Magnetization reversal processes in layered high-temperature superconductors with ferromagnetic impurities

The self-consistent interaction of a vortex system of a high-temperature superconductor and ferromagnetic impurities, including single impurities and their clusters, has been considered in the model of a layered high-temperature superconductor. For different temperatures and concentrations of ferromagnetic impurities, the magnetization reversal loops have been calculated by the Monte Carlo method taking into account an ensemble of ferromagnetic particles with different orientations of their easy magnetization axes with respect to the direction of an external magnetic field and for different magnetic anisotropy energies. It has been demonstrated that there is a nonlinear interaction of the high-temperature superconductor with ferromagnetic impurities, in which the initially thermodynamically reversible character of the magnetization reversal of the ferromagnetic ensemble can become irreversible. For a periodic lattice of clusters of ferromagnetic impurities, the magnetization curves of the high-temperature superconductor have been calculated for different sizes and configurations of the clusters. It has been revealed that, when extended defects are oriented parallel to the direction of the entrance of vortices in the sample, the length of the defects does not affect the remanent magnetization. It has been shown that the inclusion of the interaction between the magnetic moments inside the impurity cluster leads to a decrease in the magnetization reversal loop, the coercivity, and, accordingly, the energy loss due to magnetization reversal.     

Features of magnetization reversal in LCMO/YBCO heterostructures

The change in the magnetic domain structure due to the proximity of a superconductor has been experimentally investigated for the first time. The complex character of magnetization reversal at temperatures below critical, caused by the mutual long-range effect of a superconductor and a magnet, has been shown. In particular, it is found that even magnetization reversal of the heterostructure by an in-plane field leads to the formation of Abrikosov vortices in the superconductor, carrying a flux perpendicularly to the film plane. It is shown that this is a consequence of the transformation of narrow domain walls into wide stripes due to the interaction with scattering fields from the superconductor. In turn, after penetration of the magnetic flux into the superconductor at some depth, the scattering fields cause backward magnetization reversal of the external film edge, as a result of which vortices with oppositely directed fluxes enter the crystal and propagate in the superconductor bulk in the form of chains along twins, as in the case of magnetization by a perpendicular magnetic field. Thus, at longitudinal magnetization, the flux enters the superconducting film in the form of wide stripes with alternating perpendicular induction, which is explained by the long-range interaction of the scattering fields of the superconductor with the manganite magnetization.     

Effect of the soft layer thickness on magnetization reversal process of exchange-spring nanomagnet patterns

A systematic study of the magnetization reversal behavior in the regular arrangement of L1₀-FePt based exchange-spring nanomagnets with different thicknesses of the Co soft magnetic layer is presented. The magnetic property of the hard magnet is compared to two tuned exchange-spring magnets: its systems of 20 nm L1₀-FePt/3 nm, and 7 nm Co. In particular, we focus on the switching field distribution. The exchange coupling showed narrower SFD, in spite of the decoupled part switches earlier. The magnetization switching mechanism of exchange-spring nanomagnets patterns has been revealed with a first-order reversal curves technique and the switching field distribution. Further, the microscopic results using magnetic force microscopy show that the spin rotation of the non-interacting part in the thicker soft layered exchange-spring magnet. The part influences the magnetization reversal process. According to the experimental results, exchange coupling strength can be tuned by the thickness of the soft magnetic layer.     

Spin-injection mechanism of magnetization reversal and hysteresis of current in magnetic junctions

A novel mechanism is proposed for magnetization reversal by the current of magnetic junctions with two metallic ferromagnetic layers and thin separating nonmagnetic layer. The spin-polarized current flows perpendicularly to the interfaces between the ferromagnetic layers, in one of which the spins are pinned and in the other they are free. No domain structure is formed in the ferromagnetic layers. The current breaks spin equilibrium in the free layer, which manifests itself in the injection or extraction of spins. The nonequilibrium spins interact with the magnetization of the lattice due to the effective field of s-d exchange, which is current dependent. At currents exceeding a certain threshold value, this interaction leads to magnetization reversal. Two threshold currents for magnetization reversal have been obtained theoretically, which are reached as the current increases or decreases, respectively. Thus, the phenomenon of current hysteresis is found. The calculated results are in good agreement with experiments on magnetization reversal by current in three-layer junctions of composition Co(I)/Cu/Co(II) prepared in a pillar form.     

