Measurement of theg-factor of the 21 + state of192Pt in an external magnetic field

Theg-factor of the 2₁ ⁺ state of¹⁹²Pt has been measured by the IPAC technique in an external magnetic field as:g(2₁ ⁺,¹⁹²Pt)=+0.287(17). An additional IPAC experiment with an¹⁹²IrFe sample was performed with the same level in order to investigate the hyperfine field. The result:ω _L τ(2₁ ⁺,¹⁹²PtFe)=0.1115(9) gives the hyperfine field:B _hf ^4.2k (PtFe)=126.8(71) T. The result of an LTNO experiment with the same level is compatible with the assumption that 100% of the¹⁹²Ir atoms were on unique sites.     

Hyperfine interaction of Ce and La in 3-d ferromagnets

NMR/ON measurements on¹⁴¹CeFe show the sign of the hyperfine field of CeFe to be negative. For the¹⁴¹Ce nucleus a g-factor of ¦g_N¦=0.311±0.011 is found. With this g-value a hyperfine field of H_hf=?41±2 T for CeFe is derived. Low temperature nuclear orientation experiments on¹⁴¹CeCo and¹⁴⁰LaFe yield ¦H_hf¦=30±3 T and ¦H_hf¦=46±5 T respectively. The valence of cerium impurities in Fe, Co and Ni is discussed.     

g-factor of the 4 1 + rotational state of160Dy

By use of Ge-detectors of the OSIRIS-collaboration [1] in connection with the 12 detector IPAC apparatus of our laboratory [2] a precise measurement of theg-factor of the 4 ₁ ⁺ rotational state of¹⁶⁰Dy was performed. The directional correlations of the threeγ-γ cascades, 1003-197 keV, 1103-197 keV and 1115-197 keV, which are weakly populated in the decay of 72.3 d¹⁶⁰Tb were observed simultaneously. The integral rotations in the static hyperfine field of DyTb at 4.2 K were measured. Theg-factorg(4 ₁ ⁺ )=+0.350(20) was derived. By comparison with the magnetic splitting of the 2 ₁ ⁺ rotational state observed in the same environment by a Mössbauer experiment [3] the ratio of the twog-factors was derived as g(4 ₁ ⁺ )/g(2 ₁ ⁺ )=+ 0.91(5). For the high energy lines we derived from the measured directional correlations the E1/M2 mixing parameters: δ(1003 keV)=+0.005(4); δ(1103 keV)=?0.020(22), and δ(1115 keV)=+0.010(4)     

Hyperfine fields in the 5sp series studied by the low temperature nuclear orientation of83Rb,83Sr,85Sr and85Ym in iron

The hyperfine fields B_hf (RbFe), B_hf (SrFe) and B_hf (YFe) have been determined by the low temperature nuclear orientation of dilute samples of⁸³Rb,^83,85Sr and⁸⁵Y^m in an iron lattice to be B_hf (RbFe)=+54 (10) kG, B_hf (SrFe)=(?)100 (30) kG and B_hf (YFe)=?226 (10) kG. These results are compared with recent calculations for these fields (1), (2).     

Gyromagnetic ratios of 4+ and 6+ states in156Gd and158Gd

The followingg-factors have been derived from time integral measurements of γ-γ angular correlations in the static magnetic hyperfine field of magnetized gadolinium metal probes:¹⁵⁶Gd:g(4 ₁ ⁺ )=+0.310(19)g(6 ₁ ⁺ )=+0.25(21)g(4 ₃ ⁺ , 1511 keV)=+0.809(27)¹⁵⁸Gd:g(4 ₁ ⁺ )=+0.409(15). The 5.35d ¹⁵⁶Tb sources were produced by the reaction¹⁵⁶Gd(d, 2n)¹⁵⁶Tb in our cyclotron. A carrier-free 150y ¹⁵⁸Tb source was obtained from ISOLDE/CERN. In comparison with the precisely knowng-factors of the 2 ₁ ⁺ states,g(2 ₁ ^su+ ,¹⁵⁶Gd) =+0.386(4) andg(2 ₁ ⁺ ,¹⁵⁸Gd)=0.381(4), we observe a large reduction for the¹⁵⁶Gd 4 ₁ ⁺ state whereasg increases slightly for¹⁵⁸Gd. The half-life of the 4 ₁ ⁺ state of¹⁵⁸Gd was remeasured as¹⁵⁸Gd:T _1/2(4 ₁ ⁺ )=148(2) ps. A measurement of the rotation in the 4 ₃ ⁺ state of¹⁵⁶Gd in external magnetic fields of various strengths up toB _ext=9.5 T did not confirm the anomalous dependence of the magnetic hyperfine field in gadolinium metal on the external field, which has been reported by Persson et al. [29].     

