Studies on coherent and incoherent spin dynamics that control the magnetic field effect on photogenerated radical pairs

Since 1970s, magnetic field effects (MFEs) on photogenerated radical pairs have been the centre of focus in the field of spin chemistry. The MFE attributes to quantum mechanical interconversion between the singlet and triplet radical pair states and subsequent spin-selective recombination reactions. In this New View article, the author picks up two hot topics studied during the last two decades, which are (i) so-called low field effect (LFE) and (ii) 2J-resonance MFE on fixed distance donor–acceptor linked molecules. In both of the topics, quantum mechanical explanations are given referring to recent reports, and some novel calculations have been carried out for bridging theoretical and experimental data for long-lived radical pairs. For the first topic, time domain calculations of coherent state mixing have been carried out for elucidation of hyperfine (HF) structure dependence of the LFE. For the second topic, Monte Carlo simulations of the torsional motion of polyaromatic linker unit have been carried out for the demonstration of fast decoherence in such rigid molecules. From these considerations, future possibilities of MFE studies on photo-functional materials and biomolecules have been indicated.     

Spin precession of a charged particle in a uniform magnetic field on a static space-time

We investigate the ratio of spin precession frequency to orbital frequency for a spinning charged particle confined to circular orbit in the equatorial plane of a compact object, with a uniform magnetic field, as described by the Wald and the Ernst potentials. In order to see the difference in behaviours for particles with differentg values we consider the cases of electron and proton separately.     

Single-molecule spectroscopy of radical pairs,a theoretical treatment and experimental considerations

ABSTRACT

In this work, we propose to extend the scope of single-molecule spectroscopy to spin chemistry investigations of single radical pairs. A consistent theory of single-molecule spectroscopy on single radical pairs is proposed, which allows one to show that bunching phenomena are affected by singlet–triplet interconversion in radical pairs, which is, in turn, affected by local and external magnetic fields. A detailed study on the feasibility of such experiments with single flavin adenine dinucleotide, FAD, molecules is presented. We conclude that the observation of magnetic field effects on single FAD molecules is feasible but experimentally challenging for measurements on integrated fluorescence intensity and fluorescence event statistics.     

磁场微重力效应的研究

将导电的液体置于磁场中,使导电液体中浮力驱动的自然对流减弱甚至消失,在导电液体中制造出了二级微重力效应,将这种情况称为磁场微重力效应.通过研究导电液体自然对流驱动力的无量纲Grashof数的变化,发现微重力效应的水平可以用公式g_m＝（β₀/β_m）（ν₀ /ν_m）²g₀ 计算,如果略去一次项,则可用g_m＝（ν₀ /ν_m）²g₀来估算.测量研究了不同磁场条件下硅熔体的磁黏度,估算不同磁场强度对应的磁场微重力水平后,发现估算结果与实验结果基本符合. 关键词： 磁场 二级微重力效应 Grashof数 微重力水平     

用磁致旋光效应估测二维磁场分布

为了克服现有测量磁场方法只能单点测量的局限性,基于法拉第磁光效应原理,提出利用磁致旋光估测磁场的方法,提高了磁场测量的效率,获得了磁场的直观分布.建立磁致旋光估测磁场的实验装置,测量了永磁体的磁场,用CCD采集了偏振光通过磁场的图像,通过程序处理可获得磁铁产生的局部磁场二维分布图,并可求得二维分布图上任意点的磁感应强度.     

Estimation of the chiral magnetic effect considering the magnetic field response of the QGP medium

The magnetic field plays a major role in searching for the chiral magnetic effect in relativistic heavy-ion collisions. If the lifetime of the magnetic field is too short, as predicted by simulations of the field in vacuum, the chiral magnetic effect will be largely suppressed. However, the lifetime of the magnetic field will become longer when the QGP medium response is considered. We give an estimate of the effect, especially considering the magnetic field response of the QGP medium, and compare it with the experimental results for the background-subtracted correlator H at RHIC and LHC energies. The results show that our method explains the experimental results better at the top RHIC energy than at the LHC energy.     

The effect of 2.1 T static magnetic field on astrocyte viability and morphology

The viability and a number of morphological properties of in situ astrocytes of rat spinal cord cultures including changes in surface area and migration of both cell body and nucleus were investigated at magnetic field intensities comparable to those currently used for magnetic resonance imaging. Viability of rat spinal astrocytes was studied after up to 72 hours of 2.1T static magnetic field exposure. Surface areas and two-dimensional centroids of both soma and nucleus after 2 hours of magnetic field exposure were determined and compared with those of the same cells before magnetic field exposure. Cell membrane ruffling was quantified using fractal analysis.     

Reversal of coherent‐state spins in square magnetic nanodots induced by a magnetic microwave field

We study the coherent state excitation of spins in square nanodots induced by a magnetic microwave field. We present a new mechanism of spin reversal in nanodots. That is, the microwave field directly induces the reversal of the coherent‐state spins instead of indirectly through the magnetic vortex. We obtain the space distribution of coherent‐state spins in terms of a quantum theory, and calculate the time of spin reversal. This spin‐reversal process may be used to serve as a storage mechanism of binary information.     

强磁场中超冷费米气体的相对论效应

由单粒子的弱相对论能谱及泊松公式,导出强磁场中费米气体的热力学势函数.在此基础上,运用热力学关系求解低温条件下系统的统计特征量的解析式,分析相对论效应对统计性质的影响机理.研究表明,磁场愈强,相对论效应愈明显.相对论效应引发的单调项与相应的振荡项的振幅相比,对总能,单调项远大于振幅;对化学势及磁矩,单调项与振幅几乎同一量级. 关键词： 强磁场 费米气体 相对论效应     

光磁共振实验中抵消地磁场垂直分量的方法

介绍了光磁共振实验装置的各磁场线圈,分析了光磁共振实验中抵消地磁场垂直分量传统方法的缺陷,利用垂直磁场对磁共振信号的影响,提出了一种重复性较好的抵消地磁场垂直分量的方法,减小了传统实验方法产生的误差.这种方法也可用于测量地磁场垂直分量的大小.     

