Effects of transverse field on the magnetization and initial susceptibility of a molecular-based magnet

The molecular-based magnet system consists of mixed spin-2 and spin- 5/2 honeycomb lattices with ferrimagnetic interlayer coupling. Within the framework the effective-field theory with self-spin correlations and differential operator technique, the effects of the transverse field on the magnetization and initial susceptibility have been studied in detail.     

Critical properties of the biaxial Ising model with both the longitudinal crystal field and the transverse dilution crystal field

Within the effective field theory (EFT), the critical properties of the biaxial Ising model with both longitudinal crystal field and transverse dilution crystal field are investigated for a simple cubic lattice. The tricritical point (TCP) and its trajectory are discussed in T-D_x and T-D_z space. A new phenomenon of two TCPs is found in T-D_x space. There exists a second-order line between two first-order lines, separated by two TCPs. The change of dilution concentration leads to a complex relation of the trajectory of the TCP. The degenerate patterns at the ground state appear by changing the longitudinal crystal field. The range of the ordered phase for transition lines labelled as a positive or (negative) value of D_x/J becomes larger or (smaller) with the decrease of t_x in T-D_z space. Some results have not been revealed in previous works.     

Ground-state magnetic properties of the spin-2 transverse Ising model

The ground-state magnetic properties of the spin-2 transverse Ising model with a longitudinal crystal field are studied within the framework of mean-field theory (MFT) and effective-field theory (EFT), respectively. The phase diagrams and magnetization curves are examined in detail. It is found that the system exhibits a tricritical behavior in the ground-state phase diagrams. Some interesting phenomena have been found, especially the first-order phase transition from one ordered phase to the other ordered phase, which is due to the high spin. The spin correlation has important effect on the magnetic properties of the system. We also find that the ground-state phase diagrams of the spin-2 transverse Ising model are very different from those of the spin-3/2 transverse Ising model.     

The phase diagrams of a spin-1 transverse Ising model

The phase diagrams of the spin-1 transverse Ising model with the presence of a crystal field is investigated by using an effective-field theory (EFT). We give a method to calculate the Gibbs free energy numerically at finite temperature within the EFT. The first-order transition lines are obtained by comparing the Gibbs free energy. The phase diagrams and the Gibbs free energy are also compared with those given using the mean-field theory (MFT).     

Dynamics of the one-dimensional random transverse Ising model with next-nearest-neighbor interactions

The dynamics of the one-dimensional random transverse Ising model with both nearest-neighbor (NN) and next-nearest-neighbor (NNN) interactions is studied in the high-temperature limit by the method of recurrence relations. Both the time-dependent transverse correlation function and the corresponding spectral density are calculated for two typical disordered states. We find that for the case of bimodal disorder the dynamics of the system undergoes a crossover from a collective-mode behavior to a central-peak one and for the case of Gaussian disorder the dynamics is complex. For both cases, it is found that the central-peak behavior becomes more obvious and the collective-mode behavior becomes weaker as K_i increase, especially when K_i>J_i/2 (J_i and K_i are the exchange couplings of the NN and NNN interactions, respectively). However, the effects are small when the NNN interactions are weak (K_i<J_i/2).     

Frequency dependence of the complex susceptibility for a spin-1 Ising model

The complex susceptibility or the dynamic susceptibility (χ(ω)=χ′(ω)−iχ″(ω)) for a spin-1 Ising system with bilinear and biquadratic interactions is obtained on the basis of Onsager theory of irreversible processes. If the logarithm of the susceptibilities is plotted as a function of the logarithm of frequency, then the real part (χ′) displays a sequence of plateau regions and the imaginary part (χ″) has a sequence of maxima in the ordered or ferromagnetic phase. On the other hand, only one plateau region in χ′ and one maximum in χ″ is observed in the disordered or paramagnetic phase. Argand or Cole-Cole plots (χ″−χ′) for a selection of temperatures are also shown, and a sequence of semicircles is illustrated in the ordered phase and only one semicircle for the disordered phase in these plots.     

Magnetic relaxation in a spin-1 Ising model near the second-order phase transition point

The magnetic relaxation of a spin-1 Ising model with bilinear and biquadratic interactions is formulated within the framework of statistical equilibrium theory and the thermodynamics of irreversible processes. Using a molecular-field expression for the magnetic Gibbs energy, the magnetic Gibbs energy produced in the irreversible process is calculated and time derivatives of the dipolar and quadrupolar order parameters are treated as fluxes conjugate to their appropriate generalized forces in the sense of Onsager theory. The kinetic equations are obtained by introducing kinetic coefficients that satisfy the Onsager relation. By solving these equations an expression is derived for the dynamic or complex magnetic susceptibility. From the real and imaginary parts of this expression, magnetic dispersion and absorption factor are calculated and analyzed near the second-order phase transition.     