Measurement of theg-factor of the 4 1 + -state of202Pb

Theg-factor of the 4 ₁ ⁺ -state of²⁰²Pb was investigated by the IPAC-technique. Inspite of the long half-life, which was measured as:T _1/2(4 ₁ ⁺ -state)=1.97(2)ns and the strong applied external magnetic field of 95.0 kG no rotation of the 787 keV-(422keV)-961 keVγ-γ angular correlation could be observed. Theg-factor must therefore be very small. A computer fit gave the limits:g(4 ₁ ⁺ -state)=+0.002(4). This smallg-factor can be understood by the assumption of an accidental cancellation of a positive contribution by the main [f _5/2 ² ]₄-configuration and several negative contributions by admixtures of all other possible two neutron configurations.     

NMR/ON of206BiFe produced by decay of cold implanted206Po

²⁰⁶Po was implanted into iron at T<0.2 K. After electron capture decay to²⁰⁶Bi nuclear magnetic resonance of oriented²⁰⁶BiFe was observed with an asymmetric resonance line shape. Evaluation of the data with the superposition of two Gaussian lines results in ν=693.7(2) MHz for the center frequency of the narrow one of the two lines at external field zero. From this B_hf (BiFe)=119.0(1.3) T is derived. The effective spin-lattice relaxation time of²⁰⁶BiFe at T=13 mK was measured as Ti=0.94(5) s.     

Gyromagnetic ratios of excited states in186W

The gyromagnetic ratios of the 4 ₁ ⁺ , 6 ₁ ⁺ , and 2 ₂ ⁺ states in¹⁸⁶W were measured relative to that of the 2 ₁ ⁺ level by means of the transient field implantation perturbedγ-ray angular distribution technique. The nuclei in the states of interest were Coulomb excited using a beam of 220-MeV⁶³Cu projectiles and recoiled swiftly through a thin, polarized Fe foil. The present measurements yielded ratiosg(4 ₁ ⁺ )/g(2 ₁ ⁺ )=1.04±0.07,g(6 ₁ ⁺ )/g(2 ₁ ⁺ )=1.03 ±0.20 andg(2 ₂ ⁺ )/g(2 ₁ ⁺ )=0.63±0.13. The sizable disparity between the measuredg-factors of the ground- and excited-band is examined within the context of the interacting boson approximation model.     

Investigation of gamma-ray transitions in56Ni

Angular correlation measurements for the⁵⁴Fe(³He,n γ)⁵⁶Ni reaction were performed at \(E_{3_{He} } = 12.5\) MeV. Method II of Litherland and Ferguson was used to determine the multipole mixing ratio of theγ-radiation and the spins of the excited levels at 3925 and 3956 keV. As the most probable spin assignments we deduced 4⁺ (3925 keV) and 0⁺ (1,2) (3956 keV). The mixing ratio found for the 1225 keV transition from 4⁺→2 ₁ ⁺ isδ(M3/E2)=+0.21 _?0.16 ^+0.23 This result is compared with a shell model calculation.     

Untersuchung des Zerfalls von134Cs durch γ-γ-Winkelkorrelationsmessungen

γ-γ-angular correlation measurements with Ge(Li) detectors and NaJ(Tl) detectors provided theE2/M1 mixing ratios of the following gamma transitions: 3 ₁ ⁺ →2 ₂ ⁺ (475.3 keV), 2 ₂ ⁺ →2 ₁ ⁺ (563.3 keV), 4 ₂ ⁺ →4 ₁ ⁺ (569.4 keV), 3 ₁ ⁺ →2 ₁ ⁺ (1,039 keV). The angular correlation measurements were only consistent with spin 3 of the 1,643 keV level. The half life of the 1,401 keV level was determined by delayed coincidence techniques to beT _1/2 (1,401 keV)≦30 ps.     

Perturbed angular distribution of recoil implanted F19-nuclei in a nickel-environment

Magnetic hyperfine fields acting on F¹⁹ in a Nickel lattice have been investigated. Time-dependent spin rotation has been observed following the excitation and recoil implantation with a pulsed proton beam using the reaction F¹⁹(p,p′)F¹⁹?. Two hyperfine fields were detected at 290 °K:H _hf ⁽¹⁾ =+17.6 ± 0.5 kGH _hf ⁽²⁾ =+91 ± 3 kG. The variation of the effective fields with the external polarizing field was studied. The mean life of the 197 keV level has been remeasured as τ=128±2 nsec.     

