共振简并四波混频光学相位共轭的研究

本文考虑了非线性极化强度对cos(k·r)的依赖关系,对共振增强简并四波混频的半经典处理提出了修正,得到相位共轭反射率满足的Riccatti方程.使用可调谐连续波CO_2激光器和SF_6气体作非线性介质作了实验研究.获得了(0.2～0.8)×10~(-4)的反射率.     

Collision induced and resonantly enhanced extra resonances in four-wave mixing in inhomogeneously broadened four level systems

Role of collisions in inducing and enhancing extra resonances in non-linear generation by four-wave mixing in inhomogeneously broadened four level systems is studied. It is shown that collision induced three and two-photon resonances can be enhanced further by tuning to exact one photon (non-absorbing) transitions between unpopulated upper levels. In addition we also find existence of collision induced interference dip at the three-photon resonance that arises due to complete cancellation of signal at the line center.     

Nonresonant tripling and sum-frequency mixing in Hg

Nonresonant frequency tripling and sum-frequency mixing of pulsed dye-laser radiation generates in Hg vapor continuously tunable coherent vuv radiation in the wavelength range _vuv=132-185nm. Laser pulse powers of 1–2 MW produce vuv light pulses of 0.6–1.5 W (2–4.8×10⁹ photons/pulse).     

Noise characteristic of sum-frequency mixing orange solid-state laser

A laser-diode-pumped Nd:YVO₄ orange solid-state laser is described in this paper. The fundamental wavelengths at 1064 and 1342 nm oscillate simultaneously and generate the 593.5 nm wavelength by intracavity sum-frequency mixing in a KTP crystal using type II phase matching. The noise characteristic of laser output has been measured and analyzed at different pumping powers. The relationship between the amplitude noise of sum-frequency mixing output and the longitudinal modes of fundamental frequency has been investigated. The results show that the sum-frequency mixing output has low noise if one of the fundamental wavelengths is single longitudinal mode. The experiment shows that amplitude noise of the intracavity sum-frequency mixing laser is lower than that of intracavity frequency doubled laser with the same structure.     

LD泵浦全固态608.1nm和频激光器

本文报道了一种全固态腔内和频608.1 nm激光器。在激光谐振腔两个分臂中,两支激光二极管分别泵浦Nd: YVO₄和Nd: YAG晶体,分别选择1 342 nm波长(Nd: YVO₄晶体的⁴F_3/2-⁴I_13/2谱线)与1 112 nm波长(Nd: YAG晶体的⁴F_3/2-⁴I_11/2谱线)振荡并进行腔内和频。通过优化谐振腔设计,腔内两个波长获得了较好的模式匹配。在两个分臂的交叠部分,利用LBO I类相位匹配进行和频,获得和频608.1 nm激光输出。实验表明,当Nd: YVO₄与Nd: YAG晶体泵浦功率分别为600和740 mW时,获得了功率为23.8 mW、波长为608.1 nm激光输出,激光输出稳定、噪声低。利用本文提出的和频结构是获得608.1 nm激光输出较为有效的方法。     

Transient sum-frequency mixing with temporally tailored laser pulses

We discuss the possibility of using temporally tailored pump laser pulses to control the temporal width and shape of optical pulses generated in a process of transient sum-frequency mixing in crystals with second-order nonlinearity. Specific calculations performed in a model crystal in the case of fifth-harmonic generation are presented.     

Efficient sum-frequency mixing through transparency induced by autoionization

It is shown that efficient sum-frequency mixing is possible through transparency induced by autoionization. Tuning the incident laser frequencies to the absorption minimum of an autoionizing resonance for the generated wave greatly reduces the linear absorption of the generated wave while third-order susceptibility is still enhanced. The proposed scheme does not require any strong radiative couplings and would be particularly useful for the generation of short-wavelength radiation.     