Mean field study of the mixed Ising model in a random crystal field

The magnetic properties of a mixed Ising ferrimagnetic system, in which the two interacting sublattices have spins σ, (±1/2) and spins S, (±1,0) in the presence of a random crystal field, have been studied with the mean field approach. The obtained results show the existence of some interesting phenomena, such as the appearance of a new ferrimagnetic phase, namely, partly ferrimagnetic phase and consequently the existence of four topologically different types of phase diagrams. Furthermore, compensation behaviour and re-entrant phenomenon are found for appropriate ranges of crystal field. Thermal magnetization behaviour and phase diagrams have been discussed in detail.     

Phase diagram of the two-dimensional Ising model with random competing interactions

An Ising model with ferromagnetic nearest-neighbor interactions J₁ (J₁>0) and random next-nearest-neighbor interactions [+J₂ with probability p and −J₂ with probability (1−p); J₂>0] is studied within the framework of an effective-field theory based on the differential-operator technique. The order parameters are calculated, considering finite clusters with n=1,2, and 4 spins, using the standard approximation of neglecting correlations. A phase diagram is obtained in the plane temperature versus p, for the particular case J₁=J₂, showing both superantiferromagnetic (low p) and ferromagnetic (higher values of p) orderings at low temperatures.     

Magnetic properties of the bond and crystal field dilution Blume-Emery-Griffiths model in the presence of magnetic field

The magnetic properties of the spin-1 bond and crystal field dilution Blume-Emery-Griffiths (BEG) model in the presence of magnetic field are investigated on a simple cubic lattice by using effective field theory (EFT). In the M-H plane, the common action of bond and crystal field dilution leads to the exhibition of an irregular initial magnetization curve and slows down the magnetization process. The peak of the susceptibility curve has an explicit decline and shows a distinct shift toward the direction of increase of magnetic field. On the other hand, in the M-T plane, the magnetization curves show a discontinuity and a vertical leap in the small range of magnetic field when the negative crystal field is larger and the ratio of biquadratic and exchange interaction is positive (α>0). These results have not been revealed in previous works.     

Comparative study between a two-dimensional anisotropic Heisenberg antiferromagnet with easy-axis single-ion anisotropy and one with easy-axis exchange anisotropy

Generally, in literature, easy-axis single ion anisotropy and easy-axis exchange anisotropy was treated in indistinct way. In this work we propose to perform a comparative study of the effects of these two easy-axis anisotropies on the behavior of the magnetization and the critical temperature (_Tc)$(T_{\mathrm{c}})$ in the 2D classical Heisenberg antiferromagnetic model. In order to study the low-temperature thermodynamics of this model, we should consider the contribution of anisotropic spin waves, using a self-consistent harmonic approximation (SCHA) theory. We compare the predictions of SCHA with numerical simulations on L×L$L\times L$ square lattices using Monte Carlo (MC) simulations, which include effects due to all thermodynamically allowed excitations. Our SCHA results are in good agreement with our MC simulations results and have shown that the strong K$K$ limit gives two different Ising-like behavior. In the exchange anisotropic case, the dependence of _Tc$T_{\mathrm{c}}$ on anisotropic parameter K$K$ becomes linear and in the single-ion anisotropic case, _Tc$T_{\mathrm{c}}$ becomes independent of K$K$. Also, using MC simulations and finite size scaling, we show that the critical exponents in the two anisotropic case are compatible with the 2D Ising values α=0.125$\alpha =0.125$ and γ=1.75$\gamma =1.75$.     

The phase diagrams and compensation behaviors of mixed spin Blume-Capel model in a trimodal magnetic field

The phase diagrams and compensation behaviors of mixed spin-1/2 and spin-1 Blume-Capel model in a trimodal magnetic field are investigated in the framework of the effective field theory on simple cubic lattice. The change of negative crystal field and trimodal concentration can affect the TCP, the second-order phase and the magnetic field degeneration at ground state in T-H space. In T-D space, the trajectory of the TCP takes on the acre curve and there exist the two TCPs under certain condition. In addition to giving one or two compensation temperature points in M-T space, the mixed spin Blume-Capel model also provides one or two novel compensation magnetic field points in M-H space. Some results are not revealed in previous works.     

Kink solutions of the classical transverse field Ising chain

We investigate stationary and travelling wave solutions of the classical one-dimensional transverse field Ising model. Results are given on the existence, shape and stability of kink solutions and periodic solutions. We review recent analytical results (e.g., the proof of existence of a one-parameter family of stationary kink solutions and the proof of existence of travelling wave kink solutions with nonzero velocity c≠ 0) and extend them by the use of numerical methods. Small oscillations arising in the tails of travelling kink solutions are investigated numerically. In the end, stability analysis puts some light on pinning effects. Received 23 February 2001 and Received in final form 4 October 2001     

Monte Carlo analysis of critical properties of the two-dimensional randomly site-diluted Ising model via Wang-Landau algorithm

The influence of random site dilution on the critical properties of the two-dimensional Ising model on a square lattice was explored by Monte Carlo simulations with the Wang-Landau sampling. The lattice linear size was L=20-120 and the concentration of diluted sites q=0.1,0.2,0.3. Its pure version displays a second-order phase transition with a vanishing specific heat critical exponent α, thus, the Harris criterion is inconclusive, in that disorder is a relevant or irrelevant perturbation for the critical behaviour of the pure system. The main effort was focused on the specific heat and magnetic susceptibility. We have also looked at the probability distribution of susceptibility, pseudocritical temperatures and specific heat for assessing self-averaging. The study was carried out in appropriate restricted but dominant energy subspaces. By applying the finite-size scaling analysis, the correlation length exponent ν was found to be greater than one, whereas the ratio of the critical exponents (α/ν) is negative and (γ/ν) retains its pure Ising model value supporting weak universality.     