Magnetization reversal mechanisms in hybrid resin-bonded Nd–Fe–B magnets

The magnetic properties of isotropic epoxy resin-bonded magnets prepared by mixing a hard magnetic powder made from melt quenched Nd–Fe–Co–B ribbons and a soft magnetic iron powder have been examined. The magnetization reversal processes and the magnetic parameters have been studied by the measurement of the virgin magnetization curves, the major and minor hysteresis loops and sets of recoil curves. From these recoil curves the field dependence of the reversible and irreversible magnetization components during the magnetization and demagnetization processes has been derived. The remanence relationship was used to study the nature of magnetic interaction between the grains. A study of interaction domains was conducted using optical microscopy. Groups of domains, each over several grains, were observed. It was found that the reversal process in the samples investigated involves the rotation of magnetization vectors in the iron powder grains and pinning of domain walls at the MQP-B grain boundaries.     

The study of ultrafast magnetization dynamics induced by femtosecond laser pulses in GdFeCo amorphous film

The time-resolved magneto-optical Kerr spectroscopy technique is used to study the ultrafast magnetization dynamics induced by femtosecond laser pulses in GdFeCo amorphous film. We study concretely the influence of the different pump fluence and the different external magnetic field on magnetization dynamics of ultrafast demagnetization, magnetization reversal and magnetization recovery. The pump fluence dependence magnetization dynamics shows that the degree of demagnetization, the degree of magnetization reversal and the time of magnetization recovery increase with pump fluence, which can be interpreted by the “three-temperature” model. The external magnetic field dependence magnetization dynamics shows that the rate of magnetization reversal increases with the external field, which accord with the magnetization reversal mechanism based on the reversed magnetic domain nucleation and domain-wall motion.     

Nonlinear interaction of a ferromagnet with a high-temperature superconductor

The interaction of an Abrikosov vertex with a ferromagnetic substrate is taken into account in the model of a layered high-temperature superconductor (HTSC). The magnetization reversal loops are calculated by the Monte Carlo method for various values of the magnetic moment of the substrate and at various temperatures. The nonlinearity of the interaction of the superconductor with the ferromagnet is demonstrated. The magnetization of HTSC films on magnetic and nonmagnetic substrates is measured. It is found that the ferromagnetism of the substrate strongly affects the shape and magnitude of the magnetization of the HTSC-substrate composite. Experimental data are found to correlate with the results of calculations.     

Domain wall nucleation in epitaxial exchange-biased Fe/IrMn bilayers with highly misaligned anisotropies

The angular dependence of the magnetization reversal in epitaxial Fe/IrMn bilayers with collinear and non-collinear cubic and unidirectional anisotropies is investigated. Multistep loops with different magnetization reversal processes are observed for either positive or negative angles with respect to the Fe easy axis. The angular dependence of the switching fields displays the broken symmetry of the induced non-collinearity. The experimental results are reproduced with a generalized domain wall nucleation model that includes the induced anisotropy configuration and the peculiar asymmetric magnetic switching behavior. These results highlight the importance of the relative angle between anisotropies in epitaxial exchange bias systems with incoherent rotation reversal mechanism, opening a new pathway for tailoring the magnetic properties of such systems.     

Study of the magnetic interaction in nanocrystalline Pr-Fe-Co-Nb-B permanent magnets

The magnetic properties of an isotropic, epoxy resin bonded magnets made from Pr-Fe-Co-Nb-B powder were investigated. The magnetization reversal process and magnetic parameters were examined by measurements of the initial magnetization curve, major and minor hysteresis loops and sets of recoil curves. From the initial magnetization curve and the field dependencies of the reversible and irreversible magnetization components derived from the recoil loops it was found that the magnetization reversal process is the combination of the nucleation of reversed domains and pinning of domain walls at the grain boundaries and the reversible rotation of magnetization vector in single domain grains. The interactions between grains were studied by means of δM plots. The nonlinear behavior of δM curve approve that the short range intergrain exchange coupling interactions are dominant in a field up to the sample coercivity.The interaction domains and fine magnetic structure were revealed as the evidence of exchange coupling between soft α-Fe and hard magnetic Nd₂Fe₁₄B grains.     

