Use of an electrical aerosol detector (EAD) for nanoparticle size distribution measurement

Recently, Nanoparticle Surface Area Monitor (NSAM, TSI model 3550) and EAD (EAD, TSI Model 3070A) have been commercially available to measure the integral parameters (i.e., total particle surface area and total particle length) of nanoparticles. By comparison, the configuration of the EAD or NSAM is similar to that of electrical mobility analyzer of the early generation for particle size distribution measurement. It is therefore possible to use the EAD or NSAM as a particle sizer. To realize the objective of using the EAD as a sizer, we characterized the average electrical charges of monodisperse particles passing through the EAD particle charger and ion trap set at voltages ranging from 20 to 2500 V. The average charge data collected at different ion-trap voltages were then summarized by the empirical correlation using the parameter of Z _p *V, where Z _p is the particle electrical mobility and V is the ion-trap voltage. A data-reduction scheme was further proposed to retrieve the size distribution of sampled particles from the EAD readout at different ion-trap voltages. In the scheme, the functional format of each mode in a number size distribution of particles was assumed as log-normal, but the number of modes in an entire size distribution is not limited. A criterion was used to best fit the simulated EAD readouts with experimental ones by varying the count median diameter (CMD), geometric standard deviation (σ _g), and total particle number (N _t ) of each mode in a particle size distribution. Experiments were performed to verify the proposed scheme.     

Evaluation of an electrical aerosol detector (EAD) for the aerosol integral parameter measurement

The performance of an electrical aerosol detector (EAD; TSI Model 3070A) was experimentally evaluated for measuring the integral parameters of particles (i.e., total length concentration of particles, and the total surface area concentrations of particles deposited in a human lung). The EAD consists of a unipolar diffusion charger with an ion trap, and aerosol electrometer. We first evaluated the performance of the EAD charger. Both polydisperse and monodisperse particles of Ag, NaCl, and oleic acid (with the dielectric constants of infinite, 6.1 and 2.5) were then generated to evaluate the particle material effect on the EAD readout.     

Cooling and trapping polar molecules in an electrostatic trap

An electrostatic trap for polar molecules is proposed. Loading and trapping of polar molecules can be realized by applying different voltages to the two electrodes of the trap. For ND3 molecular beams centered at ～10 m/s, a high loading efficiency of ～67% can be obtained, as confirmed by our Monte Carlo simulations. The volume of our trap is as large as ～3.6 cm3, suitable for study of the adiabatic cooling of trapped molecules. Our simulations indicate that trapped ND3 molecules can be cooled from ～23.3 m K to 1.47 m K by reducing the trapping voltages on the electrodes from 50.0 k V to1.00 k V.     

Behaviors of absolute instabilities of electrostatic ion cyclotron waves in an ion beam-plasma system

Experimental results are presented for behaviors of the temporal growth and the threshold beam density of the absolute instability of the electrostatic ion cyclotron waves excited in an ion beam-plasma system, and compared with the linear theory.     

Deceleration and electrostatic trapping of OH radicals

A pulsed beam of ground state OH radicals is slowed down using a Stark decelerator and is subsequently loaded into an electrostatic trap. Characterization of the molecular beam production, deceleration, and trap loading process is performed via laser induced fluorescence detection inside the quadrupole trap. Depending on the details of the trap loading sequence, typically 10(5) OH (X2Pi(3/2),J=3/2) radicals are trapped at a density of around 10(7) cm(-3) and at temperatures in the 50-500 mK range. The 1/e trap lifetime is around 1.0 s.     

Novel wet electrostatic precipitator for collection of fine aerosol

A novel wet electrostatic precipitator (WESP) is designed for effective control of fine aerosol from humid gases. It operates on the principle of unipolar particle charging in the corona discharge and particle precipitation under the field of their own space charge. The new precipitator is characterized by high gas velocity in the ionizing stage. Tests were carried out for gas with (NH₄)₂SO₄, HCl and (NH₄)Cl aerosol at particle number concentration up to 5·10⁷#/cm³ and mass concentration 10–1000 mg/Nm³. For test conditions one-field WESP ensures mass collection efficiency 90–97% and two-field electrostatic precipitator up to 99%.     

Compensating for excess micromotion of ion crystals

A new method of compensating for the excess micromotion along two directions in three-dimensional Coulomb crystals is reported in this paper; this method is based on shape control and optical imaging of a Coulomb crystal in a sectioned linear ion trap. The characteristic parameters, such as the ion numbers, temperatures, and geometric factors of different ion crystals are extracted from the images and secular motion excitation spectra. The method of controlling the shape of the ion crystals can be used in cold ion experiments, such as sympathetically cooling, structural phase transitions,and selective-control of ions, etc.     

Absolute and convective instabilities of electrostatic ion cyclotron waves excited in an ion beam-plasma system

Experimental results are presented for the observation of the absolute and convective instabilities of the electrostatic ion cyclotron waves excited in an ion beam-plasma system.     

Demonstration of three-dimensional electrostatic trapping of state-selected Rydberg atoms

A three-dimensional trap for Rydberg atoms in selected Stark states has been realized experimentally. H atoms seeded in a supersonic expansion of Ar are excited to the low-field seeking n=30, k=25, |m|=0, 2 Rydberg-Stark states, decelerated from a mean initial velocity of 665 m/s to zero velocity in the laboratory frame and loaded into a three-dimensional electrostatic trap. The motion of the cold Rydberg atom cloud in the trap and the decay of the trapped atoms have been studied by pulsed electric field ionization and imaging techniques.     