Magnetic properties of a mixed spin- 1/2 and spin- 3/2 transverse Ising model in a longitudinal magnetic field

The mixed spin- 1/2 and spin- 3/2 transverse Ising model in a longitudinal magnetic field is studied within the framework of the effective-field theory with correlations. In this approach the effective-field equations are derived by using a probability distribution method based on the generalized but approximated van der Waerden identities. The total longitudinal and transverse magnetizations, the transverse susceptibility and longitudinal susceptibility and the critical temperatures are obtained. We find a number of interesting phenomena in these quantities, due to the applied transverse field and the longitudinal field.     

Critical behaviors of bond and crystal field dilution Blume–Emery–Griffiths model

The critical behavior of the spin-1 bond and crystal field dilution Blume–Emery–Griffiths model have been investigated on simple-cubic lattice within the framework of the effective field theory. In particular, both bond dilution and random crystal field are considered at the same time. The interplay between bond and crystal field dilution constructs rich and interesting phase diagrams. Significant distinctions are exhibited. When positive ratio α changes in a certain range, there exist double tricritical points in phase-transition lines in T–D plane. Moreover, this first-order phase transition is enlarged with increasing of ratio α at a fixed crystal field dilution concentration, while this first-order phase transition will shrink when bond dilution concentration is fixed. In addition, we observe that there exist two bond percolation thresholds for negative crystal field and α>0 in T–P plane.     

Critical properties of the three-dimensional Ising model with quenched disorder

The static critical properties of the three-dimensional Ising model with quenched disorder are studied by the Monte-Carlo (MC) method on a simple cubic lattice, in which the quenched disorder is distributed as nonmagnetic impurities by the canonical manner. The calculations are carried out for systems with periodic boundary conditions and spin concentrations p=1.0; 0.95; 0.9; 0.8; 0.7; 0.6. The systems of non-linear sizes L×L×L, L=20-60 are researched. On the basis of the finite-size scaling (FSS) theory, the static critical exponents of specific heat α, susceptibility γ, magnetization β, and an exponent of the correlation radius in a studied interval of concentrations p are calculated. It is shown that the three-dimensional Ising model with quenched disorder has two regimes of the critical behavior universality in a dependence on nonmagnetic impurities.     

Critical behavior of the 3D Ising model on a poissonian random lattice

The single-cluster Monte Carlo algorithm and the reweighting technique are used to simulate the 3D ferromagnetic Ising model on 3D Voronoi-Delauney lattices. It is assumed that the coupling factor J varies with the distance r between the first neighbors as J(r)∝e^−ar, with a≥0. The critical exponents γ/ν, β/ν, and ν are calculated, and according to the present estimates for the critical exponents, we argue that this random system belongs to the same universality class of the pure 3D ferromagnetic Ising model.     

Geometrical aspects of the Z-invariant Ising model

We discuss a geometrical interpretation of the Z-invariant Ising model in terms of isoradial embeddings of planar lattices. The Z-invariant Ising model can be defined on an arbitrary planar lattice if and only if certain paths on the lattice edges do not intersect each other more than once or self-intersect. This topological constraint is equivalent to the existence of isoradial embeddings of the lattice. Such embeddings are characterized by angles which can be related to the model coupling constants in the spirit of Baxter's geometrical solution. The Ising model on isoradial embeddings studied recently by several authors in the context of discrete holomorphy corresponds to the critical point of this particular Z-invariant Ising model.     

Ground-state phase diagrams of Ising metamagnet in a mixed longitudinal and transverse magnetic field

The ground-state magnetic properties of a two-sublattice Ising metamagnet in a mixed longitudinal and transverse magnetic field are studied within the effective-field theory. A parameter j₂=J₂/J₁ is introduced, which reflects the strength ratio of spin coupling between adjacent planes and in each plane. In addition to the second-order transition lines, the first-order transition lines are also presented, since the ground-state energy can be calculated numerically. The ground-state phase diagrams in h_x–h_z are presented. The results show that when j₂<0 the phase transition of the system is always first-order for h_x<2.751, and when −1000?j₂<0 it is always second-order for h_x>4.36. For the given h_x (0<h_x<14.71), the longitudinal critical magnetic field increases as j₂ decreases. The reentrant phenomenon occurs in the range of j₂<−11.89, h_x>14.71. There is no fourth-order critical point in the phase diagrams given by using EFT as found by using mean field theory (MFT).