Interaction of neutrons with layered magnetic media in oscillating magnetic field

New experimental possibilities of investigating layered magnetic structures in oscillating magnetic fields are discussed. Spin-flip and nonspin-flip neutron reflection and transmission probabilities show a frequency dependency near the magnetic neutron resonance condition. This allows to increase the precision of the static magnetic depth profile measurements of the magnetized matter. Moreover, this opens new possibilities of measuring the induction of the oscillating field inside the matter and determining the magnetic susceptibility of the oscillating magnetic field. Refraction of neutrons as they pass through a magnetic prism in the presence of an oscillating magnetic field is also investigated. A non-polarized neutron beam splits into eight spatially separated neutron beams, whose intensity and polarization depend on the strength and frequency of the oscillating field. Also, it is shown that the oscillating magnetic permeability of an angstrom-thick layer can be measured with a neutron wave resonator.     

Generation of an external magnetic field with the spin orientation effect in a single layer Ising nanographene

In this work, the magnetic properties of the single layer Ising nanogaphene (SLING) are investigated by using Kaneyoshi approach (KA) within the effective field theory for different spin orientations of its magnetic atoms. We find that the magnetizations of the SLING has no phase transition, certain Curie temperature and distinct peak of susceptibility at T_c for the some spin orientations at the zero external magnetic field (H=0.0). Because these behaviors occur at H≠0.0, we suggest that the SLING generates an external magnetic field and behaves as an external magnetic field generator for these spin orientations. However, the SLING exhibits ferromagnetic behaviors for only one spin orientations. But, it exhibits antiferromagnetic behaviors for the others. For the AFM cases, diamagnetic susceptibility behaviors and type II superconductivity hysteresis behaviors are obtained. We hope that these results can open a door to obtain new class of single layer graphene and graphene-based magnetic field generator devices with the spin orientation effect.     

光磁共振实验中扫场的作用和影响

讨论了方波和三角波扫场对光抽运信号和磁共振信号的作用和影响,阐明了应如何选择方波和三角波扫场信号的大小和方向,才能得到理想的光抽运信号和磁共振信号的方法．     

两种均匀磁介质分界面上有长载流导线的场和电流分布

分析两种均匀磁介质分界面上有长载流导线的场和电流分布，指出磁感应强度B=B(r)φ径向对称分布是由径向对称分布的总电流j=j(r)ez(包括传导电流和磁化电流)所激发,探讨了传导电流的分布与磁感应强度B、磁场强度H和磁化电流的分布的关系。     

带电粒子在地磁场中的运动

用计算机模拟的方法研究了地磁场中带电粒子的运动特性,绘制了粒子轨迹曲线,对粒子运动进行了分析,解释了地磁场的磁瓶效应和辐射带.     

The effect of toroidal field on the rotating magnetic field current drive in rotamak plasmas

A rotamak is one kind of compact spherically shaped magnetic-confinement device. In a rotamak the plasma current is driven by means of rotating magnetic field （RMF）. The driven current can reverse the original equilibrium field and generate a field-reversed-configuration. In a conventional rotamak, a toroidal field （TF） is not necessary for the RMF to drive plasma current, but it was found that the present of an additional TF can influence the RMF current drive. In this paper the effect of TF on the RMF current drive in a rotamak are investigated in some detail. The experimental results show that addition of TF increases the RMF driven current greatly and enhances the RMF penetration dramatically. Without TF, the RMF can only penetrate into plasma in the edge region. When a TF is added, the RMF can reach almost the whole plasma region. This is an optimal strength of toroidal magnetic field for getting maximum plasma current when Bv and radio frequency generator power are fixed. Besides driving current, the RMF generates high harmonic fields in rotamak plasma. The effect of TF on the harmonic field spectra are also reported.[第一段]     

Second-harmonic generation in asymmetric quantum dots in the presence of a static magnetic field

The second-harmonic generation(SHG) coefficient in an asymmetric quantum dot(QD) with a static magnetic field is theoretically investigated.Within the framework of the effective-mass approximation,we obtain the confined wave functions and energies of electrons in the QD.We also obtain the SHG coefficient by the compact-density-matrix approach and the iterative method.The numerical results for the typical GaAs/AlGaAs QD show that the SHG coefficient depends strongly on the magnitude of magnetic field,parameters of the asymmetric potential and the radius of the QD.The resonant peak shifts with the magnetic field or the radius of the QD changing.     

磁象法在解静磁场边值问题中的应用

讨论了静磁场中B的唯一性定理及其应用——磁象法,介绍了用磁象法解静磁场边值问题的方法．     

Increase in temperature of a ferromagnetic substance in rf magnetic field

If one applies an rf magnetic field parallel to a strong static field, temperature of a ferromagnetic substance rises due to ferromagnetic resonance. This phenomenon finds immediate application in the field of hyperthermic oncology. In this work, we have found expression for the increase in temperature when a ferromagnetic material is placed under a static and a varying magnetic field of high frequency through spin wave approach. The numerical value of this increment of local temperature has been estimated for yttrium iron garnet (YIG). We also have examined the possibility of enhancing the temperature of a ferromagnetic material only by applying a strong static field.     

The effect of rotating fields in magnetic resonance

The phenomenon of magnetic resonance is studied by considering the transverse oscillatory field as superposition of two oppositely rotating fields. One of the rotating fields is taken as strong and the other relatively weak.