Ultrasensitive femtosecond two-photon detector with resonantly enhanced nonlinear absorption

We report on two-photon detection based on nonlinear absorption between subbands in quantum wells. Resonantly enhanced nonlinear absorption, 6 orders of magnitude higher than that of typical bulk semiconductors, leads to a threshold power density for quadratic detection as low as 0.1 W/cm2 and to femtosecond time resolution. The approach facilitates dynamic characterization of the optical light field of infrared emitters with unprecedented sensitivity. We also present a new method for determining the intersubband and intrasubband scattering times by means of autocorrelation measurements.     

Walk-off and phase-compensated resonantly enhanced frequency-doubling of picosecond pulses using type II nonlinear crystal

We propose enhanced frequency-doubling inside an external ring-cavity using type II nonlinear crystal. A KTP type II twin-crystal device is implemented for compensation of both walk-off and phase-shift between ordinary and extraordinary fundamental waves. Starting from an 850 mW diode-pumped actively mode-locked Nd:YAG laser at 1.064 μm with 100 MHz repetition rate and 25 ps pulse duration, we performed 54% harmonic conversion efficiency in the green. Received: 31 August 1998 / Revised version: 10 February 1999 / Published online: 19 May 1999     

LBO腔内和频593 nm激光器

报道了LD纵向泵浦NdYVO4晶体,经腔内和频得到593 nm激光输出的实验研究.采用一个线性平凹腔实现了1 064 nm和1 342 nm双波长连续波振荡,利用LBO腔内和频产生593 nm激光输出.在泵浦功率为1.4 W时得到593 nm的输出功率为70 mW.593 nm光束远场发散角小于1 mrad,光斑椭圆度为0.999,且具有低噪声输出特性.实验结果表明,该结构激光器是获得衍射极限全固体黄激光器的实用方法.     

All-solid-state doubly resonant sum-frequency mixing laser at 555 nm

We report for the first time a coherent radiation at 555 nm by intracavity sum-frequency generation of 946 nm Nd:YAG laser and 1343 nm Nd:LuVO₄ laser. Yellow-green laser is obtained by using a doubly folded cavity, type-II critical phase matching KTP crystal sum-frequency mixing. With total pump power of 31.9 W (13.7 W pump power for 1343 nm Nd:LuVO₄ laser and 18.2 W pump power for 946 nm Nd:YAG laser), TEM₀₀ mode yellow-green laser at 555 nm of 2.35 W is obtained.     

Generation of continuous-wave 243-nm radiation by sum-frequency mixing

We have generated tunable cw radiation near 243 nm with a linewidth of less than 4 MHz by sum-frequency mixing the 351 nm radiation from an argon-ion laser with the 789 nm radiation from a ring dye laser in a crystal of ammonium dihydrogen phosphate held at moderate temperature. An external ring cavity, resonant with the dye laser, gives a power enhancement of about 12 in the sum-frequency generated radiation. Thermal lensing due to laser heating of the nonlinear crystal, distorded the 351 nm mode structure. This effect could limit the efficiency of the sum frequency mixing process.     

Internal resonantly enhanced frequency doubling of continuous-wave fiber lasers

In this Letter we describe a simple method for frequency doubling in high-power CW fiber lasers that offers the prospect of very high conversion efficiency and high power in the visible wavelength regime. Our approach is based on second harmonic generation in an enhancement resonator within the fiber laser cavity and does not require active cavity length stabilization. This technique has been applied to a cladding-pumped Yb-doped fiber laser to generate 19 W of linearly polarized CW green output at 540 nm, with excellent temporal stability for 90 W of absorbed diode pump power at 975 nm. The prospects for further improvement in performance with respect to conversion efficiency and output power are considered.     

All-solid-state continuous wave doubly linear resonator sum-frequency mixing yellow laser

We report a continuous-wave (CW) yellow laser emission by sum-frequency mixing in Nd:YVO4 crystal. Using type-II critical phase-matching KTP crystal, a yellow laser at 593.5 nm is obtained by 1064 and 1342 nm intracavity sum-frequency mixing. The maximum laser output power of 2.1 W is obtained when an incident pump laser of 18.2 W is used. At the output power level of 2.1 W, the output stability is better than 3.2%.     

