-phase imaging resolution comparable to that of high field clinical instruments. At 20.6 G, we have imaged laser-polarized (3)He (Larmor frequency of 67 kHz) in both sealed glass cells and excised rat lungs, using approximately 0.1 G/cm gradients to achieve approximately 1 mm(2) resolution. In addition, we measured (3)He T(2)(*) times greater than 100 ms in excised rat lungs, which is roughly 20 times longer than typical values observed at high ( approximately 2 T) fields. We include a discussion of the practical considerations for working at low magnetic fields and conclude with evidence of radiation damping in this system.     

激光冷却获得高亮度的亚稳态惰性气体原子束和原子阱

高强度的亚稳态惰性原子束流在原子分子物理实验研究中具有广泛的应用.使用射频电离方法和激光横向冷却技术制备了高强度的亚稳态氪原子束流,并使用数值模拟方法对横向冷却激光场中的原子径迹进行了分析.通过激光诱导荧光光谱方法测量原子束的束流特性,结果显示,横向冷却后在束流源下游230 cm处的原子束流强度达1.6atoms/(s*sr),束流强度提高了两个量级.利用这种高强度原子束流,我们成功囚禁了1.3×10¹⁰个亚稳态⁸⁴Kr原子,同时冷原子装载速率达到了3.0×10¹¹atoms/s;并利用该装置成功地实现了高亮度的亚稳态氩原子束和原子阱. 关键词： 横向冷却 原子束 原子阱 惰性气体     

Investigation of GEM-Micromegas detector on X-ray beam of synchrotron radiation

To reduce the discharge of the standard bulk Micromegas and GEM detectors, a GEM-Micromegas detector was developed at the Institute of High Energy Physics. Taking into account the advantages of the two detectors, one GEM foil was set as a preamplifier on the mesh of Micromegas in the structure and the CEM pream- plification decreased the working voltage of Micromegas to significantly reduce the effect of the discharge. At the same gain, the spark probability of the GEM-Micromegas detector can be reduced to a factor 0.01 compared to the standard Micromegas detector, and an even higher gain could be obtained. This paper describes the performance of the X-ray beam detector that was studied at 1W2B Laboratory of Beijing Synchrotron Radiation Facility. Finally, the result of the energy resolution under various X-ray energies was given in different working gases. This indicates that the GEM-Micromegas detector has an energy response capability in an energy range from 6 keV to 20 keV and it could work better than the standard bulk-Micromegas.     

Investigation of GEM-Micromegas detector on X-ray beam of synchrotron radiation

To reduce the discharge of the standard bulk Micromegas and GEM detectors, a GEM-Micromegas detector was developed at the Institute of High Energy Physics. Taking into account the advantages of the two detectors, one GEM foil was set as a preamplifier on the mesh of Micromegas in the structure and the GEM preamplification decreased the working voltage of Micromegas to significantly reduce the effect of the discharge. At the same gain, the spark probability of the GEM-Micromegas detector can be reduced to a factor 0.01 compared to the standard Micromegas detector, and an even higher gain could be obtained. This paper describes the performance of the X-ray beam detector that was studied at 1W2B Laboratory of Beijing Synchrotron Radiation Facility. Finally, the result of the energy resolution under various X-ray energies was given in different working gases. This indicates that the GEM-Micromegas detector has an energy response capability in an energy range from 6 keV to 20 keV and it could work better than the standard bulk-Micromegas.     

环戊酮C_5H_8O的同步辐射真空紫外光电离解离研究

利用同步辐射光源,研究了环戊酮(C5H8O)在真空紫外105～140 nm波段的光电离和光解离过程.通过质谱测量各离子的光电离效率曲线,得到了该分子的垂直电离能及主要碎片离子的出现势.从理论上利用G3方法,计算了母体和中性及离子碎片的结构和能量,估算了各解离通道所需的解离能.结合实验测量值和理论计算值,指认出环戊酮分子可能的光电离解离通.     

第四代同步辐射光源的光束线站及其应用

随着第四代同步辐射光源的兴起,得益于X射线亮度和相干性的大幅度提升,同步辐射实验技术在谱学、散射和成像等方面取得了显著进步。这些技术能够探测复杂非均匀体系和动态变化过程中的物质结构、成分、化学价态、电子态和磁性等关键信息,在基础科学领域和应用基础研究中发挥关键作用。文章旨在介绍第四代同步辐射光源的线站技术优势,并结合具体例子探讨其在若干物理研究中的应用,同时也讨论了当前存在的工程技术挑战。希望人们能够了解第四代同步辐射光源的光束线站的特点和应用潜力,以促进其在各个科研领域的推广。