Dynamics of sandwich domain structure in Co-based amorphous ribbons with helical magnetic anisotropy: Part I

The distribution of axes of easy magnetization close to a homogeneous distribution is revealed in each half-thickness of a ribbon after annealing it in a helical magnetic field. The transition from magnetic reversal of a ribbon by the displacement of two domain walls formed near a middle plane of a ribbon to magnetic reversal of a ribbon by displacement of two domain walls formed near to the main surfaces of a ribbon is found out during each half-period of a magnetic reversal.     

Dynamics of magnetic charges in artificial spin ice

Artificial spin ice has been recently implemented in two-dimensional arrays of mesoscopic magnetic wires. We propose a theoretical model of magnetization dynamics in artificial spin ice under the action of an applied magnetic field. Magnetization reversal is mediated by domain walls carrying two units of magnetic charge. They are emitted by lattice junctions when the local field exceeds a critical value Hc required to pull apart magnetic charges of opposite sign. Positive feedback from Coulomb interactions between magnetic charges induces avalanches in magnetization reversal.     

Magnetotransport properties of patterned magnetic Ni wires of submicrometric dimensions

Submicrometric Ni wires have been obtained by electron beam lithography to study their magnetic behavior by magnetotransport measurements. The magnetization reversal of these patterned nanostructures is driven by a combination of two mechanisms: coherent rotation processes, that govern the rotation when the magnetization direction of the lines is away from wire axis, and incoherent curling mechanisms that drive the reversal when the magnetization is closely parallel to line direction.     

Fe掺杂La0．8Sr0．2Co1-xFexO3磁性的研究

利用溶胶-凝胶法制备了一系列的La0.8Sr0.2Co1-xFexO3样品.通过研究在不同外加磁场下磁化强度和温度变化的关系发现,在较高的外场下La0.8Sr0.2Co1-xFexO3样品的磁性反转现象没有被观察到;在低场下La0.8Sr0.2Co1-xFexO3系统磁性反转现象被实现.这说明Fe的掺杂引起了La0.8Sr0.2Co1-xFexO3样品中铁磁和反铁磁之间的竞争,导致了La0.8Sr0.2Co1-xFexO3样品磁性反转;同时外加磁场的强弱影响了La0.8Sr0.2Co1-xFexO3系统磁性反转现象的发生,外加磁场增大使得在La0.8Sr0.2Co1-xFexO3样品中Co离子的自旋平行趋势更强,在铁磁和反铁磁之间的竞争中铁磁耦合占主导优势,因此在较高的外场下磁性反转现象没有被观察到.     

Element-selective nanosecond magnetization dynamics in magnetic heterostructures

We have developed a new original technique to study the magnetization reversal dynamics of thin films with element selectivity in the nanosecond time scale. X-ray magnetic circular dichroism measurements in pump-probe mode are carried out taking advantage of the time structure of synchrotron radiation. The dynamics of the magnetization reversal of each of the layers of complex heterostructures (like spin valves or tunnel junctions) can be probed independently. The interlayer coupling in the studied systems has been shown to play a key role in the determination of the magnetization reversal of each individual layer.     

Evidence for noncollinearity between surface and bulk magnetization in ultrathin Co films

The magnetization reversal of ultrathin Co films on Cu(001) has been investigated by grazing ion scattering and magneto-optical Kerr effect. Differences in the behavior of surface and bulk magnetization are found and attributed to the reduced coordination and site symmetry at the surface. The reversal behavior of the surface magnetization depends on the chemical surface composition. For pure Co films, the reversal of the bulk magnetization is preceded by a complete reversal of the surface magnetization. A particular magnetic state of the surface is suggested as a precursor for magnetization reversal.     