Gyromagnetic ratios of the 4+ and 6+ rotational states of184W

The nuclear Larmor precession has been observed for the 2⁺, 4⁺ and 6⁺ rotational states of¹⁸⁴W in the hyperfine field of WFe by application of the TDPAC and the IPAC techniques. A carrier free radioactive source of^184m Re alloyed with high purity iron was used for all three measurements. From the Larmor precession observed in the 2⁺ state by TDPACω _L = 944(15) MHz and the knowng-factor the hyperfine fieldB _{300 K} ^hf (WFe)=?69.6(27)T was derived. The deviation from the result of a spin echo experiment with¹⁸³WFe extrapolated to room temperature may be caused by the Bohr-Weisskopf effect (hyperfine anomaly). IPAC measurements with the same sample polarized in an external magnetic field of 1.6T gave for the 4⁺ and 6⁺ rotational states: ω _L τ(4⁺)=0.0609(22) andω _L τ(6⁺)=0.00735(102). By use of experimentalB(E2)-values theg _R -factors were derived asg _R (4⁺)=+0.276(26) andg _R (6⁺)=+0.281(45). The directional correlation of the 537?384 keVγ-γ cascade has been analysed in terms of anE1/M2/E3 mixture for theK-forbidden 537keV transition. We obtained the mixing ratiosδ(M2/E1)=±0.086(16),δ(E3/E1)=?0.028(5) with the sign convention of Krane and Steffen.     

Frequency dependence of the freezing temperature in spin glasses: A comparative study of (La,Gd)B6, (Y,Gd)Al2 and (La,Gd)Al2

The frequency dependence of the freezing temperatureT _f(ν) is determined for the dilute spin glass systems (La, Gd)B₆ and (Y, Gd)Al₂ in the frequency range 10–1,000 Hz. While for (La, Gd)B₆,T _f(ν) is found to be weak, for (Y, Gd)Al₂ T _f(ν) is even stronger than for the previously studied system (La, Gd)Al₂. Both, measurements of the temperature dependence of the susceptibility nearT _f and calculations of the RKKY pair interaction, suggest that this difference is correlated with a different sign of the nearest-neighbor interaction, which appears to be antiferromagnetic for (La, Gd)B₆ and ferromagnetic for (Y, Gd)Al₂ as well as (La, Gd)Al₂.     

Microscopic foundation of the interacting boson model in thes d-shell nuclei

Starting from an isospin invariant shell-model hamiltonian, we describe a method for deriving microscopically the IBM-hamiltonian appropriate to lights d-shell nuclei. The key ingredients of our approach are:a) the Belyaev-Zelevinsky-Marshalek (BZM) bosonization procedure;b) two successive unitary transformations that extract the “maximally decoupled” collective bosons with angular momentaJ=0(s _ππ ⁺ ,s _νν ⁺ ,s _πν ⁺ ) andJ =2(d _ππ ⁺ ,d _νν ⁺ ,d _πν ⁺ (T=0),d _πν ⁺ (T=1)). The method is applied to obtain the low-energy spectra and the electron scattering form factors for the 0 ₁ ⁺ →2 ₁ ⁺ transitions in²⁰Ne and²⁴Mg. Good agreement with the exact shell-model results is achieved. The inclusion of proton-neutron bosons (s _πν ⁺ ,d _πν ⁺ (T=1),d _πν ⁺ (T=0)), as well as the renormalization of boson parameters due to the non-collective degrees of freedom, are shown to play a crucial role.     

Transition probabilities and the structure of some negative-parity states in126,130Xe and132Ba

The lifetimes of several negative-parity states in^126,130Xe and¹³²Ba have been determined by means of the generalized centroid-shift method. The reactions^124,128Te(α,2n) and¹²²Sn(¹³C, 3n) have been used. Following results were obtained:T _1/2(2758 keV)=1.3±0.2 ns in¹²⁶Xe,T _1/2(2060 keV)=0.20±0.10 ns,T _1/2(2104 keV)=0.50±0.10 ns,T _1/2(2376 keV)=0.30±0.10 ns andT _1/2(2973 keV)=4.6±0.4 ns in¹³⁰Xe as well asT _1/2(2120 keV)=0.40 _?0.10 ^+0.20 ns in¹³²Ba. A systematics of the B(E2; 7 _? ¹ ?5 ₁ ^? ) values in theN=76 nuclei is presented. Electric dipole and quadrupole transition rates are discussed in terms of octupole and quadrupole collectivity. The structure of the 5 ₁ ^? and 7 ₁ ^? states is considered. Nuclear reactions:^124,128Te(α, 2 _n ),E=26 MeV,¹²²Sn (¹³C, 3n),E=53 MeV; measuredE _γ I _γ , γ-r.f. DeducedT _1/2, B(σL) in^126,130Xe and¹³²Ba. Ge detectors. Generalized centroid-shift analysis.     