Diode-Pumped Nd:YAP sum-frequency mixing orange-red laser at 616 nm

We report for the first time a coherent orange-red radiation at 616 nm by intracavity sum-frequency generation of the 1080 and 1433 nm laser-lines of two Nd:YAP lasers. Orange-red laser is obtained by using a doubly linear resonator, type-II critical phase matching KTiOPO₄ (KTP) crystal sum-frequency mixing. With a total diode pump power of 26.5 W (8.7 W pump power for 1080 nm Nd:YAP laser and 17.8 W pump power for 1433 nm Nd:YAP laser), TEM00 mode orange-red laser at 616 nm of 127 mW is obtained. The power stability in 30 min is better than 3.3%.     

All-solid-state CW doubly resonant sum-frequency mixing red-orange laser at 611 nm

We report for the first time a continuous wave (CW) coherent radiation at 611 nm by intracavity sum-frequency generation of 1064 nm Nd:YVO₄ laser and 1433 nm Nd:YAP laser. Red-orange laser is obtained by using a doubly cavity, type-II critical phase matching KTP crystal sum-frequency mixing. With total pump power of 27.9 W (17.8 W pump power for 1433 nm Nd:YAP laser and 10.1 W pump power for 1064 nm Nd:YVO₄ laser), TEM₀₀ mode red-orange laser at 611 nm of 1.15 W is obtained. The red-orange power stability in 30 min is better than 4.3%.     

Development of laser photoelectron spectroscopy based on resonantly enhanced multiphoton ionization

This review article is mainly concerned with laser photoelectron spectroscopy based on REMPI (resonantly enhanced multiphoton ionization), consisting of two parts. One is associated with the measurement of photoelectron kinetic-energy distribution and the other is associated with the measurement of zero-kinetic-energy (ZEKE) photoelectrons in very high resolution. These two techniques are complementary to each other. During the last three decades, the author and co-workers have carried out photoelectron spectroscopic studies of molecules in the gas phase, using the HeI 584 Å resonance line and a nanosecond tunable UV–visible laser. In this article, firstly the author’s background in the field of molecular photoelectron spectroscopy is described briefly, by mentioning three topics of HeI photoelectron spectroscopy. Secondly, the principle and characteristics of laser photoelectron kinetic-energy spectroscopy and its application to several typical topics, namely, one-photon forbidden states (O₂), autoionization from a super-excited state (NO), and small van der Waals molecules (NO–Ar and the NO₂ dimer), and some others. Thirdly, the principle and characteristics of ZEKE photoelectron spectroscopy are described, together with its application to the following several topics: (1) rotational spectra of NO⁺, (2) vibrational coupling of (naphthalene)⁺, (3) large-amplitude torsional motion of (tolane)⁺, (4) rotational isomers of (cis and trans n-propylbenzene)⁺ and structural isomers of (2-hydroxypyridine)⁺, (5) proton tunneling of (tropolone)⁺ and (9-hydroxyphenalenone)⁺, (6) intramolecular vibrational redistribution of trans stilbene, and (7) cation van der Waals molecules of aniline–Ar_n (n=1,2) and azulene–Ar. All the results mentioned as examples are those obtained in the author’s laboratory.     

Diode-laser-pumped continuous-wave doubly linear resonator sum-frequency mixing red laser at 689 nm

We report for the first time a coherent red radiation at 689 nm by intracavity sum-frequency generation of the 1319- and 1444-nm laser-lines of two Nd:YAG lasers. Using type-II critical phase matching KTP crystal, 689-nm red laser was obtained by 1444- and 1319-nm intra-cavity sum-frequency mixing, and output power of 156 mW was obtained. At the output power level of 156 mW, the output power stability is better than 5.0% and laser beam quality M ² factor is 1.23.     

Properties of the resonantly enhanced electric field in inhomogeneous laser-generated plasma

A numerical calculation is presented of the time-resolved response of a cold, inhomogeneous, one-dimensional plasma to obliquely incident laser radiation. The results of the simulation are compared with hard X-ray measurements taken from picosecond pulse laser-generated plasma and are shown to be in good agreement with the experimental data.