Domain wall dynamics and interlayer interactions in magnetic trilayer systems studied by XMCD-PEEM

We have used time-resolved x-ray magnetic circular dichroism combined with photoemission electron microscopy (XMCD-PEEM) to investigate the layer-resolved microscopic magnetization reversal in FeNi/X/Co (with X=Cu, Al₂O₃) trilayer systems. These measurements were performed in pump-probe mode, synchronizing magnetic pulses with synchrotron x-ray pulses. The good magnetic contrast observed for most samples reveals that in many cases the magnetization reversal is reproducible. We have used the measurements to obtain domain wall propagation speeds as a function of applied magnetic field, and to investigate the influence of domain wall interactions on the magnetic switching.     

In-plane current-induced magnetization reversal of Pd/CoZr/MgO magnetic multilayers

High critical current density ($> 10^{6}$ A/cm$^{2})$ is one of major obstacles to realize practical applications of the current-driven magnetization reversal devices. In this work, we successfully prepared Pd/CoZr(3.5 nm)/MgO thin films with large perpendicular magnetic anisotropy and demonstrated a way of reducing the critical current density with a low out-of-plane magnetic field in the Pd/CoZr/MgO stack. Under the assistance of an out-of-plane magnetic field, the magnetization can be fully reversed with a current density of about 10$^{4}$ A/cm$^{2}$. The magnetization reversal is attributed to the combined effect of the out-of-plane magnetic field and the current-induced spin-orbital torque. It is found that the current-driven magnetization reversal is highly relevant to the temperature owing to the varied spin-orbital torque, and the current-driven magnetization reversal will be more efficient in low-temperature range, while the magnetic field is helpful for the magnetization reversal in high-temperature range.     

垂直自由层倾斜极化层自旋阀结构中的磁矩翻转和进动

在理论上研究了垂直自由层和倾斜极化层自旋阀结构中自旋转移矩驱动的磁矩翻转和进动.通过线性展开包括自旋转移矩项的Landau-Lifshitz-Gilbert方程并使用稳定性分析方法,得到了包括准平行稳定态、准反平行稳定态、伸出膜面进动态以及双稳态的磁性状态相图.发现通过调节电流密度和外磁场的大小可以实现磁矩从稳定态到进动态之间的转化以及在两个稳定态之间的翻转.翻转电流随外磁场的增加而增加,并且受自旋极化方向的影响.当自旋极化方向和自由层易磁化轴方向平行时,翻转电流最小;当自旋极化方向和自由层易磁化轴方向垂直时,翻转电流最大.通过数值求解微分方程,给出了不同磁性状态磁矩随时间的演化轨迹并验证了相图的正确性.     

Magnetization reversal in granular thin films

The paper discusses the physics of magnetization reversal in granular magnetic films. It gives an overview of the key physical properties that determine the collective and macroscopically observable magnetization reversal behavior. In particular, the multitude of observable hysteresis loops is reduced to three key physical quantities, namely the single grain switching field distribution D(h_s), the inter-granular exchange coupling constant J_ex, and the magnetostatic interaction constant J_ms. By varying the relative influence of these quantities, many different shapes of hysteresis loops can occur, which is documented by experimental examples. The regime of partially and strongly correlated reversal is discussed in detail, and minor loop measurements are presented that show scaling behavior for strongly correlated magnetization reversal in the vicinity of hysteresis loop criticality.     

GdFeCo磁光薄膜中RE-TM反铁磁耦合与激光感应超快磁化翻转动力学研究

使用飞秒时间分辨抽运-探测磁光克尔光谱技术,研究了激光加热GdFeCo磁光薄膜跨越铁磁补偿温度时稀土-过渡金属(RE-TM)反铁磁交换耦合行为和超快磁化翻转动力学. 实验观察到由于跨越铁磁补偿温度、净磁矩携带者交换而引起的磁化翻转反常克尔磁滞回线以及在同向外磁场下,反常回线上大于和小于矫顽力部分的饱和磁化强度不同,显示出GdFeCo中RE与TM之间的非完全刚性反铁磁耦合. 在含有Al导热底层的GdFeCo薄膜上观测到饱和磁场下激光感应磁化态翻转及再恢复的完整超快动力学过程. 与剩磁态的激光感应超快退磁化过 关键词： 补偿温度 磁化翻转 反铁磁耦合 GdFeCo