Transition probabilities and the structure of some negative-parity states in 126,130Xe and 132Ba

The lifetimes of several negative-parity states in ^126,130Xe and ¹³²Ba have been determined by means of the generalized centroid-shift method. The reactions ^124,128Te(α, 2n) and ¹²²Sn(¹³C, 3n) have been used. Following results were obtained: T_1/2(2758 keV) = 1.3 ± 0.2 ns in ¹²⁶Xe, T_1/2 (2060 keV) = 0.20 ± 0.10 ns, T_1/2 (2104 keV) = 0.50 ± 0.10 ns, T_1/2 (2376 keV) = 0.30 ± 0.10 ns and T_1/2 (2973 keV) = 4.6 ± 0.4 ns in ¹³⁰Xe as well as T _1/2(2120 keV) = 0.40 _?0.10 ^+0.20 ns in ¹³²Ba. A systematics of the B(E2; 7 ₁ ^? ? 5 ₁ ^? ) values in the N = 76 nuclei is presented. Electric dipole and quadrupole transition rates are discussed in terms of octupole and quadrupole collectivity. The structure of the 5 ₁ ^? and 7 ₁ ^? states is considered. Nuclear reactions: ^124,128Te(α, 2n), E = 26 MeV, ¹²²Sn (¹³C, 3n), E = 53 MeV; measured E_{gg}, I_{gg}, γ-r.f. Deduced T_1/2, B(σL) in ^126,130Xe and ¹³²Ba. Ge detectors. Generalized centroid-shift analysis.     

g-factors of the ground state rotational band of158Dy

Theg-factors of the four lowest states of the ground state rotational band of¹⁵⁸Dy have been determined asg(2 ₁ ⁺ )=+0.362(23),g(4 ₁ ^su+ )=+0.340(20),g(6 ₁ ^su+ )=+0.207(36) andg(8 ₁ ^su+ )=+0.21(11). Theg-factors of the 2⁺ and 4⁺ states were measured by the IPAC method with radioactive samples of 2.4 h¹⁵⁸Er in external magnetic fields. To investigate the higher states, for the first time an on-line γ—γ IPAC experiment was performed with the reaction¹⁵⁶Gd(α, 2n)¹⁵⁸Dy by use of the static hyperfine field of DyGd.     

Remeasurement of the lifetime of the 4 1 + -state of156Gd and recalculation of itsg-factor

The half-life of the 4 ₁ ⁺ -state of¹⁵⁶Gd has been remeasured by the delayed coincidence technique. The excellent time resolution which can now be achieved by use of small BaF₂ detectors allows a more reliable determination than with previously applied methods. The resultT _1/2(¹⁵⁶Gd,4 ₁ ⁺ )=108(2) ps is smaller than previously published data, but it fits well into the systematics of theB(E2) values of the rotational transitions of this nucleus. A recalculation of the previously measuredg-factor of the same state givesg(¹⁵⁶Gd,4 ₁ ⁺ ) =0.327(19). This value is still smaller than theg-factor of the 2 ₁ ⁺ state, but the magnitude of the reduction can now easier be interpreted by nuclear structure calculations.     

Transition probabilities and hole-core coupled configurations in107In

The nucleus¹⁰⁷In was studied by in-beam spectroscopic methods in (HI, xn yp) reactions. Spin and parity values of some levels were determined by conversion electron andγ-ray measurements. Using the generalized centroid shift method, the half-lives T_1/2(19/2⁺, 2003.6 keV)=0.6±0.2 ns and T_1/2(17/2⁺, 1853.4 keV)=1.7±0.3 ns were measured. The systematics of the lowest members of the multipletπg ₉ ^2/?1 ×6 ₁ ⁺ in^111,109,107In is discussed     

Gyromagnetic ratios of collective states of166Er

The static hyperfine field ofB _hf ^4.2k (ErHo) = 739(18)T of a ferromagnetic holmium single crystal polarized in an external magnetic field of ± 0.48T at ～4.2K was used for integral perturbed γ-γ angular correlation (IPAQ measurements of the g-factors of collective states of¹⁶⁶Er. The 1,200y ^166m Ho activity was used which populates the ground state band and the γ vibrational band up to high spins. The results: $$\begin{gathered} g(4_g^ + ) = + 0.315(16) \hfill \\ g(6_g^ + ) = + 0.258(11) \hfill \\ g(8_g^ + ) = + 0.262(47)and \hfill \\ g(6_\gamma ^ + ) = + 0.254(32) \hfill \\ \end{gathered}$$ exhibit a significant reduction of the g-factors with increasing rotational angular momentum. The followingE2/M1 mixing ratios of interband transitions were derived from the angular correlation coefficients: $$\begin{gathered} 5_\gamma ^ + \Rightarrow 4_g^ + :\delta (810keV) = - (36_{ - 7}^{ + 11} ) \hfill \\ 7_\gamma ^ + \Rightarrow 6_g^ + :\delta (831keV) = - (18_{ - 2}^{ + 3} )and \hfill \\ 7_\gamma ^ + \Rightarrow 8_g^ + :\delta (465keV) = - (63_{ - 12}^{ + 19} ). \hfill \\ \end{gathered}$$ The results are discussed and compared with theoretical predictions.