Nonlinear amplitude osçillations of absolutely unstable electrostatic ion cyclotron waves in an ion beam-plasma system

We have observed experimentally the amplitude oscillations of absolutely unstable electrostatic ion cyclotron waves in an ion beam-plasma system due to nonlinear interaction between the beam ions and electrostatic ion cyclotron waves.     

Behaviors of electrostatic ion cyclotron waves excited in ion beam-plasma systems

Experimental results are presented for a behavior of the electrostatic ion cyclotron waves excited in an ion beam-plasma system. This wave appears as forward and backward waves with respect to the propagating component along the magnetic field.     

Deuterium excess in precipitation of Alpine regions - moisture recycling

The paper evaluates long-term seasonal variations of the deuterium excess (d-excess = delta(2)H - 8. delta(18)O) in precipitation of stations located north and south of the main ridge of the Austrian Alps. It demonstrates that sub-cloud evaporation during precipitation and continental moisture recycling are local, respectively, regional processes controlling these variations. In general, sub-cloud evaporation decreases and moisture recycling increases the d-excess. Therefore, evaluation of d-excess variations in terms of moisture recycling, the main aim of this paper, includes determination of the effect of sub-cloud evaporation. Since sub-cloud evaporation is governed by saturation deficit and distance between cloud base and the ground, its effect on the d-excess is expected to be lower at mountain than at lowland/valley stations. To determine quantitatively this difference, we examined long-term seasonal d-excess variations measured at three selected mountain and adjoining valley stations. The altitude differences between mountain and valley stations ranged from 470 to 1665 m. Adapting the 'falling water drop' model by Stewart [J. Geophys. Res., 80(9), 1133-1146 (1975).], we estimated that the long-term average of sub-cloud evaporation at the selected mountain stations (altitudes between about 1600 and 2250 m.a.s.l.) is less than 1 % of the precipitation and causes a decrease of the d-excess of less than 2 per thousand. For the selected valley stations, the corresponding evaporated fraction is at maximum 7 % and the difference in d-excess ranges up to 8 per thousand. The estimated d-excess differences have been used to correct the measured long-term d-excess values at the selected stations. Finally, the corresponding fraction of water vapour has been estimated that recycled by evaporation of surface water including soil water from the ground. For the two mountain stations Patscherkofel and Feuerkogel, which are located north of the main ridge of the Alps, the maximum seasonal change of the corrected d-excess (July/August) has been estimated to be between 5 and 6 per thousand, and the corresponding recycled fraction between 2.5-3 % of the local precipitation. It has been found that the estimated recycled fractions are in good agreement with values derived from other approaches.     

Fluorine in silicon: diffusion,trapping, and precipitation

The effect of vacancies on the behavior of F in crystalline Si has been elucidated experimentally for the first time. With positron annihilation spectroscopy and secondary ion mass spectroscopy, we find that F retards recombination between vacancies (V) and interstitials (I) because V and I trap F to form complexes. F diffuses in the V-rich region via a vacancy mechanism with an activation energy of 2.12+/-0.08 eV. After a long annealing time at 700 degrees C, F precipitates have been observed by cross-section transmission electron microscopy which are developed from the V-type defects around the implantation range and the I-type defects at the end of range.     

Production of nonisothermal electrons and Langmuir waves because of colliding ion holes and trapping of plasmons in an ion hole

We present new simulation studies exhibiting production of nonisothermal electron distributions and Langmuir waves by colliding ion holes and trapping of plasmons in an ion hole. We find that, during head-on ion hole collisions, streams of accelerated electrons are produced by the electrostatic potentials supporting the ion holes. Subsequently, Langmuir waves are excited by a two-stream instability involving energetic electron beams. The resulting Langmuir waves can be trapped in an ion hole. The present ion-hole-Langmuir wave interactions are unique kinetic phenomena which can be dealt with a Vlasov code, which we developed recently. The results can have relevance to the understanding of particle and field data that are forthcoming from different spacecraft missions in Earth's auroral ionosphere and the magnetosphere.     

In situ discovery of an electrostatic potential, trapping electrons and mediating fast reconnection in the Earth's magnetotail

Anisotropic electron phase space distributions, f, measured by the Wind spacecraft in a rare crossing of a diffusion region in Earth's far magnetotail (60 Earth radii), are analyzed. We use the measured f to probe the electrostatic and magnetic geometry of the diffusion region. For the first time, the presence of a strong electrostatic potential (1 kV) within the ion diffusion region is revealed. This potential has far reaching implications for the reconnection process; it accounts for the observed acceleration of the unmagnetized ions out of the reconnection region and it causes all thermal electrons be trapped electrostatically. The trapped electron motion implies that the thermal part of the electron distributions are symmetric around v( parallel)=0: f(v( parallel),v( perpendicular)) approximately f(-v( parallel),v( perpendicular)). It follows that the field aligned currents in the diffusion region are limited and fast magnetic reconnection is mediated.     

Ra+ ion trapping: toward an atomic parity violation measurement and an optical clock

A single Ra⁺ ion stored in a Paul radio frequency ion trap has excellent potential for a precision measurement of the electroweak mixing angle at low momentum transfer and as the most stable optical clock. The effective transport and cooling of singly charged ions of the isotopes ²⁰⁹Ra to ²¹⁴Ra in a gas filled radio frequency quadrupole device is reported. The absolute frequencies of the transition 7s²S_1/2–7d²D_3/2 at wavelength 828 nm have been determined in ^212–214Ra⁺ with ≤19 MHz uncertainty using laser spectroscopy on small samples of ions trapped in a linear Paul trap at the online facility Trapped Radioactive Isotopes: µicrolaboratories for fundamental Physics (TRIµP) of the Kernfysisch Versneller Instituut.